heavy water production. industrial process and plants

Comitato Nazionale Energia Nucleare

HEAVY WATER PRODUCTION. INDUSTRIAL PROCESS AND PLANTS

(A Bibliography - 2nd Rev, Edition)

D. LAVRENCIC

Comitato Nazionale Energia Nucleare

H~AVY WATER PRODUCTION. INDUSTRIAL PROCESS AND PLANTS

(A Bibliography - "nel Rei'. Edition)

D. LAVRENCIC

Testo pervenuto nel febbraio 1974

Edito dai Comitato Nazionale Energia Nucieare, Divisione Affari Internazionali e Studi Economici, Ufficio Edizioni Scientifiche - Viale Regina Margherita, 125 Roma.

Stampato in formato UNI presso la Tipolitografia RANCOS - Roma

I N D E X

I. Genera l pag. 1

II. Bibl iographies

III. Determinat ion and Analyses of Heavy Water

IV. Heavy Water Production

A - Reviews of Production P r o c e s s e s B - Patents Review (Brévatome, Pa r i s ) C - Actual Industr ia l P r o c e s s e s D - Production P lan ts and Equipment E - Technical and Economic Aspects F - Potent ial Product ion P r o c e s s e s

V. Heavy Water Reac to r s " 279

VI. Main Conferences Held on Heavy Water

and HWRs • " 2 9 9

Subject Index " 307

Authors Index " 3 1 1

Societ ies Index " 377

I I

It

II

II

II

II

II

II

II

31

41

73

75 97

137 195 227 237

Annex

Introduction

This work aims at outlining a status of the heavy water production processes and fabrica'!^-1 plants.

The bibliography contains references from the scientific and technical l i terature on analysis and production of heavy water and on the role of irWIl in nuclear power p rograms . It does not include refe rene us to survey biological effects oi' deuterium and heavy water.

The material is arranged under the following main i tems:

I. General: general information on the principal subject of the bibliography and on related ones.

II. Bibliographies: bibliographies on deuterium and heavy water and on related arguments .

i l l . Determination and analyses of deuterium and heavy water: various methods for the following analysis of hydrogen and for water production are reported.


A: Reviews of various production processes ;

B: Review of patents on heavy water production (Patents selected by Brévatome, Par is) ; Addendum with patents reported on Nuclear Science Abstracts (1972 - 1973, Oct. 15 t h);

C: Actual industrial p rocesses : chemical exchange (bithermal exchange between hydrogen sulphide and water; single tempera ture ammonia-hydrogen exchange; hydrogen-water exchange);

ID: Production plants and equipment: conceptual studies on designs; description, operation and equipment of fabrication plants and projects. A sheet of plants and projects ordered by country is also included;

E: Reviews on technical and economic aspects of industrial heavy water production; consumption and demand of D 2 0 ;

IT

F. : Potential production processo«: chemical exchange processes between other substances than those mentioned above; physical separation processes (distillation, absortive fractionation, absorbtion, diffusion etc. ) and others.

V. Heavy water reactors

A. : A table of research, test and power heavy-water-moderated reactors is included. For the bibliography on this reading, reference is made to heavy water x-eactors bibliography, .edited by IAEA, Vienna, in January, 1970. (ST1/PUB/21/37)

13.: HWlts in Nuclear Power Programmes: nuclear strategy studies with HW/ls performed in different countries; heavy water and fuel requirements for HWlt.

VI. Main Conferences on Heavy Water and Heavy Water Reactors are also listed.

Under each subject, references are listed from the first to the most recent one. The magazines where the year, only'is "indicateti are listed in alphabetical order.

In cases where the exact title is not known, a title containing the subject of reference is given in brack test. Works are given in English language, unless otherwise marked.

Author index is included. Authors of the patents listed in the Addendum are not included in this index.

The main sources of information are the Nuclear Science Abstracts from 1946 to 1973; the Chemical Abstracts, as well as the available bibliographies and status report from USA, USSR, France, Canada, India, Germany, Italy and Romania are also been examined.

I l l

R e f e r e 11cos

Nuclear Science Abs t rac t s 194G-19r/:>. (Oct. 15, 197:-!)

Bibliography of Research on Heavy Water Compounds. A. II. Kimball Comp, H. C. Urey, 1. Kirshenbaum eds , 1st ed. McGraw-Hil l Book Co. , lnc 1949, ( N"NES-ri[~4C).

Isotope Separat ion and Isotope Exchange. G. M. Begun, R . E . Allen Comps. TID-3 036 (Revised). June 1954.

Production of Heavy Water . G. M. Murphy, II, C. Urey, 1. Kirshenbaum eds . 1st ed. McGraw-Hil l Book Co. , Inc. New York - Toronto - London. 1955. (NNES-4F)

Heavy Water Product ion. J , J, Jacobs comp. TID-3091 (Suppl. .1) June 1964.

Deute r ium and Heavy Water . A Selected Bibliography. G. I-I. Vasa ru , A. Mihaila, P . Szentgyorgyi. May 1970.

I - G E N E R A L

3

I - G E N l'I II A T,

1. THE HYDROGEN ISOTOPE OF MASS 2. Kallmann H. , Easarcfi ' W. Naturwisscnseh. 20, 472, 1932.

2. A HYDROGEN ISOTOPE OF MASS 2. Urey U . C . , Bviekwoi.Ule F . G. , Murphy G. M. I'Jiya.' Jiev. 39, 164-5, 1032.

3. ISOTOPE OF HYDROGEN OF MASS 2. A Review. Landsberg G. S. Uspekhi F i z . Nauk 12, 343-50, 1932. (In Russian)

4. HEAVY WATER. Boahouffer K. F. Angew. Chcm. 46, 776-9, 1933.

5. ISOTOPE OF HYDROGEN AM) ITS 1 'JlOPURTiES. Mikolic S.S. Bull. Soc. Chini. Roy. Yougoslave 4, 227-35, 1933.

6. ISOTOPES. A Review. Kaptein A . J . G. Gliom, vveekblad 30, 695-701.. 1933.

7. ISO'J.'OPLOS OF HYDROGEN. Lewis G.N. ,J. Amur . C h e m . S ü e . 55, 1207-8 ,1933.

8. THEORETICAL CONSIDERATIONS CONCERNING THE SEPARATION OF ISOTOPES. Eyving I I . , She rman A. J . Clicm. Phys . 1, 345-0, 1933.

9. HEAVY HYDROGEN AND HEAVY WATER.. A Review. Naturo 132, 5:3GJO:}:j.

10. SEPARATION OF Til LO ISOTOPES OF HYDROGEN. Collie C . l l . Nature 132, 5G8-9,1033.

11 . EXPERIMENTS ON HEAVY HYDROGEN. P a r k a s A. , F a r k a s L. Nature 132, 894 ,1033 .

12. HEAVY HYDROGEN. Rutherford E. Nature 132, 955-G, 1933.

13. THE RELATIVE ABUNDANCE OF HYDROGEN ISOTOPES. Bleakney W. , Gould A . J . Phys . Rev. 44, 2G5-8, 1933.

14. THEORETICAL AND PRATICAL STUDIES OF ATOMIC AND MOLECULAR FORMS OF THE HYDROGEN ISOTOPES. Taylor H . S . , E y r i n g II. P r o c . Am . P h i l . Soc. 72, 255-64, 1933.

5

15. CHEMICAL PROPERTIES OF THE HYDROGEN ISOTOPES. Urey U .C . Rev. Sci. Instr . 4, 423-5 , 1933.

16. SEPARATION AND PROPERTIES OF THE ISOTOPES OF HYDROGEN. Urey U . C . Science 78 ,506-71 , 1933.

17. RECENT ADVANCES IN SCIENCE;PHYSICAL CHEMISTRY. A R e view. Wanribrough-Jones O.II . Science P r o g r e s s 28 ,107-15 ,1933 .

18. HEAVY WATER. A Review. Domange L. Ann. pha rm, franc. 4 1 , 144-8,1934.

19, HEAVY HYDROGEN AND THE WORK OF HAROLD C. UREY. A Review. Harkins W.D. Chem.'Bull. '(Chicago) 21 , 83-7, 1934.

20. HEAVY HYDROGEN OR DEUTERIUM, AND HEAVY WATER. A Review. Boutàr ic A. Genie civil. 104,444-6, 1934.

21. HEAVY WATER. A Review. Lindner J . Scientia F a r m . 5, 24-9 , 1934.

22. HEAVY HYDROGEN AND HEAVY WATER. A Review. Ouellet C. Natural is te canadj.en 61 , 205-11, 1934.

23. HEAVY HYDROGEN AND HEAVY WATER. A Review. Nature 133, 197,1934.

24. PHYSICAL AND CHEMICAL PROPERTIES OF HEAVY WATER. A Review. I l ideal E .K. Nature 134,504, 1934.

ft

THE HYDROGEN ISOTOPE AND HEAVY WATER. A Review. F r e r i c h s R. N a t u r w i s s e n s c h a l t e n 22, 1 1 3 - 8 , 1934.

THE HEAVY HYDROGEN ISOTOPE. F a r k a s L. Na turwissenschaf ten 22, G14-23;640-G;G58-G2, 1934.

THE HYDROGEN ISOTOPE O F MASS 2. A Review. Haant jes J . Nede.rl. T i j d sch r . Na tuurk . 1, 33-4 0 ,1934.

HEAVY WATER. Dominik W. Pol ish A y r . F o r e s t . Ann. 33 , 359-70 , 1934.

METHODS AND RESULTS OF RESEARCH ON ISOTOPES. Mattauch J . Phys ik . Z . 3 5 , 5 0 7 - 0 2 1 , 1934.

EXPERIMENTS ON HEAVY HYDROGEN. F a r k a s A , , F a r k a s L . P r o c . Roy. Soc. (London) A144, 467-80 , 1934.

ISOTOPES OF HYDROGEN AND THEIR SEPARATION. A Review. V e i l S . Rev. Sci . 72, 174-7 , 1934.

THE NEW HYDROGEN. Science 8 0 , 2 1 - 5 , 1934.

THE NEW HYDROGEN. An A d r c s s . Ru the r fo rd E . Sc ient ia Milan 5 5 , 3 4 1 - 9 , 1 9 3 4 .

HEAVY HYDROGEN. Chit tock C. School Sc i . Rev . 16, 132, 1934.

7

35. HEAVY WATER. A Review. Cignoli F . Semana méd. (Buenos Aires ) 1,2008-71, 1934.

3ß. ISOTOl'Y OF HYDROGEN. HliJAVY WATER. A Review. Hamann E. Süddeutsche Apotli. Ztg. 74, 1,15-G, 1934.

37. HYDROGEN ISOTOPE AND HEAVY WATER. Vasi l 'ov A. M. T r a n s . Kirov Inst. Chcm. Tcchnol. (Kazan) No. 2, 129-49, 1934. (In Russian)

38. ISOTOPE OF HYDROGEN AND HEAVY WATER. Tcmkin M. Uspekhi Khini. 3, 217-35, 1934. (In Russian)

3 9. 1SOTOPY OF HYDROGEN, HEAVY WATER. A Review. Bochme J. Z. physik. c hem. Unterr icht 47, 216-23, 1934. (In German)

40. STUDY ON PROBLEMS: HEAVY WATER, HEAVY HYDROGEN AND GRAVITATION. Har tmann J. U. 1934. (In German)

4 1 . HEAVY WATER. Mark H. Ed. F . Dcuticke, Leipzig.

42. SOME THERMODYNAMIC PROPERTIES OF HYDROGEN AMD DEUTERIUM. Nobel Lec tu re . Urey II. C. Angew. Chem. 48, 315-20, 1935.

43 . DEUTERIUM AND ITS COMPOUNDS. A Review. Darmois F . Bull. Soc. Chini. (France) (5) 2, 1513-44, 1935.

44. HEAVY HYDROGEN AND HEAVY WATER. A Review. Malan-Nelson A. M . G i o r n . fa rm. chim. 84, 108-17, 1935.

3

il RA VT HYDROGEN Alvi.) HEAVY WATER. A liuviow. Ciay , ] . Ingenieur (Utrecht) 5 0 A , 2 2 0 - 3 , J935 .

ISOTOiTC EXCHANGE EQUILIBRIA. Urey l i . C. , Croi IT L , Y. ,J. A i a . . CliOJn.Soc. 57, 321-7 , HJo'5.

HYDROGEN ISOTOPES AND DEUTERIUM OXIDE OH HEAVY WATER, P r o s o v i t s P. Keemiu Touted 2, 50-liO, 1Ü35.

HEAVY WATER IN CHEMISTRY, Pulanyi M, Naturo 135, 19-26, 1JJ35.

ISOTOPES. A Review. Aston E. W. Na tu re 135,080-7 ,11)35.

DEUTERIUM, A NEW TOOL POR. CHEMISTS. A Review. Greene C I L NUCIOUK 12, J7Ü-2, 1.935.

HEAVY HYDROGEN AND 20th CENTURY CHEMISTRY. A L e c t u r e . P h a r m . J .1:54,88, 1935.

OUR PRESENT KiX'OWLEDCE OP HEAVY HYDROGEN AND HEAVY WATER. Mark I I . , Wuld IVI. Pi-utuplasinu 20, 109-27, 1935.

HYDROGEN AND OXYGEN ISOTOPES AND HEAVY WATER. A Review. I.unelund H. Tek . Poe i -en . i Pinkuid P o c r h . 55, 35-ÌÌ, 11)35.

9

54., ISOTOPY OF THE ELEMENTS. A Review. Mattauch J. Z.VDI 79, 1140-4,1935. -

&5. DATA ON HEAVY WATER. Reitz O.Junk. , The Hague 1935. (In German)

56. ORTOHYDROGEN, PARX AHYDROGEN, AND HEAVY HYDROGEN. F a r k a s A. Cambridge Universi ty P r e s s , London 1935. (The McMillan Co. New York 1935)

57. THE SEPARATION OF ISOTOPES. Champet ier G. Bull. soc . c him. (France) 3 (5) 1701-27,1936.

58. HEAVY HYDROGEN, THE ISOTOPE OF HYDROGEN'AND HEAVY WATER. Champet ie r G. Bull, soc , encour . ind. nat i . 135, 237-49, 1936.

59. HEAVY HYDROGEN - HEAVY WATER. A Review. Stoeckl K. 'Med. Klim.32, 1105-9, 1936.

60. HEAVY WATER. A Review. Bueno O. G. Pol i tecnica , (Quito, Ecuador) 1 ,306-12,1936.

61 . RECENT ADVANCES IN SCIENCE:GENERAL AND ORGANIC CHEMISTRY. ISOTOPES. Brady O. L. Science P r o g r e s s 31 , 100-3,1936.

62. THE HEAVY HYDROGEN ISOTOPE. A Review:Wir tz K. Z .phys ik . ehem. Unterr icht 49, 14-28, 1936.

63 . VAPOR PRESSURE AND HEAT OF VAPORIZATION OF HEAVY WATER. Riesenfeld E. H . , Chang T. L. Z. physik. Chem. B 33, 120-6,1936.

to

THE PHYSICAL CHEMICAL AND BIOLOGICAL QUALITIES OF HEAVY WATER. A Review. Indovina R.,Citarda A. Bipchim. e T e r a p . s p e r . 2 4 , 2 3 6 - 4 7 , 1 9 3 7 .

RECENT RESEARCH ON HEAVY WATER AND ITS OCCURRENCE IN NATURE. Riesenfeld E. II. Sveiisfckem. TM. 49, 113-23, 1937.

HEAVY WATER. Seijo E. Rev. cent ro estud. farm, y biochim. 27, 92-107,1937.

DEUTERIUM AND HEAVY WATER. A Review. Borocco A. L. Rev. chim. ind. (Par i s ) 46, 322-9, 1937.

REACTIONS IN HEAVY WATER. A Review. Suess H. Ö s t e r r . Chem. Ztg.(Wien) 40 ,239-43 ,1937 .

GENERAL AND INORGANIC CHEMISTRY OF DEUTERIUM. A Review.Einecke.E. Chem. Ztg. (Wien) 4 1 , 331-40;355-9;371-6; 395-400,1938.

CONCENTRATION OF THE HEAVY ISOTOPES OF OXYGEN AND THE ISOTOPIC ANALYSIS OF WATER.Skar re O.K. , Brodskii AjI .Dokl . AkacT. Nauk. SSR 20, 565-8, 1938. (Rept. L . V.' P i sa rzhevsk i i Inst.' P h y s . Chem. Sci. Acad. Sci. Ukr. SSR 11, 75-98,1938)

ISOTOPES. A Review. Souza-Reis F . de, Moggi S. Rev.quim. e farm. Rio de Jane i ro 3, 34-40, 1938..

NEWS ABOUT HEAVY HYDROGEN. A Review. Royen P . Umschau 42 ,207-9 , 1938.

DEUTERIUM AND ITS COMPOUNDS. (Deuterium and composes de deuter ium. Tables annuelles de constantes . No. 1) Hermann Cie, P a r i s 1938. (In French)

11

74, HEAVY WATER, A Review. Kilde G. Dansk. Tids . F a r m . 13, 69-92, 1939.

75. SEPARATION OF ISOTOPES. Walcher W. Ergeb. exakt. Naturwiss . IB', 155-228, 1939.

76. HEAVY WATER. A Review, Steinert B. Wallerstein Labs. Com.-muns. 2 ,21-4 , 1939.

77. THE SEPARATION OF ISOTOPES. Urey II. C. Pub. Am. Assoc . Advance. Sci. No. 7, Recent Advances in Surface Chemis t ry and Chem. Phys . 73-87, 1939. (Reports on P r o g r e s s in Physics VI, 48-87,1939)

78. SEPARATION OF ISOTOPES .Urey H .C . Phys. Soc. Reports on P r o g r e s s in Physics 6 ,48-77, 1940.

79. SEPARATION AND USE OF STABLE ISOTOPES. Uréy H . C . J . Appi. Phys . 12, 270-7, 1941.

80. 'IEAVY WATER. A Review. Selwood P . W. J . Chem. Education 18, 515-20, 1941.

81. ISOTOPE REVIEW FOR 1940. Flu egge S. , Mattauch J . Physik. Z . 42 ,1 -5 , 1941.

82." PROPtBAlS FOR CONCENTRATION OF DEUTERIUM. Cohen K. Columbia Ser ia l No. 4R-133, Aug. 194.1.

83.' PROPOSALS FOR CONCENTRATION OF DEUTERIUM. Cohen K. SAM Rep. A-118, June 1941.'

84. THE THEORY OF RATE PROCESS. Glasstonc S. , Laidlor K. J . , Eyring J-I. McGraw-Hill , Now York, 1941,

8 5 ; CHEMICAL ENGINEERS' HANDBOOK, J, II, P e r r y Ed. McGraw Hill Book Co. Inc. New York 1941. (pp.'2542, 2550-G2)

8G. REPORT ON ISOTOPES, 1941. Flügge S , , Mattauch J, Physik. Z. 43, 1-5, 1942.

87. SEPARATION FACTOR. Cohen K. , Mayer H. L, SAM Rep, 4M-11 , ' Jan , 13, 1942,

88. THE HYDROGEN ISOTOPES;THERMODYNAMIC PROPERTIES OF THEIR COMPOUNDS. MDDC-149(>. Sept. 1942. Deci. Nov. 25, 1947.

89. MATERIALS OF CONSTRUCTION. Hiskey C. F . SAM Rop, 100XR-lC52.Nov.-10, 1942.

90. THE THEORY OF ISOTOPE SEPARATION BY EXCHANGE REACTIONS. Waldmann L. Naturwiss . 31, 205-6, 1943.(In German) (AEC-tr-1911)

91. THE PHENOMENA OF SEPARATION PROCESSES. Klemm A. Z. Physik 123, Nos. 1-2 ,10-27,1944.

92. METALLURGICAL PROJECT REPORT. F e r m i E . , Zinn W. H. , Wattenberg A. CP-1827. June 1944.

93. HEAVY WATER. Kirshenbaum I . , Graff J . , Fors t a t H. SAM Rep. A-2193.Aug.T7, 1945.

http://100XR-lC52.Nov.-10

13

94. APPLICATIONS OF ISOTOPES IN CATALYTIC REACTIONS AT SURFACES. Taylor PI. S. F ron t ie r s in Chemistry 3, 19-42,1945.

95. SYMPOSIUM ON ATOMIC ENERGY AND ITS IMPLICATIONS. 50 YEARS OF ATOMIC PHYSICS. METHODS AND OBJECTIVES IN THE SEPARATION OF ISOTOPES. Urey II. C. P roc . Am. Phil . Soc.90, No. 1, 30-5, 1946.

96. THE THERMODYNAMIC PROPERTIES OF ISOTOPIC SUBSTANCES. A Review. Urcy U.C. J . Chora. Soc. 502-31,.1947.

97. ISOTOPE SEPARATION FOR THE PURPOSE OF PRODUCTION OF NUCLEAR ENERGY. Groot S.'lt. de.Nedcrland Tijdsch. Naturk. 13,113-20, 1947.

98. SEPARATION OF STABLE ISOTOPES. Steward D..W. Nucleonics 1, 18-26, 1947.

99. ; SEPARATION AND PHYSICS OF ISOTOPES. A Review. Paemel O. van. Tech. Wetenschap. Tijdsch. 10, 56-9, 1947.

100. THE SCIENCE AND ENGINEERING OF INfUCLEAR POWER. Goodman C. Ed Addison Wesley, Cambridge Mass. 1947-4 8.

101. THE SEPARATION OF STABLE ISOTOPES. Par ravano G. Chimica e Industr ia 30,296-301,1948.

102. SEPARATION OF ISOTOPES. Dunlap G. W., Lichtenstein R. M. Elee. Eng. N. Y. 65, 469-74, 1948.

14

FIAT Rev. German Science 1939-46: \

103. SEPARATION OF UNWEIGHTABLE AMOUNTS OF SUBSTANCES (ISOTOPES) AND USE OF THE PRODUCT OBTAINED. Inorg. C h e m . P t . 1.113-20, 1948;

104. SEPARATION OF ISOTOPES. Dickel G. Inorg. Chem. P t . I . 121-3,1948;

105. SEPARATION OF ISOTOPES IN SMALL QUANTITIES. Walcher W. Nuclear Phys ics and Cosmic Rays . P t . I I , 94-107, 1948;

106. INACTIVE ISOTOPES, THEIR SEPARATION AND APPLICATIONS. Dickel G. Phys . Chem. 7-17, 1948;

107. ISOTOPE EXCHANGE EQUILIBRIA; Suess H. Phys . Chem. 19-24, 1948.

108. ISOTOPE SEPARATION BY UREY'S METHOD. Muylle R. L ' indus t r i e Chemique Beige 13 ,17-23 , 1948.

109. SOME RECENT WORK ON THE SEPARATION AND USE OF STABLE ISOTOPES. Lauder I. J . P r o c . Roy. Soc. N. S. Wales 82, 183-95, 1948.

110. COMPILATION OF THERMAL PROPERTIES OF HYDROGEN IN ITS VARIOUS ISOTOPE AND ORTO-PARA MODIFICATIONS. Wooley H. W. , Scott R. B . , Brickwedde F . G. J . Res . Natl. Bur. Stds. 4 1 , 379-475, 1948.

15

111. FUNDAMENTALS OF ISOTOPE SEPARATION. A Review. Cohen K. Nucleonics 6 ,2 ,3 -9 ,1948 .

112. ATOMIC ENERGY FOR MILITARY PURPOSES. Smythe H.D. Princeton University P r e s s , Princeton N, J. 1948.

113. ON THE SEPARABILITY OF ISOTOPES IN SOLUTION. Martin H. Proc. of the German Buns en Soc. for Applied Phys. Chemistry Meeting, Stuttgart. Oct. 7-10, 1948. Angew.'Chem. 61, 297-305, 1949. (In German)

114. HEAVY WATER. Ba r r F . T. AECD-2871, Nov. 23,1949. Deci. Jan. 20, 1950.

115. THERMODYNAMICS. Guggenheim E. A. North-Holland Publishing Co. Amsterdam. 1949.

116. ISOTOPE ENRICHMENT THROUGH EXCHANGE REACTIONS. Clusius K. Chimia . (Switzerland) 4,275-84, 1950.

117. ISOTOPE EXCHANGES. RECENT PROGRESS. Haissinsky M. J. chim. phys. 47, 957-82,1950.

118. ISOTOPES IN THE STUDY OF CHEMICAL REACTIONS. Arnstein H. R. V . , Bently R. Nucleonics 6, No. 6, 11-27, 1950.

119. THE SEPARATION OF ISOTOPES. A Review. Hoang T. F . Rev. questions sci . 1.1/378-88, 1950.

16

120. SEPARATION OF ISOTOPES. Groth W. Umschau 50, 402-4 , 1950. (In German)

121. SEPARATION OF ISOTOPES AND THEIR USE IN EXPERIMENTATION. Clusius K. Verhandl. Schweiz. Naturforsch. Ges. 33-52, 1950.

122. SEPARATION TUBE METHOD AND CHEMICAL EXCHANGE PROCESS FOR THE SEPARATION OF ISOTOPES. Becker E. W, Angew. Chem. 62 ,121-5 , 1950. (In German)

123. CHEMICAL EXCHANGE AS A VERSATILE ISOTOPE SEPARA TION PROCESS. Clcwctt G. H. Y-683 , Nov. 7, 1950.

124. SEPARATION OF ISOTOPES. Langer A . , Stephens W. E. Official Gazette 64, 305, 1951.

125. UTILIZATION OF HEAVY WATER. Kirshenbaum I . , Murphy G. M. , Urcy II. C. (Columbia Univ. New York. Substitute Alloy Mater ia ls Labs . USA). TID-5226. 1951. Deci. Feb . 27, 1957. (NNES-III-4B).

12G. THE THEORY OF ISOTOPE SEPARATION. Cohen K. National Nuclear Energy Ser ics - I I I , McGraw-Hil l Book Co. Inc. New York 1951.

127. PHYSICAL PROPERTIES AND ANALYSIS OF HEAVY WATER. Kirshenbaum I. ed. G. M. Murphy, H. C. Urey. McGraw-Hil l Book C o . , I n c . , N e w York 1.951. National Nuclear Ene rgy S e r i e s III, Vol. 4A. (NNES-III-4A) falso Ch. HI)

17

128. ISOTOPES. B ige l e i s en J . Ann. Rev, P h y s . C h e m . 3 , 39-5G, 1952.

129. MEASUREMENT OF THE DEUTERIUM CONCENTRATION IN CONDENSED WATER VAPOR O F BORACIFERUS SOFFIONE A T LARDERELLO. C e r r a i E . , Marche t t i C . , S i l v e s t r i M. Nuovo Cimento(.9), 9, 511-6 , June 1952. (In Italian) (a lso Ch III)

130. THE CONTINUOUS ISOTOPIC ENRICHMENT BY CASCADES. Walen R. Ree , t r a v . ins t . r e c h e r c h e s s t r u c t u r e m a t i é r e (Be lgrade) 1-, 3 5 - 6 7 , 1 9 5 2 .

131 . ISOTOPES. Bigele iscr i J . Ann. Rev. of Nuc lea r Sc ience V o l . 2 , Annual Rev. Inc. Stanford, Calif. (USA). 1953. (p. 221-39)

132.. CHEMICAL SEPARATION OF S T A B L E ISOTOPES. Clèwet t G. H. Ann.. Rev. of Nuc lea r Science Vol . 1. Annual Rev.Int ì . Stanford Calif. (USA) 1953. (p. 293-300)

i S S . . CHEMICAL ENGINEERING ASPECTS OF NUCLEAR POWER. Benedic t M. Indus t r . and Engng. Chem. 45, No. 11, 2372, 1953.

134. THERMAL CONDUCTIVITY O F HEAVY WATER. Meyer F . , E igen M. Z. Na tu r fo r sch . 8a, 5 0 0 - 1 , 1953. (In German)

135. A COMPILATION O F VAPOR PRESSURE DATA O F DEUTERIUM COMPOUNDS. A r m s t r o n g G. T. NBS-2306. F e b . 2 4 , 1 9 5 3 .

136, HEAVY WATER. Augood D. R. I ndus t r i a l Chemis t 30, No. 359, 585 ,1954 .

18

137. R E P O R T FROM GENEVA. REACTOR MATERIALS. Nucleonics 13, No. 9, G4-7.1, Sept. 1955.

138. LAWS ül<* EQUILIBRIUM DEUTERIUM DISTRIBUTION IN HYDROGEN-ISOTOPE EXCHANGE REACTIONS. Va r shavsk i i Ya. M . , Va i sbe rg S. E. Dokl. AN SSSR 100, 97-100, 1955 . ( [ n Russ ian)

139. • ALTERATIONS OF HEAVY WATER IN NUCLEAR REACTOR. Germagno l i E . , Mongini L . E n e r g i a N u c l e a r e (Milan) 2, No. 15, 323-31 , 1954-1955.(In Italian)

140. CHEMICAL ENGINEERING COST ESTIMATION. A r i e s and Newton. McGraw-Hi l l Book Co. New York . 1955.

"ATOMRUNDSCHAU". A Review. IGLefoth W. A t o m k e r n e n e r g i e 1, No. 9, 328, 1956.'(In German)

142. THE ANALYSIS AND PRODUCTION OF STABLE ISOTOPES. Roth E . CEA Rep. No. 536. 1956. (Chimic Analyt iquc No. 1, 3-14, 1956)

143. PROGRESS IN NUCLEAR ENERGY. SERIES IV. TECHNOLOGY AND ENGINEERING. R. Hurs t , S . McLain Eds . McGraw-Hi l l Book Co. Inc. , New York , 1956.

144. THEORY OF SEPARATION OF STABLE ISOTOPES. Tü rk in V. K. Trudy Moskov. Khim. Technol . Inst . i m . D . I . Mendeleeva No. 22 247-51 ,1956 .

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145, HEAVY WATER (Schweres W a s s e r ) . Kruse E. Orion-ßUcher , Murnau 105G. (In German)

14G. CHEMISTRY AND SEPARATION OF ISOTOPES. Panchenkov G. M. , Semiokhin I . A . , Akishin P . A . Vestnik Moskov. Univ.Ser . Mat. Mec. As t ron . F i z . K h i m . 12, 190-214, 1957.

147. TABLES OF PROPERTIES OF HEAVY WATER AT SATURATION TEMPERATURES. Howieson J. Nei-77, 1957. (AECL-1055)

148. ISOTOPIC ANALYSIS OF WATER. Shatenstein A. I . , Yakovleva E. A. , Zvyagintseva E. N. , Varshavski i Ya. M. , Izrai levich E. A. , Dykhno N...M. lad. AN SSSR. Moscow 1957. (German T r a n s l . VEB Deutsch.Verlag Wis s . Ber l in 1960;AEC-tr-4136,1957) (In Russian)

149. INDUSTRY TOWARDS NUCLEAR ENERGY (L ' indus t r ie devant l ' ene rg ie nuc léa i re ) . Baumgar tner R . , Bishop A . S . et a l . P a r i s 1957. (p. 237-47) (In French) OECE P a r i s . Vol. I 1957;Vol. II 1958.

150. NUCLEAR CHEMICAL ENGINEERING. Benedict M. , Pigford R. McGraw-Hil l C o . , I nc . , New York, 1957.

1 5 1 « SEPARATION OF ISOTOPES.Klemm A. Atomwirtschaft 12, No.8/9 , 341-2, 1958. (In German)

152. N E W HORIZONTS FOR STABLE ISOTOPES. Ruder man I. W. 20, P/801(USA) 2nd Geneva Conf. 1958.

153. CONCEPTIONS OF THE MODERN PHYSICS:ISOTOPES, HEAVY WATER. P u r c a r u C . I . Buchares t 1958.

1 5 4 . SOME PROBLEMS OF ISOTOPE SEPARATION THEORY. Rozen A. M. Trv.dy Vses.Konf. P r i m . Izotopov. Moscow 1958. (In Ruffian/

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155, PROCEEDINGS OF THE INTERNATIONAL SYMPOSIUM ON ISOTOPE SEPARATION, Amsterdam, Apr. 1957. J . Kistemaker J . Bigeloisen, A. 0 . C. Nier Eds,-North-Holland Pubi. Co. Amsterdam 1058.

156. HEAVY WATER. Suslov B.' N. Gosud. Izd. Teklmiko-Tcoret. Lit . Moscov 1958. (In Russian)

1 5 7 . NUCLEAR FUSION. Kurchatov I.V. Atomizdat, Moscow 1958. (In Russian)

158. CHEMICAL ENGINEERING AROUND THE WORLD. E. L. Piret ed. New York, 1958.

159. ISOTOPIC SEPARATION FACTOR OF SLOW DISCHARGE MECHANISM OF HYDROGEN ELECTRODE REACTION. II. Kodera T. (Hokkaido Univ. Sapporo, JAPAN) J. Research Inst. Catalysis , Hokkaido Univ. 7, 75-6, Sept. 1959.

160. CISE - Centro Informazioni Studi Esper ienze . Isotope Separation-Heavy Water. Milano, Jan 1959. (p. 87-90) (In Italian)

161, HEAVY WATER, lladulcscu C. Ed. Technica, Bucharest , 1959.

A RESEARCH ON ISOTOPIC COMPOSITION OF EVOLVED HYDROGEN MOLECULES WITH SPECIAL REFERENCE TO THE MECHANISM OF NICKEL CATHODE, llirota K., I-Iisano T. (Osaka Univ. JAPAN) Bull. Chcm. Soe. Japan 33, 1019-20, July 1960.

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1.G3, HEAVY WATER. Sekowski S. Chemik (Gliwice) 13 ,306-8 ,1960.

164. KINETICS OF ELECTROLYTIC KYDROGEN AND DEUTERIUM EVOLUTION. Conway B. E . (Univ. of Ottawa, CANADA) P r o c . Roy. Soc. (London) A256, 128-44, May 31,1960.

1G5. REACTOR HANDBOOK. SECOND EDITION REVISED AND ENLARGED. VOLUME I. MATERIALS. Tipton C. R. J r . New York, In te rsc ience Pub l i she r s , Inc. 1960.

16G. DESIGN AND CALCULATION IN THE CHEMICAL INDUSTRY. (Projekt i rung und Vorkalkulation in der chemischen Industr ie) Springer Ver lag, Heidelberg 19G0. (In German)

167.. THE THEORY OF ISOTOPE ENRICHMENT BY HOT-COLD METHODS. P r i ebsch J . Acta Phys . Aus t r i aca 14 ,347-57 ,1961 .

168. OVERVOLTAGE DEPENDENCE OF DEUTERIUM SEPARATION FACTOR ON PLATINUM. Horiuti J . , Fukuda M. (Hokkaido Univ. Sapporo, JAPAN) Shokubay (Tokyo) 3, No. 2, 115-7 ,1961,

169. ISOTOPE PRODUCTION AND DEVELOPMENT. Pe i sach M. , Walter A. I s r a e l AEC, 685, G3-G, 1961.

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170. HEAVY WATER. Prat t H. R. C. AERE, CE/R 735, 1961.

171. NUCLEAR FUELS AND MATERLALS DEVELOPMENT. (Division of Reactor'Development, USAEC). TID-11295. Feb. 1961.

172. THERMAL FEEDBACK IN COUNTER-CURRENT PROCESSES. Pohl H. A. (Du Pont'do Nemours E. I. & Co. At. En. Div. Wilmington, Del. and Princeton Univ. N. J , P las t ics Lab. ) Par t . I. Technical Rep. 61 A. TID-12452. Apr. 1, 1961. Part . II. Technical Rep. 61 B. TID-12453. Apr. 1, 1961.

173. PROGRESS IN NUCLEAR ENERGY. SER. IV. ENGINEERING AND SAFETY. C. M. Nicholas Ed. Pcrgamon P r e s s , London 1961.

174. SEPARATION OF STAPT ,E ISOTOPES. Johnson F . A. Encyclopaedic Dictionary of Physics. J . Thcwlis Ed. Vol. 4. Pergamon P r e s s , London 19G1.

175. SEPARATION OF ISOTOPES. London H. Ed. Newness, London 1961.

176. ISOTOPE SEPARATION. De Michelis B. , Villani S. Politecnico di Milano. Istituto di Fis ica . CISE-Segrate (Milano). Milano 1961. (In Italian)

177. ATOMIC ENGINEERING. TOME. IV.'NUCLEAR MATERIALS. (Inst. Nat. des Sci. et Tech, Nucl. and P a r i s P r e s s e s Univers i ta i res de France) Vol. 1 and 2. 1961. (In French)

178. THE PRESENT STATE OF THE RESEARCH IN THE FIELD OF ISOTOPE SEPARATION IN EUROPE AND USA. Kakihana H.' J .A t .En .Soc . Japan 4, 716-9,19.62.

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179, SEPARATION FAC TOR OF DEUTERIUM ON PLATINUM HYDROGEN ELECTRODE IN AQUEOUS SULPHURIC ACID. Fulcuda M.', Horiuti J . J . R e s . Inst . Ca ta lys i s , Hokkaido Univ. 10, 43-72, July 1962.

180. POWER REACTOR TECHNOLOGY. Zinn. W. H. Vol. 5. No. 4, Sept. 1962.

181. ISOTOPE SEPARATION METHODS. Gazith M. USAEC. LS-101 . 1962.

182, THEORETICAL BASIS OF THE ISOTOPE CHEMISTRY. Roginskii S . S . , V E B Deutsch. Verlag Wiss . Ber l in 1962. (In German)

183. HEAVY WATER ENRICHMENT IN SEA SALT MANUFACTURE. Weingaer tner E . ,Dat ta R. L. Dechema Monograph. 47, 317-32, 1962.

