III. Challenges Deriving integrative results of ExUTLS chemical observations Diagnosing the key...

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III. Challenges• Deriving integrative results of ExUTLS

chemical observations

• Diagnosing the key processes that maintain and control the chemical structure

• Reconciling physical models and definitions of the extratropical tropopause

Challenges (1): Deriving integrative results of ExUTLS chemical observations

• How/what do we use the aircraft observations to quantify? – Fine structure? STE? Transport barriers and pathways?

• What are the “right” quantities to be used as effective metrics for evaluations and constraints of CCMs?– “flux” “budget” and “age spectra”, tracer correlations

• What are the effective coordinates for integrating UTLS observations? – Eql-q, Trop rel Alt., wind speed/jet

Hintsa et al., 1998

The use of tracer correlations

Marcy et al., 2004

Laura Pan, 3/4/08 O3-CO relationship for tropospheric intrusions

All

RF01

RF01,08,09,14

Pittman et al., in progress

Integrative tracer correlations

Atlas et al., Vogel et al., in progress

START08 workshop 6January 8-9, 2008

Age spectrum derived using NMHC, Ehhalt et al., 2007

Information from tracers of different lifetimes

Age and age spectrum

Ray et al., TuesdayAtlas et al., Wednesday

Examples of using EqL in the UTLS region for compiling tracer climatology: [Hoor et al.,

2004]

Coordinates for integrating data:

Tilmes et al., submitted

Profiles in tropopause referenced Rel. Alt

Coordinates for integrating data:

Dynamical coordinates: wind field/Jet streams:

Ray et al., 2004

Brioude et al., 2004

Combine Jet and Rel Alt, in progress:

Tilmes et al., Manney et al.,

Challenges (2): diagnosing the key processes that maintain and control the chemical structure

• How do we identify the roles and interactions of multi-scale dynamical processes (i.e., planetary, synoptic, meso-scale including convection and GW)?

– Are small scale processes important?

• How do we identify, model and quantify mixing?

Stone et al., in progress

Vogel et al., Konopka et al, Tuesday

DTP and TIL: are they results of the same process?

Challenges (3): Physical models and Definitions of the extratropical tropopause (ExTP)

• How do we best characterize the ExTP as a transport boundary?

• How do we reconcile the multiple existing conceptual models/definitions of the ExTP?

• What processes control the occurrence and spatial extent of multiple tropopauses?

The Dichotomy of the Tropopause Definitions

Palmen & Newton, 1969 Shapiro & Keyser, 1990

“The Thermal Tropopause” “The Dynamical Tropopause”

(WMO, 1957) (Reed, 1955, Danielsen, 1968; Shapiro, 1980; WMO, 1986; Holton et al., 1995;…)

Adapted from Chapter 2 WMO (2002), Law, Cox & Haynes

Extratropical Transition Layer - ExTL?

Chemical Tropopause using tracer correlations?

Zahn, 2003

Statistical “Chemopause” or ExTL

Pan et al., 2007

ExTL vs TTL

Tropics: Two physical boundaries

Extratropics: one physical boundary

Gettelman and Foster, 2002

Birner, 2006

ExTL vs TTL – existence of multiple horizontal boundaries

Expectations to the workshop

• Emerging pictures -> Conceptual framework?

• From Mainz workshop 2005: “well defined terminology” “STE=STT/TST”, “ExTL”

• Broader picture: How is the extratropical UTLS coupled to the tropical UTLS? The processes near the subtropical break?