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Granular mixing in 2 and 3 dimensions

Rob Sturman

Department of MathematicsUniversity of Leeds

Dynamical Systems Seminar, 19 October 2007Surrey

Joint work with Steve Meier, Julio Ottino, NorthwesternSteve Wiggins, University of Bristol

Rob Sturman Granular mixing

Mixing

Mixing of granular materials:is important — Science 125th anniversary identifiedgranular flow as one of the 125 big questions in Scienceis ubiquitous — pharmaceuticals, food industry, ceramics,metallurgy, constructionwas initially explained by analogies with fluid mixing —hence terms like granular shear and granular diffusion

But the big difference is that granular materials tend tosegregate

Rob Sturman Granular mixing

Mixing

Mixing of granular materials:is important — Science 125th anniversary identifiedgranular flow as one of the 125 big questions in Scienceis ubiquitous — pharmaceuticals, food industry, ceramics,metallurgy, constructionwas initially explained by analogies with fluid mixing —hence terms like granular shear and granular diffusion

But the big difference is that granular materials tend tosegregate

Rob Sturman Granular mixing

Mixing

Mixing of granular materials:is important — Science 125th anniversary identifiedgranular flow as one of the 125 big questions in Scienceis ubiquitous — pharmaceuticals, food industry, ceramics,metallurgy, constructionwas initially explained by analogies with fluid mixing —hence terms like granular shear and granular diffusion

But the big difference is that granular materials tend tosegregate

Rob Sturman Granular mixing

Mixing

Mixing of granular materials:is important — Science 125th anniversary identifiedgranular flow as one of the 125 big questions in Scienceis ubiquitous — pharmaceuticals, food industry, ceramics,metallurgy, constructionwas initially explained by analogies with fluid mixing —hence terms like granular shear and granular diffusion

But the big difference is that granular materials tend tosegregate

Rob Sturman Granular mixing

Mixing

Mixing of granular materials:is important — Science 125th anniversary identifiedgranular flow as one of the 125 big questions in Scienceis ubiquitous — pharmaceuticals, food industry, ceramics,metallurgy, constructionwas initially explained by analogies with fluid mixing —hence terms like granular shear and granular diffusion

But the big difference is that granular materials tend tosegregate

Rob Sturman Granular mixing

Segregation

Granular materials segregate by (at least) 2 mechanisms:

Percolation — little particles fall through the gaps of bigparticlesBuoyancy — less dense particles tend to rise

The Brazil Nut effect

Rob Sturman Granular mixing

Segregation

Granular materials segregate by (at least) 2 mechanisms:

Percolation — little particles fall through the gaps of bigparticlesBuoyancy — less dense particles tend to rise

The Brazil Nut effect

Rob Sturman Granular mixing

The draft lottery

In 1969, the Selective Service Systemof the USA held a lottery to determinethe order of draft into the U.S. Army forthe Vietnam War.Days of the year numbered 1 to 366drawn once to assign lottery number,and again to determine draft number.

Rob Sturman Granular mixing

The draft lottery

In 1969, the Selective Service Systemof the USA held a lottery to determinethe order of draft into the U.S. Army forthe Vietnam War.Days of the year numbered 1 to 366drawn once to assign lottery number,and again to determine draft number.

Rob Sturman Granular mixing

The draft lottery

0

50

100

150

200

250

300

350

0 50 100 150 200 250 300 350

Lotte

ry r

ank

Birthday

Rob Sturman Granular mixing

Tumbler Mixers

Rob Sturman Granular mixing

Different tumbler geometries

Rob Sturman Granular mixing

Flow regimes

[from S. W. Meier et al., 2007]

Rob Sturman Granular mixing

Tumblers

[from S. W. Meier et al., 2007]

Rob Sturman Granular mixing

[Zuriguel, I., Gray, J.M.N.T., Peixinho, J. & T. Mullin (2006).Phys. Rev. E 73, 061302.]