184. NEW RESEARCH ON HEAVY ISOTOPES OF HYDROGEN. At. E n e r g . (USSR) 14, No. 6, 593-4, 196.3. (In Russian)

185. SEPARATION OF STABLE ISOTOPES. Chen W. Hua Hsueh Tung Pao . No. 8, 10-20 ,1963 .

186. SEPARATION METHODS FOR STABLE ISOTOPES. Vasaru G. Rev. Chim. (Buchares t ) :

I.' CHARACTERISTICS OF THE SEPARATION INSTALLATIONS. Terminology. 14(4) 223-8,1963;

II. METHODS BASED ON REVERSIBLE PROCESSES:DISTILLA-TION, ISOTOPIC EXCHANGE, CENTRIFUGATION.'14(5) 285-9, 1963;

III. METHODS BASED ON IRREVERSIBLE.PROCESSES:THERMAL DIFFUSION. 14(8) 474-8 , 1963;

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IV. METHODS BASED ON IRREVERSIBLE PROCESSES:GASEOUS DIFFUSION, MASS DIFFUSION, SEPARATION JET, MOLECULAR DISTILLATION. 14,605-9,1963. (Trans . MLM-1296 Miamisburg, Ohio. Sept. 1965)

187. BASIC TRENDS IN THE DEVELOPMENT OF METHODS FOR THE SEPARATION OF STABLE ISOTOPES. Sakodynskii K. I . , Zhavoronkow N. M. Zhur . Pr ik l . Khim. 36(12), 2564-79, 1963. (In Russian)

183. HEAVY WATER. TIIERMOPHYSICAL PROPERTIES. Kazavchinskii Ya. Z . , Kcssolman P. M., Kirillin V. A. , Rivkin S. L . , SychGV V. V . , Timrot D. L . , Sheinlin A. E . , Shpilrain E. E. V. A. Kirill in Ed. State Power P r e s s , Moscow-Leningrad 1963. (In Russian)

189. ON HEAVY ISOTOPE OF HYDROGEN AND NEUTRON. Vlasov N. A. ,Samoilov L. N. At. Energ. (USSR) 17(1) 3, 1964. (In Russian)

190. ISOTOPE SEPARATION, THE FINAL STEP IN RAW MATERIAL PRODUCTION FOR NUCLEAR TECHNOLOGY. Murrenhoff A. P . Kerntechnik 6(12), 553-4, 1964.

METHODS FOR.THE SEPARATION OF STABLE ISOTOPES. Vasaru G. Rev. Chim. (Bucharest):

V. METHODS BASED ON IRREVERSIBLE PROCESSES: ION MIGRATION, ELECTROLYSIS, BIOLOGICAL PROCESSES. 15(3) 156-9, 1964;

VI. METHODS BASED ON SPECIFIC PROCESSES:ELECTRO-MAGNETIC AND PHOTOCHEMICAL SEPARATIONS. 15(5) 291-5, 1964. (Trans. MLM-1296. Miamisburg, Ohio, Sept. 1965)

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192. ANALYSIS OF ESSENTIAL NUCLEAR REACTOR MATERIALS. C.J.Rodclen cd. 19G4.

193. STABLE ISOTOPE SEPARATION. Bottcr F . , Molinari P h . , Dir ian G. , Grünspan S. , Moncs F . , Saito E. , Lera t J . M. , Roth E . CEA Saclay Rep. No. 2047. 1964.

194. SEPARATION OF ISOTOPES. Annual P r o g r e s s Report . NYO-755-1. Sept. 1, 1964.

195. WATER AND WATER TREATMENT IN NUCLEAR POWER PLANTS. Kot A. A. Atomizdat , Moscow 1964. (In Russ ian . I s rae l T r a n s l . 1966)

19G. A RKVIEW OF NUCLEAR. INDUSTRY CHEMICAL TECHNOLOGY. Neumann L. Rypar V. SNTL Prague 1964. (In Czech)

197. CHEMICAL PROCESSING IN THE ATOMIC ENERGY INDUSTRY. Copper A. It. London, Ilii'fo Books Ltd. 1964.

198. THERMODYNAMIC PROPERTIES OF HEAVY WATER. A Compilation of Available Data. Lundkvist B . , P e r s s o n T. Brcnnstoff-Wärme-Kraf t 17(7) 356-G2, 1965.

199. HEAVY HYDROGEN ISOTOPES AND THEIR PREPARATION. Kiss I. (HUNGARY) F i z . S z e m l e 15(10) 311-5, 1965.

200. SPECIAL METHODS OF STABLE ISOTOPE ANALYSIS.-Müller G. Kernenerg ie 8(5) 265-83, 19G5.(In German)

201. SEPARATION OF ISOTOPES:INTRODUCTION AND SUMMARY. Taylor T. I. Separat ion of Isotopes . Annual P r o g r e s s Report 1905. NYO-755-2. Pape r 1.

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202. ISOTOPE ANALYSIS.DETERMINATION OF.HEAVY WATER AND OF URANIUM. Roth E. , Bir R. Gonio Atomique Vol. V. 1965, (p. 395-435) (also Ch. Ill)

203. SEPARATION OF ISOTOPES. Senvar C. B. Turk. At. En. Comm,. Sci. Pubi. Sor. B, Vol. VI. 1965.

204. SEPARATION OF NATURAL ISOTOPES. Selecki A. Panstwowe Wyclawn. Nauk., Warsaw 1965. (iti .Polish)

205» INTERACTIONS BETWEEN THE HYDROGEN ISOTOPES AND THEIR ORTHO- AND PARA-MODIFICATIONS. Knaap II. F . P . ot al . Disc. Faraday Soc. 40, 135-9, 1965.

206. ATOMIC ENGINEERING. VOLUME V. PRODUCTION OF BASIC NUCLEAR MATERIALS. PRODUCTION AND UTILIZATION OF ARTIFICIAL ELEMENTS. Second Edition Review and Addenda to Pa r t of Volume IV; (Inst. Nat. des Sci. et Tech. Nucl. Saclay). P a r i s P r e s s e s U n i v e r s i t ä r e s , 1965. (In French)

207. TECHNICAL DEVELOPMENT IN EQUIPMENT CONSTRUCTION FOR HEAVY-CHE MIC AL INDUSTRY. P laskura W. Chom. (Gliwice) Wkladka No. 2, 1-8, 1965;No. 1, 1-6, 1966.

208. SEPARATION OF ISOTOPES. Blum J . M. Ene rg . Nucl. 8, 207-11, 1966.

209. THE INSTITUTE OF STABLE ISOTOPES AT LEIPZIG. MUhlenpfordt J . Isotopenpraxis 2, 113-6,1966. (in German)

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210. PROGRESS IN PRODUCING STABLE ISOTOPES. Wetzel K. Isotopenpraxis 2,277-84, 1966. (In German)

211. HEAVY WATER. Gryson H. Rev. Ind. Minerale 48, No. 3, 182-91, 1966.

212. SEPARATION OF THE ISOTOPES OF URANIUM BY THE SEPARATION NOZZLE PROCESS. Becker E . W . , Bier K., Bier W. , Schnette R. , Seidel D. Angew. Chem. Inst. Ed. 6, 507-18, 1967.

213.. TEN YEARS OF ISOTOPE TECHNIQUE IN ROMANIA. Mercea V. Isotopenpraxis 3,239-40,1967. (In German)

214. ISOTOPE SEPARATION. Holmberg K. E. (Aktiebolaget Atomenergi, Stockholm, SWEDEN) Svensk.Kem. Tidskr . 79, No. 2, 89-93, 1967. (In Svedish)

215. IMPROVED GAS-LIQUID CONTACTING IN CO-CURRENT FLOW. Voyer R. D. /Mi l le r A. I. AECL-2765. 1967.

216. PRODUCTION OF BASIC MATERIALS FOR THE NUCLEAR INDUSTRY. Annual Report 1967. CEA. (CEA, P a r i s , FRANCE). (In French) (NP-17597. 1967. p. 109-35)

217. PRODUCTION OF DEUTERIUM. Jül -Bibl . - 7 . May 1967. Inf. No. 262

218. PROGRESS REPORT (on Deuterium Separation). Jan. 1, 1967-Oct. 1, 1967.NYO-3783-3.

HERMETICALLY SEALED WATER PUMPS IN NUCLEAR POWER PLANT INSTALLATIONS. Sinev N. M. , Udovichenko P . M. Atomizdat, Moscow 1967. (In Russian)

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220. OPTIMIZATION OF SEPARATION PROCESS. Dickol G. Isotopenpraxis 4,419-214, 1968. (In German)

221. THE COMING AGE OF NUCLEAR ENERGY. Weinberg A. M. Nuclear News 11, No. 7, 30-4, July 1968.

222. A LYMAN'S GUIDE TO HEAVY WATER. AECL-3034. 1968.

223. STANDARDIZATION OF THE DEUTERIUM CONTENT OF HEAVY WATER. Baer t sch i P . , Rosatzin H. (Eidgenossisches Inst , fuer Reaktorforschung, Wuerelingen, SWITZERLAND). EIR-142. Oct. 1968. (In German)

224. PHYSICAL PROPERTIES OF HYDROGEN ISOTOPES. Shtukkenberg Yu. M. Yu.I. Moskalev Ed. Atomizdat, Moscow 1968. (In Russian)

225. ISOTOPES IN CHE M S TRY. Duncan J . F . , Cook G. B. Clarendon P r e s s , Oxford, 1968.

226. MODERATORS. Gauthron M. (Inst. Nat. des Sci. et Tech. Nucl. Sac lay ;Par i s P r e s s e s Unive r s i t a i r e s , P a r i s , FRANCE). Genie Atomique 27-43, Tome II. 1968. (In French)

227. STABLE ISOTOPES. Väsaru Gh. Ed. Technica, Buchares t 1968.

22 8. STANDARDS FOR A PRATICAL SCALE OF pD IN HEAVY WATER. Paabo M. , Bates R. G. (NBS, Washington, D. C. USA). Anal. Chem. 41 , 283-5, Feb . 1969.

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WESTERN COAL DEPOSITS: A NATIONAL SOURCE OF POWER. Steinberg M.,.Powell J . , Manowitz B. (Brookhaven National Lab . , Upton, N. Y. ).'BNL-50187. NOV. 1969.

ANNUAL REPORT, 1968-1969. (Atomic Energy of Canada Ltd. , Ottawa, Ont. CANADA). AECL-3326.'1969.

CHEMISTRY AND MATERIALS DIVISION. P r o g r e s s Report, Oct. 1-Dec. 31, 1969. AECL. (CRNL. Chalk River, Ont. CANADA) AECL-3521 (PR-CMa-11)

REACTOR DAY 1969 OF THE GERMAN ATOMFORUM. Winnacker K. (Deutsches Atomforum e. V., Dusseldorf, W. GERMANY)NP-17899. Apr. 16, 1969. (In German)

REVIEW OF FUEL PROCESSING TECHNOLOGY PRESENTED AT THE 1964 GENEVA CONFERENCE. Gresky A. T.(ORNL, Tenn. USA) . P r o g r . N u c l . Energy Ser. Ill, 4, 3-34, 1970.

HEAVY WATER AND ORGANIC FLUIDS AS NEUTRON MODERATOR AND REFLECTOR MATERIALS. Ayres J . A. (Battelle Northwest, Richland, Wash. USA). Trilling C.A. Nucl. Eng. Des. 14, 363-89, Feb. 1971.

SPECIFIC HEAT AND ENTHALPY OF LIQUID HEAVY WATER. Rosta P . Z . (Atomic Energy of Canada Ltd . , Sheridan Park (Ontario)). AECL-3689. May 1971. (TDAI-43).

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BIBLIOGRAPHIES

DEUTERIUM. A Bibliography. Chem. Eng. News 12, 11, 1934.

BIBLIOGRAPHY OF DEUTERIUM (as of Aug. 1, 1934). Young A . R . Perm. State Coll. (USA)

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BIBLIOGRAPHY OF RESEARCH ON HEAVY HYDROGEN COM POUNDS. Kimball A. 11. comp. Urey H. C. , Kirshenbaum I. E d s . New York, McGraw-Hil l , 1949. (NNES-HI-4C)

THERMAL DIFFUSION. A Bibliography. AERE-Inf /Bib-59. Feb . 1950.

DEUTERIUM AND HEAVY WATER-PHYSIOLOGICAL AND BIOLOGICAL ACTION. Bibliography of Published L i t e r a t u r e . CAERE, Harwel l Be rks , UK). AERE -Inf /Bib -60 . Feb . 1950.

34

9. SELECTED BIBLIOGRAPHY ON ISOTOPE .SEPARATION METHODS. Morphew A . T . T I D - 4 5 7 . F e b . 1951. (UCRL-Bibl-5116)

10. ISOTOPE SEPARATION. A Bibl iography of Separa t ion Methods . Whetsel II. B . , Mills G . F . K- 814. Oct. 1951. (UCRL-Bib-5116 . Pt . II)

11. BIBLIOGRAPHY ON DISTILLATION. Lawrence S. J . , Givens E . j KAPL-588 . Aug. 1951. !

I I

12. A REVIEW OF THE PROPERTIES OF DEUTERIUM COMPOUNDS: | ANNUAL BIBLIOGRAPHY-1946. Brown L . M. , Beckett C. W. | NBS-1527. May 1, 1952. J

13. A REVIEW OF THE PROPERTIES OF DEUTERIUM COMPOUNDS: ANNUAL BIBLIOGRAPHY-1947. Brown L. M . , Beckett C. W. NBS-1631. June 1, 1952.

14. A REVIEW OF THE PROPERTIES OF DEUTERIUM COMPOUNDS: ANNUAL BIBLIOGRAPIIY-1948. Brown L . M . , Becket t C. W. NBS-1685. Ju ly 21, 1952.

15. A REVIEW OF THE PROPERTIES OF DEUTERIUM COMPOUNDS: ANNUAL BIBLIOGRAPHY-1949. Brown L. M . , Goldstein J . M . , Beckett C .W. NBS-1721. Aug. 1, 1952.

16. A REVIEW OF THE PROPERTIES OF DEUTERIUM COMPOUNDS: ANNUAL BIBLIOGRAPHY-1950. Brown L. M . , Goldstein J . M. P a r k J . L. , Beckett C .W. NBS-1777. Sept. 1, 1952.

; ,- ' r / l - r .

35

THE BIOLOGICAL E F F E C T S OF DEUTERIUM COMPOUNDS. Morowitz H.J . . , Brown L.' M.(NBS, USA).NBS-2179. Jan . 14, 1953.

BIBLIOGRAPHY OF RESEARCH ON THE PROPERTIES OF THE ISOTOPES OF MOLECULAR HYDROGEN; F r i edman A . S . , Beckett C. W. NBS-2266. Mar. '15, 195 3.

A CRITICAL REVIEW OF THE LITERATURE RELATING TO THE VAPOR PRESSURE OF AMMONIA AND TRIDEUTEROAM-MONIA. Arms t rong G.'T. (Nat. Bur . of Stand. , USA) NBS-2626. June 30, 1953.

A REVIEW OF THE PROPERTIES OF DEUTERIUM COMPOUNDS: ANNUAL BIBLIOGRAPHY-1951. Brown L. M„Fr iedman A . S . (NBS,USA)NBS-2529. Aug. 1,1953.'

A REVIEW OF THE PROPERTIES OF DEUTERIUM COMPOUNDS. BIBLIOGRAPHY OF UNCLASSIFIED GOVERNMENT REPORTS: 1947-1952. Brown L. M. , F r i e d m a n A . S. NBS-2492. Sept. 1, 1953.

BIBLIOGRAPHY ON DEUTERIUM SEPARATION METHODS. Drews W:'P.NYO^6084. Dec. 4, 1953. Deci . Oct. 28, 1955;(SöA-159)

A .REVIEW OF THE REACTION KINETICS OF DEUTERIUM COMPOUNDS. I. DECOMPOSITION REACTION OF INORGANIC COMPOUNDS. Brown L . M . , F r i e d m a n A . S ; NBS-3091.March 15, 1954.

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24. A REVIEW OF THE PROPERTIES OF DEUTERIUM COMPOUNDS: ANNUAL BIBLIOGRAPHY-1952. Brown L. M., Fr iedman A.S. NBS-3144. March 1954.

25. ISOTOPE SEPARATION AND ISOTOPE EXCHANGE. Bibliography of Unclassified Li tera ture . Begun G. M. (ORNL), Allen R. E. (Techn. Inf. Service USA) comps. TID-3036 (Rev.) June 1954. (TID-3036, Jan. 23, 1953)

26. NUCLEAR SCIENCE:A Bibliography of Selected Unclassified Literature. TID-3070. Apr. 1955.

27. A REVIEW OF THE PROPERTIES OF DEUTERIUM COMPOUNDS: ANNUAL BIBLIOGRAPHY-1953. Brown L. M., Fr iedman A. S. NES-3985.Sept. 1,1955.

28. BIBLIOGRAPHY OF RESEARCH ON DEUTERIUM AND TRITIUM COMPOUNDS 1945 TO 1952. Brown L. M., Fr iedman A . S . , Beckett C.W. (NBS, USA).NBS-C-5G2.Jan.27, 1956.

29. HEAVY WATER. Bibliography of British,Canadian and American Reports etc, and a Selected References to the Published Li terature. Clarke R. AERE-Inf/Bib-87. (Suppl. 5). June 1957.

30. BIBLIOGRAPHY OF RESEARCH ON DEUTERIUM AND TRITIUM COMPOUNDS 1953-54. Johnson V. R. , Brown'L. M. , Fr iedman A.S. NBS-C-562(Suppl. D.July 1957.

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A REVIEW OF THE PROPERTIES OF DEUTERIUM AND TRITIUM COMPOUNDS. ANNUAL BIBLIOGRAPIIY-1955. Johnson V.R. NBS-5446,Oct . 30, 1957.

GASEOUS THERMAL DIFFUSION. I. Bibliography of Open L i t e r a ture 1940-57.11. A Bibliography of the Report L i t e ra tu re , 1941-57. ( F r o s t F . E . ) McFadden C. UCRL-511G. Jan. 1958.

AN ANNOTATED BIBLIOGRAPHY ON HEAVY WATER AND HEAVY WATER REACTORS. Curran A. T. (Babcock and Wilcox Co. Atomic Energy Div . , Lynchburg, Va. USA). BAW-47. Feb . 1958.

A REVIEW OF THE PROPERTIES OF DEUTERIUM AND TRITIUM COMPOUNDS. ANNUAL BIBLIOGRAPHY-1956. Johnson V . R . , Oppenheim I. NBS-5092.May 1958.

LITERATURE SURVEY ON ISOTOPE SEPARATION. LS-2 3. Nov. 1958.

THERMAL DIFFUSION. A Bibliography. Grove G.R. MLM-1088. June 1959.

ISOTOPE SEPARATION AND ISOTOPE EXCHANGE. A Bibl iography with A b s t r a c t s . Begun G. M. ORNL-2 852,Oct. 2 8, 1959.

THE HYDROGEN SULPHIDE-DUAL-TEMPERATURE PROCESS. A Bibliography of Selected Report L i t e r a t u r e . Jacobs J . M . TID-3091. Oct. 1959.

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BIBLIOGRAPHY ON GAS SEPARATION BY C E N T R I F U G E . T h o m a s J . R . , M a u g h a n G . I . DEGIS-48(R). Nov. 1959.

ISOTOPIC EXCHANGE REACTIONS B E T W E E N AMMONIA AND HYDROGEN OR SOME HYDROGEN COMPOUNDS. H o u b e r g e r M.', Botter F. C E A - S a c l a y - B i b . No. 3. 1959.

ISOTOPE SEPARATION BY GASEOUS DIFFUSION AND C E N T R I -FUGATION.A L i t e r a t u r e S e a r c h . J a c o b s J . J . T1D-3554. May 1960.

NEUTRON AGE MEASUREMENTS IN WATER, D2O, W A T E R - M E TAL MIXTURES, GRAPHITE, VARIOUS ORGANICS AND ORGANIC- ' M E T A L MIXTURES AND SLOWING DOWN P R O P E R T I E S OF VARIOUS MEDIA FOR NEUTRONS. UNCLASSIFIED BIBLIOGRAPHY. Chapman M . J . (Atomic In t e rna t iona l Div. Of Nor th A m e r i c a n Avia t ion, I n c . , Canoga P a r k , Calif. USA). N A A - S R - M e m o - 5 5 4 6 . Aug. 1, 1960.

HEAVY WATER REACTORS AND TIIK P R O P E R T I E S , ANALYSIS, HANDLING, AND E F F E C T S OF HEAVY WATER. A BIBLIOGRAPHY. Duke D. M. (Bab'cock and Wilcnx Co. Atomic Ene rgy D i v , , Lynchburg , Va. USA). BAW-1209. D e c . 1960.

A BIBLIOGRAPHY SEARCH ON RADIOACTIVATION ANALYSIS. Gada F . CISE R e p . No. 83. J an . 1961 .

APPLICATION O F CHEMICAL EXCHANGE METHODS TO ISO-TOPIC SEPARATIONS. D r u r y J . S. (ORNL, Tenn . USA). P r o g r . in Nucl . E n e r g y , S e r . IV, 4, 308-4.8, 1961 .

ISOTOPE SEPARATION METHODS. Annotated Bib l iography . Gazi th M. ( I s r a e l AEC) L S / 1 0 1 . J u n o 1962.

39

47. PHYSICAL CONSTANTS OF ISOTOPIC SUBSTITUTIONS IN WATER (Ol7 -Ol8 -D-T) .D i r i anG. (CEA, Centre d 'Etudes Nucl . , Saclay, FRANCE). CEA-Bib-15. 1962.

48. HEAVY WATER PRODUCTION. An Annotated Bibliography of Selected L i t e r a tu re . Jacobs J . M. , comp. (Division of Technical Information Extension, USAEC). TID-3091,(Suppl. 1) June 1964.

49. ABSTRACTS OF CANADIAN PATENTS ON THE PRODUCTION OF HEAVY WATER, Armst rong F . i; (AECL, Chalk River . Ont. CANADA). AECL-2279. July 1965.

50. BIBLIOGRAPHY OF REFERENCES FOR THE THERMOPHYSICAL PROPERTIES OF 4 I Ie , H, D, HD, Ne, Ar, N, O, C02, CII4, C2H6 , Kr AND REFRIGERANTS 13, 14, AND 23.Dimiduk P . W. AFML-65-338. 196 5.

51 . PHYSICAL AND CHEMICAL PROPERTIES OF AMMONIA. Bibliographic Compilation, Jacolin O. CEA-Bib. No. 57. 19G5.

52. BIBLIOGRAPHY OF HEAVY WATER PRODUCTION. Shah P . G . S . (Pakistan AEC). AECL-CHEM-103. 1966.

53. LIST OF UNCLASSIFIED REPORTS AND PAPERS PUBLISHED BY STAFF OF THE ISOTOPE RESEARCH DIVISION. 1950-1965. AERE-Bib. 127(Rev. 1). 1966.

54. MOLECULAR PHYSICAL PROPERTIES OF THE HYDROGEN ISOTOPES AND THEIR ISOTOPIC COMBINATIONS. Biblio-graphycal Compilation. Guizouarn L. CEA-Bib-87. 1967.

55. .METHODS FOR HEAVY WATER PRODUCTIONS.(Foreign Patents ) . Bakin V.O. Moscow TNIIPI, 1967.

40

56. THERMAL DIFFUSION. A Bibliography. Vasaru Gh. Räp. I. IAEA, Vienna, STI /PUB/21/28 .1968.

57. LIST OF PATENTS OF I-I2S-ri20 EXCHANGE, OF DUAL TEMPERATURE SYSTEMS AND ABSTRACTS OF H 2 S-H 2 0 PATENTS. Vasaru Gh. IFA-AG-4.May 1970. (Unpublished Report)

58. HEAVY WATER REACTORS. Bibliographical Ser ies No. 37. STI/PUB/21/37.IAEA, Vienna, 1970.

59. DEUTERIUM AND HEAVY WATER. A Selected Bibliography. Vasaru Gh., Ursu D . , Szentgyórgyi P . , Mihaila A. (Academia R .S .R . Cluj ,Inst .de Fizica Atomica, ROMANIA) Cluj 1970.

6u. STABLE ISOTOPES. Vasaru Gh. (Academia R . S . R . Cluj, Insti tululde Fizicä Atomica) CEA-Bib-136.Sept . 1970.

61 . BIBLIOGRAPHY ON PRODUCTION OP HEAVY WATER. Nagrathna R. A. (comp). Bhabha Atomic Research Center , Bombay (India) . BARC-BIB-3. 1970

Ill - DETERMINATION AND ANALYSIS OF DEUTERIUM

AND HEAVY WATER

43

III - DETERMINATION AND ANALYSIS OF DEUTERIUM AND HEAVY WATER

1. ADDITIONAL EVIDENCE FOR AN ISOTOPE OF HYDROGEN OF MASS 2.Bleakney W. Phys. 'Rev. '39, 536, 1932.

2. MASS SPECTROSCOPHIC RESEARCH ON HYDROGEN AND HELIUM. Kallmann H. , Lasaref f W. Naturwissenschaf ten 20, 206,1932.

3. ISOTOPIC ANALYSIS OF WATER. C r i s t R. H. , Murphy G. M. , UreyH- .C . J . Am. Chem. Soc. 55, 5060-1, 1933.

4, MICROPYCNOMETER, FOR THE DETERMINATION OF D I F FERENCES IN THE ISOTOPIC RATIO OF WATER. GÜfülan E . S. J r . ,-PoIanyi M. Z. Physik . Chem. A 166 ,254-6 ,1933 .

5. THE USE OF THE INTERFEROMETER IN THE ISOTOPIC ANALYSIS OF WATER. C r i s t R. H . , Murphy G. M. , Urey H. C. J . Chem. Phys . 2, 112-5, 1934.

6. AN EXAMINATION OF WATER FROM VARIOUS NATURAL SOURCES FOR VARIATIONS IN ISOTOPIC COMPOSITION. Washburn E. W. , Smith E . R . Bur. Standards J . Resea rch 12, 305-11,1934.

44

PREPARATION OF PROTIUM OXIDE AND THE DETERMINATION OF THE PROPORTION OF DEUTERIUM IN THE HYDROGEN OF NORMAL WATER. Ingold E. I I . , Ingoici C. K. , Whitaker H. , Whytlawgray R. Nature 134,661,1934.

MICRO-METHOD FOR THE DETERMINATION OF HEAVY WATER. Goldfinger P . , Scheepers L. Compt. Rendu. 198, 1916-8, 1934.

THE DETERMINATION OF THE DEUTERIUM CONTENT OF THE DILUTE HEAVY WATER BY FLOATING METHOD. Harada M. J. Chem.Soc. Japan 5G, 811-8, 1935.

INTERFEROMETRIC ANALYSIS OF HEAVY WATER. Filippova N.S . ,S lu t skaya M. M. Acta Physicochim. USSR 5, 131-6, 1936.

INTERFEROMETRIC ANALYSIS OF HEAVY WATER. Filippova N. S. , Slutskaya M. M. J . Phys . Chem. USSR 8, 468-71,1936.

PRODUCTION OF LIGHT WATER AND THE DETERMINATION OF THE DEUTERIUM CONCENTRATION OF ORDINARY WATER. Morita N . , Titani T. Bull. Chem.Soc . Japan 11,403-13,1936.

A MICRO METHOD FOR THE ACCURATE DETERMINATION OF D 2 0 IN WATER. F e u g e r - E r i k s e n K. , Krogh A . , Ussing II. Biochem. J. 30, 1264-9, 1936.'

A METHOD OF ANALYSIS OF HEAVY WATER. F a r k a s A. T r a n s . Faraday Soc. 32 ,413-5 , 1936.

45

A SIMPLE METHOD FOR THE DETERMINATION OF D 2 0 CONTENT OF- SMALL QUANTITIES OF WATER. Fromherz H. , Sonderhoff R. , Thomas H. Ber . 70B, 1219-23, 1937.

A METHOD FOR THE ANALYSIS OF HEAVY WATER. Filippova N. S., Slutskaya M, M. Trudy Dnepropetrovsk. Khim. -Tekh. Inst. 14-24, 1938. (Khim, Referat. Zhur. 2, No. X, 9, 1939)

MEASUREMENT OF THE DEUTERIUM CONTENT IN MIXTURES OF H2O AND D2O.Lindersti'oem-L)ng K., Jacobsen O. ', JohansenG. Compt. Rend. Trav. Lab. Car lsberg, Sér. chim. 23, 17-25, 1938.

PRECISION DETERMINATIONS OF THE DENSITIES OF DEUTERIUM OXIDE AND WATER.ELECTROLYTIC SEPARATION OF THE OXYGEN ISOTOPES. Tronstad L . , Brun J. Trans, Faraday Soc. 34, 766-73, 1938.

DETERMINATION OF HEAVY HYDROGEN. Harteck P . Z .E lec t ro -chem. 44, 3-8, 1938.

A MODIFIED MICROPIPET FOR DENSITY DETERMINATIONS IN HEAVY WATER ANALYSIS. Rosebury F. , van Heyningen W.E . Anal, Chem. 14, 363-4, 1942.

A MASS SPECTROMETER FOR ROUTINE HYDROGEN ISOTOPE ANALYSES:SUPPL. No.l. Nier A.O.C.,Stevens C.'M.', Rustad B. AECD-2767. Mar, 17, 1943. Deci. Jan, 3, 1950.

46

MODIFICATION OF APPARATUS FOR DEUTERIUM OXIDE DETERMINATION BY THE FALLING DROP. F e t c h e r J r . F . S . I n d . E n g . C h e m . A n a l . E d . T G , ^ , 1944.

CHEMICAL RESEARCH-ANALYTICAL REPORT FOR MONTH ENDING JULY 1, 1944. (Chicago Univ, Meta l lu rg ica l Lab. USA). CC-1915. Aug; 11, 1944. 'Deci. Jan . 30, 195G.'(A-2803)

METALLURGICAL PROJECT R E P O R T . F i s c h e r R . B . , P o t t e r R . À . , V o s k u y l R . J . MUC-DHT-103.

THE SPECTROGRAPHIC ASSAY OF HEAVY WATER. (Based on CC-24G7) .Tomkins F . S . , F r e d M. (ANL^ 111. USA). AECD-3100; ANL-HDY-577. Deci . Mar . 21 ,1951 .

METALLURGICAL PROJECT R E P O R T . Brayson J . A, M-CP-1928 , July 1944.

ANALYSIS OF HEAVY WATER BY EQUILIBRATION. F i s c h e r R . B . , P o t t e r R . A . , V o s k u y l R . J . (Univ. Meta l lu rg ica l Lab. Chicago, USA). CC-2994. May 15, 1945. Deci . Dec. 15, 1955.

STANDARDIZATION OF THE pD SCALE. 'F i sche r R. B . , Po t t e r R. A .CC-3271 .Sep t . 12, 1945.

47

29. DETERMINATION OF DEUTERIUM IN WATER; A MASS SPECTROM E T R Y METHOD. F i s c h e r R. B . , Po t te r R. A. , Voskuyl R. J . Anal. Chem. 20/571, June 1948. (MDDC-1208, deci . Aug. 8, 1947).

30, DETERMINATION OF DEUTERIUM IN WATER. CONVERSION TO METHYL DEUTERIDE AND METHANE AND MEASUREMENT BY MASS SPECTROMETER. Orchin M . , Wender I. ; F r i ede l R. A. Anal. Chem. 21, 1072, 1949.

31 . THE DETERMINATION OF HEAVY WATER. Puddington I. E . Can. J . R e s . 2 7 B , 1-5, Jan. 1949.

32. ANALYTICAL CHEMISTRY AND STANDARDS FOR NUCLEAR PURITY. Gueron J . A t o m e s 4, 53-6, Feb . 1949.

33. THE RELATION OF APPARENT TO TRUE pH IN DEUTERIUM SOLUTIONS. Hart R. G.(Nat. Res . Council of Canada). CRE-423. June 1949.

34. ANALYSIS OF HEAVY WATER WITH A HIGH DEUTERIUM OXIDE CONTENT BY GRAVIMETRIC METHODS. Viallard R. Bull . Soc. Chim. F r a n c e , Nos . 5-6, 265-71 , May-June 1949. (AERE-T r a n s - l l / 3 / 5 / 2 1 1 ; A E C - t r - 1 2 9 9 )

35, DETERMINATION OF HEAVY WATER. Thomas B. W. Anal. Chem. 22 ,1476 ,1950 .

36. HEAVY WATER PICNOMRTllY. C o r r a i -E., Orsoni L. , Sii vos t r i M.CISE-10. 1950. (In Italian)

48

DETERMINATION OF ISOTOPE RATIOS OF KNOWN DEUTERIUM-HYDROGEN SAMPLES USING A MASS SPECTROMETER. Alfin Sla ter R . B . , R o c k S. M . , Swislochi M. Anal . Chem. 22, 421-3 , Mar . 1950.

A SIMPLE METHOD FOR THE DENSIOMETRIC DETERMINATION OF HEAVY WATER. Sapir s te in L . A. J . Lab, Clin; Med. 35, 793-4 , May 1950.

INFRARED SPECTROMETRIC DETERMINATION OF DEUTERIUM OXIDE IN WATER. Thorn ton V . , Condon F . E. Anal . Chem. 2? 690-1 , May 1950.

DETERMINATION OF THE ABSORBED WATER BY EXCHANGE WITH DEUTERIUM OXIDE. EXTENSION OF THE EXCHANGE METHOD TO STUDY OF MACROMOLECULAR STRUCTURES. Vi l lani R. J . C h i m . Phys . 48, 372, 1951. (AEC-t r -1887)

ANALYSIS OF HYDROGEN-DEUTERIUM MIXTURES AND OF MIXTURES OF HEAVY-WATER AND LIGHT-WATER BY MEANS OF A MASS SPECTROMETER. Chenouard J . , Gueron J . , Roth E . (Commissa r i a t à l 'Ene rg ie Atomique, FRANCE). CEA-87. July, 1951.

CONTROL OF THE PURITY OF HEAVY WATER BY ELECTRIC CONDUCTIVITY MEASUREMENTS. Se lmi L. (CISE, Milan, ITALY). CISE-28, 1952. (In Italian) (CEA- t r -X-405)

MEASURING THE CONCENTRATION OF DgO IN AQUEOUS SOLUTIONS OF HEAVY WATER. C e r r a i E . , Marche t t i C . , S i lves t r i M. CISE-31 , 1 952.

/

44. THE COLORIMETRIC DETERMINATION OF TRACES OF BORON IN HEAVY WATER. F izzo t t i C. ,Selmi L. (Chimica e Industr ia , Milan,-I taly) . 34 ,265-6 ,1052 . (In Italian) (AEC-tr-1960)

45 , ON THE CONCENTRATION OF HEAVY WATER IN GLACIER ICE. SandstrBem A . E . A r k i v . F y s i k , 3 /549-56,1952.

46 . INFRARED DETERMINATION OF DEUTERIUM IN LIQUID WATER. T renne r N . R . , Walker R . W . T h e P e r k i n - E l m e r Instrument News 4, No. 1, 1, 1952.

47 . APPLICATION OF A FLOAT METHOD TO RAPID MEASUREMENT OF D2O CONCENTRATION IN AN AQUEOUS SOLUTION OF HEAVY WATER. C e r r a i E. , Marchetti C. , S i lves t r i M. , Nuovo Cimento (9), 9, 530-4, June 1952. (In Italian)

4 8 # THE ISOTOPIC ANALYSIS OF HYDROGEN IN VARIOUS COMPOUNDS. Bigeleisen J . , Pe r lman M. L. , P r o s s c r H. C. Anal. Chem. 24, 135G-7, 1952. (BNL-1058)

49 . MASS SPECTROMETRIC DETERMINATION OF DEUTERIUM IN WATER. Goodall C. A. , Alki re G.'J. HW-25258. Aug. 20, 1952.'

50. CONVERSION OF HYDROGENIC MATERIALS TO HYDROGEN FOR ISOTOPIC ANALYSIS. Bigeleisen J . , P e r l m a n M. L. P r o s s e r U . C . Anal. Chem. 24, 135G,Aug. 1952.

51.'PRECISION DETERMINATION OF DEUTERIUM IN H 2 0 - D 2 0 'MIXTURES BY A PICNOMETER METHOD. Si lverman L... Gossen W.NAA-SR-236, 1953.

50

52. MEASUREMENT OF DEUTERIUM OXIDE CONCENTRATION IN WATER SAMPLES BY THE MASS S P E C T R O M E T E R . Washburn H . W . , B e r r y C . E . , I I a l l L. O. Anal . Chem. 25, 130-4, J a n . 1953.

5(3. INFRARED S l 'ECTRA OF HEAVY WATER ADSORBED ON SILICA GEL. P it tu; il lui Ci. C. , Garland C. W . , J u r a G. J . Am. C h e m . Soc. 75 , 803-5 , F e b . 2 0 , 1 9 5 3 .

54. ISOTOPIC PROPORTION OF WATER BY MEASUREMENT OF ABSORPTION IN THE INFRARED. L e c o m t e J . , Cecca ld i M . , Roth E . J . Chini . P h y s . 50, 1G6, M a r . 1953.

55. USE OF HEAVY WATER AS SOLVENT FOR SPECTROSCOPIC INVESTIGATION IN NEAR I N F R A R E D . E v s t i g n e e v V. B.Doklady A k a d . N a u k . S . S . S . R. 8 9 , 1 0 5 - 8 , M a r . 1 ,1953 .

56. DETERMINATION OF HEAVY WATER WITH THE HOT WIRE GAGE, l l a ldeman 11. G. Ana l . C h e m . 25, 787-90, May 1953.

57. INFRARED SPECTRA .AND MOLECULAR STRUCTURE OF SOME GROUPS VI 11EXAFLUORIDES. Canni J . A E R K - C / U - 1264, Oct . 22, 1953.

