Fallout radionuclides to investigate soil erosion:An overview
Lionel Mabit Institute of Environmental Geosciences, University of Basel
Soil Degradation
80% of degraded land is located in developing countries !!!
From: Oldeman et al. (1990)
Methods for erosion measurement
Modeling (USLE, Erosion 3D, Eurosem, AGNPS..)
Erosion pins Erosion plots
Indirect methods (sediment deposits)
Nuclear techniques(radioisotopes)
Reasons for using radioisotopes
The fallout is universal
Strongly fixed to soil particles
Integration of climatic variability
Only one sampling required to estimate erosion processes
Sediment budgets can be calculated at different scales
Radioisotopes for erosion studies
Nuclide Origin Half-life γ-Energy
137Cs Artificial 30 y 661 keV
7Be Natural 53 d 477 keV
210Pb Natural 22 y 46 keV
Guiding principle of 137Cs method
Initial fallout of 137Cs
Reference site (RS) e.g: 2000 Bq/m²
Erosion
Stable
Deposition
♦ Samples
137Cs level higher than RS e.g: 3000 Bq/m²
137Cs level lower than RS e.g: 1600 Bq/m²
137Cs level around RS e.g: 2100 Bq/m²
In the field : Sampling with soil corer or cylinder
Establish a sampling strategy1 - Vertical and horizontal sampling (transect..)
Pennock and Appleby, 2002
Grid Sampling
Pennock and Appleby, 2002
Transect Sampling
Lab 1 (pre-preparation) : Drying and sieving
Lab 2 (measurement) : Gamma spectroscopy
Gamma detector
Gamma spectroscopy analysis
Conversion Bq/m² ± t/ha/yr (Models)
Conversion Bq/kg Bq/m²
Case study on the application of FRN (137Cs)
180ha
From: Bernard et al. (1998); Mabit et al. (1998 and 1999)
180 ha
Temperate Climate
~ 700 mm/yr
~ 140-150 m
Slopes ~ 2 %
Silty loam
Land use
Openfield
Dry thalweg
Vierzy watershed land use
Potato 10 %
Other 15 % Winter wheat 45 %
Sugar beet 30 %
AugustJune
December–May(Bare Soil)
October / November
(Harvest)
March
September-February
(Bare Soil)
June
November-May(Bare Soil)
August
Map of the soil movement in
Vierzy
Model
Sampling and geostatistical
analysis
-18 -15 -12 -9 -6 -3 0 3 6 9 12 15 18 20 2
154 m
146 m
154 m
Mouvement des sols en tonnes/hectare/an
500 m
N
EROSION DEPOSITION
Soil movement in t/ha/yr
-18 -15 -12 -9 -6 -3 0 3 6 9 12 15 18 20 21
154 m
146 m
154 m
Mouvements des sols en tonnes/hectare/an
500 m
N
EROSION DÉPOSITION
Soil movement in t/ha/yr
Eroding area% total area 45Mean erosion (t/ha /yr) 6
Sedimentation area% total area 15Mean deposition (t/ha /yr) 7
Total areaNet output (t/ha/yr) 2SDR (%) 60
Stable area% total area 40
2 t/ha/yr
Sediment budget of the watershed
OM (%) = 0,0002 137Cs (Bq m-2) + 0.96 (n = 30 ; r = 0,79 ; p < 0,001)
1.01.11.21.31.41.51.61.71.81.92.0
1000 1500 2000 2500 3000 3500 4000 4500
137Cs (Bq/m2)
OM
(%)
ErosionStableDeposition
Erosion vs soil quality
From: Mabit and Bernard (1998)
Boyer River watershed ~ 200 km2
60% of the basin area is cultivated
Affected by a degradation of the soil and water resources
Boyer River watershed (Canada)
0102030405060708090
61 63 65 67 69 71 73 75 77 79 81 83 85 87Year
Ton
s
Use of GIS and 137Cs
5 Soil–slope combinations
GIS: identify sectors with similar agri-environmental conditions (soil, slope, land use)
MBM + IDW2
Land use: forest and agricultural area
14 reference areas (n=42)
2860 Bq m-2 ; CV of 21% (n = 42)
Min 3 representatives fields / isosector
3 transects ~ 10 samples/transect
Summary of results
GIS/137Cs
Overall sediment production = 2.8 t ha-1 yr-1
28% of the arable lands of the watershed present erosion rateshigher than 6 t ha-1 yr-1
Sediment production per isosectors
Conclusion and perspectivesFRNs are very useful tools for improving knowledge about erosion processes;
The use of 137Cs as soil tracer in Alpine areas : current status
(ii) Test 239+240Pu more homogenous distribution - Nuclear bomb tests origins
(i) Re-sampling method for 137Cs based on the samples collected in 2007
(i) to localize degraded area and (ii) to quantify the magnitude of soil erosion
Heterogeneity of the initial fallout originating from Chernobyl
Successfully applied in 2010 and 2012 (e.g. Schaub et al., 2010)
Meusburger et al., 2010
i. Bernard, C., Mabit L., Wicherek, S., Laverdière, M.R. (1998). Long-term soil redistribution in a small French watershed as estimated from 137Cs data. Journal of Environmental Quality, 27(5), 1178-1183.
ii. Mabit, L. (2011). Erosion/deposition data derived from fallout radionuclides (FRNs) using geostatistics. In: Impact of soil conservation measures on erosion control and soil quality. IAEA-TECDOC-1665. pp. 185-194.
iii. Mabit, L., Benmansour, M., Walling D.E. (2008). Comparative advantages and limitations of Fallout radionuclides (137Cs, 210Pb and 7Be) to assess soil erosion and sedimentation. Journal of Environmental Radioactivity, 99(12), 1799-1807.
iv. Mabit, L., Bernard, C. (1998). Relationship between soil inventories and chemical properties in a small intensively cropped watershed. Comptes Rendus de l’Académie des Sciences, Série IIa, Earth and Planetary Sciences, 327 (8), 527-532.
v. Mabit, L., Bernard, C., Laverdière, M.R. (2007). Assessment of erosion in the Boyer River watershed (Canada) using a GIS oriented sampling strategy and 137Cs measurements. Catena, 71(2), 242-249.
vi. Mabit, L., Bernard, C., Laverdière, M.R., Wicherek, S. (1999). Assessment of water erosion in a small agricultural basin of the St.Lawrence river watershed. Hydrobiologia, 410, 263-268.
vii. Mabit, L., Bernard, C., Laverdière, M.R., Wicherek, S. (1998). Spatialisation et cartographie des risques érosifs à l’échelled’un bassin versant agricole par un radio-isotope (137Cs). Étude et Gestion des sols, 5 (3), 171-180.
viii. Zupanc, V., Mabit, L. (2010). Nuclear techniques support to assess erosion and sedimentation processes: preliminary results of the use of 137Cs as soil tracer in Slovenia. Dela, 33, 21-36.