Rob Sturman Granular mixing

Tumblers

Modelling percolation and buoyancy

[from S. W. Meier et al., 2007]

Rob Sturman Granular mixing

2D circular tumblers

In the bulk

r = 0, θ = ω

In the flowing layer

x = γ(δ(x)+y), y = ωxy/δ(x)

The flowing layer hasshape

δ(x) = δ0

√1 − x2/L2

Rob Sturman Granular mixing

Constant rotation rate

At constant rotation rateparticle streamlines form closed loops passing throughflowing layersteady, divergence-free, integrablecan transform to action–angle coordinates ρ, φtrajectories in action–angle coordinates given by:

ρ = 0φ = 2π/T (ρ)

taking a time τ -map gives a twist map

P(ρ, φ) = (ρ, φ+ 2πτ/T (ρ))

Rob Sturman Granular mixing

Constant rotation rate

At constant rotation rateparticle streamlines form closed loops passing throughflowing layersteady, divergence-free, integrablecan transform to action–angle coordinates ρ, φtrajectories in action–angle coordinates given by:

ρ = 0φ = 2π/T (ρ)

taking a time τ -map gives a twist map

P(ρ, φ) = (ρ, φ+ 2πτ/T (ρ))

Rob Sturman Granular mixing

Constant rotation rate

At constant rotation rateparticle streamlines form closed loops passing throughflowing layersteady, divergence-free, integrablecan transform to action–angle coordinates ρ, φtrajectories in action–angle coordinates given by:

ρ = 0φ = 2π/T (ρ)

taking a time τ -map gives a twist map

P(ρ, φ) = (ρ, φ+ 2πτ/T (ρ))

Rob Sturman Granular mixing

Constant rotation rate

At constant rotation rateparticle streamlines form closed loops passing throughflowing layersteady, divergence-free, integrablecan transform to action–angle coordinates ρ, φtrajectories in action–angle coordinates given by:

ρ = 0φ = 2π/T (ρ)

taking a time τ -map gives a twist map

P(ρ, φ) = (ρ, φ+ 2πτ/T (ρ))

Rob Sturman Granular mixing

Constant rotation rate

At constant rotation rateparticle streamlines form closed loops passing throughflowing layersteady, divergence-free, integrablecan transform to action–angle coordinates ρ, φtrajectories in action–angle coordinates given by:

ρ = 0φ = 2π/T (ρ)

taking a time τ -map gives a twist map

P(ρ, φ) = (ρ, φ+ 2πτ/T (ρ))

Rob Sturman Granular mixing

Variable rotation rate

Break the integrability by varying the rate of angular rotationSinusoidal forcing has been well-studied.

[Fiedor and Ottino, JFM 255 2005]

Rob Sturman Granular mixing

Variable rotation rate

[Fiedor and Ottino, JFM 255 2005]

Rob Sturman Granular mixing

Variable rotation rate

Key idea is that streamlines changes and cross

[Fiedor and Ottino, JFM 255 2005]

Rob Sturman Granular mixing

Piecewise constant rotation rate

Simplify the forcing by using a blinking flow

ω =

ωb = ω + ω for iτ < t < (i + 1/4)τωa = ω − ω for (i + 1/4)τ < t < (i + 3/4)τωb = ω + ω for (i + 3/4)τ < t < (i + 1)τ

Alternate the angular velocity between ωa and ωb.

Rob Sturman Granular mixing

Poincaré sections

N = 2 N = 4

N = 6 N = 8

Rob Sturman Granular mixing

Blinking experiments

Rob Sturman Granular mixing

Linked Twist Maps on the plane

Domain is two intersect-ing annuli with two dis-tinct regions of intersec-tion

Rob Sturman Granular mixing

Linked Twist Maps on the plane

The action of a twist mapis to take a line...

Rob Sturman Granular mixing

Linked Twist Maps on the plane

... and twist it around theannulus.Then do the same withpoints in the other annu-lus.

Proof of ergodic mixing due to Burton & Easton (1980),Devaney (1980), Wojtkowski (1980), Przytycki (1983)

Rob Sturman Granular mixing

Linked Twist Maps on the plane

... and twist it around theannulus.Then do the same withpoints in the other annu-lus.

Proof of ergodic mixing due to Burton & Easton (1980),Devaney (1980), Wojtkowski (1980), Przytycki (1983)

Rob Sturman Granular mixing

Linked Twist Maps on the plane

... and twist it around theannulus.Then do the same withpoints in the other annu-lus.

Proof of ergodic mixing due to Burton & Easton (1980),Devaney (1980), Wojtkowski (1980), Przytycki (1983)

Rob Sturman Granular mixing

The Blinking Vortex

Rob Sturman Granular mixing

The Blinking Vortex

Rob Sturman Granular mixing

The Blinking Vortex

Rob Sturman Granular mixing

The Blinking Vortex

Rob Sturman Granular mixing

Microfluidics — patterned walls

from [Stroock, A. D. et al., Science 295, 647–651 (2002)]

Rob Sturman Granular mixing

Microfluidics — electroosmotic flow

from [Qian, S. & Bau, H. H., Anal. Chem., 74, 3616–3625 (2002)]

Rob Sturman Granular mixing

Streamline crossing structure

Rob Sturman Granular mixing

3-dimensional spherical tumbler

An obvious way to introduce some transversality...