58. THE DETERMINATION OF THE. DgO CONTENT OF HEAVY WATER BY A MASS S P E C T R O M E T E R . Reynolds P . , Love r idye B. A. (AERE, Harwe l l , B e r k s , UK). A E R E - G P / R - 1 2 8 2 . Oct.. 26, 1953.

59. FINAL R E P O R T COVERING THE PERIOD JUNE 15, 1948 TO DECEMBER 31 ,1953 . C a r p e n t e r R. B . , McDonough R . , P a t t e r s o n W. A. (Bairtl A s s o c i a t e s , Inc . USA). NP-501 5.

51

GO. T H E D E T E R M I N A T I O N O F T H E D2O C O N T E N T OF HEAVY WATER BY INFRARED S P E C T R O M E T R Y . S t e v e n s W. I I . , T h u r s t o n W. M. (AECL, Chalk R i v e r , Ont. CANADA). A E C L - 2 9 5 . 1954.

6 1 . DENSITY O F HEAVY W A T E R E N R I C H E D IN OXYGEN ISOTOPES DETERMINED BY ELECTROLYTIC METHOD. Isberg P . , Luiidberg L. Z . Naturforsch. 9 ,472-3 , 1954.(In German) (CEA-tr-A-955)

62. A METHOD FOR THE ANALYSIS OF MICROSCOPIC QUANTITIES OF HEAVY WATER. Mardaleishvil i R. E. , Lavrovskaya G. K., Voovodskii V. V. Zhur. Fiz. Khim. 28, 2195-8, 1954. (In Russian)

63. RECORDING DIFFERENTIAL HEFRACTOMETER. Campbell D. N . , Fel lows C . G . , Spraklen S .B .e t a l . Ind. Eng. Chem.46, 1409, 1954.

64. A SIMPLE INFRARED GRATING SPECTROMETER FOR USE IN ANALYSIS. Gaunt J . AERE-C/R-13D8. Apr. 9, 1954. .

65; A MASS SPECTROMETER FOR THE ISOTOPIC ANALYSIS OF HYDROGEN CONTAINING A LOW CONCENTRATION OF DEUTERIUM. Reynolds P . -AERE-CP/R-1449, Aug. 1954.

66. THE DETERMINATION OF DEUTERIUM OXIDE BY INFRA-RED SPECTROMETRY.Gaunt J . (Atomic Energy Res . Es t ab l . , Harwell, Berks , UK). Analyst 79, 580-5, Sept. 1954.

07. A DIFFUSION-EQUILIBRATION METHOD AS A STAGE IN THE DETERMINATION OF THE DEUTERIUM OXIDE CONTENT IN 1-2 MICROLITRES OF FLUID. Lars Garby (Univ. of Uppsala, SWEDEN). Acta Chem.Scand. 9, ,\... 2, 339-41, 1955.

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68. DETERMINATION OF SMALL QUANTITIES OF NITROGEN AND OXYGEN OCCURRING AS IMPURITIES IN tJYDROGEN AND HELIUM. Zinovyeva N. P . Zavodskaya Lab . 1, 1955. (In JUissian)

69. CONTINUOUS ANALYSIS OF ORTHO-PARA-HYDROGEN MIXTURES. Woitzcl D. I I . , Wlüte L . E . Rcv. Sci . I n s t r . 26, 290, M a r . 1955..

P roceed ings of the In terna t ional Conference on tlie Peaceful Uses of Atomic Energy , Geneva 1955.

70. INFRA-RED METHODS FOR ANALYSIS OF HEAVY WATER. Gaunt J . 8, P/410(UK).

71. ON METHODS O F ISOTOPIC ANALYSIS OF HEAVY WATER. V lad imi r sk i i K. V . , Kats M. Y a . , S tasevich B . M. 8, P /63KUSSR) .

72. ISOTOPIC ANALYSIS OK WATER EY NEAR INFRA-RED S P E C T R O PHOTOMETRY. SillM-rnuiii K .8 , P/1010(ARGENTINA).

73. DETERMINATION OK SMALL AMOUNTS OF DEUTERIUM OXIDE IN-WATER BY INFRA-RED SPECTROSCOPY. Berg lund-L a r s s o n U. (Nobel Inst , of C h e m i s t r y , Stockholm, SWEDEN). Acta Chem.Scand . 10, No. 4, 701-2, 1956.

74. THE ANALYSIS OF HEAVY WATER BY INFRA-RED S P E C TROMETRY. Gaunt J . (Atom*« Ene rgy R e s . E s t a b l . . H a r w e l l , Didcot, B e r k s , UK). Spect.rochim. Acta 8, 57-65, 1956. (AERE-C / l t - IfiSti. Apr. 25, l!)5fi).

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75. AN APPARATUS FOR CONTINUOUS ISOTOPIC ANALYSIS OF HYDROGEN-DEUTERIUM MIXTURES. Si lves t r i M. , Adorni N. Nuovo Cimento X-4, 1610, .1956.

INVESTIGATION OF "BITTERNS" AS A SOURCE FOR HEAVY WATER. Weingaer tncr E . , Datta R. L. (Indian Inst, of Sc i . , Bangalore , INDIA). J . Indian Inst. Sci . 38, 73-86, Jan . 195G.'

77_ THE ANALYSIS OF HEAVY WATER. Bryant F . J. (United Kingdom Atomic Energy Authority. Res . Group. Chem. Div. , Woolwich Outstation, UK). Mar . 1956.

78. ISOTOPE SPECTRAL ANALYSIS. Stziganov A. R. Uspekhi F i z . Nauk 58, 365-414, Mar. 1956. (In Russian)

79. A MICROFLOTATION METHOD OF ANALYZING HEAVY WATER. Gragcrov I. P . (L. V. P isarzhevsky Inst, of Phys . Chem. USSR). Zhur Anal .Khim. 11, No. 3, 264-8, May-June 1956. (In Russian) (English t ranslat ion)

80. CONTINUOUS MEASUREMENT OF DEUTERIUM CONCENTRATION BY MEANS OF TI1KRMAL CONDUCTIVITY. Si lvest r i M. , Adorni N. Rev. Sci. [n.str. 27, 388, June 1956.

81. THE-DETERMINATION OF DEUTERIUM BY THE MASS-SPEC-TROMETRIC METHOD. MnrDonald A.., Reed R. I. (Univ. of Glasgow,•UK). Analyst 81, -I0I- 3,July 1956.

54

82. APPLICATION OF FLOAT METHOD FOR PRECISION MEASUREMENT O F DENSITY OF WATER BETWEEN 3, 7 AND 4, 2PC AND FOR DENSITY MEASUREMENTS OF VERY SMALL SAMPLES OF SOLID SUBSTANCES. Spaepen J . Mededcl Konik l . V l a a m . Akad. W e t e n s c h a p . B e l g . K l . Wetenschap , 19, No. 5, 1957. ( A E C - t r - 3 8 4 7 ) .

83. ANALYSIS OF D 2 0 / H 2 0 BY THE I N T E R F E R O M E T E R . Namba S. (Sei. R e s . I n s t . , L t d . , Tokyo, JAPAN) . R e v . Sci . I n s t r . 27, 872 -3 , Oct. 1956.

84. METHODS FOR ISOTOPIC ANALYSIS OF WATER. I . NEW A P PARATUS FOR THE FALLING D R O P METHOD OF ISOTOPIC ANALYSIS OF WATER. Sha tens te in A. Y. , V a r s h a v sk i i ' Y;i. AI. (Karpov Moscow P h y s i c o - C h e m i c a l Inst . ). Zhur Ana l . Khim. 11, No. 6, 746-8 , Nov. - D e c . 1956.(In Russ i an )

85. MEASUREMENT OF LOW DEUTERIUM CONCENTRATION IN WATER BY-MEANS OF FLOAT METHOD. Br igo l i B . , C e r r a i E . , S i l v e s t r i M. (CISE L a b s . , Milan, ITALY). E n e r g i a N u c l e a r e 4, 43 -9 , F e b . 1957.

86. MEASUREMENT OF DEUTERIUM CONTENT IN HIGHLY ENRICH ED SAMPLES OF HEAVY WATER BY MEANS O F A FLOAT METHOD. A d o r n i ' N . , B r i g o l i B . , S i l v e s t r i M. E n e r g i a N u c l e a r e , (Mili.ui)4, 31.5-8, Aug , 1957.

87. ISOTOPIC ANALYSIS OF HEAVY WATER BY NUCLEAR R E S O NANCE. Goldman M. (Savannah R i v e r L a b . , Aiken, S. C. USA). A r c h . Sci . ,(Geneva) 10 ,247 -0 , 1957. ( A E C - t r - 5 3 2 8 )

88. APPARATUS FOR STANDARD MEASURING OF DEUTERIUM ISOTOPIC EXCHANGE RATE B E T W E E N HYDROGEN AND STEAM AT ATMOSPHERIC PRESSIIUK AND 100°C. S i l v e s t r i M . , Adorn i N. Nuovo Cime-ilio V. (Ser ie X)-2fi(i, 1957. (In Ital ian)

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89. THE DEUTERIUM OXIDE CONTENT OF WATER SAMPLES FROM OIL-FIELDS. Cziké K . / F o d o r P . Acta geol.-Acad.Sci. Hung. 4, 331-9, 1957. '

90. DETERMINATION OF THE CONTENT OF HEAVY WATER IN A MIXTURE OF HEAVY AND NORMAL WATER. For t A. (Karlovy Univ. , P rague , CZECHOSLOVAKIA). Czcchoslov. J . Phys. 7, 740-4, 1957. (In Czech)

91. THE DETERMINATION OF DEUTERIUM OXIDE IN WATER BY FREEZING POINT MEASUREMENTS. Fodor P . , C z i k e K. Magyar Kein. Folyci.-.-ut (;;}, No. 2 -3 , 95-6, 1957. (In Hungarian)

92. A STUDY ON THE FALLING-DROP METHOD OF ANALYSIS OF HEAVY WATER. Ching-Lien Chang, Chih-Hsiang Cheng, Hui-P i l l s u . Sci. Record (Peking) 1,417-19, 1957.

93. A METHOD FOR THE SPECTRAL QUANTITATIVE ANALYSIS OF THE ISOTOPIC COMPOSITION OF IlHAVY WATER. Dontsov P . Yu. , Striganov A.R. Zhur. Analit. Khim. 12, 6-9, Jan. - F e b . 1957. (In Russian)

94. METHODS FOR ISOTOPIC ANALYSIS OF WATER. II. NEW LIQUIDS FOR THE DROPPING METHOD OF THE ISOTOPIC ANALYSIS OF WATER WITH A DEUTERIUM CONCENTRATION UP TO 100%. Shatenstein A. I . , Yakovleva E. A. , GP.adkova E. N. , Suzdaltseva S. F . , Antipova N . P . Zhur Anal. Khim. 12, No. 1, 115-7, J a n . - F e b . 1957. (In Russian)

9S\ ANALYSIS OF MIXTURES OF LIGHT AND HEAVY WATER BY MEANS OF A SIMPLE INFRARED PHOTOMETER. Berton A. , Ceccaldi M. Chini. Anal. No. 3, 102-3, Mar; 1957. (In French)

96. METHODS FOR ISOTOPIC ANALYSIS OF WATER. III. THE COMPLETE ISOTOPIC ANALYSIS OF WATER BY DECOMPOSING WITH IRON. SJiatenshtein A. I . , Varshavski i Ya. M. (Karpov Moscow Phys ico-Chemica l Inst. USSR). Zhur. Annlit. Khim. 12, 236-9, Mar . -Apr. 1957. (In Russian)

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97. • METHODS FOR ISOTOPIC ANALYSIS OF W A T E R . IV. METHOD FOR C O M P L E T E ANALYSIS O F W A T E R . S h a t e n s t e i n A. I. , Yako-v leva E . A . , S u z d a l l s c v a S. F . , Ant ipova N. P . Z h u r . A n a l . K h i m . 12, No. 3, 3 9 8 - 4 0 1 , M a y - J u n e 1957. (In R u s s i a n )

08. METHODS FOR ISOTOPIC ANALYSIS OF W A T E R . V. A F L O A T METHOD FOR MEASURING DENSITY D I F F E R E N C E WITH AN ACCURACY WITHIN +0, 2 . S h a t e n s t e i n A. I. , Z v y a g i n t s e v a E . I. Z h u r . Anal . Khim. 12, No.4 . 5.16-22, J u l y - A u g . 1957.

99. MASS S P E C T R O M E T R Y IN THE ISOTOPIC ANALYSIS O F D E U TERIUM. B r i g o l i B . E n e r g . N u c l . (Milan) 4, No 5, 4 11-9 , Oct . 1 957. (In I ta l ian)

1 0 0 A NEW BALANCING D R O P METHOD FOR THE D E T E R M I N A TION O F THE DENSITY OF HEAVY WATER. Yosh ih ide Nai to (Tokyo Me t ropo l i t an U n i v . , Sc t agaya , J A P A N ) . Bul l . C h e m . Soc . J a p a n 30, 939-40 , Dec . 1957.

101. DENSIMETRIC METHODS FOR ISOTOPIC ANALYSIS O F D E U T E RIUM. B r i g o l i B . E n c r g . Nucl . (Milan) 4 , 4 8 3 - 9 1 , D e c . 1957. (In I tal ian)

102. A P P A R A T U S FOR THE CONTINUOUS ANALYSIS O F MIXTURES OF O R T H O - P A R A HYDROGEN AND D E U T E R I U M . V a s i l y e v D . I . , Shalnikov A. I. P r i b o r y i tekh. e k s p . 4 , 1958. (In R u s s i a n )

103. MASS Sl 'K( T R O M E T R I C ANALYSIS O F SOME HYDROGEN OXIDES. Kei-win I. L. , Col tin M. Can . J . P h y s . 3(i, 1 8 4 - 9 1 , F e b . ] 958.

57

P r o c e e d i n g s of the 2nd United In t e rna t iona l Confe rence on the p e a c e f u l Uses of A tomic E n e r g y , Geneva 1958:

104. HEAVY WATER MONITORING BY INFRARED SPECTROSCOPY. S tevens W. H. Bayly I. G. 28, P / 1 8 8 (CANADA);

105. QUANTITATIVE DETERMINATION BY NUCLEAR MAGNETIC RESONANCE. Ionel Solomon. (CEA, P a r i s ) . 28, P / l 154 (FRANCE);

106. THE NUCLEAR MAGNETIC MOMENT AS A TOOL FOR D E T E C TION, ANA LYSIS AND STRUCTURE OF CHEMICAL COMPOUNDS. D h a r m a t t i S. S. , Kaneka r C . R . , M a t h u r S . C . ( T a t a Ins t , of F u n d a m e n t a l R e s . , Bombay, <y Atomic E n e r g y E s t a b l i s h . , T r o m b a y ) . 28, P / 1 6 2 8 . (INDIA);

107. NON DISPERSIVE I N F R A - R E D ANALYSIS MIXTURES O F WATER AND HEAVY WATER. B o s s e l a a r C. A . (Stichting voo r F u n d a m e n -t e e l Ondcrzock dor M a t e r i e , U t r ech t ) . 28, P / 2 2 5 0 . (NETHERLAND)

108. DETERMINATION O F DEUTERIUM OXIDE IN WATER BY MEASUREMENT O F F R E E Z I N G POINT. R e a s e r P . B . , Burch G . E , (Tu lane Univ. and C h a r i t y Hospi ta l of L u i s i a n a , New O r l e a n s USA). Sc ience 128, 4 1 5 - 6 , Aug. 22, 1958.

109. MEASUREMENT O F SMALL AMOUNTS OF H2O IN D ? 0 BY NEAR-INFRARED ABSORPTION SPECTROSCOPY. B i g g e r s R . E . (Oak Ridge Nat. L a b . , Term. USA). C F - 5 8 - 1 2 - 1 4 3 . Dec . 8, 1958.

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HO. DETECTION OF THE LEAKS OF HEAVY WATER FROM A REACTOR INTO THE LIGHT WATER OF ITS EXCIIANGFRS. Julliot C. , Lousiart A. , Nordemann D. (CEN, Saclay, FRANCE). "Nuclear Elec t ronics I. "p. 435-40. P r o c . Int.Symp. P a r i s 1958. IAEA 1959.

111. ANALYSIS OF HEAVY WATEu. IN CONCENTRATIONS A P PROXIMATE TO THAT EXISTING IN NATURAL WATER. Otero de la Gandnrn J. L. ,Gisper t M.G. Anales Real Soc .Espan. F i s . y Qium. (Madrid) S e r . B 55B, 73-82, 1959. (In Spanish)

112. SIMPLIFIED FLOAT METHOD FOR THE DETERMINATION OF THE D 2 0 CONTENT OF WATER. Baer tschi P . , Thllrkauf M. (Univ. of Basel, SWITZ. ). Hclv. Chim. Acta 42, 282-93, 1959. (CEA-tr-A-GGG)

113. TEMPERATURE-FLOAT METHOD FOR ISOTOPIC ANALYSIS OF HEAVY WATER WITHIN LOW CONCENTRATION RANGES Weingaertncr E . , Datta R. L. , Kumar R., MJiacbvan E . .G . Indian Inst. of. Sci. Golden Jubilee R e s . Volume 1909-1959, p. 170-80,1959.

114. SEMI-MICROMÉTHOD FOR ISOTOPIC ANALYSIS OF SUBSTANCES CONTAINING ABOUT 100% OF DEUTERIUM. Shatcnshtcin A. I . , Antnnchik Yu.I . (Karpov Physico-Chemical Ins t . , Moscow, USSR). Zhur. Anal. Khim. 14, 100-3, Jan . -Feb. 1 1959. (In Russian)

115. MEASUREMENT OF THE PURITY OF GRAPHITE AND HEAVY WATER. Hering H. (Commissar ia t à l 'Energ ie Atomique, P a r i s , FRANCE). CEA-1094. Feb. 1959.

HB# ANALYTICAL CHEMISTRY DIVISION ANNUAL PROGRESS REPORT FOR PERIOD ENDING DECEMBER 31 , 1958. (Oak Ridge Nat. Lab. , Term. USA). ORNL-2662. Mar. 3, 1959.

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n , 7 ( AN EXPERIMENTAL DETERMINATION OF SPECIFIC VOLUMES OF HEAVY-WATER. Kirillin V. A. , Oulibin S. A.Teploenerge-tikaNo. 4, 67-72, Apr. 1959. (In Russian) (CEA-tr-R-1579)

Proc .o i the 6th Tr ipar ' i te Instrumentation Conf., Chalk River, Ontario, Canada, Apr. 1959. AECL-801:

118. RECENT DEVELOPMENTS IN THE INFRA-RED ANALYSIS OF HEAVY WATER. Bayly J . , Stevens W. H. (Atomic Energy of Canada Ltd. , Chalk River, Out. CANADA). AECL-801;. p. 39-41;

119. DETECTION OF D 2 0 LEAKAGE IN HEAT EXCHANGERS. Gruber G. 1-1. (Du Pont de rumours E . I . tv Co.Savannah River Plant, Aiken S.C. USA). A E C . 301,: p. 73-6.

120. THE SPECTROGRAPHIC DETERMINATION OF IMPURITIES IN HEAVY WATER. Webb R. J. (United Kingdom Energy Authority. Res . Group Chemistry Div., Woolwich Outstation, UK). AERE-AM-8. Apr. 1959.

121. ISOTOPIC ANALYSIS OF WATER. Kats M. Ya. , Lapteva F. S. Zhur. Anal.Khim. 14, No. 2,227-33, Mar. -Apr. 1959. (In Russian)

122. ANALYSIS OF HgO AND D 2 0 MIXTURES BY INFRA-RED SPECTROSCOPY. DETERMINATION OF MOLECULAR EXTINCTION COEFFICIENTS. Ceccaldi M. (Centre d'Etudes Nuel. , Saclay, FRANCE). Rev. Universelle Mines(9)15,May 1959. (CEA-1285; AEC-tr-5270)

123. TRITIUM GENERATION IN D 2 0 SYSTEMS OF PRTR. Regimbal J. J . , Hayward W. H. (General Electric Co. Hanford Atomic Products Operation,. Richland, Wash. USA).HW-61151. July20, 1959.

124. DETERMINATION OF LOW CONCENTRATION OF DgO IN WATER BY THE FLOTATION METHOD. Report No. 27. Canna vale L. (Comisìon Nacional de Energia Atòmica,. Buenos Aires, ARGENTINA). I960.

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125., DEUTERIUM CONTENT OF THE U. S. NATIONAL BUREAU OF STANDARDS ISOTOPE REFERENCE SAMPLES. Yoshio Horibe , Mituko Kobayakawa, (Tokyo Metropoli tan Univ . , Tokyo, JAPAN). Bu l l .Chem. Soc. Japan 33, 116-7, Jan . 1960.

12G. THE ANALYTICAL PROBLEMS AND THE PRODUCTION OF HEAVY WATER. Niof G. Bull. Inform. Sci. et Tech . (Par is ) No. 40, 19-23, May 19G0. (In F rench )

127. ISOTOPIC ANALYSIS OF HEAVY WATER OF THE REACTOR. Sandroni S. (CNRN, Ispra , ITALY). CNI-33. May 1960.

128. ANALYSIS OF HEAVY WATER BY DENSITOMETRIC METHODS Ching-Lien Chang (Univ. of Peking, CHINA). Kernenergie 3, 892-7, Sept. I960.

129. DETERMINATION OF THE CONCENTRATION OF HEAVY WATER IN THE NATURAL WATERS OF CHILE. la. WATERS OF THE REGION OF CONCEPCION. Fighet t i C . ,Schenke l G. et a l . (Univ. de Concepcion, CHILE). Boi. Soc. Chilena Qu im. , 10, 1-5, Dec . 1960. (In Spanish)

130. ANALYSIS BY MASS SPECTROMETRY OF SAMPLES OF LIGHT WATERS ENRICHED WITH D 2 0 UP TO 1%. B a r b i e r i W., Chiesa A. et al . (CNRN, Ispra , ITALY). CNI-42. (In Italian)

131. ANALYSIS OF D 2 0 / H 2 0 INTERFEROMETER. Vers ino B . (CNRN CSN, I spra , ITALY). CNI-46. (In Italian)

132. ISOTOPIC ANALYSIS OF LIGHT WATER. Sandroni S . , B a r b i e r i W. (CNRN;CSN, Ispra , ITALY). CNI-46. (In Italian)

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133; THE SPECTROGRAPHS ANALYSIS OF INORGANIC IMPURITIES IN HEAVY WATER. Artaud J . , N o r m a n d J . , Vie R. (Commissar ia t a l 'Energ ie Atomique. Contro d 'Etudes Nucl. ,Saclay, FRANCE). CEA-1027. 19G1.

134. A NON-DISPERSIVE INFRARED ANALYZER AND ITS USEFULNESS FOR THE ANALYSIS OF MIXTURES OF WATER AND HEAVY WATER. Bosse laa r C. G. A. Thes i s , Utrecht, Ri jksuniversi te i t , 10G1. (In Dutch)

135. PROGRESS REPORT FOR 1961. Stichtag voor Fundamental Onderzoek, Utrecht;Stiching Institut voor Kernphysisch Onderzoek, Ams te rdam. NP-12208, 1961.

136. THE COULOMETRIC DETERMINATION OF BORIC OXIDE IN HEAVY WATER. P a r k e r A. , T e r r y E . A. (UK Atomic Energy Author i ty .Res . Group Chemis t ry Div. , Woolwich Outstation, UK). AERE-AM-72. Jan. 1961.

137. ANNUAL.REPORT OF ICPP ANALYTICAL SECTION FOR 1960, Shank R. C. (Phill ips Pe t ro leum Co. Atomic Energy Div. Idaho F a l l s , Idaho, USA). IDO-14547. Apr. 14, 1961.

138. HEAVY WATER ANALYSIS IN THE 1% TO 99% D 2 0 RANGE BY INFRARED SPECTROPHOTOMETRY. Stevens W. H. , Bayly J . G. et al , (Atomic Energy of Canada Ltd. , Chalk River , Ont . , CANADA). AECL-1391 . Sept. 1961. (CRDC-1051)

139. ON THE EXPERIMENT ON THE ANALYSIS OF THE HEAVY WATER BY INFRA-RED SPECTROMETRY. Okabe T. ,Denki Shikensho Iho25, 679-86, Sept. 1961. (In Japanese)

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140. . DETERMINATION OF DEUTERIUM CONCENTRATION UM HEAVY WATER BY THE REACTION 0*6(d, n ) F J ' I N D U C E D BY REACTOR NEUTRONS; Amie l S. , P e i s a c h M. (Atomic E n e r g y Commiss ion , Tel Aviv, ISRAEL). IA- 692. Oct. 1961.

141. HEAVY WATER ANALYZER WITH INTERFERENCE F I L T E R . CeccaJdi M , , Goujon P . (CEA, CEN, Saclay, FRANCE) ,T ID-7629 : p . 91-109.(ÖRNL, USA). Analyt ical C h e m i s t r y in Nuclear R e a c t o r Technology. 5th Conf. Gat l inburg Term. USA. Oct. 1961.

142. ANALYSIS OF HEAVY WATER AT NEAR NATURAL WATER CONCENTRATIONS. PART II. O te ro de la Gandara J . L . , G i s p e r t M. (.'<. Anales Real Soc. Espan . F i s . y Quim. (Madr id)Ser . B, 57, 827 :?2,Dec. 1961.

14 3, A S I M P L I F I E D WAY OF DETERMINING DEUTERIUM IN WATER BY THE FALLING UHOP METHOD. Zlotowaki J. , Wrob lewska M. (Univ. of Warsaw, POLAND). Nukleonika 7, 775-88, 1962. (In Pol i sh)

144, RECORDING HYDROMETER FOR LIQUIDS ESPECIALLY A D A P T ED TO THE CONTINUOUS MEASUREMENTOF HEAVY WATER. Chate l S . ,N ie f G. (CEN, Saclay, FRANCE). CEA-2184. 1962. (In F rench)

145. EXPERIMENTAL DETERMINATION O F HEAVY WATER D E N SITY A T HIGH PRESSURES AND T E M P E R A T U R E S . Rivkin S. L . , Akhundov T. S. (All-Union Inst , of T h e r m a l T e c h . , USSR). Tep loenerge t ika , No. 5 , 6 2 - 5 , 1962. (In Russ i an ) .

146, THE DETERMINATION OF THE D 2 0 CONCENTRATION IN HEAVY WATER BY THE FLOAT METHOD. K u m m e r e r K. (Kern-forsch i ingszent rumn, K a r l s r u h e , GERMANY). Z . Physik 169, 166-77, 1962. (In German)

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147. DETERMINATION OP HEAVY WATER PURITY BY INFRARED ABSORPTION. Abernathey R. M. , Morgan T. D. (Phillips Pe t ro leum Co. Atoivu: Energy Div. , Idaho Fa l l s , Idaho, USA). IDO-14576. •l.-m. 16, 1962.

148. \ \ AUTOMATIC TIMER FOR DETERMINATIONS OF D 2 0 CONCENTRATIONS IN WATER BY MEASUREMENTS ON DROPS FALLING IN O-FLUOROTOLUENE. Jason A . C . , Lees A. (Ücpt.of Sclent, and Ind. R e s . , Aberdeen, Scotland, UK). J . Sci. Ins t r . 39, 1G2-4, Apr . 1962.

149. AN IMPROVED INFRA-RED METHOD OF MONITORING I1FAVY WATER. Bayly J . G., Booth R. J . , Stevens W. H. (Atomic Energy of Canada L td . , Chalk River , Ont. CANADA). CRRP-1099. July 1962.

t (.lloquium on Heavy Water . Madrid, Dec. 1962. (JEN Madrid and EAES P a r i s ) . NP-13766:

150. THE "TWO-IMAGE" FLOAT METHOD AT TEMPERATURE BELOW 25°C. Otero J . L. , Gisper t M. , Rojas J . L. NP-13766, p ,155-66 .

151. A DOUBLE SLOW NEUTRON SPECTROMETER. Bondarenko I. I. , Liforov V. G. , Nikolaev M. N. , Orlov V„ V . , Parfenov V. A. , Semenov V .A. , Smirnov B. I. Turchin V. F . Inelast ic Scattering of Neutrons in Solids and Liquids. Vol. I. 127-37. IAEA 1963. (In Russian)

152. A RAPID INFRARED METHOD FOR THE QUANTITATIVE DETERMINATION OF D 2 0 - H 2 0 MIXTURES. Fochler H .S . . (Standard Oil Co. of Ohio, Cleveland, USA). Appi. Spect ry . 17, 105-6; 1963. :

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153. USE OF MEASUREMENTS OF DEUTERIUM CONTENT IN THE STUDY OF METEOROLOGICAL AND GEOLOGICAL PHENOMENA, Roth E . J . Ch i r r t ;Phys . GO, 3 3 9 - 5 0 , 1 9 6 3 . (In F r e n c h )

154, DETERMINATION OF DEUTERIUM OXIDE BY THE FALLING DROP METHOD, Te -Ch iu Chin,ChingV Lien Chang (Peking Univ. GHINA).Acta Chim. Sinica 29 ,266 -76 , 1963.

155. NON-DISPERSIVE INFRA.-RED ANALYSIS OF MIXTURES OF WATER AND HEAVY WATER. B o s s e l a a r C. A. ( P h i l i p s ' G loeüampenfab r i cken , Ni jmegen, NETHERLANDS). Appi . Sci . R e s . , Sect . B, 10, 137-56, 1963.

156. SPECTROCHEMICAL ANALYSIS OF H 2 0 - D 2 0 MIXTURES BY MEANS OF BAND S P E C T R A . Dunken H. , Mikkeleit W. Haucke G. Glas . Hem. D r u s . (Beograd)28, No-8-9, 429-38 , 1963. ( N P - t r - 1 3 0 9 , p . 2 1 - 8 . )

157, NEW MEDIUM FOR THE FALLING DROP METHOD OF ANALYSIS OF DILUTE HEAVY WATER. Te -Ch iu Chin,Chircg-LienChang (Peking Univ. CHINA). Sci . Sinica, (Peking) 12, 147-8 , J an . 1963. (In Engl i sh)

158. THE E X P E R I M E N T A L DETERMINATION OF THE SPECIFIC V O LUME OF HEAVY WATER A T HIGH TEMPERATURES AND P R E S SURES. Rivkin S. L. , Akhundov T . S. At . Energy(USSR) 14, 581-2 , June 1963. (In Russ ian)

159. DETERMINATION OF THE ABSOLUTE CONCENTRATIONS OF I - I 2 0-D 2 0 MIXTURES USING THE INCREASE IN SENSITIVITY OF INFRARED ABSORPTION MEASUREMENTS. Ceccalcli M. (CBA,-CEN.'Saclay, FRANCE) . C E A - R - 2 4 4 1 . 1964.

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160, INVESTIGATION OF TA-' ACCURACY OF THE DROP METHOD ANALYSIS OF HEAVY WATER HAVING A LOW CONCENTRATION OF DEUTERIUM. Wei Chung-Wu, Liu Tien-Ch' iu. Ch'ing Hua Ta Hsueh Hsueh P a o l i , 61-71 , 1964.

161. INVESTIGATION OF THE ACCURACY OF DROP-METHOD ASSAY OF HEAVY WATER WITH A LOW CONCENTRATION OF DEUTERIUM. II. INVESTIGATION OF THE MOVEMENT OF LARGE DROPS. Lo Ch ' i -Fang , Liu Tien-Ch'iu X h ' i n g Hua Ta Hsueh Hsueh Pao 11, 73-80, 1964.

162. IMPROVEMENT OF THE REPRODUCIBILITY OF THE F A L L ING-DROP METHOD BY INCLINATION OF THE TUBE. P r o k s c h E . , Bi ldstein II. et a l . (Os te r re ich i sche Studiengesellschaft i'llr Atomenergie G. m. b . II. Inst. für Chemie, Seibersdorf,. AUSTRIA). SGAE-CH-6/1964 . (In German)

16 3. AN'INFRARED METHOD FOR DETERMINING VARIATIONS IN THE DEUTERIUM CONTENT OF NATURAL WATER. Bayly J . G. , Stevens W. I I . , Thurston W. M. (Atomic Energy of Canada L td . , Chalk River , Ont . , CANADA). AECL-2076, Jan . 1964. (CRDC-1141)

1G4. DETERMINATION OF THE DEUTERIUM CONTENT OF A SAMPLE OF DEUTERIUM OXIDE BY THREE METHODS. Goldblatt M. , Jones W , M . (Los Alamos Seien. L a b . , N. Me's. USA) Anal. Chem. 36, 431-2, Feb . 19C4. (LADC-5874)

165. SEQUENTIAL ANALYSIS OF RADIO-NUCLIDES IN HEAVY WATER MODERATOR. Holcomb II. P . (Du Pont de Nemours E . I. &Co.Savannah River L a b . , Aiken, S .C. USA).DP-886. May 1964. *

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166. CONTINUOUS INFRA-RED MEASUREMENT USING AN INTERFERENCE FILTER. ANALYSIS OF H 2 0 - D 2 0 MIXTURES. Ceccal-di M., Coujon P. (Commissariat a l 'En'ergie Atomique; Centre d'Etudes Nucleaires, Saclay, FRANCE). CEA-R-2440. May 1964.

157. ANNUAL REPORT OF DIVISION ANALYTICAL BRANCH FOR 19G3. Shank R . C . e t a l . (Phillips Petroleum Co. Atomic Energy Div. .Idaho Fa l l s , Idaho, USA). IDO-14636. June 1964.

168. SPECTROPIIOTOMETRIC DETERMINATION OF HYDROGEN CONTENT IN HEAVY WATER. Gordon G. , Yamatera H. (Univ. of Maryland College Park; USA). Anal. Chem. 36, 1866-7, Aug. 1964.

169 RAPID DETERMINATION OF D 2 0 CONTENT IN WATER USING A VAPOUR PRESSURE OSMOMETER. Lazzarini E . (CSN, E . Fe rmi , Po l i t ec . , Milano, ITALY). Nature 204, 87 5-6, Nov. 28, 1964.

1 7 ° . HEAVY WATER. Anderson C. E . , Ebeiihack.D. G. (Du Pont de Nemours E . I . & Co. Savannah River Plant , Aiken, S. C. USA). Analysis of Essent ia l Nuclear Reactors Materials(C. J . Rodden Ed. 1964) (p. 629-57)

171. ANALYSIS OF HEAVY WATER IN CONCENTRATIONS NEAR TO(THAT IN) NATURAL WATER. III. Otero de la Gandara J . L . , Gispert M., Rojas J . L. An. Real Soc ; Espan. F i s . yQuim (Madrid) Ser .B,61, 1155-62, 1965. (In Spanish)

172. DETERMINATION OF THE ISOTOPIC COMPOSITION OF WATER BY FALLING-DROPLETS METHOD. Blaga L.", Blaga L . , Chifu A. (Inst, of Atomic Phys . ,'Cluj, ROMANIA). Stud. Cer-cet. F i z . 17, 765-7-3, 1965.

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173. THE HANDLING OF DEUTERATED WATER AND SPECIFIC PROBLEMS OF DEUTERIUM ANALYSES. Chifu A. (Inst,of Atomic Phys . , Cluj, ROMANIA). Acad. Repub. Pop. Rom. Stud. Cercet . Fix. 17, 574-610, 19G5. (In Rumanian)

174. A SIMPLE METHOD FOR DETERMINATION OF THE H/D RATIOS FROM FIELD ION-MASS SPECTRA OF 1 I 2 0 / D 2 0 OR NII3/ND3 MIXTURES.Richter E. L . , Schmidt W. A. (Max-Planck-GeseUschaft, Berlin, GERMANY). Z. Naturforsch. 20a, 317-19, Feb . 1965. (In German)

175. GAS-CHROMATOGRAPHIC DETERMINATION OF THE DEUTERIUM CONTENT (99 to 100 at. percent) IN HEAVY WATER. Jaege r K. (Gesellschaft i'uer Linde's Eismaschinen AG, Hoel l r iegels-kreuth, W. GERMANY). Kerntechnik 7, 221-4, May 1965. (In German)

176. APPLICATIONS OF ATOMIC ABSORPTION SPECTROSCOPY. Wheat'.J. A. (Du Pont de Nemours E . I . &Go. Savannah River L a b . , Aiken S.C. USA).DP-980. July 1965.

177. STUDIES ON THE PRODUCTION OF HEAVY WATER. IH. ANALYTICAL CONTROL OF THE PRODUCTION INSTALLATIONS. Olero"de ; 'la Ganclara J . L . , Gispert M. , Rojas de Diego J . L . (J - .E.N. , Madrid, SPAIN). Energia Nu ci . (Madrid) 9, 248-55, July-Aug. 1965. (In Spanish)

173. AUTOMATED ANALYSES FOR THE CHARACTERIZATION OF HEAVY WATER MODERATOR. Gaddy R. H. (Du Pont de Nemours E. Ì. &Co. Savannah River Lab . , Aiken, S. C. USA). Technicon'Analytical.Symposium Aug. 3, 1965. (CONF-650919-2)

179. A I I I G H S E N S I T T V Ì T Y HEAVY WATER LEAK DETECTOR. Bayly ' J . G. (Atomic. Kiuu-g.y or Cannda Ltd., Chalk River, Ont. CANADA).

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180. ANALYSIS OF DEUTERIUM" OXIDE-WATER MIXTURES AND MEASUREMENT OF THE DEUTERIUM ISOTOPE E F FECT ON THE ACID-BASE EQUILIBRIUM OF N, N-DIME-THYLBENZYLAMINE USING NUCLEAR MAGNETIC RESONANCE. Leyden D . E . , Reilley C. N. (Univ. of N. C. , Chapel Hill, USA). Anal. Chem. 37, 1333-8, Oct. 1965.

