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...G/,IC79Q G/,IR =D R C79Q -M & + #( * ( C79Q F $% 1J 48A 1J N48G;En1J !'" 1J L48A 1J L48A 1J $%...

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Page 1: ...G/,IC79Q G/,IR =D R C79Q -M & + #( * ( C79Q F $% 1J 48A 1J N48G;En1J !'" 1J L48A *1J L48A *1J $% P; !'" P; < 48 O8D G/,I(CT):D G/,I:D CT2> K5 G/,IC79Q N@ 3 G; 6 0B ...

Page 2: ...G/,IC79Q G/,IR =D R C79Q -M & + #( * ( C79Q F $% 1J 48A 1J N48G;En1J !'" 1J L48A *1J L48A *1J $% P; !'" P; < 48 O8D G/,I(CT):D G/,I:D CT2> K5 G/,IC79Q N@ 3 G; 6 0B ...

-

Page 3: ...G/,IC79Q G/,IR =D R C79Q -M & + #( * ( C79Q F $% 1J 48A 1J N48G;En1J !'" 1J L48A *1J L48A *1J $% P; !'" P; < 48 O8D G/,I(CT):D G/,I:D CT2> K5 G/,IC79Q N@ 3 G; 6 0B ...

Page 4: ...G/,IC79Q G/,IR =D R C79Q -M & + #( * ( C79Q F $% 1J 48A 1J N48G;En1J !'" 1J L48A *1J L48A *1J $% P; !'" P; < 48 O8D G/,I(CT):D G/,I:D CT2> K5 G/,IC79Q N@ 3 G; 6 0B ...

Page 5: ...G/,IC79Q G/,IR =D R C79Q -M & + #( * ( C79Q F $% 1J 48A 1J N48G;En1J !'" 1J L48A *1J L48A *1J $% P; !'" P; < 48 O8D G/,I(CT):D G/,I:D CT2> K5 G/,IC79Q N@ 3 G; 6 0B ...

Page 6: ...G/,IC79Q G/,IR =D R C79Q -M & + #( * ( C79Q F $% 1J 48A 1J N48G;En1J !'" 1J L48A *1J L48A *1J $% P; !'" P; < 48 O8D G/,I(CT):D G/,I:D CT2> K5 G/,IC79Q N@ 3 G; 6 0B ...

Page 7: ...G/,IC79Q G/,IR =D R C79Q -M & + #( * ( C79Q F $% 1J 48A 1J N48G;En1J !'" 1J L48A *1J L48A *1J $% P; !'" P; < 48 O8D G/,I(CT):D G/,I:D CT2> K5 G/,IC79Q N@ 3 G; 6 0B ...

12

(12 )

Page 8: ...G/,IC79Q G/,IR =D R C79Q -M & + #( * ( C79Q F $% 1J 48A 1J N48G;En1J !'" 1J L48A *1J L48A *1J $% P; !'" P; < 48 O8D G/,I(CT):D G/,I:D CT2> K5 G/,IC79Q N@ 3 G; 6 0B ...

Page 9: ...G/,IC79Q G/,IR =D R C79Q -M & + #( * ( C79Q F $% 1J 48A 1J N48G;En1J !'" 1J L48A *1J L48A *1J $% P; !'" P; < 48 O8D G/,I(CT):D G/,I:D CT2> K5 G/,IC79Q N@ 3 G; 6 0B ...

-

Page 10: ...G/,IC79Q G/,IR =D R C79Q -M & + #( * ( C79Q F $% 1J 48A 1J N48G;En1J !'" 1J L48A *1J L48A *1J $% P; !'" P; < 48 O8D G/,I(CT):D G/,I:D CT2> K5 G/,IC79Q N@ 3 G; 6 0B ...

15%

10 0kJ/mol

XH••• CH•••nCH•••

Page 11: ...G/,IC79Q G/,IR =D R C79Q -M & + #( * ( C79Q F $% 1J 48A 1J N48G;En1J !'" 1J L48A *1J L48A *1J $% P; !'" P; < 48 O8D G/,I(CT):D G/,I:D CT2> K5 G/,IC79Q N@ 3 G; 6 0B ...

C-H

( 1kJ/mol)

Page 12: ...G/,IC79Q G/,IR =D R C79Q -M & + #( * ( C79Q F $% 1J 48A 1J N48G;En1J !'" 1J L48A *1J L48A *1J $% P; !'" P; < 48 O8D G/,I(CT):D G/,I:D CT2> K5 G/,IC79Q N@ 3 G; 6 0B ...

Page 13: ...G/,IC79Q G/,IR =D R C79Q -M & + #( * ( C79Q F $% 1J 48A 1J N48G;En1J !'" 1J L48A *1J L48A *1J $% P; !'" P; < 48 O8D G/,I(CT):D G/,I:D CT2> K5 G/,IC79Q N@ 3 G; 6 0B ...

n

* *

(CT)

CT

Page 14: ...G/,IC79Q G/,IR =D R C79Q -M & + #( * ( C79Q F $% 1J 48A 1J N48G;En1J !'" 1J L48A *1J L48A *1J $% P; !'" P; < 48 O8D G/,I(CT):D G/,I:D CT2> K5 G/,IC79Q N@ 3 G; 6 0B ...

H-

) ace-to-

face

ring-over-

ring):(ring-over-bond)

Page 15: ...G/,IC79Q G/,IR =D R C79Q -M & + #( * ( C79Q F $% 1J 48A 1J N48G;En1J !'" 1J L48A *1J L48A *1J $% P; !'" P; < 48 O8D G/,I(CT):D G/,I:D CT2> K5 G/,IC79Q N@ 3 G; 6 0B ...

-( )

Page 16: ...G/,IC79Q G/,IR =D R C79Q -M & + #( * ( C79Q F $% 1J 48A 1J N48G;En1J !'" 1J L48A *1J L48A *1J $% P; !'" P; < 48 O8D G/,I(CT):D G/,I:D CT2> K5 G/,IC79Q N@ 3 G; 6 0B ...

K = zV0/V

K

Page 17: ...G/,IC79Q G/,IR =D R C79Q -M & + #( * ( C79Q F $% 1J 48A 1J N48G;En1J !'" 1J L48A *1J L48A *1J $% P; !'" P; < 48 O8D G/,I(CT):D G/,I:D CT2> K5 G/,IC79Q N@ 3 G; 6 0B ...

(a) -

(b),c) -

a), b)

Page 18: ...G/,IC79Q G/,IR =D R C79Q -M & + #( * ( C79Q F $% 1J 48A 1J N48G;En1J !'" 1J L48A *1J L48A *1J $% P; !'" P; < 48 O8D G/,I(CT):D G/,I:D CT2> K5 G/,IC79Q N@ 3 G; 6 0B ...

r-6 r-3

- -

Page 19: ...G/,IC79Q G/,IR =D R C79Q -M & + #( * ( C79Q F $% 1J 48A 1J N48G;En1J !'" 1J L48A *1J L48A *1J $% P; !'" P; < 48 O8D G/,I(CT):D G/,I:D CT2> K5 G/,IC79Q N@ 3 G; 6 0B ...

-

-

1,4-

-

Page 20: ...G/,IC79Q G/,IR =D R C79Q -M & + #( * ( C79Q F $% 1J 48A 1J N48G;En1J !'" 1J L48A *1J L48A *1J $% P; !'" P; < 48 O8D G/,I(CT):D G/,I:D CT2> K5 G/,IC79Q N@ 3 G; 6 0B ...

-

CH3CN> H3N> (CH3)3N

sp2 sp3

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