Rob Sturman Granular mixing

Rotation about the z-axis

Solid body rotation in the bulk:

x = ωyy = −ωxz = 0

Shear in the flowing layer:

x = γ1(δ1(x , z) + y)

y = ω1xy/δ1(x , z)

z = 0

Boundary of flowing layer and bulk:

δ1(x , z) = δ0

√1 − x2/L2

=√ω1/γ1

√R2 − x2 − z2

Rob Sturman Granular mixing

Rotation about the z-axis

Solid body rotation in the bulk:

x = ωyy = −ωxz = 0

Shear in the flowing layer:

x = γ1(δ1(x , z) + y)

y = ω1xy/δ1(x , z)

z = 0

Boundary of flowing layer and bulk:

δ1(x , z) = δ0

√1 − x2/L2

=√ω1/γ1

√R2 − x2 − z2

Rob Sturman Granular mixing

Rotation about the z-axis

Solid body rotation in the bulk:

x = ωyy = −ωxz = 0

Shear in the flowing layer:

x = γ1(δ1(x , z) + y)

y = ω1xy/δ1(x , z)

z = 0

Boundary of flowing layer and bulk:

δ1(x , z) = δ0

√1 − x2/L2

=√ω1/γ1

√R2 − x2 − z2

Rob Sturman Granular mixing

Rotation about the x-axis

Solid body rotation in the bulk:

x = 0y = −ωzz = ωy

Shear in the flowing layer:

x = 0y = ω2zy/δ2(x , z)

z = γ2(δ2(x , z) + y)

Boundary of flowing layer and bulk:

δ2(x , z) = δ0

√1 − z2/L2

=√ω2/γ2

√R2 − x2 − z2

Rob Sturman Granular mixing

Rotation about the x-axis

Solid body rotation in the bulk:

x = 0y = −ωzz = ωy

Shear in the flowing layer:

x = 0y = ω2zy/δ2(x , z)

z = γ2(δ2(x , z) + y)

Boundary of flowing layer and bulk:

δ2(x , z) = δ0

√1 − z2/L2

=√ω2/γ2

√R2 − x2 − z2

Rob Sturman Granular mixing

Rotation about the x-axis

Solid body rotation in the bulk:

x = 0y = −ωzz = ωy

Shear in the flowing layer:

x = 0y = ω2zy/δ2(x , z)

z = γ2(δ2(x , z) + y)

Boundary of flowing layer and bulk:

δ2(x , z) = δ0

√1 − z2/L2

=√ω2/γ2

√R2 − x2 − z2

Rob Sturman Granular mixing

Dynamical properties I

TheoremIf ω1/γ1 = ω2/γ2 then motion of a particle is constrained to asingle hemispherical surface.

Rob Sturman Granular mixing

Dynamical properties II

TheoremPeriod 1 points for rotation about the x-axis form a bowl in theshape of a prolate spheroid.

Rob Sturman Granular mixing

Intersection of bowl and spheroid

Rob Sturman Granular mixing

Experiments

Experiments...are hard — how do you see what’s happening inside a spherefilled with a granular material?

Rob Sturman Granular mixing

Experiments

Experiments...are hard — how do you see what’s happening inside a spherefilled with a granular material?

Rob Sturman Granular mixing

Rob Sturman Granular mixing

Rob Sturman Granular mixing

Piecewise isometries

[Goetz, 2003]

Rob Sturman Granular mixing

Outstanding problems

3 dimensional transport through the hemispherethe role of segregationthe role of the dynamics of piecewise isometrieshow to measure, or even see, all the above in anexperiment

Rob Sturman Granular mixing

Outstanding problems

3 dimensional transport through the hemispherethe role of segregationthe role of the dynamics of piecewise isometrieshow to measure, or even see, all the above in anexperiment

Rob Sturman Granular mixing

Outstanding problems

3 dimensional transport through the hemispherethe role of segregationthe role of the dynamics of piecewise isometrieshow to measure, or even see, all the above in anexperiment

Rob Sturman Granular mixing

Outstanding problems

3 dimensional transport through the hemispherethe role of segregationthe role of the dynamics of piecewise isometrieshow to measure, or even see, all the above in anexperiment

Rob Sturman Granular mixing