181. DETERMINATION OF THE D2O CONTENT IN WATER BY INFRARED SPECTROMETRY. Knezevic Z .V . (Boris Kidrich Inst, of Nucl. Sc i . , Belgrade, YUGOSLAVIA). Isotopenpraxis 1, 69-71, Nov. 1965.

18?. ISOTOPIC ANALYSIS OF HEAVY WATER BY INFRARED SPECTROMETRY. Rojas J . L. Energ . Nucl. (Madrid.)9, 453-8 , Nov.-Dec. 1965, (In Spanish)

183. AUTOMATIC SPECTROPHOTOMETRY ANALYSIS OF DEUTERIUM OXIDE FOR VARIOUS IONS PRESENT IN CONCENTRATIONS OF THE ORDER OF PARTS PER 109 . Bri t t R. D. J r . (E. I. Du Pont de Nemours & C o . , Aiken, S. C. USA). Tech. Eau (Brussels) No. 238, 29-33, 1966. (In French)

184. THE DETERMINATION OF HEAVY WATER WITH THE UR-10 •. SPECTROPHOTOMETER. Kocent A-, ,Vasatkova J . (Cancur

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186. METHOD OF ISOTOPIC ANALYSIS OF OXYGEN IN MICROQUANTI-TIES OF WATER. DETERMINATION'OF. EQUILIBRIUM DISTRIBUTION COEFFICIENTS OF 1 8 0 BETWEEN H 2 0 AND CO2 AND D 2 0 AND CO2. Majzoub M. (CEN Saclay, FRANCE). J . Chem. Phys . 63, 563-8, Apr. 1966. (In French)

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1'87. ANALYTICAL PROCEDURES (1966) FOR THE HEAVY WATER AND HELIUM SYSTEMS OF THE NRX AND NRU REACTORS. PART I, II, AND III. (Atomic Energy of Canada Ltd. , Chalk River, Ont. CANADA). AECL-2596. June 1966.

188. ISOTOPE DILUTION ANALYSIS WITH STABLE ISOTOPES. PART I. EXPERIENCES IN DETERMINATION OF WATER CONTENT BY ISOTOPE DILUTION ANALYSIS WITH D 2 0 . Krumbiegel P. , Huebner H. , Rolle W. (Inst, fuer Stabile Isotope, Leipzig. Deutschen Akad. der Wissenschaften, Berlin, GERMANY). Isotopenpraxis 2, 220-4, June 19G6. (In German)

189. INFRARED DETERMINATION OF RESIDUAL HYDROGEN IN DE-UTERATED INORGANIC COMPOUNDS. Whateley T. L . , Whittem R.N. (Australian-Atomic Energy Commission Res . Es t ab l . , Lucas Heights,AUSTRALIA). AAEC-TM-326. May 1966.

190. DETERMINATION OF DEUTERIUM ION CONCENTRATION IN DILUTE UNBUFFERED DEUTERIUM OXIDE SOLUTIONS. Baumann E.W. (Du Pont de Nemours E . I . &Co., Aiken, S. C. USA). Anal. Chem. 38, 1255-7, Aug. 1966.

191. USE OF DIMETHYL SULPHOXIDE AS A SOLVENT FOR THE RAPID ISOTOPIC ANALYSIS'OF WATER BY INFRARED SPECTROMETRY. Mahadevan E.'G. (Columbia Univ. , New York, USA). Analyst, 92, 717-8, 1967. ,

192; ANALYSIS OF HEAVY WATER BY THE FLOAT METHOD OVER THE ENTIRE CONCENTRATION RANGE. Gispert M. , Rojas J. L . , Otero de la Gandara J . L. (J. E . N . , Madrid, SPAIN). A n . R e a l . S o c . E s p a n . F i s . y Quim. (Madrid) Sor. B, 63,479-84,

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193. FUNDAMENTAL CALCULATION OF ACCURACY IN HEAVY WATER STANDARDS..Rowland P . R. (Atomic Energy E s t a b l . , Winfrith, Eng. UK). AEEW-M-745. May 1967.

194.PHOTOMETRIC DETERMINATION OF THE 1SOTOPIC CONTENT OF HEAVY WATER. Feue r s t e in II. (Kernforschungszentrum, Kar l s ruhe , W. GERMANY). KFK-570. May 1067. (In German)

195 WATER QUALITY CONTROL IN THE HFBR. P ro t t e r S.R. (Brook-haven Nat. Lab. , Upton, N. Y. USA). P.N.L- II 56.1. June 196 7.

196. METHOD FOR THE DETERMINATION OF OXYGEN ISOTOPIC RATIOS IN HEAVY WATER. Robinson B. K. , Symons W. J . (Atomic Energy Establ . , Winfrith, UK). AEEW-R-550. Sept. 1967.

197. RAPID WIDE-RANGE DETERMINATION OF HEAVY WATER BY CUT-OFF PYCONOMETER. Rowland P . R. t Wright C. R . , Knott A . R . AAEW-M746.19G7.

198. MtCllOCHEMICAL ANALYSIS SECTION: SUMMARY OF ACTIVITIES, JULY 196G-.IUN13 1937. Taylor J . K. (Nat. Bur. of Stand. , Washington, D . C . USA). NBS-TN-425. Out. 1967.

199. DETERMINATION OF WATER-HEAVY WATER MIXTURES BY 1 9 F NUCLEAR MAGNETIC RESONANCE. Devcrel l C . , Schaumburg K. (Nat. Res . Council, Ottawa, CANADA). Anal. Cliem.

•39, 1879-80, Dec. 1967.

200. FUNDAMENTAL PROBLEMS OF HEAVY WATER'DOSIMETRY IN NUCLEAR I IE ACTORS. David L . , Tomaskova LÙUstav Jadcrncho Vy/Jumui, Prague, CZECHOSLOVAKIA). Jad. E n e r g . 1 4 , 11 -20, Jan . 1968. (In Czech)

71

2 0 1 . STANDARDIZATION OF THE DEUTERIUM CONTENT OF HEAVY WATER. B a e r t s c h i P . , Rosa tz in H. (E idgenöss i sches Inst, fuer Reak to r fo r schung , Wuerel ingen,SWITZERLAND). Oct. 1968. (In German)

2 02. STANDARDS FOR A PRATICAL SCALE OF pD IN HEAVY WATER. Paabo M . , Bates R. G. (NBS. Washington, D. C. USA). Anal. C h e m . 4 1 , 283-5 , F e b . 1969.

2 03. DENSIMETRIC ISOTOPIC ANALYSIS OF LIGHT AND HEAVY WATER BY USE OF OXYGEN EXCHANGE BETWEEN CARBON DIOXIDE AND WATER. S taschewski D. (Kern fo r schungszen t rum K a r l s r u h e , GERMANY). B e r . Bunsenges , P h y s . Chem. 73, No. 1, 59-65. M a r . 1969. (In G e r m a n )

2 J 4 . INTERFEROMETRIC DETERMINATION O F SMALL AMOUNTS OF D 2 0 AND H 2 0 . Mercea J. ( Inst . Atomphysik , Cluj , ROMANIA). Chem. -Ing. - T e c h . 4 1 , 508-10, A p r . 1969. (In G e r m a n )

205. A CALORIMETER APPARATUS T O MEASURE THE ENTIIAL-PIIY DIFFERENCE OF HEAVY WATER. Nowak E . S . , Chan. J . (Univ. of W e s t . O n t . , London, CANADA). J . Heat T r a n s f e r 91 , 235-40, May 19S9.

206. INFRARED ANALYSIS OF HEAVY WATER-WATER MIXTURES O F INTERMEDIATE (3 TO 97 PERCENT) CONCENTRATION. Kimbrough D. J r . , Askins R. W. (Georgia Inst , of T e c h . , Atlanta, USA). A;ud, Chem. 4 1 , 1147-8, Ju ly 1969.

207. DEUTERIUM ANALYSIS BY PHOTONEUTRON DETECTION. George K. D. , K r a m e r H. (Ster l ing F o r e s t R e s . Cen te r , Tuxedo, N . Y . U S A ) . N u c l . App i .Techno l . 7, 385-8 , Oct. 1969.

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208. IN-LINE D 2 0 ANALYSIS. Stutheit J . S . , Rampey W. P . (Du Pont de Nemours E . I. & Co . , Aiken, S. C. USA). Nucl. Ins t rum. Methods 75 ,43-4 ,1969 .

209, CHEMISTRY AND MATERIALS DIVISION; P r o g r . Rep. Oct. 1 -Dec. 31, 1969. (AECL, CNRL, Chalk River,"Ont. CANADA).

210. DETERMINATION OF DEUTERIUM IN HEAVY WATER BY SECONDARY DEUTERON ACTIVATION. P re to r iu s R . , Wainerdi E . R. (Texas A and M Univ. College Station, USA).Talanta 17, 51 -9 , Jan. 1970.

211. A COMPARISON OF ANALYSES OF HIGH-PERCENTAGE HEAVY WATER SAMPLES BY DENSITY MEASUREMENTS AND BY INFRARED SPECTROSCOPY. Moravec J . , S a r a V. , Vagner J , , Kysela J . (Inst. Nucl. R e s . of CSAV-Re2-CSSR) J a d e r n a energ ie 17, No. 1,28-30, 1971;

f1

I V ' HEAVY WATER PRODUCTION

75

REVIEWS OF PRODUCTION PROCESSES

THE NEED OF ADEGUATE PROVISION FOR THE QUANTITY PRODUCTION OF DEUTERIUM WATER. Washburn E. W. Science 78, 555-6 , IÖ33.

THE MANUFACTURE OF DEUTERIUM AND ITS COMPOUNDS. Webb W.A. Ind. Eng .Chem. News Ed. 12, 63, 1934.

COMMERCIAL PRODUCTION OF HEAVY WATER. An Editor i a l . Nature 133, G04, 1934.

THE PREPARATION OF HEAVY WATER. Schachert F . P r i r o d a 28, 226-34,1935.

THE ELECTROLYTIC SEPARATION OF HYDROGEN AND DEUTERIUM AND THE CATALYZED EXCHANGE REACTION HD+H2O-H2+HDO. Butler J .'A. V. Z. E lek t rochem. 44, 55-G2, 1938.

EXCHANGE REACTIONS BETWEEN LIGHT AND HEAVY HYDROGEN. A, Review. Ingolfi O . K . , Wilson C, L. Z . E lck t ro-•chem. 44, 62-72, 1938.

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INDUSTRIAL MANUFACTURE AND APPI-ICATIONS OF HEAVY WATER AND OF DEUTE.RIUM DERIVATES. A Review. Da rmoi s E. Tccli. Ind. Chi-n. ;\jo. 284 bis , 16-8 , 1939.

(On DuaL T e m p e r a t u r e Exchange).Edmonds S. M. , ßix-baum N. Ind. Eng . Gliom. Anal . Ed. 12, GO, 1940.

(On Dual T e m p e r a t u r e P r o c e s s ) . Shaw A . J . Ind. Eng . Chem. Anal . Ed. 12, 668, 1940.

SEPARATION OF ISOTOPES BY CHEMICAL MEANS. Urey II. C. J . Wash. Acad. Sci . 30 ,277-94 , 1940.

A COMPARISON OF THE METHODS OF PREPARING HEAVY WATER. Brodskii A. I. Zhur . P r i k l a d Khim. 13, 6 70 -5 , 1940. (In Russian)

ON PRODUCTION OF HEAVY WATER. F a r k a s A. SAM R e por t . A-84 . J an . 11, 1942.

(On Dual T e m p e r a t u r e P r o c e s s ) . Kimbal l G. E . , S tockmayer W . U . Col . Univ. Rep. A-144 . Apr . 7, 1942.

(On Dual T e m p e r a t u r e P r o c e s s e s ) . S p e v a c k J . S. Col . Univ. Rep. A-393.DCC. 3, 1942.

(On Dual T e m p e r a t u r e P r o c e s s ) . Kimbal l G. E . , S tockmayer W. II. Col . Univ. Rep. 100XR-1G57. Oct. 14, 1942.

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IG. (On Dual T e m p e r a t u r e P r o c e s s e s ) . Spevack J . S. Col. Univ. Monthly Repor t . Nov. 11, 1942.

17. (ON Deuter ium Separat ion by Means or Exchange Reactions). Mayer II. Col. Univ. Memo. Nov. 21 and 26, 1942.

18. (On Dual T e m p e r a t u r e P r o c e s s ) . Ki rshcnbaum I. Col. Univ. Thes i s . 1942.

19. (On D2O Product ion) . Webb G. M.A L e t t e r to J . E. Ahlberg Col. Univ. Sept. 3, 1942.

2 0. REPORT ON PRELIMINARY ANALYSIS OF THE EXCHANGE PLANT. Chopin J . H . , Urey U . C . SAM Report 3R-23 (A-501) Jan . 5, 1943.

21 . (On Dual T e m p e r a t u r e P r o c e s s e s ) . Brown F . B . Col. Univ. Rep, A-566. Mar. 12, 1943.

22. (On Dual T e m p e r a t u r e P r o c e s s e s ) . Brown F . B. Col. Univ. R e p . A - 5 9 1 . Apr. 14, 1943.

23. (On D 2 0 Product ion) . Ahlbcrg J . E. , Blair T . S. , Bcthuno A. J . de, Koracli JVI., Urban J . , Vona J . Col. Univ. Rep. A-1214. Nov. 5, 1943.

24. (On Separat ion P r o c e s s e s ) . Cohen K. , Mayer H. L. SAM Memo. 4M-10. Jan . 2, 1943.

25. OPTIMUM DESIGN OF CATALYTIC TOWERS. Mayer H. L. SAM Rep. 4R-34 . Mar . 12, 1943.

78

THE PHENOMENOLOGY OF TWO PROCEDURES FOR S E PARATING ISOTOPES. K l e m m . A. Z . Na tu r fo r sch . 1 ,252-7, 194G.

SURVEY ON HEAVY WATER AND ITS PRODUCTION. S i lve s t r i M. CISE-2 .1946 . (In I tal ian)

MULTISTAGE SEPARATION PROCESSES. Benedict M. Am. I n s t . C h c m . E n g r s . 4 3 , No. 2 , 4 1 - 6 0 , 1947.

CALCULATION OF EQUILIBRIUM CONSTANTS FOR ISO-TOPIC EXCHANGE REACTIONS. Bige le i sen J . , Mayer M. G. J . Chem. P h y s . 15, 261-7 , 1947.

SEPARATION OF ISOTOPES BY THERMAL DIFFUSION. A Review. Wolczek O. Widomosci- Chem. 7 / 9 , 1, 2 1 - 5 , 1947. (In Pol i sh)

THE DUAL TEMPERATURE PROCESS FOR ISOTOPE S E PARATION. MDDC-89. ADD, 1, 547 .Dec i . F e b . 26, 1947.

CHEMICAL METHODS OF ISOTOPE SEPARATION. Reid A. F . U. S. Naval Med. Bull . SuppL205-8 , 1948.

PRELIMINARY STUDY OF POSSIBLE PROCESS TO P R E P A R E HEAVY WATER. P e r p é r o t II. Mem. P o u d r e s 32 ,429 -36 , 1950.

REVIEW OF THE PRESENT STATUS OF ISOTOPIC SEPARATION METHODS. Grotli W. (Bunsenges . fUr phys ik . Chemie , GERMANY).ZtGchr.Elektfochem. 54, 5-12, 1950. (In G e r m a n )

LABORATORY STUDIES FOR SEPARATION P R O C E S S E S . . Gidinoff M. L . , J o r i s G. G . , T a y l o r E . H . , T a y l o r H. S . , U r e y H . C . NNES4II-4D. 1951.

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3G. CHEMICAL EXCHANGE REACTIONS FOR THE PRODUCTION OF HEAVY WATER. Bigclc isen J . et al . BNL-107. 1951.

37. DEUTERIUM CONCENTRATION BY CHEMICAL EXCHANGE. Bigeleisen J . et a l . BNL-118. 1951.

3 8 SEPARATION OF STABLE ISOTOPES. THE ROLE OF ENGINEERING IN NUCLEAR ENERGY DEVELOPMENT. Benedict M. 3rd Ann. Oak Ridge Summer Symp. Aug. 27 to Sept. 7, 1951. T lD-5031 .Dec . lD51 .

HEAVY WATER. Brim J . T i d s s k r . Kjemi, Borgvson. Mot. 13, 156-G1,1953.

HEAVY WATER. C e r r a i E . E n e r g i a Nucleare (Milan) No. 5, 96 9G-103, Dec.20, 1952.

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42. STATUS OF HEAVY WATER PROCESSES.Thayer V.R. (Du Pont de Nemours E . I. &Co, Atomic Energy Div. , Wil-minghton.Del . USA). TID-2504. (Del. )(Suppl. 1) (DPW-G6G2. Del . )

43. HEAVY WATER. A REVIEW OF PROCESSES AND PLANTS FOR LARGE-SCALE PRODUCTION. Selak P . J . / F i n k e J . Chem. Eng. P r o g r . 50, 221-9, May 1954.

44. ON PROPERTIES AND PREPARATION OF HEAVY WATER. Baer t sch i P . , Kuhn W. Techn. Rundschau 52, 1954. (In German)

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ON DEUTERIUM DISTRIBUTION IN HYDROGEN ISOTOPIC EXCHANGE. Varshavskii Ya. M. , Vaisberg S. E. ZhürvFiz . Khim.-22, No. 3, 52 3-32, Mar. 1955.

REPORT FROM GENEVA. REACTOR MATERIALS. Nuc leonics 13,No. 9,G4-71.Scpt. 1955.

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SOME ASPECTS OF THE HEAVY WATER PREPARATION DESIGNED FOR A SWITZERLAND REACTOR, dc Haller P . P /923 . ( SWITZERLAND). 1st Geneva Conf. 1955. (Abstract only)

GENERAL ASPECTS ON INDUSTRIAL SEPARATION OF ISOTOPES. Gueron J . CEA-Saclay Rep. 456. 1955.

THE THEORY OF ISOTOPE SEPARATION BY COUNTER-CURRENT CHEMICAL EXCHANGE. Marcus W.C. De, Halle E. von. K-1190. Jan. 19,1955.

DEUTERIUM SEPARATION STTJDYProgrcss Report No. 2. Drews W. P. (Esso Res. and Eng. Co . , Linden, N. J . USA). NYO-G085.Aug. 1, 1955. Deci. Mar. 4, 1957.

DEUTERIUM SEPARATION STUDY. P rogres s Report No. 4. (Final Report on HEAVY WATER MANUFACTURE SURVEY). Bar r . F . T . , Drews W. P. (Esso Res. and Eng. Co. , Linden, N. J . USA). NYO-7523. Oct. 14, 1955. Deci. Mar. 25, 1957. (SOA-188)

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53. PRODUCTION OF HEAVY WATER. NATIONAL NUCLEAR ENERGY SERIES, DIVISION III, VOLUME 4 F . G. M. Murphy, I-I. C. Urey, I. Kirshenbaum, eds. New York, McGraw-Hill Book Co . , Inc. 1955. (NNES-III-4F)

54, THE PRODUCTION OF HEAVY WATER. Becker E . W. Angew. Chem. 68, 6-13,1956. (In German)(AERE-Lib/Trans r 734; AEC-tr -2808)

55. OPTIMUM CONDITIONS FOR THE ENRICHMENT OF HEAVY WATER IN HOT-COLD COLUMNS. I. THE SINGLE HOT-COLD SYSTEM. Bier K. Chem. Ing. Tech. 28, 265-88, 1956. (In German) (AEC-tr-2887)

56. PRODUCTION OF HEAVY WATER. Sojka, J . Chem. Prumysl . 6, No. 4, 170-2, 1956, (In Czech)

57. THE ANALOGY BETWEEN ISOTOPE 'XCHANGE IN COUNTER-CURRENT COLUMNS AND ADSORPTION PROCESSES. Rozen A. M. Doklady Akad/Nauk SSSR 108, 122,1956. (In Russian)

58. HEAVY WATER PRODUCTION. D2O BEHAVIOUR IN REACTORS. Roth E. Chim. &Ind., Suppl. Energie Nucléaire 75, No. 2 ,42-52, 1956.

59. ISOTOPIC E F F E C T IN THE LIQUID-VAPOR EQUILIBRIUM OF BINARY SYSTEMS CONTAINING DEUTERIUM COMPOUNDS. Rabinovich I. B . , Nikolaev P. N . , Gochaliev Z. E . , Tretyakova N. N. ( Lobachevskii ' Gorkii State Univ. USSR). Doklady Akad. Nauk SSSR, 110, 241-4, Sept. 11, 1956. (InRussian)

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PREPARATION OF HEAVY WATER. Fe l lner -Fe l ldeg H. Gas und Wasserfach 97, No. 24, 1017-9, 1956. (In German)

PILOT-PLANT-SCALE MANUFACTURE OF HEAVY WATER.' Cziko K» , Fodor P. Magyar Tudomanyos Akad.Központi Fiz . Kulat(!) Intezetcnek Közlcmenyei 4, 68-75, 195G.(In Hungarian)

HYDROGEN ISOTOPE EXCHANGE. Augood D. R. Nature 178, 754-5,1956.

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PROBLEMS CONNECTED WITH THE PRODUCTION OF HEAVY WATER IN ITALY. Silvestri M.p . 315-34; (In Italian)

PROBLEMS CONNECTED WITH THE PRODUCTION OF HEAVY WATER IN THE UNITED KINGDOM. Pra t t H . R . C , p.315-34;

PROBLEMS CONNECTED WITH THE PRODUCTION OF HEAVY WATER IN FRANCE. Roth E. p. 335-52. (In French)

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69. SURVEY OF HEAVY WATER PRODUCTION PROCESSES. Benedict. M. (MIT, Cambridge, Mass . USA). P r o g r e s s in Nuclear Energy. Ser ies IV. Technology and Engineering. R. I-Iusrt, S. McLain eds. New York, McGraw-Hill Book Co. , Inc . , 195G. (p.3-56)

70. HEAVY WATER IN GERMANY. Atomics 8, No. 11, 428-30, Nov. 1957.

71. THE PREPARATION OF GRAPHITE AND HEAVY WATER. Beckmann R. Atompraxis 3, (2), 60, 1957.

72. METHODS OF OBTAINING HEAVY WATER. Otero de la Gandara J . L. Energia Nuclear (Madrid) 1, No. 2 ,45-58 , A p r . - J u n e 1957. (In Spanish)

73. SPECIAL MATERIALS FOR NUCLEAR INDUSTRY. Cerra i E. Energia Nucleare (Milan) Suppl.Vol. 3, 82-92, 1957.

74. NEW RESEARCH DEVELOPMENTS FOR INDUSTRIAL SCALE ISOTOPE SEPARATION. Villani S. Energia Nucleare (Milan) 4 ,187-95,1957.

75. METHODS OF PRODUCTION OF HEAVY WATER. Nuklconika 2 , N o . l , 111-30, 1957. (In Polish)

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ISOTOPE SEPARATION BY MULTISTAGE METHODS. Johns T . F . P rogr . Nucl. Phys .6 , 1-25, 1957.

THE PRODUCTION OF DEUTERIUM OXIDE AND THE DETERMINATION OF ITS DENSITY. Shatenstein A. I . , Yakimenko L. M. , Kalinachonko V. R. , Yakovleva E . A.. Zhur. Neorg. Khim. 2, 985-94, 1957. (In-Russian) (CEA-R-367; JPRS-2499)

AN INVESTIGATION OF TECHNIQUES FOR THE SEPARATION OF HYDROGEN AND DEUTERIUM. PART I.ZONE REFINING OF MIXTURES OF ORDINARY AND HEAVY WATER. PART II. THE REACTION OF IRON WITH MIXTURES OF ORDINARY AND HEAVY WATER. PART III. GAS CHROMATOGRAPHY WITH HYDROGEN AND DEUTERIUM SAMPLES. Thomas C. O. Thes is , Univ. of Tennessee, Knoxvillo, 1957.

Proceedings of the Int. Symp. on Isotopie Separation, A m s t e r dam, Apr. 1957. North Holland Pubi. Co. Amsterdam 1958.

EVALUATION OF ISOTOPE SEPARATION PROCESSES. Garret G. A. ,Shacter J . (p. 17-32);

THE SIGNIFICANCE OF THE PRODUCT AND SUM RULES TO ISOTOPE FRACTIONATION PROCESSES. Bigele isen.J . (BNL, Dept. Chem. , Upton L. I . , N. Y. USA), p. 121-57;

ENRICHMENT OF ISOTOPES BY THE DIFFERENCE IN RATES OF ISOTOPIC REACTIONS. Bernstein R. B. (Univ. Mich., Ann Arbor, USA), p . 313-15;

ISOTOPE SEPARATION BY FRACTIONAL DISTILLATION. London H.. p. 319.

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METHODS OF HEAVY WATER PRODUCTION. Stouls L. , Enex-gie Nucléaire 2 ,4 , 397-407, 1958.

CHEMICAL EXCHANGE. Augood D. R. Ind. Chem. 34, No. 404, 533, 1958.

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METHODS FOR THE SEPARATION OF STABLE ISOTOPES. Blanc D. A cero y onci-gia, Barcelona IG, 92, 54-6 0, 1959. (In Spanish)

INDUSTRIAL PRODUCTION OF HEAVY WATER. Sakodynskii K. I, Atomnaya Encrg. 6, 14-20, Jan. 1959. (In Russian)

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K6

PERFORMANCE CHARACTERISTICS OF DEUTERIUM EXCHANGE PROCESSES. Dietze M. , Pilz S.' Chem.Tech. (Berlin) 11,544-6,1959.

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OPTIMUM CONDITIONS FOR THE DUAL-TEMPERATURE EXCHANGE PROCESS OF PRODUCING HEAVY WATER. Mizushina T . , Takainatsu T, , Yoshida A . , Nakanishi A . , Kono M., Sayama H. Kagaku Kogaku 23, 71-80,1959.'(In Japanese)

INDUSTRIAL METHODS FOR THE PRODUCTION OP HEAVY WATER. Zhavoronkov N. M., Sakodynskii K. I. Khiiri; P rom. No. 3, 35-48, 1959. (In Russian) ( JPRS-50G4)

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PRODUCTION OF HEAVY WATER. Hannerz K. Tekn. Tidskr . 89, No. 7, 151-6, 1959.

HEAVY WATER PRODUCTION IN ROMANIA. Mercea V . , Peculea M. , Grecu E. Rep.IFA (Bucharest) A4, 1959.

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P roc .o f the Joint Symposium on Instrumentat ion & Computation in P r o c e s s Development and Plant Design, London, ICE, 19G0.

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107. INDUSTRIAL MANUFACTURE OF HEAVY WATER. Zhavoronkov N. M. , Sakodynskii K. I. (Karpov Inst, of Physic and Chemis t ry , Moscow, USSR). Kernenergie 4, No. 12, 893-904, Dec. 19G1. (In German) (JPRS-42164)

108. APPLICATION OF CHEMICAL EXCHANGE METHODS TO 1SOTOPIC SEPARATIONS. Drury J . S. (ORNL) P r o g r . in Nucl. Energy, Ser.. IV, 4, 308-48, 1961.

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109. THEORY OF ISOTOPE SEFARATIONIN COLUMNS. llozon A.M. Atomizdat, Moscow 19G0. (In Russian)

110. GENERALITIES ON THE PHYSICAL CHEMISTRY OF THE PROCESSES FOR HEAVY WATER PRODUCTION. Dirian G. Bull. Inform. Sci. et Tech. (Par is) No. 40, 24-35, May 1960. (In French)

111. SEPARATION AND USE OF STABLE ISOTOPES. I. SEPARATION OF STABLE ISOTOPES BY CHEMICAL EXCHANGE. Wetzel K., Krctzchmann G. Chem. Tech. 12, 26 3-6, 196 0. (In German)

112. PRODUCTION OF HEAVY WATER FOR REACTORS. Bolhar-Nordonkampf F. Electroteeh. u. Maschinenbau, 77, 387-90, Sept. 1, 19C0. (In Gentian)

113. HEAVY WATER PRODUCTION. Favre I. Energie nucléaire 2,108,1960.

114. PRODUCTION OF HEAVY WATER IN THE UNITED STATES. Walker P. T. Ind. Chemist 36, 373-6, 1960.

115. HEAVY WATER PRODUCTION IN THE .U. S.A. Thayer .V. Nucl. Power 5, No. 46, lOOrll , 1960.

11G. PRACTICAL USABLE METHODS FOR ISOTOPE SEPARATION. Walker W. Physik. BlHtter 16,61-72, 19G0.

89

11Y. CONTROL OF THE DUAL TEMPERATURE EXCHANGE PROCESS FOR THE MANUFACTURE OF HEAVY WATER. Morr is J. "W., Scotten W. C. Chem. Eng. Progr . , Symp. Ser. 58(39), 26-38, 19G2.

118. STABLE ISOTOPE SEPARATION. II. PRODUCTION PROCESSES. Linders t roem-Lang C. U, (Atomenergikommissiones Forsogsanlaeg, Riso, DENMARK). Dansk. Kemi 43, 165-71, 1962. (In Danish)

119. SEPARATION OF HEAVY WATER BY ISOTOPIC EXCHANGE. Roth E. Energia Nucleare 4, 332-42,1962.

120. THE SEPARATION OF HEAVY WATER. Brancker A. V. Ind. Chem. 38, 14-22,1962.

121. APPLICATION OF CHEMICAL EXCHANGE METHODS TO ISOTOPE SEPARATION.DruryJ .S. J . Nucl. Energy Pt. B . , Reactor Technol. 3, 120-GO, 1962.

\12.. DEVELOPMENT DIRECTIONS IN THE PERFECTION OF METHODS FOR THE SEPARATION OF STABLE ISOTOPES. Zhavoronkov N. M. , Sakodynskii K. I . Kernenergie 5,211-9, 1962. (In German)

123. HEAVY WATER PRODUCTION. Becker E. W.A. (Inst. fUr Kernverfahrenstechnik, Kar l s ruhe , W. GERMANY). STI /PUB/ 15/21. IAEA, Mar. 1962.

124. ISOTOPE SEPARATION BY MEANS OF ION TRANSPORT, DISTILLATION AND THERMAL DIFFUSION. Clusius K;

• Cheni. Ing. Tcchn. 35, 422-8, 1963.

90

125. THE HYDROGEN ELEMENT AND THE PREPARATION OF HEAVY WATER. Jcnn J . T . , Akar P . Energie Nucl. 5, 98-114, Mar. rApr . 1963. (In French)

126.. THE PRESENT STATE AND THE PROBLEMS OF HEAVY WATER MANUFACTURING. Kur ihara Y. Genshiryoku Kogyo 9, No. 8, 57-62;Aug. 1963. (In Japanese)

127. THE PRESENT STATE AND PROBLEMS OF TECHNOLOGY FOR HEAVY WATER PRODUCTION. (PART)2. Kur ihara Y. Genshiryoku Kogyo 9, No. 9, 17-20, Sept. 196 3. (In Japanese)

128. SOME FEATURES OF THE DUAL TEMPERATURE METHOD OF SEPARATION OF HYDROGEN ISOTOPES. Vaisberg S. E . , Varshavski i Ya. M. (Inst, of Radiation Phys ics , Chemis t ry and Biology, Academy of Sciences , USSR). Zhur . F i z . Khim. 6 0, 115-23, J a n r Feb . 1963. (In Russian)

129, SEPARATION OF ISOTOPES, ANNUAL PROGRESS REPORT. Taylor T . I . TID-19592, Sept. 1, 19G3.

130. ENRICHMENT AND USE OF STABLE ISOTOPES. Groth W. 2nd Wiss . Tag. Deut. Atomforums Munich 1963. (p. 239-51; pubi. 19G4)

131. ISOTOPE SEPARATION BY DISTILLATION AND CHEMICAL EXCHANGE. Murrenhoff 'A. P . Kerntechnik 6(12), 554-7, 1964.

132. INDUSTRIAL PRODUCTION OF DEUTERIUM. Murrenhoff A . P . ' K e r n t e c h n i k 6(12), 558-60, 1964.

133. PRODUCTION OF DEUTERIUM AND OF HEAVY WATER BY ISOTOPIC EXCHANGE. Mer ie l Y. Sci. p r o g r . Nat. (Pa r i s ) No. 3352,305-10, 1964.

91

3rd International Conference on Peaceful Uses of Atomic Energy. Geneva 1Ì3G4:

134. STUDY OF THE PRODUCTION OF HEAVY WATER IN FRANCE. Lefrancois I I . , Lerat J . 'M. , Roth E. P / 9 1 . (FRANCE). 3rd Geneva Conf. 1964. (CEA-R-2G46)

135. STUDIES ON THE PRODUCTION OF HEAVY WATER AT J. E. N. P/49G. Alvarez J . , Gispert M. , Maria A. Otero J. L . , Rojas J. L. 3rd UN Geneva Conf. 1964.

136. . PRODUCTION OF HEAVY WATER. Roth E . , Rostaing M. Genie Atomiquc Vol. V. 1965. (p. 317-49)

137. CALCULATIONS OF THE DUAL TEMPERATURE SEPARATION OF ISOTOPES BY EFFECTIVE CONCENTRATION METHOD. Filippov G. G. ,Sakodynskii K. I . , Zelvenskii Ya. D. Khim. Prom. 1, 10-14, 1965. (In Russian)

138. A REVIEW OF HEAVY WATER PRODUCTION PROCESSES. Rae H.K. (AECL, Chalk River, Ont. CANADA). AECL-2503, 1965.

139. PRODUCTION OF HEAVY WATER. Ice C. PI. Research Materials Coordination and Planning Meeting, Nov. 14-J 5, 19G3. ORNL-TM-1047. 1965.

92

j.40. METHODS OF SEPARATING STABLE ISOTOPES. I. -VI. Vasari! Gli. MLM-129G. Sept. 1965. (English t ranslat ion)

141. MULTISTAGE SEPARATION PROCESSES. I. IDEAL AND SQUARED OFF CASCADES. II. THERMODYNAMIC E F FICIENCY OF SEPARATION PROCESSES. P ra t t I-I.' R. Univ. of Madras 1966.Indian Chem. Eng. 8, 6 0-82, 19GG.

142. CHEMICAL EXCHANGE PROCESSES FOR HEAVY WATER. Rao IF. K. AECL-2555. 19G6.

143. INFORMATION ON HEAVY WATER PRODUCTION. Pcculea M. , Sampalcanu L. IFA Report , Buchares t , Jan . 19GG. (Unpublished)

144. THE PRODUCTION AND THE APPLICATIONS OF STABLE ISOTOPES. Vasaru Gli. IFA Report , Buchares t , 15-3G, 19GG.

145. A REVIEW OF THE SEPARATION OF STABLE ISOTOPES. Gverdis i te l i I. G. Abh. Deut. Akad. Wiss . Ber l in , Kl . Math. Phys . Tech. 1, 79-85, 19G7.

146. THE HEAVY WATER PRODUCTION IN CANADA. Energ ie Nuclóairc 9, 343, 1967.

147. ADVANCES IN THE FIELD OF SEPARATING STABLE ISOTOPES BY CHEMICAL EXCHANGE. Cir ic M. , K r e l l E . , Kulicke P . , Missbach D . , Mühle K. ,Schuetze H . , Stiehl G . , Thiel S . , Weise G. , Wetzel K. Isotopenpraxis 3 ,21 -6 ,1967 . (In German)

93

148. CONSIDERATION O F PROCESSES IN SEPARATION COLUMNS F R O M THE POINT OF VIEW O F THE A P P R O A C H TO EQUILIBRIUM. M e r c c a V., P a l i b r o d a N . , Grecu E . K e r n e n e r g i e 10, 5 4 - 9 , 1967. (In German)

149. THE SEPARATION OF ISOTOPES IN D U A L - T E M P E R A T U R E SYSTEM WITH OPEN CIRCUITS. M e r c c a V . , Grecu E . , Olar iu A. Rev. Roura. P l iys . 12, 29-42 , 19C7.

150. CHEMICAL RESEARCH A T THE SWEDISH ATOMIC ENERGY COMPANY. Svenke E . (Aktiebolaget A t o m e n e r g i , S tockholm, SWEDEN). Svcnsk Kern. T i d s k r . 79, No. 2, 89 -93 , 19G7. (In Swedish)

151. A B R I E F SURVEY OF PROCESSES FOR HEAVY WATER PRODUCTION. Ryan R. K. ( A u s t r a l i a n Atomic E n e r g y C o m m i s s i o n R e s . E s t a b l . , L u c a s Heigh ts , AUSTRALIA). A E C / T M - 3 G 8 . F e b . 19G7.

152. SEPARATION O F ISOTOPES. S u m m a r y of the R e s u l t s of the D u a l - T e m p e r a t u r e P r o c e s s for Concen t ra t ing D e u t e r i u m by the Methy l -Ace ty lene and the PI2S Exchange Reac t ions with W a t e r . Goldfrank J . C. C U - 7 5 5 - 4 , P a p e r III C. 1967.

153.. COMPARISON OF ME TI IY LAC E T Y LENE AND I-I2S EXCHANGE WITH H 2 0 FOR CONCENTRATING DEUTERIUM*IN A DUAL T E M P E R A T U R E SYSTEM. Goldfrank J . C . C U - 7 5 5 - 5 , Sec t . III. Sept. 20, 19G8.

154. ON HEAVY WATER PRODUCTION IN ROMANIA. IFA Repor t , B u c h a r e s t , 19G7. (Unpublished)

94

155. PRESENT PROBLEMS OF HEAVY WATER PRODUCTION. Mihaila A . , Vasaru G. IFA Report , Buchares t , 1967. (Unpublished)

156. CONTINUOUS TECHNIQUES FOR THE SEPARATION OF STABLE ISOTOPES. Selcclri A. Isotoponpraxis , 4, 293-7, 1968. (In German)

157. HEAVY WATER PRODUCTION. Law C .A . Nuclear Eng. 13, 145, 510-2 ,1968.

158. PHYSICAL METHODS FOR THE SEPARATION OF ISOTOPES. Kokoh A. Rev. Chini. Miner. 5, 645-82,1968.

159. ORIENTATIVE STUDIES ON PROFILE AND EMPLACEMENT OF A HEAVY WATER PLANT. Manciulescu A. IPRAN Report IFA, Buchares t , 1968.

160. HEAVY WATER PRODUCTION IN ROMANIA. Mercea V. IFA Report , Buchares t , Oct. 1968. (Unpublished)

161. ISOTOPE SEPARATION PRACTICE. Bigeleisen J . Advan. Chem. S e r . N o . 89, 1-24, 1969.

162. HEAVY WATER. Malleroy A. Atomes 24, 265, 322-5 ,1969.

1G3. HEAVY WATER EXPERIENCE AT HALDEN. Wood J.' I . , Wullum T. Nucl. Eng. Int. 14, 338-42, 1969.

164. PRODUCTION OF HEAVY WATER. Status Repor t . Ayres J . A. (Batel le-Northwest , Richland, Nash. Pacific Northwest Lab. USA) BNL-884. Mar . 1969.

95

Ì65 . REVIEW OF HEAVY WATER PRODUCTION PROCESSES. Rae II. K. (Atomic Energy of Canada Ltd. .Cha lk River (Ontario)) . AECL-2503 . Aug. 1969.

1G6. REVIEW OF F U E L PROCESSING TECHNOLOGY PRESENTED AT THE 1964 GENEVA CONFERENCE. Gresky A. T. (ORNL) P r o g r . Nuc'l. Energy Sur . Il l 4, 3-34.1970.

1G7. HEAVY WATER PRODUCTION. A REVIEW OF PROCESSES. Lewins D. M. (Austra l ian Atomic Energy Commission^ R e s e a r c h Es tab l i shment , Lucas Heights) . AAEC/TM-562 . Sept. 1970.

16&. STUDIES OF HEAVY WATER PRODUCTION IN FRANCE. Roth E . . Rostaing M. (CEA. FRANCE). CNEN Symp. on the Technical and Economic Aspec t s of Heavy Wate r Product ion . Tur in . I taly. Sept. 30 - Oct. 1. 1970.

169. STRUCTURAL ACTION OF CHROM1A FOR INCREASING THE CATALYTIC PROPERTIES OF NIKEL IN THE HYDROGEN-HEAVY WATER ISOTOPIC EXCHANGE. Olar iu A. (Inst, of Nuclear P h y s i c s , Buchares t ) . Stud. C e r c e t . F i z . 22, 953-85. 1970. (In Rumanian)

170. VERSATILE HEAVY WATER. Swaroop J . (Bhabha Atomic Resea rch Cen t re , Bombay) . Vaigyanik 3, No. 1 .8-12. Mar . 1971. (In Hindi)

171. STUDIES O F PRODUCTION PROCESSES AND HEAVY WATER PLANTS USING THE FRENCH PROCESS. Roth E . , T r a o u r o u d e r R . , V i r a t e n e J . , Lefrancois B . P /607 (FRANCE) 4th Geneva Conf .1971.

1 7 2 . INDUSTRIAL PRODUCTION OF HEAVY WATER. Kortus J . , Zoch O. (Czech Atomic Energy Commiss ion , P r a g u e ) . Jad . Ene rg . 17, No. 9, 291-6 . Sep. 1971. (In Czech)

96

173. HEAVY WATER PRODUCTION.Lewins D . M. , Alfredson P . G. (Austral ian Atomic Energy Commiss ion , Coogee). At. Energy Aust . 15, No. 3, 2 - 1 1 , Ju l . 1972.

174. CHEMICAL PROCESS ENGINEERING. FLUORIDE PROCESS AS AN ADVANTAGEOUS PROCESS IN F U E L REPROCESSING. 7. CHEMICAL PROCESSES IN THE DEVELOPMENT OF NUCLEAR TECHNOLOGY. Lanius E. II. VDJ, Nachr". 2G, No. 14, 14, 1972. (In German)

175. PLANTS AND PROCESSES FOR THE PRODUCTION OF HEAVY WATER. Nitschkc E. Atomwirtschaft 18, No. 6, 274-80, June 1973. (In German)

97

B - PATENTS REVIEW (Breva tome , P a r i s )

The patents have been se lec ted from the files of Breva tome -Serv ice de Documentation - 44, Avenuo du Pres iden t Kennedy -75, P a r i s IGC (tal. 527. 07. 45) who is in possess ion of the full set of the mentioned documents and can furnish them on r eques t . B reva tome publishes fu r the rmore a nuclear patent magazine:

La ProprLété Indust r ie l le Nucléa i re - Atomic Pa ten t s A b s t r a c t s .

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Open to public inspection DA Germany F. R. Patents granted DB

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Patents BR U. S.S.R,

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(Information received as of .January 22,1971)

1

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99

BREVATOME/ DOCUMENTATION'

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Heavy water Production by Chemical Exchange H2S-HDO Fabrication d'eou lourdo par óchango chiciique H-S - HDG

1 - US 2 787 526 du 9 . 1 1 . 1 9 4 3 U . S . A . E . C .

"r-lethod of i s o t o p e c o n c e n t r a t i o n "

BP 845 501 4 . 1 0 . 1 9 4 4 S . P . E . V . A . C . K . CP 574 293 7 .10 .1944 A . E . C .

2 - US 2 776 263 du 1 6 . 0 4 . 1 9 4 5 U . S . A . E . C .

"Corrosion i n h i b i t o r s f o r deuter ium exchange process"

. 1 - US 2 741 543 du 2 2 . 0 5 . 1 9 4 5 U . S . A . E . C .

"Process f o r the product ion of deuter ium ox ide"

CP 558 985 2 6 . 0 4 . 1 9 4 6 A .E .C . BP 837 730 2 5 . 0 4 . 1 9 4 6 U .K .A .E .A .

4 - US 2 895 803 du 2 9 . 0 9 . 1 9 5 0 J . S . 5PEVACK

"Procède et i n s t a l h t i o n de c o n c e n t r a t i o n d ' i s o t o p e s "

BF 1 232 316 2B .05 .1957 BP 865 705 2 3 . 0 4 . 1 9 5 7 BP 865 706 2 3 . 0 4 . 1 9 5 7 BJ 36-13 808 9 . 0 5 . 1 9 5 7 BJ 37-11 655 9 . 0 5 . 1 9 5 7

DA 1 235 272 2 8 . 0 5 . 1 9 5 7 CP 612 0 8 7 1 4 . 0 8 . 1 9 5 7 CP 763 347 9 . 0 1 . 1 9 6 1 CP 780 298 9 .01 .1961

5 - US 2 954 279 du 2 3 . 0 2 . 1 9 5 4 RENSSELAER POLYTECHNIC INSTITUTE

"Method of manufactur ing heavy water"

BP 81 e 777 DA 1 047 753

18 .06 .1956 2 0 . 0 6 . 1 9 5 6

6 - US 2 952 525 du 2 0 . 1 0 . 1 9 5 5 RENSSELAER POLYTECHNIC INSTITUTE

"Procède de f a b r i c a t i o n d'eau l o u r d e "

BF 1 157 971 11 .09 .1956 DA 1 050 319 2 1 . 0 6 . 1 9 5 6 BP 818 421 1 8 . 0 7 . 1 9 5 6

du 1 2 . 0 1 . 1 9 5 7 C E . A . 7 - BF 1 164 729

"• Per fect ionnement aux procédés d1 enr ich issement i s o t o p i q u e par échange b i therme " .

BS 347 172 CP 592 261 BP 870 036 DA 1 080 073 BJ 35 B488

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100

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PF 1 164 750 du 15 .01 .1957 C E . A .

" P e r f ect ionnei i ten t nux procèder, d ' e n r i c h i s s c m e n t i s o t o p i q u e por échange b i t h e n n e " .

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CP 600 007 16 .01 .1958 BI 583 609 16.01.1958 BS 34B 956 1 4 . 0 1 . 1 9 5 8 BJ 35-0490 22.01.195B BP 079 4 6 7 2 1 . 0 1 . 1 9 5 0 SP 2 0 0 5 2 7 2 3 . 0 1 . 1 9 5 0 BB 564 177 2 2 . 0 1 . 1 9 5 0 IP 11 025 17.Ü1.195B MP 126 776 2 1 . 0 1 . 1 9 5 0 BLux 35 704 1 1 . 0 1 . 1 9 5 0 DA 1 206 390 2 2 . 0 1 . 1 9 5 0 BE 239 6 3 9 1 0 . 0 1 . 1 9 5 0

in - BF 1 169 140 du 5 .03 .1957 L 'AIR LIQUIDE

"Procède d'enrichissement d'un compose chimique en un element".

DA 1 055 507 1 .03.1950 BI 5Ü8 027 4.03.1950

1 1 - BF 1 175 094 du 6.06.1957 C.E.A.

"Perfectiunnement aux procédés d'cnrichissement isotopique par échange bitherme"•

19. - BF 1 170 661 du 5 . 0 7 . 1 9 5 7 S t é D'ETUÜES POUR L 'OBTENTIOtJ DU DEUTERIUM

"Perfectionnement au procede de refroidissement d'un gaz dans un échange isotopique bitherme".

BI 591 579 19.06.195D IP 11 450 15.06 .1950 5P 219 562 4 .07 .1950 DA 1 260111 2 .07 .1950

13 - DA 1 064 919 d u ? . 1 0 . 1 9 5 7 PINTSCH DAI1AG A . G .

"Verfahren zur Iso topenanreicherunq d^rch zwei temperatur - Stoffaustausche

14 - 5PD 1 169 du 7.02.1950 ALLMANNA SVENSKA ELEKTRISKA A.D.

"Method and means for heat exchange of gases".

CP 630 951 31.01.1959 DA 1 137 421 4.02.1959

15- BP 067 840 du 10.03.1950 CONSTRUCTORS JOHN BROWN Ltd. &. N.W. R0BERT5 "Improvements in or relating tD the concentration of deuterium".

101

BREVATOME / DOCUMENTATION

R 1910

16- 5PD 3 665 du 16.I LMANNA 5VEN5KA ELEKTRISKA A.B.

"Procède pour le refroiu d'un gaz en circulation dans une installation .pour l'enricl .cement de l'oau en eau lourde".

BF'1 221 479 6.04.1959 CP 616 04B 1.04.1959 DA 1 255 096 14.04.1959

17- BF 1 207 117 du 1.0B.1958 NORSK HYDRO-ELEKTRISK KVAELSTOF AKTIESELSKAB

"Procède et installation pour la fabrication d'oxyde de deuterium".

18- US 3 142 540 du 25.06.1959 J.5. SPEVACK

"Apparatus for dual temperature exchange".

19- DA 1 193 4B0 du 26.0e. 1959 K. SCHOE.NEHANN J. CONNEMANN

'"Verfahren zum Isotopenaustauach nach dem Heiss-Ka^lt-Verfahren".

20- DA 1 193 4B1 du 5.03.1960 K. SCHOENEMANN J. CONNEMANN

"Procède d'échange thernique pour la separation d'isotopes selon le procède d'échange chaud-froid".

BF'1 2B3 48C 4.03.1961 BB 61B 750 B.06.1962 BP 979 320 20.05.1962

2i- CP 727 029 du 11.03.1963 DOW CHEhlCAL Co.

"Process for istope concentration".

BF 1 463 916 15.10.1965

22- CP 7E5 690 di. 31.08.1963 CANADIAN GENERAL ELECTRIC Co.

"Dual temperature isotope concentration process".

23- BF 1 3S4 692 du 15.11.1963 CE.A.

"Installation perfectionnée pour la production d'eau lourde".

BB 654 957 2B.10.1964 CP 766 15B 14.11.1964 BP 1 050 125 13.11.1964 BS 423 730 26.10.1964

US 3 431 0e0 13.11.1964

24- BF 1 409 660 du 22.07.1964 CE.A.

"Systeme de recuperation de chalélir pour installation de production d'eau lourde par le procède d'échange isotopique bitherme".

CP 738 B67 B.07.1965 BB 665 147 9.06.1965 B5 433 209 B.06.1965 US 3 3B6 502 B.07.1965 BP 1 IIB 966 13.07.1965 DA 1 542 650 9.07.1965

25- USD 457 359 du 20.05.1965 ESSO RESEARCH L ENG.-Co. "Deuterium concentration process and apparatus".

CP e03 445 6.05.1966

102

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R 1910

9R- U5 3 437 567 du 2B. 12.1965 LUIit.US Co.

"Procède perfectionné pour récupérer l'hydrogène sulfuré dans la production d'eau lourde".

BF 1 52B 639 20.12-1966 CP 796 OBé 27.12.1966

37- U5 3 411 884 du 11.04.1967 U.5.A.E.C.

"Process for concentrating heavy water".

CP 812 696 21.06.1967

28- USD 721 674 du 16.04.196B U.S.A.E.C.

"Perf ectionnen.ents aux procédéc d'échange d'isotopes à deux .ter.-.pératures".

BF 2 010 461 15.04.1969 OS 1 916 574 1.04.196t

29- USD 721 675 du 16.Ü4.1968 U.S.A.E.C. "Perfectionnemünts aux procédés d'échange d'isotopes à deux temperatures".

BF 2 007 461 15.04.1969 C5 1 916 573 1.04.1969

3(1- U5D 721 676 du 16.U4.196E U.S.A.E.C.

"Perf ectionnemen ts aux procédés d'échange d'isotopes à deux tei.-.pératurcs".

BF 2 00: 459 14.04.1569 Do 1 916 570 1.04.1569'

31- CPD 31 19B du 30.09.1568 CANADIAN GENERAL ELECTRIC Cy Ltd. "Echangeur à tour étagée notamnicnt destine à lu production d'eau lourde".

BF 2 019 256 30.09.1969 OS 1 949 3E7 30.C9.1569

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103


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Heavy water Production by Chemical Exchange NH3-HD B.2 F a b r i c a t i o n d ' eau lou rde par échange chimique NU- - HD

1 - US 2 676 E75 du 16 .06 .1942 U.S .A .E .C.

" C a t a l y t i c appa ra tus f o r i s o t o p e exchange"

CP 519 O i l 12 .06 .1943

ü - U 5 2 650 379 du 2 1 . 1 1 . 1 942 I 1 . 5 .A .E .C .

"Proceus for production of d .utc oxide a3 a source of deuterium".

BP PGü 73Ü 11 .11 .1943 I'.K.A. CP. 53Ü 34 3 9.11 .154 3 U.ii.A. .C.

3 - US 2 787 526 du. 5. 11.1943 U.S.A.E.C.

"tfethod of isotope concentration",

BP C45 501 4.1c'. 1944 S. P.E.V. A .C. K. CP 574 293 7.10.154.1 A.E.'C.

4 - BP L07 SÜ3 du 4.C5.1956 COSTAR'- JCHfo BRUV.'N Ltd.

"PerfectionnEraunts relatifs ä un procède d'cxtrcction du deuterium de gaz renf eri;, nt de l'hydrogàne".

BF 1 174 545 3.05.1557 DA 1 051 092 4.U5.1957 CP 619 092 4.C5.1957

5 - DA 1 030 E1C du 16.06.1556 F. U.H.D.E. Gnbh.

"Verfahren zur Gewinnung von nn Deuterium angereicherter,) VJassEX zw. Wasserstoff • aiy 'jzazcr".

6 - BP G69 413 du 4.07.1956 U.K.A.E.A.

BF BI CP BB

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DP B9 558 MP 92 998 BJ 39-11 753

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"Perfectionnements concernant la pxoduction d'eau lourde".

BF 1 1P0 420 31.07.1957 BB 55'J 165 1 .08.1957 i 50J 42P 29.07.1957 D 1 129 13L 29.07.1957

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R . DA 1 036 223 du 17.00.1956 F. UHDE Grnbh

"Procède d'enrichiscement ou d'obtcntion d'eau lourde ou cours de la aynthèsa de l'ammoniac ovec échange d'isotopcs entre l'anmoniac et 1'hydrogène".

3F 1 100 973 G.06.1957 BP B70 452 7.06.1557 US 2 997 365 13.Oe.1957 EJ 39-5 912 12.00.1957

a- 3F 1 169 140 du 5.03.1957 L'AIR LIQUIDE

"Procède d' enrichissement d*un compose chimique en un element".

DA 1 055 507 1.03.1950 BI 568 027 4.03.195B

10 - BP G67 846 du 10.03/1958 CONSTRUCTORS JOHN BROWN Ltd. & N.W.ROBERTS. "Improvements in or relating to the concentration of Deuterium".

11 - ÜP_ du 14.G3.1958 OSTERREICHISCHE STICKSTOFFWERKE A.G.

"Procede de concentration du deuterium dans l'hydxogène ou 1'ammoniac".

3F 1 224 376 12.03.1559 BP 847 504 16.03.1959 DA 1 155 228 5.03.1959 LENTIA.

12 - DA 1 120 431 du 13.00.1956 F. UHDE Gobh

"Procède d'enrichissement d'eau ou d'h^drogène en deuterium, dans la synthèse de 1'ammoniac".

BF 1 237 972 13.06.1959 BP 092 067 13.08.1959 BB 561 674 13.06.1959

13 - BF 1 209 633 du 22.OB.1958 C.E.A.

"Perfectionnement aux méthodes de soutirage dans les procédés d'enrichissement isotopique pax échange bitherr.ie".

BS 359 120 18.08.1959 BP 920 227 10.08.1959 BB 581 756 17.08.1959 BLux 37 561 18.00.1959 CP 630 236 18.06.1959 IP 12 886 18.08.1959 BI 614 303 7.08.1959

14- BF 1 219 270 du 13.12.1958 HOUILLERES DU BASSIN DU NORD ET DU PAS-de-CALAIS

"Perfectionnements aux cetalyseuxs de polyméxisation et d'échange".

BP 925 923 11.12.1959 BJ 37-7 735 14.12.1959 CP 637 770 11.12.1959 US 3 133 793 10.12.1959 BB 585 501 9.12.1959 BI 621 772 12.12.1959 DA 1 124 694 11.12.1959 B5 411 356 11.12.1959

BND 246 367 12.12.1959

http://13.Oe.1957

105


R 1910

15- B5 3B3 939 du 13.03.1959 5UL2ER

"Fabrication d'hydrogène enrichi en deuterium, et pr'oduction consecutive d'eau lourde".

BF 1 249 06B 23.02.1960 BP 903 367 9.03.1960 BND 237 B67 7.04.1959

in- BF 1 237 166 du B.06.1959 CE.A.

"Perfectionnement aux procédés de preparation d'eeu lourdc par échange isotopique monotherme ammoniac et hydrogène".

CP 644 705 31.05.1960 NP 105 454 30.05'.196O BB 591 019 9.05.1960 BS 400 385 16.05.1960 05 1 417 759 3.06.1960 IP 13 933 25.05.1960 BP 952 335 25.05.1960 US 3 233 971 6.06.1960

17- BF 1 241 260 du 6.08.1959 CE.A. fi. H0UILLERES DU BASSIN DU NORD ET DU PA5-DE-CALAIS

"Perfectionnements aux procédés de recuperation des catalyseurs dans les processus d'enrichiaseraent en deuterium d'un compose hydrogéné".

BLux 39 032 1.0E.1960 BND 254 625 6.08.1960 DA 1 142 344 3.0E.1960 B5 397 610 30.07.1960 BJ 37-9 690 5.0B.196D BI . 636 9B4 6.0B.1960 CP 656 471 5.08.I960 US 3 163 589 2.0B.1960 BB 593 655 1.0B.I960 DP 96 640 6.OB.1960 BP 950 200 4.OB.1960

18- BF 1 351 353 du 2B.OB.1959 C.E.A. 1 HOUILLERES DU BASSIN DU NORD ET DU PA5-DE-CALAI5

"Procède de saturation par contact direct d'une phase gazeuse par de la v/apeur d'un liquide charge en adjuvant non non v/olatif".

19

20

CP BB BE ILux BP BJ DP

BF

BE BI

BF

656 855 593 857

. 260 836 -' 39 063 951 791

38-18 650 96 109

1 243 843

14.09.1960 5.0B.1960

13.08.1960 6. OB.1960 25.OB.1960 29.OB.1960 25.08.1960

du 5.09.

"Perfectionnement aux p par échanc

260 791 626 119

1 243 945

e bitherme

3.09.1960 2.09.1960

du 11.09

US 3 098 020 NP 104 396 OS 1 417 782 B5 405 244 US 3 214 243 BI 636 154

BND 255 253

1959 C.E.A.

11 12 29 6 11 17 27

rocédés d'enrichissement NH3-H2».

BLux 39 119 BB 594 323

1959 CE.A.

.31 '29

OB.1960 OB.1960 OB.1960 08.1960 OB.1960 OB.1960 OB.1960

isotopi

.08.1960

.OB.1960

"Perfectionnement aux procédés d'enrichissement isotopique par échange bitherme à Systeme de contact d"épuisement".

BE BI

260 827 626 119

6.09.1960-2.09.1960

BLux BB

39 132 594 524

2.09.1960 29.OB.1960

106


R 1910

21 - US. °u 1.10.1959 NORSK HYDRO-ELEKTRISK KVAELSTOFAKTIESELSK'A

"Process for the concentration of heavy water".

BP 867 736 3.12.1959

22 - BPD 33 906 du 6.10.1959 U.K.A.E.A.

"Procède d'échange thermiquc".

BF 1 268 977 4.10.1960

23 - DA 1 145 5e5 du 18.11.1959 BADISCHE ANILIN &. SODA-FABRIK A.G. "Procède pour la production d'hydrogène lourd".

BF 1 273 612 14.11.1960 US 3 100 138 15.11.1960 BND 258 003 16.11.1960 BS 40,7 963 21.10.1960

24 - BP 896 269 des 4.02. et 22.09.1960 U.K.A.E.A.

"Procède de concentration du deutériun".

DA 1 152 999 4.02.1961 CP 653 188 4.02.1961 SP 192 252 3.02.1961 BF 1 281 601 4.02.1961 BI 632 580 3.01.1961 US 3 377 135 6-02.1961 BS 401 931 4.02.1961 NP 100 74e 3.02-1961

25 - DA 1 171 398 du 11.03.1960 F. UHDE Gmbh

"Method of recycling a catalyst used for isotope exchange".

CP 672 392 22.01.1962

26 - DA 1 171 399 du 11.03.1960 F. UHDE Gmbh "Method of recycling a catalyst used for isotope exchange".

CP 672 s'91 22.1.1962

27 - BF 1 269 472 du 14.12.1960 C.E.A..HOUILLERES DU BASSIN DU NORD ET DU PAS-de-CALAIS., Cie de CONSTRUCTION HECA-NIQUE, PROCEDE SULZER ET L'AIR LIQUIDE

" Perfectionnement aux procédès de preparation d'eau lourde par échange isotopique monotherme NH3 - H_".

BLux 40 923 7.12.1961 BB 611 155 5.12.1961 DA 1 168 395 12.12.1961 US 3 239 310 7.12.1961

BND 272 357 8.12.1961 NP 105 455 5.12.1961 OP 231 958 13.12.1961 BS 412 825 5.12.1961 CP 701 779 8.12.1961 BI 660 563 13.12.1961 BP 9G5 782 6.12.1961

28 - DA 1 200 789 du 2X01.1961 F. UHDE Gmbh

"Procède pour l'obtention d'isotopes, à deux ou plusieurs Stades".

BF 1 314 170 24.01.1962 OP 230 329 23.01.1962 BP 999 618 .24.01.1962 BI 663 166 23.01.1962 US 3 503 710 17.01.1962

107


R 1910

29 - I5P 15 941 du 25 .08 .1vul F. KLEIN et K. BAR-ELI

"Precedes d'enrichissement du deuterium".

BF 1 331 779 CP 719 200

30 - DA 1 198 799

17.08.1962 8.08.1962

BP 994 303 US 3 457 041

10.08.1962 11.U5.1967

du 16.02.1963 F.UHDE Gmbh

"Verfahren zur Verminderung der Deuterium - veri iste beim Isotopen ouBtausch mit Flüssigkeitskreislauf".

31 - BF 1 3B3 743 du 13.03.1963 C.E.A., HOUILEERE'J DU BASSIM DU NORD ET DU PA5-DE-CALAIS, CUMPANIE DU CONSTRUCT ION MECANiqUE - PRUCEDEb 5ULZER ET L'AIR LIGUIH

"Perfectionnements au procède d'échange isotopique ammoniac -hydrogèi «_•" .

DA 1 253 683 BB 645 204 CP 780 2B8 BP 1 023 859 BS 426 750 NP 107 115

6.03.1964 13.03.1964 13.03.1964 12.03.1964 12.03.1964 7.03.1564

0P 245 532 BLux 45 65U US 3 342 550 IP 20 940

BND 6 402 667

12.03.19 64 13.03.1964 26.03.1964 9.03.1964 13.03.1964

32 - BF 1 373 686 du 1U.U6.1963 C.E.A., HOUILLERE . DU BAbSlN DU MORD ET !)U PAS-DE-CALM'i, Ci" le CUN5TRUCTIUN f-ECAIII-ÜUE - PR0CEDE5 SULZ'JR et 1 «AIR LIQUIDE

" Plateau perfectionné pour colcnnes de contact rjdz-liquide" .

OS 1 442 718 BB 648 900 CP 778 760

BND 6 406 508 BS • 426 729

9.06.1964 5.06.1964

'10.06.1964 9.06.1964 9.06.1964

OP 254 140 ' 1Ü.U6.1964 BP 1 063 443 9.G6.1964 US 3 394 927 1U.06.1964 NP 111 900 8.06.1964

33 - PAP U 10 B3B du 24.06.1964 F. UHDE Gmbh S. Ges, für KERNFORSCHUNG mbh

"Procède pour l'épuration de l'hydrogène ou du mélange d'azote et d'hydrogène av/ant son introduction dans une installation destinée à la concentration du deu+érium".

BF 1 44B 234 CP 773 480

23.06.1965 23.06.1965

BP 1 105 498 23.06.1965

34 BF 1 4Q9 860 du 22.07.1964. C.E.A.

"Systeme de recuperation de chaleur pour installation de productiun d'eau lourde par le procède d'échange isotopique bitherriiu".

CP 73B 867 BS 433 209 BP 1 118 966

35

9.07.1965 8.06.1965 13.07.196 5

BF 1 433 444 . du 15.02.1965

BB 665 147 US 3 386 502 DA 1 542 650

F. UHDE Gmbh

9.06.1965 B.07.1965 9.07.1965

"Procède permettant de diminuer les pertes de deuterium lore de la production de D_0".

.../...

108


R 1910

36 - BP 1 066 470 du 1 0 . 0 3 . e t 1 0 . 1 2 . 1 9 6 5 U . K . A . E . A .

"P rocède pour l a f a b r i c a t i o n de m a t i è r e s e n r i c h i e s en d e u t e r i u m " .

BF 1 476 887 9 . 0 3 . 1 9 6 6 US 3 437 442 7 . 0 3 . 1 9 6 6 CP 782 9B7 7 . 0 3 . 1 9 6 6 05 1 567 871 9 . 0 3 . 1 9 6 6

37 - BF 1 450 643 du 3 0 . 0 6 . 1 9 6 5 C E . A .

"P rocède d ' e n r i c h i s s o m e n t i s o t o p i q u e par échange b i t h e r m e i inuiuninr -h y d r o g è n e " .

BP 1-084 940 2 7 . 0 6 . 1 9 6 6 BB 681 121 1 6 . 0 5 . 1 9 6 6 SP 225 302 2 9 . 0 6 . 1 9 6 6 US 3 464 789 2 8 . 0 6 . 1 9 6 6 OP 262 233 1 3 . 0 6 . 1 9 6 6 CP 813 262 2 4 . 0 6 . 1 9 6 6 BS 454 811 1 8 . 0 5 . 1 9 6 6 DA 1 567 417 1 5 . 0 6 . 1 9 6 6

38 - BF 1 462 290 du 2 4 . 0 9 . 1 9 6 5 C E . A .

"P rocède d ' e n r i c h i s s e m e n t i s o t o p i q u e de 1 ' h y d r o g è n e " .

BP 1 125 670 2 1 . 0 9 . 1 9 6 6 BS 455 720 2 4 . 0 0 . 1 9 6 6 BB 685 905 2 4 . 0 8 . 1 9 6 6

39 - BP 1 100 991 du 7 . 0 1 . 1 9 6 6 U . K . A . E . A .

"Procède et appareil de production de matières enrichies en deuterium".

BF 1 507 428 3.01.1967 U5 3 505 016 4.01.1967

40 - BF 1 494 264 du 27.07.1966 C.E.A., H0UILLERES DU BASSIN DU l'URD ET DU PA5- de - CALAIS, L'AIR LIQUIDE t= t Cid dt. CONSTRUCTION MECANIQÜE, PROCEDES5ÙLZER

"Procède amélioré d'échange isotopique pour 1'utilisation d'un cycle d'échange monothern.e ammoniac-hydrogène" .

BB 700 925 5.07.1967 BLux 54 176 26.07.1967 BS 464 866 26.07.1967 US 3 479 140 21.07.1967 BND 6 709 695 17.07.1967 NP 116 905 6.07.1967 BP 1 149 729 27.07.1967 CP 820 786 26.07.1967

41 - BF 1 515 B90 du 16.08.1966 CE.A., HOUILLERES DU BASSIN DU NORD ET DU PAS-DE-CALAIS, L'AIR LIQUIDE et Cie DE CONSTRUCTION liECANIQUE, PROCEDES 5ULZER

"Procède amélioré pour la realisation d';s échsnges isotopiques suivent le procède monotherme".

BB 700 892 4.07.1967 US 3 471 257 28.07.1967 DP 1 150 405 18.07.1967 NP 116 904 6.07.1967 BLux 54 046 6.07.1967

42 - BF 1 509 0B9 du 17.10.1966 CE.A., HOUILLERES DU BASSIN DU NORD ET DU PAS-DE-CALAIS, L'AIR LIQUIDE et tie DE CONSTRUCTION MECANIQUE, PROCEDES SULZER

"Amelioration du procède monotherme d'échange isotopique entro ammoniac et deuterium".

BLux 54 046 6.07.1967 US 3 471 257 28.07.1967

.../...

109


R 1910

43- BF 1 522 400 du 14.03.1967 C.E.A.

"Plateau a plaques perforéos pour colonnes u'uchanges".

44- BF 1 523 472 du 24.03.1967 C.E.A.

"Procède et dispositif d'échantillonnage d'une solution liquide sous prsasion".

45-Bf ft 92 590 / 1 494 264

du 15.06.1967 CiE.A,, H0UILLERES DU BASSIN DU NuRD ET PA5-DE-CALAIS, L'AIR LIQUIDE et Cie DE CONSTRUCTION t'ECANIQUE, PRUCEDES SULZE

"Procède amélioró d'échange isotopique pour 1'utilisatiun d'un cycle d'échange monotherme ammoniac-hydrogène".

I R - CP D 1 5B6 du 3.10.1967 A.E.C. Ltd.

"Colonne à plateaux à courants paralleles pcur échanije entre liquide^ et gaz".

BF 1 5B7 797 3.10.196B 0b 1 B00 990 3.10.196B BND 6 B14 162 3.10.1968

4"? - B5D 6 671 du B.05.1968 SULZER

"Procède et appareil de traiteraent d'ammoniac deutérié".

BF 2 008 061 7.05.1969 BB 732 350 30.04.1969

110


R 1910

Heavy water Product ion by Chemica l .Exchange H2O-HD B t 3 P r o d u c t i o n d ' e a u l o u r d e pBr /échange ch i rn ique H_0 - HD

1 - Ql du 6 . 1 2 . 1 9 3 4 F. HANSGIRG

" Improvemen ts i n o r r e l a t i n g t o a p rocess f o r t h e p r o d u c t i o n o f w a t e r e n r i c h e d w i t h heavy w a t e r " .

BP 462 191 4 . 1 1 . 1 9 3 5 DA 674 965 1 2 . 0 3 . 1 9 3 5 US 2 134 249 3 . 1 2 . 1 9 3 5

2 - Of? du 2 3 . 1 2 . 1 9 3 5 F. HANSGIRG

" Improvemen ts i n o r r e l a t i n g t o t h e p r o d u c t i o n o f heavy w a t e r " .

BP 4B7 066 2 2 . 1 2 . 1 9 3 6 US 2 156 851 1 0 . 1 1 . 1 9 3 6

3 - US 2 6B9 7B2 du 2 7 . 0 2 . 1 9 4 2 U . S . A . E . C .

" P r o d u c t i o n o f heavy w a t e r " .

BP '795 920 1 3 . 0 3 . 1 9 4 3 U . K . A . E . A . CP 539 823 1 9 . 0 2 . 1 9 4 3 A . E . C .

4 - US 2 676 875 du 1 6 . 0 6 . 1 9 4 2 U . S . A . E . C .

" C a t a l y t i c a p p a r a t u s f o r i s o t o p e e x c h a n g e " .

CP 519 811 1 2 . 0 6 . 1 9 4 3

5 - US 2 690 379 du 2 1 . 1 1 . 1 9 4 2 U . S . A . E . C .

" P r o c e s s f o r p r o d u c t i o n uT d e u t e r i u m o x i d e as a sou rce o f d e u t e r i u m " .

BP 800 730 1 1 . 1 1 . 1 9 4 3 U . K . A . E . A . CP 530 343 9 . 1 1 . 1 9 4 3

fi - US 2 787 526 U . S . A . E . C . du 9 . 1 1 . 1 9 4 3

"Method o f i s o t o p e c o n c e n t r a t i o n " .

BP 845 501 4 . 1 0 . 1 9 4 4 S . P . E . V . A . C . K . CP 574 293 7 . 1 0 . 1 9 4 4 A . E . C .

7 - US 2 690 380 du 4 . 0 5 . 1 9 4 4 U . S . A . E . C .

"Production of deuterium oxide".

CP 520 374 4.05.1945 BP 748 991 3.05.1945

8 - US 2 677 668 du 11.01.1945 U.S.A.CC.

"Stabilization of reduced metal catnl st".

CP 514 229 11A01.1946

Ill


R 1910

q - US 2 677 6P9 du 11.01.1945 U.S.A.E.C.

"Stepwise stabilization of raduced metal catalysts",

CP 514 230 11.01.1946

10 - »5 2 851 427 du 22.03.1945 U.S.A.E.C.

"Method of purifying catslysts".

11 - BI 493 492 du 31 :07.1952 C.I.S.E.

"Procède pour enrichir l'eau en deuterium".

BF 1 0B6 502 30.07.1953 BB 521 B32 30.07.1953

12 - DA 1 003 690 du 8.09.1954 E.W.A. BECKER

"Procède d'obtention d'eau ou d'hydrogène enrichis en deuterium".

BF 1 138 776 26.08.1955 US 3 087 791 1.09.1955 BP 803 274 25.06.1955 BS 341 481 3.08.1955 BN 108 803 17.OB.1955 CP 616 561 6.09.1955

13 - B_S du 3.08.1955 E.W.A. BECKER

"Verfahren zur Gewinnung von mit Dauterium angereichertem Wasser oder WasBarstoff".

DA 1 052 960 29.10.1955

u - JJ£ du 18.11.1955 N0R5K HYDRO-ELEKTRISK KVAELSTOFAKTIESELSKAB

"Procède d'extraction du deuterium è partir d'hydrogène mélange à d'autree gaz".

BF 1 179 985 19.11.1956

15 - US 2 967 0B9 du 25.11.1955 'H0UDRY PROCESS CORP.

"Process for making heavy wator".

is - DA 1 032 233 du 30.04.1956 E.W.A. BECKER

"Procède d'obtention d'eau ou d1hydrogens enrichis en deuterium".

BFA 71 295/1 138 776 26.4.1V57 US 2 927 003 29.04.1957 BP 834 306 30.04.1957

17 - DA 1 131 191 du 16.06.1956 F. UHDE Gmbh

PA 1 135 S65 23.01.1957 DA 1 147 203 .9.08.1956

" Procèdi de fabr icat ion d'eau,ou d'hydrogène,anrichia en deutèr i um

BF 1 179 427 14.06.1957 CP 585 604 21.06.1957 BP B64 026 17.06.1957 BB 558 414 15.06.1957

. . . / .

112

BREVATDME / DOCUMENTATION

R 1910

18- DP 869 413 du 4.07.1956 U.K.A.E.A.

"Procède de production d'eau lourde"

BF 1 17B 627 3.07.1957 BB 550 926 3.07.TJ57 BI 574 307 3.07.1957 CP 592 366 27.06. TJ57 NP 92 998 26.06.1957 DP H9 558 3.07.1957

BJ 39 11 753 4.07.1957

19- BP C69 414 du 4.07.1956 U.K.A.E.A,

"Appareil de production d'eau lourde".

BF 1 182 332 3.07.1957 BB 558 927 3.07.1957 BE 236 348 3.07.1957 DP 1 121 593 3.07.1957 NP 105 935 4.07.1957

20- DA 1 066 555 du 20.10.1956 RUHRCHEMIE A.G. 8. 5TEINBDHLEN-ELEKTRIZITAET

"Process for the production of heavy water".

BP B65 411 8.10.1957 CP 583 841 16.10.1957 B5 401 932 2.10.1957

? 1 - BP B81 941 du 9.11.1956 U.K.A.E.A.

"Procédés d'hydratation et de deshydratation de gaz".

BF 1 105 920 8.11.1957 CP 574 226 4.11.1957 U5 3 019 61.0 6.11.1957 BB 562 184 6.11.1957 DP 1 056 634 D.11.1957

99- DA 1 038 542 du B.12.1956 E.W.A. BECKER

"Process for the production of water or hydrogen having an increa -.ed deuterium content".

US 3 036-891 4.12.1957 BP 824 820 4.12.1957 BI 602 461 29.11.1957

23- BF 1 169 140 du 5.03.1957 AIR LIQUIDE

"Procède d1enrichissement d'un compose chimique en un element".

BP 1 055 507 1.03.1958 BI 588 027 4.03.1958

24- BP 877 089 du 24.04.1957 .U.K.A.E.A.

"Appareil d'échonge catalytique".

BF 1 195 063 24.04.1958 CP 5BB 262 18.04.1958 BI 588 531 22.04.1958 BB 566 990 21.04.1958

.../...

I1J

BREVATOHE / DOCUMENTATION

R 1910

25- BP B69 415 du 24.04.1957 U.K.A.E.A.

•"Procède de production d'eou lourde".

BFA 73 511 / 1 178 627 24.D4.195B

CP 592 367 1B.04.195B BB 567 DB2 24.04.1958 US 3 336 113 24.04.195B NP 97 607 24.04.195B

26 - DA 1 046 590 du 7.06.1957 DEGUSSA

"Procède de traitcment de catalysours dans des dispositifs d'échange pour 1•enrichissement de deuterium".

BF 1 196 731 7.06.195B BI 591 7B3 4.06.195B BP 889 B2B 9.06.1958

'il- DA D U 4 471 du 19.OB.1957 F. UHDE Gmbh

"Procède et dispositif pour la reduction de la concentration de deuterium dans l'humidité résiduairo imprégnant un catalyseur pulwérulent après filtration d'une suspension du catalyseur sur le g3teau de filtration".

BF 1 201 757 19.OB.1958 US 2 980 420 19.08.1958 BI 593 604 1B.OB.1958

28- DA 1 074 555 du 20.01.1958 V. BAYERL

"Procède de production de deuterium".

BF 1 213 247 du BP B96 021 DWP 19 225

90- DA 1 0B2 BB4 du 11.10.195B RUHRCHEMIE A.G.

"Process for the production of heavy water".

BP 930 606 30.09.1959 BB 503 407 9.10.1959

30- DA 1 076 093 du 11.10.195B DEGUSSA

"Verfahren zur Anreicherung von Deuterium in Wasser oder Wasserstoff".

31 - DA 1 200 261 du 22.11.195B METALLGESELLSCHAFT A.G.

"Verfahren zur Anreicherung von .Deuterium".

32- PAP 30 525 du 24.04 &. 1.1.06 1?" PEGUSSA

"Procède pour 1'enrichissement de 1 Vau ou de l'hydrogène en deuterium, e installation pour sa mise en oeuvre'

BF 1 255 667 25.04.1960 BB 509 902 19.04.1960 CP 223 170 22.04.1960 BI 617 405 23.04.1960 BN 250 700 22.04.1960

9 . D I . 1 9 5 9 13.01 .1959 2 2 . 1 2 . 1 9 5 7

CP BI

619 681 605 202

13 .01 .1959 9 .01 .1959

. . . / . . .

114


R 1910

33- BF 1 245 589 du 25.07.1959 OFFICE NATIONAL INDU5TRIEL DE L'AZOTE

"Catalyseurs destines à l'échange isotopique entr.e l'eau et l'hydrogène à haute temperature".

BP 929 653 13.07.1960 DB 593 203 22.07.1960 BN 253 147 22.06.1960

3d- DA 1 171 390 du 11.03.19ri3 F.UHDE Gmbh


CP 672 392 22.01.1962 • »

35- DA 1 171 399 du 11.03.1960 F. UHDE Gmbh


CP 672 391 22.01.1962

3P, - BF 1 278 246 du 6.12.1960 Veb Vakutronitk

"Procède de concentration de deuterium et de fabrication d'eau lourde".

DA 1 145 145 21.10.1960 DP 23 705 20.04.1960 CA 148 246 6.1-2.1960 BN 25B 064 17.11.1960 DP 98 686 1.11.196D

37- US 3 206 365 du 8.02.1963 50C0NY MOBIL OIL

"Production of heavy water".

38" DAD U 10 549 du 3.03.1964 F. UHDE Gmbh Ges.für Kernforschung m.b.H.

"Procède de regeneration de catalyseurs à base de métaux nobles empoison-nés par des oxydes inetalliques".

BF 1 425 833 1.03.1965

115

BREVATOME/ DOCUMENTATION

R 1910

Heavy water Production by Chemical Exchange: Equipment and o ther Processes j ; 4 F a b r i c a t i o n d 'eau l o u r d e par échange ch im ique : a p p a r e i l l a g e et

a u t r e s p rocédés .

oLhcr processes: a u t r e s procédés :

1 - US 2 690 3B1 du 15 .05 .1945 U .S .A .E .C .

" I s o t o p e exchange process f o r c o n c e n t r a t i n g d e u t e r i u m " .

2 - US 2 690 3e2 du 28 .05 .1945 U.S .A .E .C.

"Dua l t empera tu re i s o t o p e exchange p r o c e s s " .

CP 522 983 2 .05 .1946 BP 800 851 10.05.1946 equipment a p p a r e i l l a q e

3 - BSD 76 064 Ju 22 .07 .1959 SULZER

"Colonne de t r a n f e r t de rna t iè re p e r f e c t i o n n é e " .

BF 1 264 235 21 .07 .1960

4 - BSD 76 065 du 22.07.1959 SULZER

"Perfectionnements aux colonnes de transfert de matière".

BF 1 264 236 21.07.1960 BN 243 011 4.09.1959

5 - BS 372 645 du 29.10.1959 SULZER

"Separating devices and separating plant incorporating such devices".

BP 908 917 20.10.1960 DA 1 174 706 12.11.1959

6 - BSD 6 832 . du 15.06.1960 SULZER

"Apparatus for mass transfer between two phases".

BP 973 748 29.05.1961 BF 1 266 913 6.09.1960

7 - BSD 4 341 du 12.04.1961 SULZER

"Substance exchange columns".

BP 1 005 586 12.03.1962 BE 1 318 149 21.03.1962

8 - BSD 13 437 17.11.1961 SULZER

"Appareillage pour l'extraction des produits d'une colonne d'échange".

BF 1 '334 800 28.09.1962 BJ 39/18 003 4.10.1962

.../...

116


R 1910

9 - BSD 9 1BB/62 du 31 .07 .1962 SULZER

"Colonne pour l 'échange de substances".

BF 1 362 274 4 .07 .1963

1 0 - USD 241 494 du 3 .12 .1962 UNION CARBID&CORP.

"Cata lyseurs de r e a c t i o n chimique et son procède de p r e p a r a t i o n " .

BF 1 413 872 2 . 1 2 . 1 9 6 3 BB 640 629 20 .11 .1963 BP 1 074 129 25 .11 .1963

11 - BSD 15 547 du 19 .12 .1963 SULZER

"Colonne pour l 'échange de p r o d u i t s " .

BF 1 438 259 15 .12 .1964 DA 1 237 067 7.01.1964 BP 1 069 770 21 .12 .1964 CP 770 028 1 5 . 1 2 . 1 9 6 4

12 - BSD 11 527 du 16.OB.1967 SULZER

BSD 9 362/6B 24 .06 .1968 SULZER

"Garn i tu re pour colonne d'échange de p r o d u i t s " .

BF 1 575 344 2 .08 .1968 BB 719 499 14.08.1968 BP 1 186 647 16 .08 .1968

117

BREVATOME/ DOCUMENTATION R 1910

Heavy water Product ion by Hydrogen D is t i l l a t ion ]3_5 F a b r i c a t i o n d 'eau l o u r d e par d i s t i l l a t i o n d 'hydrogène

! - B N du 1.10.1954 STAMICARBON N.V.

"Procède pour r é f r i g é r e r de l ' h y d r o g è n e t e c h n i q u e "

BF 1 130 015 1.10.1955

2 -BN des 22.10., 13.11.1954 8. 28.02.1955 STAMICARBON N.V.

"Procède pour 1'extraction d'hydrogène lourd et d'eau lourde".

BB 542 107 20.10.1955 BF 1 139 652 22.10.1955 DA 1 018 848 2tl.10.1955 CP 561 840 22.10.1955 US 2 098 554 17.10.1955 BP 815 098 29.10.1955

3 - BN du 4.02.1955 STAI-1ICARB0N N.V.

'.'Procède pour la production ou la recuperation de froid par vaporation d'un liquide s'éveporant à très basse temperature".

BF 1 14e 002 4.02.1956 CP 587 974 2.02.1956 BP 795 270 31.01.1956

4 - B5 332 465 du 10.Ü2.1955 0ERLIKON

"Verfahren zur Gewinnung von Deuter.ùi moxyd".

5 " B5 332 466 du 12.02.1955 OERLIKON

"Procède de production de l'oxyde de deuterium".

BF 1 141 241 1C.02.1956

(i - BS 332 467 du 1.03.1955 OERLIKON

"Verfahren zur Gewinnung von Deuter.t>imoxyd".

7 - IN ' du 12.03.1955 STAMICARBON

"Procede pour l'extraction de deuterium".

DA 1 066 554 12.03.1956 BP 826 962 12.03.1956 BF 1 152 631 12.03.1956 BB 545 933 10.03.1956

CP 575 762 12.03.1956

8 - BS 340 492 du 1.03.1956 LONZA

"Verfahren zur Gewinnung von Deuter/Oj(m (D_)".

.../...

118


R 1910

9 - BP B69 412 du 19.06.1956 U . K . A . E . A .

" I n s t a l l a t i o n de d i s t i l l a t i o n de 1 • h y d r o g à n e " .

BF 1 177 343 18 .06 .1957 DA 1 144 30B 1 9 . 0 6 . 1 9 5 7 CP 596 586 19 .06 .1957 US 2 960 838 19 .06 .1957 BS 3 700 / 5 9 ' 19 .06 .1957 NP 97 806 1 9 . 0 6 . 1 9 5 7

1 0 " DA 1 026 284 du 7 .07 .1956 HOECHST

"Procède pour c o n c e n t r e r l ' h y d r o g è n e l o u r d " .

BF 1 178 228 5 . 0 7 . 1 9 5 7 CP 613 201 5 . 0 7 . 1 9 5 7 BI 577 546 6 .07 .1957

] ! - BN 99 069 du 11 .07 .1956 5TAMICARBON N.V.

" Improvements i n the low t e m p e r a t u r e s e p a r a t i o n o f gas m i x t u r e s " .

BP 823 754 4 .07 .1957

1 2 - BF 1 157 917 du 7 .09 .1956 L 'A IR LIQUIDE

"Procède de l i q u i d a t i o n d ' u n g a z " .

US 2 954 677 12 .00 .1957 CP 605 896 2 2 . 0 8 . 1 9 5 7 BP 842 471 2 0 . 0 8 . 1 9 5 7

1 3 - U5 3 004 628 du 17 .07 .1957 U . S . A . E . C .

• " R e c t i f i e d a b s o r p t i o n method f o r t h e s e p a r a t i o n o f hydrogen i s o t o p e s "

H - BP 893 057 du 25 .11 .1957 U . K . A . E . A .

" Improvements i n o r r e l a t i n g t o low t e m p e r a t u r e gas m i x t u r e s e p a r a t i o n p r o c e s s e s " .

BF 1 215 376 2 4 . 1 1 . 1 9 5 8 BI 599 214 2 0 . 1 1 . 1 9 5 8 CP 612 ODD 14 .11 .1958

1 5 - DA du 11 .12 .1957 Ges. f ü r LINDE'S,. EISMASCHINEN A.G.

" Improvements i n low t e m p e r a t u r e p u r i f i c e t i o n o f g a s e s " .

BP 894 558 10 .12 .1958

1 6 - BS du 1 .02.1958 SULZER

" P u r i f i c a t i o n o f g a s e s " .

BP 865 870 2 0 . 0 1 . 1 9 5 9

n

119


R 1910

17- DA 1 066 187 du 4.07.1958 DEGUSSA

"Procède pour 1'enrichissement de l'hydxogène lourd et dispositif pour aa mise en oeuvre".

BF 1 229 332 3.07.1959 NP 101 221 1.12.1959

18- DAD G25 088 ig- DAD G25 052 des 6 t 11.0B.195B Ges. für LINDE'S EISMASCHINEN A.G.

"A process of and an apparatus for low temperature gas separation".

BP 904 007 6.0B.1959 NP 102 742 5.0B.1959

20- DAD G25 003 du 6.0B.1958 Ges. für LINDE'S EISMASCHINEN A.G.

"A method of and an apparatus for gas treatment".

BP 907 477 6.08.1959

21 - US 3 126 267 du 24.07.1959 AIR PRODUCTS 8. CHEMICALS

"Separating isotopes of hydrogen".

22- BF 1 271 501 du 2.05.1960 CE.A.

" N o u v e l l e i n s t a l l a t i o n de d i s t i l l a t i o n d ' h y d r o g è n e " .

BL 40 059 25 .04 .1961 BN 264 254 2 . 0 5 . 1 9 6 1 BB 602 994 2 5 . 0 4 . 1 9 6 1 OP 232 958 28.04.1961 CP 660 349 2 7 . 0 4 . 1 9 6 1 DP 101 579 1 5 . 0 1 . 1 9 6 1 BP 932 178 1 . 0 5 . 1 9 6 1

2 3 - BF A 78 64B/ 1 271 501 9 .11 .1960 C E . A .

" N o u v e l l e i n s t a l l a t i o n de d i s t i l l a t i o n d ' h y d r o g è n e " .

OP 232 958 28.04.1961 US 3 216 800 1.05.1961

tv t i

120


R 1910

Heavy water Production by Water Disti l lation B.6 Fabr i ca t i on d'eau lourde par d i s t i l l a t i o n d'eau

1 - BB 490 239 du 19.07.1949 Mykola R0MANIW

"Separat ion dB l ' e a u l o u r d e " .

2 - BB 490 900 du 31.06.1949 Mykola ROMANIW

"Separat ion de l ' e a u l o u r d e " .

3 - BJ du 3.12.1954 S. YAGI, Y URAGUCHI

"Method and apparatus f o r the p u r i f i c a t i o n of heavy wa te r " .

US 2 999 795 21.11.1955

4 - DW 14 311 du 9.07.1955 V. BAYERL

"Verfahren und Vorrichtung zur Gewinnung von DeutentSi Tioxyd".

5 - US 2 79B 359 du 1.0B.1955 U.S.A.E.C.

"Steam power plant with means for heavy water concentration".

CP 567 92B 5.06.1956 BP B24 954 31.07.1956

6 - BP B06 975 du 27.10.1955 U.K.A.E.A.

"Garniture pour colonnes de distillation".

BF 1 163 919 26.10.1956 A.E.C. CP 575 971 9.10.1956 A.E.H.

.BS 34B 955 2 6 . 1 0 . 1 9 5 6 A . E . C .

7 - BF 1 152 915 du 5.04.1956 o. GRANER

"Procède et appa re i l de d i s t i l l a t i o n "

8 - BFA70 19B/1 152 915 du B.12.1956 J . GRANER

"Procède e t appa re i l de d i s t i l l a t i o n " .

9 - BF 1 1B9 393 du 31.12.1957 Sté INDUSTRIELLE L COMMERCIALE DE LA Cie DES SALINS DU MIDI

"Procède de separat ion des v a r i é t é s i so top iquas de l ' e a u " .

10 - BSD 76 063 du 22.07.1959 SULZER

"Colonne de t r a n s f e r t de m a t i è r e " .

BF 1 264 234 21.07.1960

• • • / « • •

121

HREVATOME / DOCUMENTATION

R 1910

11 - B5D 76 064 du 2 2 . 0 7 . 1 9 5 9 5ULZER

"Colonne de transfert de matière perfectionnée".

BF 1 264 235 ' 21.07.1960

12 - BSD • 76 065 d u 2 2 . 0 7 . 1 9 5 9 SULZER

"Perfectionnements aux colonnes de transfert de matière".

BF 1 264 236 21.07.1960

13 - B5D 77 752 du 3.09.1959 5UL2ER

"Distillation columns".

BP 933 281 2 4 . O B . 1 9 6 0 DA 1 123 293 2 1 . 0 9 . 1 9 5 9

14 - DW 25 046 du 21.12.1959 K. WETZEL

"Process f o r o b t a i n i n g Deuter ium-enr iched hydrogen compounds".

BF 1 253 501 18.03.1960 BP 950 627 1 4 . 0 3 . 1 9 6 0 OP 227 235 2 1 . 0 1 . 1 9 6 0 CA 148 793 3 1 . 0 3 . 1 9 6 0 DA 1 144 697 2 2 . 1 2 . 1 9 5 9 BN 249 395 1 4 . 0 3 . 1 9 6 0 CP 679 138 1 .04 .1961

.15 - BF 1 262 640 du 1 9 . 0 4 . 1 9 6 0 5 t é COMMERCIALE DE5 SALINS DU MIDI

"Per fec t ionnement aux procédés pour l a sepa ra t i on des v e r i é t é s i s o t o p i q u e s de l ' e a u " .

DA 1 274 564 19.04.1961

in - BFA' 78 919/1 152 915 du 17.12.1960 J . GRANER

"Procède et a p p a r e i i de d i s t i l l a t i o n " .

Add 70 196

17 - BFA 79 520/ 1 262 640 du 7.4.1961 Sté COMMERCIALE DE5 SALINS DU MIDI

"Perfectionnement aux procédés pour la separation des variétée isotopiques de l'eau".

DA 1 274 564 19.04.1961

18 - USD 679 916 du 1.11.1967 PACTIDECORP.

" A p p a r e i i pour augmentar l e c o n c e n t r a t i o n d'une f r a c t i o n l i q u i d e moine v o l a t i l e dans un mélange de l i q u i d e s " .

BF 1 590 459 31.10.1968 BND 6 815 610 31.10.1968 BP 1 189 608 31.10.1968

122

BREVATCME / DOCUMENTATION

R 1910

19 - BSD 6 B71 du B .05 .1966 SULZER

"Procède e t a p p a r e i l de t r a i t e m e n t d 'ammoniac d e u t é r é " .

BF 2 OOB 061 7 .05 .1969 E3 732 39C 3 0 . 0 4 . 1 9 6 9

20 - DA 1 767 700 du 6 . 0 6 . 1 9 6 8 STEINKOHLEN-ELEKTRIZITÄT A .G.

" A p p l i c a t i o n de l a c h a l e u r perdue dans des c e n t r a l e s à l ' o b t s n t i o n d ' e a u l o u r d e " .

BF 2 010 2B5 6 . 0 6 . 1 9 6 9

K a i

$ & •

123


R 1910

Heavy water Production by Ammonia Distillation B, 7'. Fabrication d'nau lourde par d i s t i l l a t i o n d1ammoniaqua"

1 - BP 807 B03 des 4.S.1956 £ 29.04.1957 COSTAIN-JOHN BROWN L td .

"Perfactionnements r e l a t i f 6 un procède d'extract ion du deuterium de gaz renferment de l1hydrogene*.

BF 1 174 545 3.05.1957 BP 1 091 092 4.05.1957 CP 619 092 4.05.1957

2 - BF 1 164 BB2 du 19.01.1957 Sta des Pioduita Azotes

"Procèdo da fabrication da l ' eau lourde".

3 - BP 867 B4B du 10.03.1958 CONSTRUCTORS JOHN BROWN Ltd . i. N.W.ROBERTS

"Improvements in or re la t ing to the concentration of deuterium".

124


R • 1910

Heavy water Production by Methane Distillation 3 ' g F a b r i c a t i o n d'ssu lourde par d i s t i l l a t i o n du i:

1 - BF 1 444 991 du . 1 4 . 0 6 . 1 9 6 5 BRITISH AMERICAN OIL Cy L t . i

"P rocède de p r o d u c t i o n ds methanes d e u l é r é s e t d ' s a u l o u r d u

CP 711 45B 14 .12 .1963 BB CS 2B9 11 .06 .1965

Heavy water Production by Distillation of Other Compounds Q g F a b r i c a t i o n d'eau lourde par d i s t i l l a t i o n d ' a u t x e s composes

1 - BF 1 191 413 du 10 .02 .1958 . K.E. (OLMBERG

"Procède pou r l a s e p a r a t i o n des i s o t . - ' ^ s . d B l ' h y d r o g è n e " .

BI 604 651 3 0 . 0 1 . 1 9 5 9

2 - BF 1 207 143 du 2 5 . 0 8 . 1 9 5 8 K.E. ÌI0LMBERG

"Procède pour la séparstion dea isotc-oss dB l'hydrogène1'.

3 - U5 3 101 256 du 28.OB.1958 qUARTZ £ SILICE

"Separation of hydrogan isotopes".

125


R 1 91 G

Heavy water Production by Electrolysis B,10 Fabrication d'eau laurda par électrol;

1- US 2 108 570 du 27.06.1933 AMERICAN SECURITY 4. TRb. LO.

"Kinds of WBtar and method of producing them".

2 - US 2 137 430 du 15.05.1934 W.A. WEBB

"ProcesB for the concentration of isotopes".

3 - DA 623 336 du 2.06.1934 I.G. FARBENINDUSTRIE A.G.

"Verfahren zur Gewinnung von Schwerem Wasser und Schwerem Wasserstoff".

4 - BF 7B9 B22 -du 25.03.1935 .A.E. KN0WLES

"Perfectionnements apportés à 1'electrolyse de l'eau".

BP 435 450 21.02.1934 US 2 044 704 29,Ü3.1935 BN 42 704 19.03.1935 DA 666 393 26.03.1935

5 - DA 915 690 des IB.10.1941, 8.05.1945 & 7.05.1950 A. KLEMM

"Verfahren zur Anreicherung von Isotopen".

6 - HP du 21.12.1942 N0RSK-HYDR0-ELEKTRISK KVAEL5T0FAKTIESELS-KAB

"Procède pour élever la concentration de l'eau lourde".

BF 922 529 18.02.1946 BP 620 837 10.01.1946

7 - BP 726 532 du 15.02.1943 U.K.A.E.A.

"Improvements in and relating to the production of heavy water".

B - BP 726 771 du 10.08.1943 U.K.A.E.A.

"Improvements in ond relating to the production of heavy, water",

CP 531 807 24.07.1944

fl - BP 581 908 du 16.11.1943 L. TR0NSTAD

"A method and apparatus for the combined preparation of hydrogen, heavy water and metals or alloys'with low carbon content".

in - US 2 695 26B du 27.01.1945 U.S.A.E.C.

•"Process for the concentration of isotopes".

CP 509 231 28.11.1944

126

BREVATGME / DOCUMENTATION

R 1910

11 - B5 328 414 du 16.08.1954 OERLIKON

"Verfahren zur Gewinnung von Deuterium oxyd".

12 - BS J32 465 du 10.02.1955 OERLIKON


13 - BS 332 467 du 1.03.1955 OERLIKON


14 - DA 1 057 585 du 31.05.1955 K. DIEBNER

"Procède relat'f à 1'enrichissement du deuterium".

15-BE du 1.06.1955 JUNTA DE ENERGIA NUCLEAR

"Procède et dispositif pour obtenir de l'eau lourde à des degrés de puraté differente".

BF 1 150 242 25.05.1956 BP 837 894 25.05.1956 BB 548 230 30.05.1956 CP 566 101 26.05.1956

16 - DA 1 058 479 du 13.08.1955 F. UHDE Gmbh

"Mit elektrolytisher kaskada arbeitendes Verfahren zur Herstellung von schwerem Wasser".

17- NP du 6.10.1955 N0R5K HYDRO-ELEKTRISK KVAELSTOFAKTIE-SELSKAB

"Procède de concentret ion de l ' e a u lourde" .

BF 1 158 105 4 .10 .1956 BS 357 379 2 .10 .1956 CP 566 397 3.10.1956

1 8 - DA 1 051 820 du 11.11.1955 RUHRCHEMIE A.G. i. STEINKOHLEN-ELEKTRIZI TAT A.G.

"Verfahren zur Anreicherung von schwerem Wasser".

CP 575 018 8.11 .1956

m - DA 1 023 017 du 18.07.1956 W. VIELSTICH

"Verfahren zur Anreicherung von schwerem WBSser in elektrochemischen Zellun".

20- BF 1 166 831 du. 1.02.1957 J.C. SEAILLES

"Procède électrolytiqua da separation d'éléments épurés notamment da l'eau lourde".

BP 882 607 30.01.1958

127


R 1910

2 1 - BJ du 2 4 . 0 8 . 1 9 5 7 ZAIDAN-HOJIN NOGUCHI KENKYU - JO

"P rocess o f c a r r y i n g o u t e l e c t r o c h e m i c a l l y e l e c t r o l y s i s " .

US 3 111 472 8 .04 .1958

22 - BF 1 203 110 du 21.07.1958 J.C. 5EAILLE5

"Procède de fabrication das isotopes de l'hydrogène et de l'eau".

93 - BF 1 207 117 du 1.08.1958 NORSK HYDRO-ELEKTRISK KVAELSTOFAKTIESELS-KAB

"Procède et installation pour la fabrication d'oxyde de deuterium".

24 - DA 1 088 932 du ' 5.03.1959 RUHRCHEMIE A.G.

"Verfahren zur Gewinnung von schewerem Wasser in elektrochemiechen Zellen".

25 - DA 1 154 443 du 12.05.1959 A. KOSSNER &. E. WICKE "Verfahren zur Steigerung der Permeabilität von Metallen gegenüber Wasserstoff".

26 - DA 1 109 653 du 22.05.1959 RUHRCHEMIE A.G. i. STEINKOHLEN-ELEKTRIZITRT

"Procède et diepositif pour l'obtention continue d'eau riche en deuterium et electrolyse de l'eau".

BF 1 256 969 17.05.1960 CP 641 333 13.05.1960 SIEMENS BB 591 026 19.05.1960

27 - BF 1 322 116 du 2B.08.1959 MQUILLERES DU BASSIN DU NORD ET DU PAS-de-CALAIS L C.E.A.

"Nouveau p rocède pour 1 * e n r i c h i e s e m e n t ou l e f r a c t i o n n e m e n t i s o t o p i q u e de l ' h y d r o g è n e " .

BP 926 488 2 5 . 0 8 . 1 9 6 0 BB 593 858 5 .08 .1960 DA 1 155 425 2 9 . 0 8 . 1 9 6 0 BI b26 113 19 .08 .1960 US 3 098 020 1 1 . 0 8 . 1 9 6 0 SP 219 359 29 .08 .1960 BN 255 292 2 7 . 0 8 . 1 9 6 0

28 - BJD 3 460 du 6 .02 .1960 I . 0BINATA

"Method o f s e p a r a t i n g and c o n c e n t r a t i n g i s o t o p e s and d i f f i c u l t - t o - s e p a r a t e e lemen ts by e l e c t r o l y s i s " .

BP 913 336 du 30 .01 .1961

29 - DA 1 183 892 du 14 .06 .1961 L. KANDLER

" C e l l u l e d * e l e c t r o l y s e pour l a d è c o m p o e i t i o n de l ' e a u " .

BF 1 329 797 1 4 . 0 6 . 1 9 6 2

128


R 1910

w - BF 1 31B 703 du 9.01.1962 C.F.T.U.

"Perfectionnementa aux procédéa de fabrication d'eou lourde".

31 - OA 1 245 337 du 26.10.1962 SIEMENS A.G. &. VARTA A.G.

"Verfahren zur elektrochemischen Deuterium 8nreicherungn.

32 - BP 973 B20 du 30.11.1962 JOHNSON,MATTHEY L Cy Ltd.

"An improved method of 8aparating hydrogen isotopes".

33 - BJD 31 166 du 21.06.1963 ASAHI KASEI KOGYO K.K. 8. H. KAKIHANA i. ATOMIC FUEL CORP.

"Procède pouz separer et anrichir des isotopes".

U5 3 425 924 17.01.1964 BF 1 403 196 19.06.1964 DA 1 232 926 19.D6.1964 BP 1 066 374 19.06.1964

34 - BJD 40 311 du 2.OB.1963 ASAHI KASEI KOGYO K.K. Ä. H. KAKIHANA

"Perfectionnements apportéa aux procédéa pour la separation d'isotopea",

BF 1 402 626 30.07.1964 BP 1 067 367 4.OB.1964 05 I 442 362 31.07.1964 US 3 414 500 27.07.1964

3 5 - CPD 952 421 du 16.02.1966 A.E.C. Ltd.

"Procède electrolytique pour la preparation da l'eau lourda".

BF 1 510 31B 27 .01 .1967 BP 1 152 094 27.01.1967 US 3 514 382 31 .01 .1967

129


R 1910

Heavy water Production by Other Processes 3 n Fabrication d'eau lourde par autraa procédés

1 - BE 485 904 du 19.11.1946 M. ROMANI«

"Separation de l'eau lourde par sa refrigeration et le décontage et l'évaporisation de l'eau légère".

2 - US 2 780 526 du 12.04.1951 UNION OIL Co. "Isotope separation process",

3 - BI 518 551 du 10.06.1954 L. BARN0CCHI "Procedimento per la produzione di acqua pesante".

4 - DA 1 091 541 des. 26.03. &. 14.06.1955 DEGUSSA

"Procède de separation de matières soua forme de gaz ou de vapeur, an particulier dea isotopes et dispositif pour sa realisation".

BF 1 230 416 18.07.1955 E.W.A. BECKER BP 794 834 7.07.1955 BB 539 578 5.07.1955

5 - BF 1 129 214 25.07.1955 CE.A.

"Perfectionnement à la separation des isotopea et des composes de mesaee moléculaires trèa voisines".

6 - BP 826 128 du 8.09.1955 U.K.A.E.A.

"Improvements in or relating to tha saparation of isotopes".

7 - DA 1.0B3 768 du 2.12.1955 SIEMENS

"Verfahren zum trennen von Isotopen".

8 - BP 825 934 du 4.02.1956 U.K.A.E.A.

"Improvements in or relating to the separation of the isotopos of hydrogen".

CP 615 400 1.02.1957

9 - DA du 9.03.1956 CASSELLA FARBWERKE

"Procède de separation de melanges liquidas".

BF 1 169 182 7.03.1957 BP 823 297 7.03.1957 BJ 35 308 8.03.1957

130


R 1910

10- SAJJ du 2.07.1956 8. 3.04.1957 SOUTH AFRICAN COAL OIL AND GAS CORP. Ltd.

"(ìocédé de concentration ou d'isolsment du deuterium ou d'eutres isotopes ou de leurs composes".

BB 558 556 20.06.1957

11 - DA 1 096 675 du 5.09.1956. DEGUSSA

"Procède de eéperation de metières sous forme de gaz ou de vapeur, en particuliex dee isotopes et dispositif pour sa realisation".

BF A 74 040 / 1 230 416 3.09.1957 E.W.A. BECKER BB 559 713 30.07.1957 BP B25 798 30.08.1957 BI 600 721 19.07.1957 US 2 951 554 3.09.1957

12 « US 2 863 526 du 17.10.1956 U.S.A.E.C.

"Method of separating hydrogen isotopes".

1 3 - D A dee 12.06. 8. 20.08.1957 CASSELLA FARBWERKE 14.08.1957 8. 6.05. 1958

"Procède de eéperation de melanges de carps".

BF 1 211 398 11.06.1958 BP 836 857 10.06.1958

u - BP 907 657 du 26.06.1957 R.J. CROSS "Improvements in the separation of light and heevy components of a fluid mixture".

15 - DA du' 12.11.1957 RfltJlRCHEMIE A.G.

"Process for producing heavy water".

US 3 019 088 10.11.1958 BP 901 713 12.11.1958

16 - U5 3 197 402 du 20.11.1957 S.L. RUSKIN

"Methode for the rapid recovery of heavy weter end other products".

17- DAD 22 349 du 14.12.1957 RUHRCHEMIE A.G.

"Process for the production of heavy water",

BP 903 257 27.11.1958

18- BF 1 188 904 du 21.12.1957 Sto INDUSTRIELLE 8. COMMERCIALE DE LA Ci( DES SALINS DU MIDI

"Procède de separation de variétés ieotopiques en phess liquide".

131


R 1910

ID - USD 745 374 du 30.06.195B WESTERN ELECTRIC Co.

"Procèda at apparali d'axtraction da 1'helium".

BF 1 227 030 11.06.1959 BP 869 047 25.06.1959 BB 579 767 17.06.1959

?.0 - BI 593 750 du 12.07.1958 G. PAOLUZI

"Parati eamiparmaabili adatta alla aaparaziona rapida dal deuterio dal comune idrogeno, o dal tritio dal deuterio".

21 -BLux D 36 315 du 4.08.1958 P. MALDAGUE

"Procèdi da production da deuterium et de ses composes eins! que d'eutres isotopee logore".

BF 1 231 593 4.08.1959 BP 923 852 29.07.1959 BB 561 198 30.07.1959 BN 241 448 21.07.1959 BI 614 914 3.08.1959

22 - DA 1 143 792 du 10.11.1959 U. SCHMIESCHEK

"Verfahren zur Anreicherung von Deuterium in Deutorium-Wasserstoff-Gomischen durch Adsorption und Dosorption an "Palladium".

?? - BI 635 056 du 1.03.1960 G. PAOLUZI

"Perfezionamento nelle pareti samipsrmeabili destinata alla separazione del Deuterio del comune idrogeno".

24 - US 3 PB1 156 du B.04.1960 FLUOR CORP.

"Separation of deutariui from hydrogen*.

E6 - US 3 05B 811 du 25.04.1960 ATLANTIC REFINING Co.

"Method for the enrichment of D-0 in solutions of 0,0 in HjO".

gB - DAD 574 558 du 29.06.19 61 SIEMENS

"Procède et installation pour la separation masaiqus da gaz rèactifs".

BF 1 375 681 27.06.1962 US 3 230 693 22.06.1962

•xi - BF 1 330 152 du 15.02.1962 G.A. RUBISS0W

"Methode da double contrifugation simultanee moyens employes st produits ainsi obtenus".

132


R 1 91 0

28 - I5P 17 6B7 du 22 .07 .1962 FERTILIZERS Ä. CHEMICALS LTD L H. AHARONI

"Procède p e r f e c t i o n n é de p r e p a r a t i o n de f r a c t i o n s d ' hyd rogène e n r i c h i e s en d e u t e r i u m " . /

BF 1 363 0B1 17 .07 .1963 CHEMICALS 8. PHOSPHATES L t d .

29 - DA 1 241 416 du 30 .05 .1964 Gos. f ü r KERNFORSCHUNG mbh.

" E i n r i c h t u n g zum t r e n n e n von I s o t o p e n " .

30 - BF 1 414 B59 du 28 .00 .1964 C.E.A.

" P e r f e c t i o n n e m e n t s au r e m p l i s s a g e dea co lonnea de a é p e r a t i o n i e o t o p i q u e p a r C h r o m a t o g r a p h i e , e t procède de p r e p a r a t i o n " .

BB 668 377 17 .08 .1965 BS 449 583 2 7 . - 8 . 1 9 6 5 OS 1 519 978 26 .08 .1965 BP 1 123 044 27 .0R. 1965

31 - US D 357 687 du 21 .09 .1964 GENERAL ELECTRIC Co.

" Improvements i n p rocess f o r t h e s e p a r a t i o n of gases by p e r m e e t i o n through a p o l y a r y l e n e o x i d e f i l m " .

BP 1 115 413 10 .09 .1965 BF 1 458 476 17 .09 .1965 BB 669 917 2 1 . 0 9 . 9 6 5

32 - US 3 368 968 du . 3 .03 .1965 A .M .F .

"Method for the deselinization of water".

33 - SA_D__2_5J12 du 11.05.1965 V. PRETORIUS, H. H. HAHN

"Improvements relating to chromatography".

BP 1 148 661 9.05.1966 BP 1 148 662 9.05.1966 US 3 493 497 10.05.1966

3^ - BF 1 478 542 du 14.03.1966 S. R.T.I.

"Procède de separation continue des isotopes de l'hydrogène d'un mélange gezeux par odsorption à contre-courant".

35 - BF 1 478 569 du 15.03.1966 S.R.T.I.

"Procède d1enrichiasement isotopique d'un mélange gazeux contenant en particulier das isotopes de l'hydrogène".

36 - BF 1 492 087 du 19.04.1966 S.N.P.A.

"Disposäif de recyclage utilissble en Chromatographie".

17 - US 3 460 318 du 14.12.1966 GULF GENERAL ATOMIC Inc.

"Centrifugal molecula separator".

133

BnEVATOME / DOCUMENTATION

R 1910

38- BF 1 583 714/ du 14.04.1967 CE.A.

"Procédés et dispositifs de separation des molecules'1,

OS 1 90B 792 IP 31 632

BND 69/02 586

21 .02.1969 16.02.1969 19.02.1969

BE BL

364 225 57 986

26.02.1969 12.02.1969

i»

134

ADDENDUM:

Lis t of Pa ten ts Reported on Nuclear Science Abst rac t from 1972 till Oct. 15; 197.3

U .S . Pa ten ts

METHOD AND APPARATUS FOR TREATING PRE-ENRICHED AMMONIA. Har tmann F . , Gisler H. R. (to Sulzer B r o t h e r s . Ltd). U . S . P a t e n t 3, 644, 093. 22 F e b . 1972. P r i o r i t y date 8 May 1968. Switzerland.

PRODUCTION OF HEAVY WATER EMPLOYING A GROUP VIII CATALYST. Mikovsky R . J . (to Mobil Oil Corp . ). U . S . Patent 3 ,681 ,021 . 1 Aug. 1972. Field 31 Mar . 1970.

PRODUCTION OF HEAVY WATER. Thayer V. R. U . S . P a t e n t 3 ,685 ,966. 22 Aug. 1972. Fie ld 4 Aug. 1969.

DEUTERIUM SULFIDE SEPARATION AND ITS CONVERSION TO DEUTERIUM OXIDE. Glew D. N . , C la rke E. C. (to Dow Chemical C o . ) . U .S . Patent 3 ,690,829. 12 Sep. 1972. Field 22 May 1970.

ISOTOPE SEPARATION WITH HEAT BALANCING. Nazzer D. B. (to Canadian Genera l E lec t r i c Co. Ltd. ). U .S . Patent 3, 690, 830. 12 Sep. 1972. P r i o r i t y date 30 Nov. 1968. Canada.

PROCESS FOR ENRICHMENT BY COUNTER-CURRENT MASS TRANSFER. Thayer V. R. U . S . Patent 3, 692,477. 19 Sep. 1972. Fiald 4 Aug. 1969.

DUAL TEMPERATURE FIXED CARBON BED HEAVY WATER CONCENTRATION PROCESS. Broughton D. B. (to Universa l Oil P roduc t s Co. ). U. S. Patent 3, 700, 417. 24 Oct. 1972. Field 4 Nov. 1968.

135

8, INCREASED RECOVERY IN DUAL T E M P E R A T U R E ISOTOPE EXCHANGE PROCESS. Babcock D . F . , Neill J . S . (to United States Atomic Energy Commiss ion ) . U . S . P a t e n t 3 , 7 1 1 , 5 9 8 . 16 J a n . 1973. Fie ld date 11 May 1971.

9. METHOD O F DECONTAMINATING HEAVY WATER COOLED AND MODERATED REACTOR. Motojima K. , Sakura i H . , Onishi H , , Sasaki Y. , Koike M. , Ueno K. (to Japan Atomic Energy R e s e a r c h I n s t . ) . U . S . Patent 3, 737, 373. 5 J a n . 1973. P r i o r i t y date 2 July 1970. Japan,

F r e n c h Pa ten t s

1. IMPROVED PROCESS FOR PREPARING HEAVY WATER BY ISOTOPIC EXCHANGE (MONOTHERMIC TYPE) BETWEEN AMMONIUM GAS-AND SINTHESIS GASES. L e s u r P . , Vi ra te l l e J . (to Socicte Chimique des Charbcmnages . C o m m i s s a r i a t à l ' E n e r g i e Atomiquc . l ' A i r Liquide. 1'Exploitation d e s ' P r o c e d e s Georges Claude . Compagnie de Cons t ruc t ion Mecanique. P r o c e d e s Su lzc r ) . F r e n c h Patent 2, 056, 050. 19 A p r . 1971. F i l ed 25 Aug. 1969. (In F rench)

2. IMPROVED METHOD FOR PREPARING HEAVY WATER USING MONOTHERMAL ISOTOPIC EXCHANGE BETWEEN AMMONIA AND A SYNTHESIS GAS. L e s u r P . , V i r a t e l l e J ; (to Societe C h i mique des Charbonnages . C o m m i s s a r i a t à l ' E n e r g i e Atomique . l 'A i r Liquide. Socicte Anonyme pour l 'Exploi ta t ion des P r o c e d e s Georges C laude . Compagnie de Cons t ruc t ion Mecanique. P r o c e d e s Su lzc r ) . F r e n c h Pa ten t 2, 074, 737. 8 Oct. 1971. F i led 22 J a n . 1970. (In F rench)

3 . ISOTOPIC ENRICHMENT OF HYDROGEN FOR HEAVY WATER PRODUCTION. Lamber t I . , Ravoi re J . , Roth E. (to C o m m i s s a r i a t à l ' E n e r g i e Atomique) . F r e n c h Pa ten t 2, 079, 708. 18 Oct . 1971. F i led 10 F e b . 1970, (In F rench )

136

Bri t i sh Patent

RECOVERY OF HYDROGEN SULPHIDE FROM WATER. Nazzer D . B . B. , Thayer V. R. (to Canadian Genera l E lec t r i c Co. Ltd. ). Br i t i sh Patent 1, 285, 077. 9Aug. 1972. Filed 27 Oct. 1969.

Germany F . R . Pa ten ts

PLANT FOR THE PRODUCTION OF DEUTERIUM-ENRICHED WATER. Kluge H . (to Ste inkohlen-Elektr iz i tae ts AG). German Patent 2. 048, 117. 20 Anr . 1972. (In German)

UTILIZATION OF WASTE HEAT FROM POWER PLANTS FOR THE PRODUCTION OF HEAVY WATER. Kluge H. (to Steinlcohlen-Elekt r iz i tae ts AG). German Patent 1,767,7001 18 May 1972. (In German)

137

C - ACTUAL INDUSTRIAL PROCESSES

1 - Chemica l Exchange

1 - B i t h e r m a l Exchange between Hydrogen Sulphide and Wate r (H2S - HDO)

1. THE CONCENTRATION OF.DEUTERIUM BY THE S-PROCESS. Spevack J.'S.' Columbia SAM Repor t A - 3 9 3 . D e c . 3 ,1942. Deci . 1957.

2. THE TEMPERATURE COEFFICIENT OF EXCHANGE CONSTANT FOR THE HYDROGEN SULPHIDE-WATER SYSTEM.' McClure D. C.', H e r r i c k C. 'E. Columbia SAM Repor t A-582. 'Apr. 8 ,1943.

3. THE E F F E C T OF TEMPERATURE AND PRESSURE ON THE MURPHREE P L A T E EFFICIENCY FOR THE DEUTERIUM E X CHANGE BETWEEN WATER AND HYDROGEN SULPHIDE. Spevack J . S . ' , Grabow ski E . J . (Columbia Univ.', New York .Div . of War R e s e a r c h , USA). A-597 .Apr . '17 ,1943 . 'Dec i . Mar.' 14, 1957.

4. THE DUAL TEMPERATURE PROCESS FOR ISOTOPIC SEPARATION, Spevack J . S . C o l u m b i a Univers i ty . MDDC-891. Deci . Feb.'26', 1947.'

5. THE IMPROVED DUAL-TEMPERATURE PROCESS FOR THE PRODUCTION OF HEAVY WATER(INCLUDING COST ANALYSIS AND PILOT PLANT PROGRAM).'Spevack J . S . NYOO-85.'Oct. '25, 1949 .Dec l . Ju ly 27, 1959.':

6. THE IMPROVED DUAL-TEMPERATURE PROCESS F p R THE PRODUCTION OF HEAVY WATER. REVIEW OF REPORT NYOO-85. Benedict M. , Golden S . , Norton W. J, (Hydrocarbon Res . I n c . , New York,USA);NYO-180. ' Jan. '6 ,1950. 'Decl . .Feb. '27, 1957. :

http://1949.Decl.July

1.18

TUE DEVELOPMENT OF TUE ".DUAL-TEMPERATURE" PROCESS FOR TUR PRODUCTION OF HRAVY WATER. New York Operation Office. Div. of Technical Advise r s AEC. iNTYOO-799. Sept. 11, 1050. Deci. Apr . P.. 15157.

CALCULATION OF REACTION EQUILIBRIUM FOR ISOTOPE EXCHANGE. Talcvskii. V. 1Y1. Zluir. F iz .Kl i im. 25, 2(N -73 , 1051. (hi Russian)

S-PROCESS PILOT P I A N T - F I K S T RESULTS AND PROCESS PRINCIPLES. Eabcock D. F . , Biii'orrl C. B . J i \ , M o r r i s J . W. (Du Poni; de Nemours E. I. &Co. Savannah River Lab. , Augusta, Ga. USA). D P - 3 . Nov. 23, .1 951. Deci . Feb . .10, 1957.

EXCHANGE REACTIONS BETWEEN HEAVY WATER AND SULFUR COMPOUNDS AND THE ASSOCIATED ISOT01TC ANALYSES. Kirshcnbaum I. (Columbia Univ. , New York, USA). TJD-5028. May 25, 1.051. Deci . Mar. 7, 1957,

PHASE BEHAVIOUR IN THE I12S-WATER SYSTEM. Scllcck F . T. , Ca rmichae l L. T. , Sage P.. 11. Ind. Eng. Choi». 44, 2219-2G, 1952.

CORROSION IN H2S-TI2O SYSTEM. Snyder .I .A. , War ren D. DP-9G. Oct. 1.95:"..

THE EQUILIBRIUM BETWEEN HYDROGEN SULPHIDE AND HEAVY WATER. Small P . A. Trans . -Faraday Soc. 33, 820-3, 1957.

HEAVY WATER PRODUCTION THROUGH THE I r ^ S / l ^ O DUAL TEMPERATURE EXCHANGE PROCESS. Weiss G. Chain. Ing. Tech. 30 ,433-40, 1950. (In German) (AEC-t r -3365)

139

15. A TWO TEMPERATURE PROCESS FOR THE SEPARATION OF BINARY MIXTURES. Sakodynslcii K. I . , Babkov S. I . , Zhavoronkov N. M. Dokl. Vyssh. Shkoly, Khim. Tcchnologiya 1, 598,1950.

16. MEASUREMENT OF EQUILIBRIUM CONSTANTS FOR THE D 2

EXCHANGE BETWEEN HYDROGEN SULPHIDE AND WATER. Haul R . A . W . , B o h n k c c H . , Die t r ich II. Angcw. Chemie 71 ,30 , .1.959.

17. PRODUCTION OF HEAVY WATER. Bcbbington W. P . (Du Pont dc Nemours E . I. &Co. , Wilmington, Del . USA), Thayer V. R. Chum. Eng. P r o g r . 55, No. 9, 70-fi, Sept. 1959.

18. HEAVY WATER PRODUCTION THROUGH TWO TEMPERATURE EXCHANGE PROCESSES, PARTICULARS THE H2S HOT-COLD EXCHANGE PROCESS. Weiss G. Declicma Monograph. 34, 148-65, 1959.

19. A K.WETIC STUDY O.F THE EXCHANGE OF DEUTERIUM B E TWEEN LIQUID WATER AND GASEOUS HYDROGEN SULPHIDE. Garancl J . , Amanr ich R. J . Chini . Phys . 56, 532-47, 1959. (NP-tr-44G)

20. SEPARATION OF HEAVY WATER BY MEANS OF A 1 I 2 S - H 2 0 ISOTOPIC EXCHANGE DUAL TEMPERATURE PROCESS. A lva rez Gonzales J . R . , Mar ia Arcocha A. M. , Ote ro tic la Ganclara J . L . , Rojas de Diego J . L. (JEN, Madrid, SPAIN). Anales r e a l soc . ospan. f i s .y qui in. (Madrid) Sor . B5G, 547-58, May I960. (In Spanish) (CEA- t r -X-410)

21 . CHEMICAL AND BIOLOGICAL STUDIES WITH DEUTERIUM. Ka tz .T . J . Am. Scient is t 48 , 544-80, Dec . 1960.

22. INDUSTRIAL' TESTS ON HEAVY WATER PRODUCTION BY H 2 S - H 2 0 EXCHANGE. Lazar t l B . (CEA), Ti l lol A.(SOD). Bull . Inform. Sci. et" Teclin. (Pa r i s ) No. 40, 14-18, May 1960. (In French)

140

SWEDISH HEAVY WATET! PROCESS. E r i k s s o n B . J . ( A l I m ü i m a Svcnska E l c k t r i s k a A. D . , Vl l s to rüs , SWEDEN). Chum. &• P r o c e s s E n g . 4 1 , f»-7, ,T:ui. l.iXiO.

SWEDISH HEAVY WATER PROCESS-2 . E r i k s s o n B . J . (Ailina'n-na Svonska E'iokt,.viska A. B , , SWEDEN). Cliom. fc. P r o c e s s Eng. 4 1 , 0:5-7, F e b . 1.9(ill.

HEAVY WATER PRODUCTION IN SWEDEN. E r i k s s o n B . J . Nuc lea r Eny. r>, 400 -12 , Sopì. IfJfiO.

1SOTOPIC EQUILIBRIUM CONSTANTS OF THE DEUTERIUM EXCHANGE DETWEEN HBO AND HuS, UoSc, AND l l2Te. Marx D. CEA-R-i:5, ')2. DK;«, (in F r e n c h )

REMARKS ON TTIE A R T I C L E BY I?.. Haul, H. Bohnke, II. D i e t r i c h , M e a s u r e m e n t of the Equ i l i b r i um Cons tan t s of the Deu te r ium Exchange be tween IT2S and HoO. Grantlcoilof. P . , Roth E. CEA-Kop . .1.4 0Q. 19(50.

THERMODYNAMICS OF THE HYDROGEN SULPHIDE-WATER SYSTEM RELEVANT TO THE DUAL T E M P E R A T U R E PROCESS FOR THE PRODUCTION OF HEAVY WATER. Tcehn . Rep . 58 ß . Pohl 11. A. T til-(>(><)(>. July 1, .1.9(50. (.1. Gliom. Eng . Data G, 5 1 5 - 2 1 , 10(j.l)

APPLICATIONS O F CHEMICAL EXCHANGE METHODS TO ISO-TOPrC SEPARATION. D r n r y J . S . (ORNL Tenn. USA). P r o g r . in Nue lea r E n e r g y 3e.r. IV 4, 308-43 ,10G1.

Ml

SOLUBILITY OF IRON SULL'llllMù'à. Tod i . r ep . No. (HC. Polii H.A. (Du Poilt tie Nemours E . 1, fc C o . , A t o m i c Energy Div . , Wilmington De l . , Princeton Univ. N. J . Plastics Lab.. USA). TID-124 51, Apr . '1,1001.'

THERMAL FEEDBACK IN COUNTER-CURRENT PROCESSES. PART I. Polii H.A. (Du Pont do Nemours E . I. & C o . , Atomic Energy Div. Wilmington, Del. and Princeton Univ. N . J . P las t i cs Lab. USA). T[D-.l2452.'Apr.' !., 1061.'

THERMAL FEEDBACK IN COUNTER-CURRENT PROCESSES. PART II. Pohl II. A. (Du Pont do Nemours E. I. & Co. , Atomic Energy Div. Wilmington., Del. and Pr inceton Univ. N. J . P las t i c s Lai). USA). T ip -12453 . Apr. 1, 1961.

SWEDISH HEAVY WATER PROCESS. Er iksson B . J . ASEA Res . J . (Sweden) 7 ,280-304,1962.

CONTROL OF THE DUAL TEMPERATURE EXCHANGE PROCESS POH THE MANUFACTURE OF HEAVY WATER. Morr i s J . W. , Scottoli W. C. (Du Pont do Nemours E . I, & C o . , Aiken, S. C. USA). Chcm. Eng. P r o g r . , Symp. Sor. 53, 26-38,19G2. (Presented at A. I. Ch. E.Meet ing, Ran F ranc i sco , Cai. USA, Dec. 1059)

MATERIALS OF CONSTRUCTION FOR THE DUAL-TEMPERATURE EXCHANGE PROCESS FOR PRODUCING HEAVY WATER. Thayer V. R . , DcLong W. B. Chom. Eng. P r o g r . , Symp. Sor. 58, 86-93,1962. (Prosontod at A. I, Ch. E . Meeting, San F ranc i s co , Cai . USA, Dec. 1959)

CATALYTIC EXCHANGE OF HYDROGEN SULPHIDE AND OF HYDROGEN WITH DEUTERIUM ON DISULPHIDE OF MOLYBDENUM AND TUNGSTEN. Wilson R. L . , Kcmball C. , Galwey A. K. T r a n s . Faraday Soc. 58, No. 3, 583-92, 1962.

142

37. CALCULATION OF THE EQUILIBRIUM CONSTANTS OF ISOTOPE EXCHANGE B E T W E E N WATER AND II2S; Katoluikov S. G . , Shlypnikov S. V. Z h u r . F i z . Kirim. 3G, No. 4 , 853-4 , 1962. (In Russ ian)

3«. EXAMINATION OF RECENT IMPROVEMENTS PROPOSED BY THE AMERICANS IN HEAVY WATER PRODUCTION BY THE IT2S PROCESS. Uostning M. Repor t of the Col loquium on Heavy W a t e r . ( JEN, Spain and EAES P a r i s ) , Madrid Deo. 1,902. (NP-13766 P.7-2G)

30. WHY THE GS PROCESS S T I L L TOPS COMPETITORS. Law C. A. Can . Nucl . Tcc lmol . 3, 30-40, 1904.

40. HEAVY WATER-OUR STAKE IN THE F U T U R E . Con. C h e m . P r o c e s s . 50, No. 5, 00, 7G, May 10GG.

4 1 . CANSO, N. S . , SITE FOR HEAVY WATER P L A N T . Can . Nucl . Tccluinl . 5, No. 4 , 30, .Tuly-Aug. .1 .!)GG.

42. P E R F O R M A N C E O F SIEVE TRAYS UNDER GS HEAVY WATER PROCESS CONDITIONS. PART 1. LOW PRESSURE OPERATION. B u r g o s s M. P . , Garv in R. G . , Scottel i W . C . (Du Pont de N e m o u r s E . I . & C o . , Aiken , S. 'C. 'Savannah R ive r Lab . USA). D P - 1 0 2 5 . J u n e 1,966.

43 . SEA-WATER TO F E E D HEAVY WATER PLANT. .Can . C h e m . P r o c e s s . 5 1 , No. 6 , 4 1 - 2 ; 4 5 - 6 , June 1967.

44. HEAVY WATER PROCESS D E V E L O P M E N T A T CHALK RIVER. Rae II. K. (Atomic E n e r g y of Canada , Ltd. Chalk R i v e r , Ont. CANADA). C h e m . Can . 19, No. 44-G, Oct. 18 ,1967 . (AECL-2895)

143

45. HEAVY WATER COMES TO NOVA SCOTIA. Chem. Eng. P rogr . 63, No. 6, 44, June 1967.

4G. PERFORMANCE OF SIEVE TRAYS UNDER GS HEAVY WATER PROCESS CONDITIONS .PART II. HIGH PRESSURE OPERATION. Garvin 11. G.', Norton E . R. (Du Pont de Nemours E. I. &. C o . , Aiken, S .C. Savannah River Lab. USA). DP-1025-II . Apr . 1967.

47. SIEVE-TRAY PERFORMANCE UNDER GS-PROCESS CONDITIONS. Garvin R.' G.', Norton E. R. , Chem. Eng. P rogr . 64, 99-106, 1968.

48. ISOTOPE EXCHANGE RATES. V. HOMOGENEOUS REACTION BETWEEN H2S AND D 2 . Burcat A . , Lifshitz A . , Lewis D. , Bauer S.II. J. Chom. Phys . 49, 1449-57, 1968.

49. PHYSICAL PROPERTIES OF H 2 S-H20 MIXTURES. Aicro J . 15, 272-5, 1969.

50. EQUILIBRIUM CONSTANTS FOR GS PROCESS REACTIONS INVOLVING TRITIUM COMPOUNDS. Jackson D. P . (AECL, CRNL, Chalk River , Ont.' CANADA). AECL-3382. Aug. 19G9.

51. COMPARISON OF METHYL ACETYLENE AND HYDROGEN SULPHIDE EXCHANGE WITH WATER FOR CONCENTRATING DEUTERIUM IN A DUAL TEMPERATURE SYSTEM. Goldfrank J. C . . New York, Columbia Univ. 1969.

52. PREDICTED PERFORMANCE OF GS PROCESS WITH SUPPLEMENTARY FEED TO THE HOT TOWER. Burgess M. P . (Du Pont de Nemours E . I . and C o . , Aiken, S. C. Savannah River Lab . ) . Apr.

• 1970.

144

53. DEVELOPMENT OP THE HYDROGEN SULPHIDE-WATER DUAL TEMPERATURE TECHNOLOGY. Spcvack J. S. CNEN Symposium on Technical and Economic Aspects of Heavy Water Production, Turin, Italy. Sept. 30-Oct. .1, 1970.

54. OBTAINING OF HEAVY WATER BY THE DUAL TEMPERATURE H2S PROCESS. Agostini J. P . (Commissar iat à l 'Energie Atomique, Sa clay, France .Centre d'Etudcs Nucleaires). CEA-R-4217. Oct. 1971. (In French)

143

45. HEAVY WATER COMES TO NOVA SCOTIA. Chem. Eng. Progr . 63, No. 6, 44, June 1967.'

46. PERFORMANCE OF SIEVE TRAYS UNDER GS HEAVY WATER PROCESS CONDITIONS.'PART II. HIGH PRESSURE OPERATION. Garvin R. G., Norton E . R. (Du Pont de Nemours E. I. &• Co . , Aiken, S.'C. Savannah River Lab. USA).DP-1025-II. Apr. 1067.

47. SIEVE-TRAY PERFORMANCE UNDER GS-PROCESS CONDITIONS. Garvin R.' G.', Norton E . R. , Chem. Eng. Progr . 64, 99-106,19G8.

48. ISOTOPE EXCHANGE RATES. V. HOMOGENEOUS REACTION BETWEEN I-I2S AND D 2 . Burcat A . , Lifshitz A. , Lewis D. , Bauer S.'H." J. Chom. Phys . 49,1449-57,1968.

49. PHYSICAL PROPERTIES OF H2S-H2O MIXTURES. Aicre J . 15,272-5,1969.'

50. EQUILIBRIUM CONSTANTS FOR GS PROCESS REACTIONS INVOLVING TRITIUM COMPOUNDS. Jackson D. P . (AECL, CRNL, Chalk River, Ont.'CANADA). AECL-3382. Aug. 1969.

51. COMPARISON OF METHYL ACETYLENE AND HYDROGEN SULPHIDE EXCHANGE WITH WATER FOR CONCENTRATING DEUTERIUM IN A DUAL TEMPERATURE SYSTEM. Goldfrank J. C. . New York, Columbia Univ. 1969.

52. PREDICTED PERFORMANCE OF GS PROCESS WITH SUPPLEMENTARY FEED TO THE HOT TOWER. Burgess M. P. (Du Pont de Nemours E . I. and Co . , Aiken, S. C. Savannah River Lab. ). Apr. 1970.

144

DEVELOPMENT OF THE HYDROGEN SULPHIDE-WATER DUAL TEMPERATURE TECHNOLOGY.'Spovack J. S. CNEN Symposium on Technical and Economic Aspects of Heavy Water Production. Turin, Italy. Sept. 30-Oct.' 1,1970.

OBTAINING OF HEAVY WATER BY THE DUAL TEMPERATURE H2S PROCESS. Agostini J, P . (Commissar ia t a l 'Energie Atomique, Saclay, France .Cent re d 'Etudes Nucleaires) . CEA-R-4217. Oct. 1971. (In French)

145

ACTUAL INDUSTRIAL PROCESSES

1 - Chemical Exchange

2 - Chemical Exchange between Ammonia and Hydrogen (Nil3 - HD)

AMMONIA - HYDROGEN EXCHANGE; Arnold H. R. Columbia Memorandum Nov. IG, 1942.

N PROCESS DESIGN. Chapin J. I I . , Quinn P . G., Reynolds T. G. SAM Report A-402. Doc. 5, 1942.

(On Deuterium Separation by Means of Exchange Reactions). Columbia University Memorandum Nov. 21 and 2G, 1942.

PROGRESS REPORT ON ISOTOPIC SEPARATION. Urey H. C. SAM Report A-170. Apr. 25, 1942.

CATALYSTS POR WATER-HYDROGEN AND AMMONIA HYDROGEN SYSTEMS. Urey II. C . , Arnold H. R. SAM Report A-330. Oct. 20,1942.

CATALYSTS FOR AMMONIA-HYDROGEN EXCHANGE. Arnold II. R. SAM repor t 2 AR-4 (A-105). Jan. 9, 1943.

EQUILIBRIUM TIME. Mayer H. L. SAM Memorandum 4 M-4. Jan. 5, 1943.

146

B. HIGH CONCENTRATION PROCESS.' Mayer H.', Bonner R. SAM Report 4 R-19. fob. 2, 1943.'

9. TPIE N PROCESS.Quinn G.F.SAM Report 3 R-16 (A-510). Jan. 4, 1943.

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11. COMPLEMENT SEARCH OF INTERCEPTION OF HYDROGEN ATOMS BY AMMONIA MOLECULES.'Mund W.', Huyskens P . , Lor ies R. Bull. Classe Sci. Acad. Roy.'Belg.'35, 995, 1949.

12. SLOW EXCHANGE OF HYDROGEN IN AMMONIA SALT SOLUTIONS. Brodski A. I . , Sulima L. V. Dokl. Akad. Nauk. SSSR 74,513-5, 1950.

13, BNL-Document C-4027. Bigcleiscn J . 1950. (Classified)

14. REACTION BETWEEN DEUTERIUM AND AMMONIA ON EVAPORATED METAL CATALYSTS.'Singleton J . II. , Roberts E. R . , Winter E . R . S.' T r a n s . Farad. 'Soc. '47, 131Ü-31, 1951.

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PROGRESS R E P O R T O F IH E CHEMISTRY D E P A R T M E N T . CONCENTRATION OF DEUTERIUM BY CHEMICAL EXCHANGE PROCESSES. I n t e r i m R e p o r t for A p r . 15-Ju ly 1 ,1951 . B i e g e l e i s e n J . , E l l io t N. , F r i e d m a n L . , I r s a A. P . , Kant A . , P e r l m a n M. L . , P r o s s e r H. C. (BNL, Upton N . Y . USA) B N L - 1 1 8 . Aug. 1951 . Dec i . J a n . 5, 1956.

AMMONIA PROCESS FOR DEUTEJIIUM.CONCENTRATION. T h o m p s o n W. I. ( F e r g u s o n I-I. K. Co. Atomic E n e r g y Div. / N e w York , USA). H K F - 1 1 3 . Sept . 4, 1951 . D e c i . F e b . 20, 1957.

P L A T E E F F I C I E N C Y IN THE EXCHANGE O F DEUTERIUM B E T W E E N AMMONIA AND HYDROGEN. P e r l m a n M. L . , B i e g e l e i s e n J . (BNL, Upton N. Y. USA) B N L - 1 4 3 . Dec . 3 , 1951. D e c i . Dec . 3 , 1955.

THE CONCENTRATION OF DEUTERIUM BY CHEMICAL E X CHANGE BETWEEN HYDROGEN AND AMMONJA. B ige le i sen J . , P e r l m a n M. L . BNL«.1.4(i. I)tic. J.5, 1051 . Dec i . Dec . 5 , 1 9 5 5 .

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DISPROPORTIONATION IN DEUTERATED AMMONIA. Bigele isen J . J . Cham. P h y s . 20 ,1945-6, 1952.

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DISPROPORTIONATION IN DEUTERIATED AMMONIA. Stedman D . F . J . Chem. Phys . 20, 718-21,1952.

CATALYSIS ON EVAPORATED FILMS. I.'THE EFFICIENCY OF DIFFERENT METALS FOR THE REACTION BETWEEN AMMONIA AND DEUTERIUM. Kembal l C. P r o c . Roy. Soc. (London) A 2.14, 413-26, 1952.

KINETIC STUDIES ON IRON UTILIZED AS CATALYST FOR AMMONIA SYNTHESIS. I. TEMPERATURE E F F E C T ON EXCHANGE REACTION RATE BETWEEN DEUTERATED . AMMONIA AND HYDROGEN. Enomoto S. Shokubai 8, 47, 1952.

REACTION OF AMMONIA AND DEUTERIUM ON EVAPORATED NICKEL CATALYST. Kemball C. T r a n s . F a r a d . Soc. 48, 254-8, • 1952.

THE MECHANISM OF THE EXCHANGE OF HYDROGEN GAS WITH SOLUTIONS OF POTASSIUM AMIDE IN LIQUID AMMONIA. Wilmarth W. K. , Dayton J . C. J . Am. Chem. Soc. 75, 4553-6, 1953. (NP-4339;U-23788)

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31. EXCHANGE REACTION BETWEEN AMMONIA AND D E U T E RIUM. Miyahara K. J . R e s . J n s t . Ca t a ly s i s , Hokkaido Univ. 4, 193-8 ,1957 .

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SOLUBILITY OF GASEOUS MIXTURE (N2+3H2) IN THE LIQUID AMMONIA. LefrahgòiV'ÌB., Vaniscot te C. Genie Chimique 83, 5 / 139-45; 1960.

SATURATION OF A GASEOUS MIXTURE (N2+3H2). WITH AMMONIA IN THE PRESENCE OF LIQUID AMMONIA AT. 300 AND ' 500 k g / c m % E T W E E N - 7 0 ° C AND +60°C. Lefrancois B . , Vaniscof-tè C.Chaleur Ind.419, 183-6, 1960. (In French)

HEAVY WATER, FRENCH RESEARCH AND PROCESSING. Paulsen F . R . N u c l . Energy, 471-3 , Oct. 1960.

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EXCHANGE OF DEUTERIUM BETWEEN HYDROGEN AND LIQUID AMMONIA. Bourke P . J . , Lee J . L. T r a n s . Inst j , Chem., :. Engrs.39, No. 156, 280, 1961.

THE ISOTOPIC EXCHANGE BETWEEN GASEOUS HYDROGEN AND LIQUID AMMONIA. PART I: THE KINETICS OF THE EXCHANGE I N A BUBBLING CONTACTOR. Rebora P . L. (L. R. S. R , , Milan, ITALY). Energ ia Nucleare 9, 388-96, July 1962. (In English)

A NEW PROCEDURE FOR THE PREPARATION OF HEAVY WATER BY ISOTOPIC EXCHANGE. Roth E . (CEN, Saclay, FRANCE) Energ ie Nucl .4 , 332-42,_Sept. -Oct . 1962. (In F rench) ...

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KINETICS OF ISOTOPE EXCHANGE BETWEEN HYDROGEN , AND LIQUID AMMONIA ON HETEROGENEOUS CATALYSTS. ' Haul R . , Blenheman D. J.' Ca ta lys i s 1(5), 432-42 ,1962 .

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SOLID-LIQUID EQUILIBRIA IN THE NHg-KNHg SYSTEM. Moreau C . L e p o u t r e G. Bull. Soc. Chcm. (France)No. 8, 1721-3, 1963. (In F rench )

DETERMINATION OF THE SEPARATION FACTOR OF DEUTERIUM BETWEEN AMMONIA AND HYDROGEN. Ravoi re J . , Grandcol lot P . , Di r ian G. (CEN, Saclay, FRANCE). J . Chini . P h y s . 60, 130-8, J a n . - F e b . 1963. (CEA-R-2244. 1963)

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HYDROGEN EXCHANGE BETWEEN D2 AND NH3 CATALYZED BY EVAPORATED Ni FILM. Mjyahara K. J.' Res . Inst ; Ca t a ly s i s , Hokkaido Univ. 11(2), 129-31 , 1963.'

1SZ

GAS ABSORPTION PERFORMANCE OF BUBBLE COLUMN-(with Special Reference to the NH3-H2 process for Deuter ium Separation).'Bourke P.'J. ' , Pepper D. Trans . Inst. Chem. Engrs . (London) 4.1(1), 40-50, 1963,

THE AMMONIA HYDROGEN EXCHANGE SYSTEM FOR THE ENRICHMENT OF HEAVY WATER.'Schindewolf U. , Walter S. Abt. Deut. Akad. Wiss .Ber l in , Kl. Chem.', Gcol. Biol. 7, 163, 1964.

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CATALYSIS BY ALKALINE AMIDES OF THE ISOTOPE EXCHANGE BETWEEN HYDROGEN AND LIQUID AMMONIA. Delmas R. , Courvoisier P . , Ravoire J . J . Chim. Phys. 62, 1423-5, Nov. -Dec. 1965. (In-French)

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DECOMPOSITION OF AMMONIA ON A NICKEL CATALYST. Tamaru K., Tanaka K. , Fukasalai S. , Ishida S. T rans . Faraday Soc. 61, No. 4, 765-72, 1965.

(On Heavy Water Production). Can. Chem. Process ing P-56 . June 1966.

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ISOTOPIC EQUILIBRIUM IN THE HYDROGEN-AMMONIA SYSTEM. Barb D . , Moraru N. Stud. Cercet . Fiz . Bucharest 19,131-9,1967.

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REPARATION FACTOR IN THE ISOTOPE EXCHANGE REACTION BETWEEN LIQUID AMMONIA AND HYDROGEN. Sakharovski Yu. A. ,Ze l ' vens id Y a . D . At .Encrg . (USSR) 25,499-503,1968.

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63. ..DjjO'FROM SYNTHESIS GAS LOOKS PROMISING. Can. Chem.' Process .52:71-4 ,Sept ; 1968.

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D20 SUPPLY ACCORDING TO THE H 2 /NH 3 DUAL TEMPERATURE PROCESS. Becker E. W., Lang G., Schindewolf U. (Univ. Karlsruhe; Kernforschungszentrum, Karlsruhe, W, GERMANY) Atomwirt. , Atomtech. 14, 257-60, May 1969. (In German)

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'.'•• 3 - Hydrogen - Water Exchange (H2Ò - HD)

CATALYTIC ACTIVITY OF ALKALI LYE FOR H2O-HD ISOTOPIC EXCHANGE. Wirtz K. , Bonhoeffer K. F . Z . physik. Chemie 117A, 1, 1936. (In German)

THE KYDROGEN-WATER VAPOR EXCHANGE REACTION ON METAL CATALYSTS. P r o g r e s s Report . A-149. March 10, 1942. Deci. Dec. 6, 1955.

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CATALYSTS FOR WATER-HYDROGEN AND AMMONIA-HYDROGEN EXCHANGE. Urey H . C . , Arnold H. R. SAM Report A-330, Oct. 20/1943.

CALCULATION OF CONVERSION EFFICIENCY. J o r i s G. G. , Hiskey C. F . , SAM Report A-36 3. Nov. 5,1942.

THE EQUILIBRIUM H2+HDO=HD+H20 AND FURTHER EXCHANGE EQUILIBRIA IN THE SYSTEM H2, D 2 , AND H 2 0 .

, Suess II. E.' Z . Naturforsch. 4a, 328-32, Aug. 1949. (In German)

HEAD LOSSES OF HYDROGEN AND STEAM MIXTURES THROUGH A CATALYST BED SUPPORTED BY ACTIVE CARBON. 'Ce r r a iE . ' ,Roseo L.' La Chimica e l ' Industr ia 36; 603,1954.' • _ l \ ; -

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8. A T H E R M A L METHOD FOR CONCENTRATING.HEAVY,WATER... C e r r a i E . , Marche t t i C . , Renzoni R . , Roseo L. ' , S i l v e s t r i M.', V i l lani S. ( L a b o r a t o r i CISE, Milan, ITALY). NUCLEAR ENGINEERING; P A R T I. C h e m . Eng . Progr . ' Sympos ium Ser . 'No. 11 , 2 7 1 - 8 0 . 1 9 5 4 . (Ene rg i a Nucleare (Mi lan) 2 , No. 14, 257-71;, 1955)- (In I tal ian)

9,' E F F I C I E N C Y OF SOME CATALYSTS IN THE EXCHANGE R E A C - ' TIONS BETWEEN HEAVY WATER AND HYDROGEN. Savie P . , R ibn ikar S . , Pav lov ic B . 8, P / 9 5 8 . ( YUGOSLAVIA).'.lst UN Geneva Conf. 1955.

. 10. CATALYSTS FOR DEUTERIUM EXCHANGE B E T W E E N HYDROGEN AND WATER. Br igo l i B . , C e r r a i E , P r e s e n t e d at Sympos ium on Heavy Wate r , Rome , Italy, Mar.' 31 -Apr. ' 2, 1955.

1 1 . THE ISOTOPIC EXCHANGE BETWEEN HYDROGEN AND WATER ON PLATINUM. RELATIVE RATES OF EXCHANGE OF ISOTOPIC HYDROGEN MOLECULES. Hannerz K. (Royal Ins t , of T e c h . , Stockholm, SWEDEN). Acta Chem. Scand. 10, No. 4, 655-66 , 1956.

13.'.. PREPARATION AND BEHAVIOR OF SOME CATALYSTS FOR DEUTERIUM ISOTOPIC EXCHANGE REACTION BETWEEN HYDROGEN AND WATER VAPOR. Br igo l i B . , C e r r a i E . , Renzo -ni R . , S i l v e s t r i M. Nuovo Cimento No. 3, Suppl. Vol. 5, S e r . X, 478, 1957. (In I tal ian)

13. THERMODYNAMIC AND KINETIC PECULIARITIES OF ISOTOPE-EXCHANGE REACTIONS OF HYDROGEN..Varshavskiy Ya. M . , V a i s b e r g S. E . Usp. Khim. 27, 1434-68, 1957. (In Russ ian)

,:;.A,' RADIATION-INDUCED EXCHANGE OF DEUTERIUM B E T W E E N HEAVY WATER AND DISSOLVED HYDROGEN. B a r d w e l l J . , Dyne P . J . Can. J . Chem. 35, 82-8 , J a n . 1957.

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P r o c . Int. Symp.' on Isotope Separation, Apr , 1957.' North Holland Pubi . 'Co. 'Amsterdam 1958:

STUDY OF CHEMICAL EXCHANGE BETWEEN HYDROGEN AND ,' WATER IN PRESENCE OF LIQUID PHASE-CATALYST.'.Montarmi, R# , Balaceànu J, 'C. ' , Dirian G. ( Inst . 'Francais du Pe t ro le , Rueil; CEN Saclay, FRANCE) p."247-71.'.(IFP-1554.'Apr.' 1957);

MASS AND PIEAT TRANSFER IN CONCURRENT. LIQUID-GAS FLOW. POSSIBLE APPLICATION TO SOME SEPARATING PROCES-. SES AND TO SOME SEPARATING UNITS. Finzi S . , Renzoni R . , .' S i lves t r i M. , Villani S. (CISE, Milan, ITALY).P- 44-61; (Energia Nucl . , Milan, 4, 211-21, June 1957).

ENRICHMENT OF HEAVY WATER IN HIGH PRESSURE EXCHANGE BETWEEN HYDROGEN AND AN AQUEOUS CATALYST SUSPENSION. PART I. Becker E . W. , HÜbener R. P . , Kess le r R.W.'. Chem. Ing .Tech . 30, 2 88-96, 1958. (In German) (AERE-Lib / t r ans -799 . 1958)

THE CATALYSIS OF THE H 2 - D 2 0 EXCHANGE BY AQUEOUS BUFFER SOLUTIONS. Miller S. L . , Rittenberg D: (Columbia Univ. NY, USA). J. Am. Chem. Soc. 80, 64-5, Jan . 1958.

EXCHANGE REACTIONS BETWEEN HYDROGEN GAS AND HYDR03ÖTL GROUPS. A CONVENIENT PREPARATION OF TRITIUM-LABE LED WATER. Swain C. G. , Kresge A. J . (Massachuset ts Inst, of Tech. .Cambr idge , USA). J , Am. Chem. Soc. 80, 5281-3, Oct. 5, 1958.

ENRICHMENT OF HEAVY WATER BY HIGH PRESSURE EXCHANGE BETWEEN HYDROGEN AND AN AQUEOUS SUSPENSION OF A CATALYST. Becker E . W . , Bier K. ,Hl lbener R. P . , Kess le r R .W. (Univ. of Marburg) . 4, P /1000. (GERMANY). 2nd UN Geneva Conf, 1958.

.' EXCHANGE OF DEUTERIUM AND HEAVY OXYGEN AMONG HYDROGEN, WATER VAPOR AND OXIDE CATALYSIS OF SPINEL TYPE.Yukio Yoneda,Akio Fujimoto, Shoji Makishima.'

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KINETICS OF CATALYZED GAS-LIQUID. REACTION IN A • STIRRED REACTOR. DEUTERIUM EXCHANGE BETWEEN' , GASEOUS HYDROGEN AND LIQUID WATER. Sai toH. ' , Moritd N. , S a t a k a O . Kagaku Kogaku 23, 45078, 1959;

THE E F F E C T OF SOME HYDRODYNAMIC FACTORS ON THE CATALYTIC DEUTERIUM EXCHANGE BETWEEN HYDROGEN AND WATER VAPOR. Selecki A. Nukleonik a 5, 513-30, 1960.

DEUTERIUM-EXCHANGE REACTION BETWEEN WATER AND HYDROGEN. Selecki A. Wiadomosci Chem. 14, 741-58; 1960.

PLATINUM CATALYSTS FOR THE HYDROGEN-WATER VAPOR ISOTOPIC EXCHANGE REACTION. Margineanu P . , P i r inger O. , Szentgyb'rgy P . IFA Report, Bucharest , 1960. (Unpublished))

ISOTOPIC EXCHANGE OF DEUTERIUM BETWEEN HYDROGEN . AND WATER IN THE VAPOR PHASE. Baran W. J. , Crete l la R . F . Arg. Com. Natl. Energia At. Informe No. 57, 1961.

INFLUENCE OF H2-D2O ISOTOPIC EXCHANGE OCCURING ON . TPIE SURFACE ON Pd-H ELECTRODES ON THEIR POTENTIAL. Bucur R.V. Rev. Physique (Bucharest) 6,269, 1961.

CATALYSTS ON THE ENRICHMENT OF HEAVY WATER BY MEANS OF EXCHANGE REACTION. Saburo Enomoto, Hiroaki Ugajin (Utsunomiya Univ. JAPAN). Shokubai (Tokyo) 3, No. 2, 126-30, 1961. (In Japanese)

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THE ISOTOPIC EQUILIBRIUM OF A HYDROGEN-WATER SYSTEM.' Barb D . , Mercea V.' IFA-IDF 13, Bucharest, 1961.

THE EQUILIBRIUM OF THE H2-H2Ó ISOTOPIC.EXCHANGE REACTION. Ciobotaru T . , Szcntgyörgy P . , Margineanu-P. IFA Report, Bucharest, 1961. (Unpublished)

ENRICHMENT OF HEAVY WATER BY HIGH PRESSURE EXCHANGE EETWEEN HYDROGEN AND AN AQUEOUS CATALYST SUSPENSION. PART III. EFFECTS ON SPECIFIC EXCHANGE PERFORMANCE OF ADDITIVES. Becker E . W . , Kessler R .W. , HÜbener R. P . (Technische Hochschule, GERMANY). Chem.Ing. Tech. 34, 105-8, 1962. (KFK-92) (In German)

DUAL TEMPERATURE SEPARATION SYSTEM FOR THE ISOTOPIC EXCHANGE COMBINED WITH VAPOR DIFFUSION. Margineanu P . , Mercea J. ' , Mercea V . , Olariu A. IFA Report, Bucharest, 1962. (Unpublished)

KINETICS OF THE CATALYTIC EXCHANGE REACTION OF DEUTERIUM BETWEEN WATER VAPOR AND HYDROGEN ON VARIOUS SURFACES. Nakhmanovich M . L . , Morozov N . M . , Buadze L . G . , Temkin M.I . (Karpov Inst, of Physics and Chemistry, Acad., of Sciences, USSR). Dokl. Akad.Nauk SSSR148, 1346-9, Feb. 21, 1963. (In Russian)

THE HOMOGENEOUS CATALYSTS OF THE ISOTOPE EXCHANGE BETWEEN HYDROGEN AND LIQUID WATER. Schindewolf U.' J. Chim. Phys. 60/124-9, 1963.

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DUAL-TEMPERATURE HYDROGEN ISOTOPE EXCHANGE BETWEEN A GAS VAPOR MKTURES AND A SOLUTION OF GAS. Vaisberg S. E . , Varshavskii Ya. M. Zh. F iz . Khim. 37;. 87-93,1963. (In Russian)

HEAVY WATER PRODUCTION BY H2-H2O ISOTOPIC EXCHANGE. Mercea V . , Peculea M. , Grecu E . , Pal ibrodaN.-IFA Report, Bucharest , 1963. (Unpublished)

THE INFLUENCE OF CAPILLARY CONDENSATION ON THE. ACTIVITY OF N i - C r 2 0 3 CATALYSTS FOR THE ISOTOPE EX-. CHANGE REACTION BETWEEN HYDROGEN AND WATER. Barb D . , Margineanu P . , Mercea V. , Olariu A. Abh. Deut. Wiss . Berl in, Kl. Chem. , Geol . , Biol. 7, 793-9, 1964.

KINETICS OF THE ISOTOPE EXCHANGE BETWEEN HYDROGEN AND WATER. (Compensation Effects). Marazan N . , Margineanu P . , Olariu A. Abh. Deut. Akad. Wiss . Berl in, Kl. Chem. , Geol. Biol. 7, 811-9, 1964.

THE ISOTOPE EXCHANGE BETWEEN HYDROGEN AND WATER. Mahadevan E . G . Indian J . C h e m . 2(1), 1-5,1964.

DEUTERIUM ENRICHMENT BY DUAL TEMPERATURE EXCHANGE REACTION BETWEEN HYDROGEN AND WATER. Sawayanagi S. , Kurihara Y. Koatsu Gasu Kyokaishi,27, 626-32,1964.(In Japanese)

NOMOGRAM FOR SOME CALCULUS FOR THE HYDROGEN-WATER ISOTOPE EXCHANGE REACTION. Szentgyörgy P . ' Stud. Cerce t . F iz . (Bucharest) I16, 729,1964.

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ISOTOPIC EXCHANGE BETWEEN HYDROGEN AND WATER VAPORS IN A-STREAM REGIME OVER A POROUS .CATALYST LAYER. Palibroda E . , Palibroda N., .IFA Report, Bucharest 19G4. (Unpublished)

LIQUID PHASE CATALYSIS OF DEUTERIUM EXCHANGE REACTION BETWEEN WATER AND DISSOLVED HYDROGEN. (S.M. Thesis) . Barthelemy R. (MIT, Mass. USA). Feb. 1964.

RATE OF EXCHANGE OF DEUTERIUM BETWEEN WATER AND DISSOLVED HYDROGEN IN PRESENCE OF DIMETIIYLAMINE. Ishida T. , Benedict M. (MIT, Mass . , USA). MIT-2249-1, Feb . 1964.

HOW D2O MAY BE MADE IN SASKATCHEWAN. Can. Chem. P rocess .49 ,71-5 ,1965 .

KINETICS OF ISOTOPE EXCHANGE BETWEEN HYDROGEN AND WATER VAPOR OVER NICKEL CATALYSTS. I. EFFECT OF TRANSPORT PROCESSES ON THE REACTION RATE.' Nedumova E. S. , Boreskov G.K. , Slin'ko M.'G." Kinetika i kataliz 6, 65-73, 1965. (In Russian)

INFLUENCE OF THE PRESSURE ON THE ACTIVITY OF Ni- „ r 2 0 3 CATALYST IN THE HYDROGEN-WATER ISOTO-PLC EXCHANGE REACTION. Margineanu P . , Mercea V . , Olariu A. IFA Report, Bucharest , 1965. (Unpublished)

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PRODUCTION OF HIGH ACTIVITY N i - C r 2 0 3 CATALYST, FOR THE HYDROGEN-WATER ISOTOPIC EXCHANGE. ' ,.. REACTION • Bolojga- M; , :Szentgy.örgyi P.' IFA ;.Reppr t; Buchare• -x, ," 1965. (Unpublished) .

THE TRITIUM BETA-RAY INDUCED REACTIONS IN DEUTERIUM OXIDE VAPOR AND HYDROGEN OR CAREON MONOXIDE AND THE EXCHANGE OF.H-ATOMS WITH WATER MOLECULES. Bibler N. E. Columbus, Ohio, Ohio State Univers i ty , 1965.

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DEUTERIUM SEPARATION BY AMMONIA DISTILLATION AND HYDROGEN-WATER EXCHANGE. Benedict M. MIT-2249-2. 1965. ' . '

HOMOGENEOUS CATALYSIS OF D 2 / H 2 0 EXCHANGE BY .Ru(III)Cl3. EVIDENCE FOR HETEROLYTIC SPLITTING OF H 2 . H a l p e r n J . , J a m e s B . J . Can. J . Chem. 44, 671-5 ,1966 .

DEPENDENCE ON pH OF THE RATE OF DEUTERIUM EXCHANGE BETWEEN HYDROGEN AND WATER ON NICKEL CATALYST. Enyo M. , Matsushima T. J . Res . ' lns t . Cata l . Hokkaido Univ. 14, 248-56, 1966.

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.DETERMINATION OF THE TRANSPORT CONSTANTS FOR CATALYZED HYDROGEN-WATER VAPOR-WATER'ISOTOPIC EXCHANGE REACTION. Hodor ' I . ', Moraru . N . , Pecu lqa M. Sampaleanu L. IFA R e p o r t , B u c h a r e s t , 1966. (Unpublished)

COMPARATIVE TREATMENT OF HYDROGEN POISSONING OF THE P t -ACTIVE CARBON AND Pd-ACTIVE CARBON CATALYSTS IN THE ISOTOPIC EXCHANGE- REACTION BETWEEN HYDROGEN AND WATER. S t rugaru D . , : Paladi '• M . , P i r i n g e r O. Stud. C e r c e t . F i z . (Buchares t ) 18, 1081, 1966.

ISOTOPE EXCHANGE AND EQUILIBRATION REACTION ON NICKEL IN THE SYSTEM DEUTERIUM-LIGHT WATER. Enyo M. J . Res . ' lns t . Catal . 'Hokkaido Univ.' 15 ,1 -20 ,1967 .

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ISOTOPE EXCHANGE O F DEUTERIUM BETWEEN HYDROGEN AND WATER" VAPOR ON ALUMINA-PROMOTED NICKEL. Olariu A.', Margineanu P . Rev.'Roum.' P h y s . 13, 823 -8 ,1968 . .

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2.1. UNSTATIONARY MASS TRANSPORT IN RECTIFICATION COLUMNS. Rozen A. M. Dokl. Akad. Nauk. SSSR 107, 295-8, 195G. (In Russian)

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43. INDUSTRIAL SCALE RECTIFICATION OF HYDROGEN. Scholz W.Kältetechnik 13,184-8,1961.

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ISOTOPIC FRACTIONATION OF WATER BY DISTILLATION. H&ll N. F . , Jones T. O. J . Am. Chem. Soc. 56, 749-50, 1934,

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CONCENTRATION OF HEAVY WATER BY SPONTANEOUS EVAPORATION. Hughes E. D . , Ingoici C. K. , Wilson C. L. Nature 134, 142, 1934.

THE ISOTOPIC FRACTIONATION OF WATER DUE TO EVAPORATION AND DISTILLATION. I-Iarada M. , Titani T. BuU. Chem. Soc, Japan 10, 41-2 ,1935.

ISOTOPIC SHIFT OF WATER BY DISTILLATION. Horiuchi J . , Oka moto G.' Bull. Chom. Soc. Japan 10, 503-5, 1935.

DISTILLATION AND RECTIFICATION OF DILUTE SOLUTIONS OF VOLATILE COMPOUNDS. I. THEORETICAL STUDY AND ..• APPLICATION TO THE CASE OF HEAVY WATER. Jau lmes P . Chimie et Industrie 33, 1045-52,1935.

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(On D2O Separation by Dist i l lat ion)Dunn C. L . , Mil ler R. W. , P icro t t i G. J . , Shires R. N . , Souclors M. J r . T r a n s . Am. Inst , Chem. Eng r s . 41 , G31-44,1945.

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ELECTROLYSIS AD A METHOD FOR THE PRODUCTION OF HEAVY WATER. Vasa ru G . , B u c u r R . V . IFA-AG-2 (Cluj) Oct. 10, 1969 (Unpublished)

ISOTOPIC FRACTIONATION OF HYDROGEN IN THE WATER-HYDRONIUM ION SYSTEM. Z n a m i r o v s c h i V. Rev .Roum. P h y s . 14, 175-81 ,1969 .

LABORATORY ENRICHMENT O F HEAVY WATER BY E L E C T R O LYSIS. 'PART I.'DESIGN O F ELECTROLYTIC CELLS AND CAL-C U L A T I O N O F THE MEAN CURRENT DENSITY. Hallaba E . , i l ly A . I . M. (Atomic Energy Es tab l i shmen t , Cai ro) . ' I so topenpraxis 7, No. 10, 427-30 , Oct . 1971.

194

89. LABORATORY ENRICHMENT OF HEAVY WATER BY E L E C T R O LYSIS. PART II. E F F E C T OF CURRENT DENSITY, CATHODE MATERIAL, AND TEMPERATURE ON THE SEPARATION FACTOR. Hallaba E . , A.ly A. I. M. (Atomic Ene rgy Es tab l i shmen t , C a i r o ) . I sotopenpraxis 7, No. 11-12, 456-9 , N o v . - D e c . 1971.

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IV. D. 1. 1 - INDUSTRIAL HEAVY WATER PLANTS AS OF FEBRUARY 1974

N. C ountry Location

Plants based on H2S/HDO Process

1.

2.

3 .

4 .

5.

USA

Canada

India

Savannah River

Glace Bay

Port Hawkesbury

Bruce

Kota

Plants based on NHs/HD Process

6.

7.

8.

India Baroda

Tuticorin

Talcher

Plants based on Hi distillation

S. India Nangal

Plants based on Electrolysis

10. Norway Rjukan

Capacity t/year

180

360

360

2x365

100

67

71

63

14

20

Constructor o'r owner

Gir ller-Lummus/Dupont

Spevack-Burns & Roe/Deuterium of Canada Ltd.

Lummus/Can. G. E. Ltd.

Lummus /Can. G. E. Ltd.

Dept. Of Atomic Energy

Group. Eau Lourde Proced. Ammoniac /Dept. of At.E nergy

Group. Eau Lourde Proced. Ammoniac/Dept. of At. Energy

Uhde/Dept. of Atomic Energy

Linde/Dept. of Atomic Energy

Norsk Hydro

Remarks

In operation since 1952 Final enrichment: H20 distillation

In trasformation Final enrichment: H2O distillation Start-up: 1975

In operation since 1970 Final enrichment: ÔdistUlation (Sulzer)

In operation since 1973

Engineering. Start-up: 1975

One temperature process Start-up: 1974

One temperature process Start-up:1974

Dual temperature process Final enrichment: H2O distillation (Sulzer) Start-up: 1975

In operation since 1962

In operation since 1934 Final enrichment: H2O distillation

(IV.A-175)

199

PRODUCTION PI-ANTS

2 - Plants based on HgS / TIPO P r o c e s s

THE OPERATION OF A DUAL-TEMPERATURE SINGLE STAGE TOWER FOR DEUTERIUM CONCENTRATION. Eidinoff M.L. , Hiskey C. F . (Columbia Univ. , New York. Div. of War Research; USA). A-718. May28, 1943. Deci . Nov. 1, 195G.

DUAL TEMPERATURE HEAVY WATER PROCESS EVALUATION OF PROPOSED TESTING AND PRODUCTION PROGRAM AT WABASH ORDNANCE WORKS. (Girdler Corp. Gas P r o c e s s e s Div. Louisville, Ky. USA). NYO-681. Apr. 21 , 1950. Deci. Feb. 27, 1957.

DANA PLANT TECHNICAL MANUAL. P a r t . I. Bebbington W. P . , Keller W. R. (E. I. du Pont do Nemours v Co. USA). DPTM-1 . Dec. 15, 1951.

THERMAL BEHAVIOUR OF COUNTER-CURRENT EQUIPMENT. Hull H . A . , Pohl H.A. (Du Pont Co.AED, Wilmington, Del. USA). D P - 9 7 . D e c . 1954. Deci . Apr. 15, 1957.

INDIANA D 2 0 PLANT OFF STREAM. Nucleonics 15, No. 1, R 12, Jan .1957 .

AMERICAN HEAVY WATER PLANT TO SHUT DOWN. Atomics 8, No. 2, 39, F e b . 1957.

200

OECD D 2 0 PLANT IN ICELAND? Atomwir t schaf t 3, No. 1, 294 , Ju ly 1958.

HEAVY WATER. Pari; 6. FLOWSHEETS, DESIGN AND COST ESTIMATION FOR 22 AND 3G t / y e a r PRODUCTION PLANTS USING II2S PROCESS. Walker P . T . , Lyon C. J . , Handley D. , Hcnsley J . D. C . , P r a t t II. R. C. A E R E - C E / R - 2 3 4 3 . 1958.

SECOND D2O PLANT. Atomwir t schaf t 4, No. 5, 222 -3 , May 1959.

A PRELIMINARY APPROACH TO THE CALCULATION OF A WATER-HYDROGEN SULPHIDE DUAL T E M P E R A T U R E DEUTERIUM SEPARATING PLANT. Br igol i B . , Villani S. (CISE, Milan, ITALY) Energ ia Nuc lea re (Milan) G, 784-92 , Dec. 1959.

PRODUCTION.OF HEAVY WATER. SAVANNAH RIVER AND DANA PLANTS. Techn ica l Manual . Bebbington W. P . , T h a y e r V. R. eds . (Du Pont de N e m o u r s E . I . &Co. Savannah River L a b . , Aiken, S. C. USA). D P - 4 0 0 J . F . P r o c t o r comp. Ju ly 1959. (TID-4500)

HEAVY WATER PRODUCTION IN THE USA. Thayer V. R. Nucl. P o w e r 5, No. 4G, 103-11 , F e b . 19G0.

FLOWSHEETS AND SUPPLEMENTARY DATA FOR THE HEAVY WATER PLANT DESCRIBED IN Chem. Eng. P r o g r . 58, 53-61, ' No. 4, Apr i l 19G2. P r o c t o r J . F . , Thaye r V. R. (Du Pont de N e m o u r s E . I. & Co. Savannah R i v e r L a b . , Aiken S. C. Wilmington, Del . USA) TID-15733. 19G2.

HEAVY WATER POWER REACTOR PROGRAM MONTHLY PROGRESS REPORT, FEBBRUARY 1SG3. (Savannah R i v e r Opera-t ions Office, AEC, USA). SRO-80. 1963.

•K^^fjr^-ît-J^J^wt»» J i n r - - T * * - T rv,"rr~-Tyû'-rTiW*^TiT-7^»* V- \-V

201

15, USAEC-AECL COOPERATIVE PROGRAM MONTHLY PROGRESS R E P O R T , JANUARY 1964. I l i lborn II. S. comp. (Du Pont de Nemours E . l . & Co. Savannali R ive r L a b . Aiken, S. C. U S A ) , D P S T - 0 4 - 3 3 - l .

lf>. USAEC-AECL COOPERATIVE PROGRAM MONTHLY PROGRESS R E P O R T , FEBRUARY 1964. I l i lborn H. S . , comp. (Du Pont de N e m o u r s E . I. &. Co. Savannah R i v e r L a b . , Aiken, S. C. USA). DPST-G4-33-2 . Mar . ID, 1964.

17. I ISAEC-AECL COOPERATIVE PROGRAM MONTHLY PROGRESS R E P O R T , MARCII.UHM. Hilborn U . S . comp. (Du Pont de Nemours E . [. & Co. .Savannah River L a b . , Aiken, S. C. USA). D P S T - 6 4 - 8 3 - 3 . Apr. 17, 19(54.

18. USAEC-AECL COOPERATIVE PROGRAM MONTHLY PROGRESS R E P O R T , APRIL 1964. Beach J . E . , comp. (Du Pont de Nemours E . I . & Co. Savannah River L a b . , Aiken, S. C.USA). DPST-G4-83-4 . May 15, 1964.

19. USAEC-AECL COOPERATIVE PROGRAM MONTHLY PROGRESS REPORT, MAY 1904. Hilborn II. S . , comp. (Du Pont de Nemours E . I . & Co. Savannah R ive r Lab. , Aiken, S. C. USA). D P S T - 6 4 - 8 3 - 5 . June 18, 1964.

20. USAEC-AECL COOPERATIVE PROGRAM MONTHLY PROGRESS REPORT, JUNE 1964. Hi lborn H. S . , comp. (Du Pont de Nemours E. ' l . & Co. Savannah River L a b . , Aiken, S. C. USA). D P S T - 6 4 - 8 3 - 6 . July 15, 1964.

21 . USAEC-AECL COOPERATIVE PROGRAM MONTHLY PROGRESS REPORT, JULY 1964. Hilborn II. S. (Du Pont de N e m o u r s E . I . &Co. Savannah River L a b . , Aiken, S. C. USA). D P S T - 6 4 - 8 3 - 7 . Aug. 24 ,1964 .

202

22. HEAVY WATER PLANT. Prospec t , T!ie Lunumis Co. Canada LUI. 1968.

23. THE STATUS OF CANADIAN CONSTRUCTION PROJECTS. PART II. HEAVY WATERAND OTHER.NUCLEAR PROJECTS. Can. Nucl. Assn. Annual Conf. June 19G9.

24. MAJOR CHANGES RECOMMENDED BEFORE DEUTERIUM'S PLANT OPERATIONAL. Chem.Can. 21, 33-4, Nov. 1969.

25. BRUCE HEAVY WATER PLANT. Robinson R. D. (Lurnmus Co. Cauda, Ltd. Don Mills, Ontario). P rog re s s Report . 70-CNA-423. May 1970.

CNEN Symposium on Technical und Economic Aspects of Heavy Water Production. Turin, Italy, Sept. 30-Ocl. 1, 1970:

20. FABBRICATION AND CONSTRUCTION EXPERIENCE. BRUCE AND PORT IIAWKESBURY HEAVY WATER PLANTS.Spray P. II .G. ( A EC L.CANADA);

27. DESIGN CRITERIA FOR HEAVY WATER PLANT BASED ON H 2 S-H 2 0 EXCHANGE PROCESS. Bhargawa R. K., Sadhukhan H. K., Scligal I. J . S . , Deslipande P. G. (Bhabha Atomic Research Center Trombuy-Bombay, INDIA).

28. BRUCE AUXILIARY STEAM SUPPLY.Kolisnyk Z . (Montreal Engineering Co. Ltd. ), Spray P . H. G. Eng. J . (Montreal) 55 ,No.4 , 22-G,Apr. 1972.

29. SINGLE UTILITY ELECTRIFIES NOVA SCOTIA. Mod. Power Eng. GG,No. 8, 56-7, Aug. 1972.

203

D - PRODUCTION PLANTS

3 - Plants Based on NII3/HD Exchange Process

1. HEAVY WATER PRODUCTION. Constructors John Brown Ltd. (UK). Brochure presented at the 2nd UN Geneva Conf.1958.'

2. ENRICHMENT OF DEUTERIUM THROUGH HIGH PRESSURE ISOTOPIC EXCHANGE BETWEEN HYDROGEN AND LIQUID AMMONIA IN A HOT-COLD PLANT. Walter S., Schindewolf U. Chcm.Ing. Tocli. 37, No. 12,1185-91, 1965,(Angew. Chemie.'77, No. 14, 620,19G5,Angew.Chcm.Inst.Ed. Eng.4,597, 1965)

HEAVY WATER FROM COAL?. Colliery Guardian 208, 212, Feb. 14, 1964.

HEAVY WATER PLANT AT MAZINGARBE. Lefrancois B.Bull. Inform. Sci. Tech. (Paris) No. 123, 11-20, Feb. 1968. (In French)

HEAVY WATER PLANT. Le Chatolier J. Bull. Inform. Sci. Tech. (Paris) No. 123, 21-5, Feb. 19G8.(In French)

?.0<t

A PILOT PLANT FOR DUAL TEMPERATURE EXCHANGE FOR STUDIES TO DEVELOP NII3- IJ2 PROCESSES. Kostaing M. Bull. Inform. Sci . Tech . (Par i s ) No. 12 3, 27-30, Fob. 1Ö6Ö.

THE HEAVY WATER, PLANT OF MAZ1NGARBE. Roth E . (CEN, Sac-Jay, FRANCE), l.'.edhome A. , Lefrancois B . , Le Chalolicr J. Tillol A. Enorg . Nucl. (Par i s ) 10, 2.1.4-1.9, May 11H>1}. (In French)

MAZ1.NCAUBE HEAVY WATER PLANT. Nu el . Eng. Int. 14, 578-80, .iLily IDfii).

THE MAZINGARBE HEAVY WATER PLANT. Société Chimique des Charbonuages . CEA. Nuolc.x 19G9.

INDIA'S AEC PROPOSES A $.1. ß-BILLION, 10-YEAR. NUCLEAR POWPIR PROGRAM. Nucleonics Week 11, No. 30, fi, Aug. G, 1070.

CNEN Symposium on Technical and Economic: Aspec ts of Heavy Watc 1- Production. Turin, Italy. Sept. 30-Oct. 1, 1970:.

OPTIMIZATION OF DEUTERIUM PRODUCTION PLANT WITH THE AMMONIA-HYDROGEN SYSTEM. SchtndcwolJ' U., Lang G. (Inst. fUr Kernverl 'a lnonstochnik, K.FK Kar l s ruhe W. GERMANY);

PROBLEMS OF DESIGN AND CONSTJÌUCTION OF A PLANT FOR THE PRODUCTION OF HEAVY WATER BASED ON THE DUAL-TEMPERATURE AMMONIA-HYDROGEN EXCHANGE SYSTEM. Waller S . , Nttschke E . (F r i ed r i ch Ulule G. ni. b. II. Dortmund, W. GEH MANY):

205

13. PROBLEMS ON A CONCEPTUAL DESIGN OF A JJEAVY W A T E R Ì

PRODUCTION P L A N T . - C O N T R I B U T I O N OF AG1P NUCLEARE. Bracc i l'orli L. , Cnbclla A . , Durant i Vnlenìiiii P . (AGTP Nuc lea re , Jlaly) ;(ln f-.i'liaii)

14.. OPERATING EXPERIENCE OP* MAZINGARBE HEAVY WATER P L A N T . i_,e!'rancni,s Jl. (Sor.. Chiiniquc clc Cliurbonnago,FRANCE) (fn P'vench).

15. CRITERIA FOR THE DESIGN OF NII3-H3 TWO-TEMPERATURE PLANT FOR HEAVY WATER PRODUCTION. Fol l i E. (CISE), P o l a s t r i F . , Vacca ro G. Energ ia Nuc lea re (JVIilaii) 17, 721-32, Doc . 1970

16. OPTIMIZATION OF HEAVY-WATER ENRICHMENT PLANT BASED ON LI2/NH3'EXCHANGE AND OPERATING BY THE HOT/COLD PRINCIPLE. Lang G. , SchindcwoH' U. Chcm. Ing. -Tech . 43 , No. 14, 004-10, Ju ly 1971. (in German)

207


4 - P lan ts Based on I-Ip.O/lID Exchange P r o c e s s

1. TRAIL REPORT. Weight M.M. Aug. 28, 1944.

2. THE PRODUCTION OF HEAVY WATER AT TRAIL B. C. Barlow E. A. (AECL, Chalk River, Ont. CANADA). CRE-374. Mar. 8, 1948. Deci. F e b . 22, 1955. (AECL-163)

CALCULATION OF THE PERFORMANCE OF EXCHANGE IN THE PRODUCTION OF HEAVY WATER. Car l son II. C . , Maloncy J. O^ A-327. Oct. 7, 1942. Deci . May 14, 1954.

4. CATALYTIC EXCHANGE ELECTROLYTIC PROCESS FOR THE ISOLATION OF HEAVY WATER AT TRAIL B. C. Maloney J. O . , Quinn G. F . , Ray II. S. Product ion of Heavy Water . G. M. Murphy, H. C. Urcy, I. Kirshenbaum eds . McGraw Hill 1955. (NNES-III-4F) p .9 -52)

5. A METHOD FOR THE GRAPHICAL CALCULATION OF THE NUMBER OF THEORETICAL PLATES IN AN ELECTROLYTIC PLANT AITH EXCHANGE TOWERS FOR THE PRODUCTION OF HEAVY WATER. DinelJi D. Energ ia Nucleare (Milan) 2, 426-33, Aug, 15, 1955. (In I ta. l ian)(AERE-Lib/trans-G06)

208

6. .CALCULATION METHODS FOR TRANSFER COLUMNS. Villani S. Energ ia Nucleare (Milan) 2, 504-18, 1955.

7. DEUTERIUM SEPARATION COLUMNS AND HEAVY WATER. S i lves t r i M . , Villani S', P r e s e n t e d at Symposium on Heavy Wate r . Rome, Italy, March 31-Apr. 2, 1955.

8. RECENT EXPERIMENTS ON THE PRODUCTION OF HEAVY WATER BY ELECTROLYSIS AND ISOTOPIC EXCHANGE REACTIONS.Finzi S.', Ronzoni R . , S i lves t r i M. Energ ia Nuclear e (Milan) 3, No. 4, 294-308, Aug. 195G.(In Italian)

9. HYDROGEN-WATER VAPOR CONDENSERS DESIGN. Finzi S . , Ronzoni R . , S i lves t r i M. , Zava t t a re l l i R. (CISE, Milan, ITALY). Energ ia Nucleare (Milan) 4, 199-210, June 1957.

10. A NEW PROCESS FOR THE MANUFACTURE OF HW WAS SHOWN. ACTIVITIES INCLUDING THE PRODUCTION OF U, Th, Z r , REACTOR FUEL ELEMENTS, CONTROL RODS & R E FRACTORIES. Degussa (Germany) . Atomics and Nuclear Ene rgy 9, No. 10, 341, Oct. 1958.

11 . DEGUSSA UHDE LARGE PILOT PLANT CONSTRUCTION. Atomkernene rg ie 3, 362, 1958.

12, DEGUSSA PLANT. Nuclear Engineer ing 3, No. 29, 352, 1958.

13. ENRICHMENT OF HEAVY WATER BY HIGH PRESSURE EXCHANGE BETWEEN HYDROGEN AND AN AQUEOUS CATALYST SUSPENSION.PART II. CONSTRUCTION AND OPERATION OF A PILOT PL-ANT. Walter S . , Nitschke E . , Bode C. ( F r i e d r i c h Uhde GmbH, Dortmund, GERMANY). Becker E. W . , Huebener R. P . , K e s s l e r R. 'A. , Schindewolf U. Chem. Ing. Tech . 3 4 , 7 - 1 0 , 1 9 6 2 .

209

14. LABORATORY PILOT PLANT FOR THE EXPERIMENTATION OF ISOTOPIC PROCESS AT HYDROGEN-WATER EXCHANGE REACTION IN A BITHERM SYSTEM. Fcculca M,, Boian M. , Fatu C . , Potior T. IFA Ilcpoi't, Buchares t , 030/19G5. (Unpublished)

15. INSTALLATION FOR HEAVY WATER PRODUCTION BY THE HYDROGEN-WATER ISOTOPIC EXCHANGE REACTION OCCURRING IN A COLUMN AND WITH PHASE CONVERSION BY ELECTROLYSIS, IN THE RANGE OF 5-99, 8% DEUTERIUM. Boian M. , Mcrcea V. , Pa l ibroda N . , Pcculea M. IFA Report , Buchares t , G9G/19G7. (Unpublished)

1C. CAUSTIC SODA SOLU'TlON AS CATALYST FOR ISOTOPIC EXCHANGE BETWEEN HYDROGEN AND WATER IN A TRANSFER COLUMN FOR TECHNICAL CONCENTRATION OF DEUTERIUM. SchindewoLl' U . , Hornke J . Chem. Ing. Tech. 40, 29-30, 1968. (In German)

17. ENRICHING COLUMN FOR THE SEPARATION OF LIGHT WATER BY ISOTOPE EXCHANGE REACTION BETWEEN HYDROGEN AND WATER. Mcrcca V . , Pa l ibroda N . , Fodor T . , Stoicovici L. Isotopenpraxis 4, 328-30, 19G8. (In German)

18. EFFICIENCY OF THE EXCHANGE SPACE WITH DIFFERENT STRUCTURES IN A CATALYZED HYDROGEN-WATER VAPOR-WATER ISOTOPIC EXCHANGE REACTION COLUMN. Boian M. , Hodor I.', Pcculea M. , St raulca R . S . IFA Report (Bucharest) IS-50-.1DG8.

211


5 - Disti l lat ion P lan ts

1. CONCENTRATION OF THE OXYGEN ISOTOPES. Urey H. C . , Peg ram G. B . , Huffman J . R. J. Chem. Phys . 4, 623, 1936.

2. DISTILLING APPARATUS FOR THE SEPARATION OF ISOTOPES. P e g r a m G. B. , Urey II. C . , Huffman J. R.- Phys . Rev. 49 ,883 , 1936.

3. SEPARATION OF OXYGEN ISOTOPES BY A FRACTIONATING COLUMN. Huffman J . R . , Urey H. C. Ind. Eng. Chem. 29, 531-5 ,1937.

4. PACKED FRACTIONATION COLUMNS AND THE CONCENTRATION OF ISOTOPES. Cohen K. J . Chem. Phys . 8, 588-97, 1940.

5. OPERATING MANUAL OF WATER-DISTILLATION UNITS. Monier J . A. 1941.

6. PRODUCTION OF HDO WATER BY DIRECT METHOD. Amick M. G. SAM Report A-394. Dec. 4, 1942.

212

7. PRELIMINARY PLANT DESIGN. Huffman J . R. SAM Report A-402. Dec. 1, 1942.

8. FRACTIONATION OF LIQUID HYDROGEN. Huffman J. R. Columbia Memo. Nov. 11, 1942.

0. (On Hydrogen Distillation). Johnston II. L. Ohio State Universi ty . P rogress Report. SAM Report A-501. Jan. 9,1943.

10. SEMIWORKS DISTILLATION TESTS. Carlson R. C. Du Pont Engng. Dopt. Report Mar. 8, 1043.

11. THE SE PARATION OF ISOTOPES BY THE DISTILLATION OF WATER. Thode H. G., Smith S. R . , Walking F . O. Can. J. Res. 22 3 ,127-36,1944.

12. A CONVENIENT AND EFFICIENT FRACTIONATING COLUMN AND ITS USE IN THE SEPARATION OF THE HEAVY ISOTOPES OF HYDROGEN. Dostrovsky I . , Hughes E.D. Nature 153, 164-5, 194G.

13. FRACTIONAL DISTILLATION AND ITS APPLICATION IN THE CONCENTRATION OF HEAVY ISOTOPES OF OXYGEN' AND HYDROGEN. Dostrovsky I . , Hughes E. D. , LleweUyn D. R. Nature 161,858-9,1948.

213

INDUSTRIAL FRACTIONATING-TOWER PACKING. Scottele! R. C. Cliem. Eng, P r o g r e s s <IG, ,405-14, 1950.

STATUS REPORT ON HEAVY WATER PRODUCTION PROGRAM. DESIGN OF PRODUCTION PLANT-HYDROGEN DISTILLATION PROCESSES, HYDRO-CARBON RESEARCH, INC., CONTRACT AT (3.0-1) -810, DESIGN OF PILOT AND PRODUCTION PLANT AND CONSTRUCTION OF PILOT PLANT-DUAL-TEMPERATURE PROCESSES, THE GIRDLER CORPORATION, CONTRACT AT(30- l ) -947.NYO-699. June 19, 1950, Deci. Jan. 15, 1959.

SOME CHARACTERISTICS OF STEDMAN PACKING IN THE DISTILLATION OF HYDROGEN AND ITS ISOTOPES.'Fooicson A. , Pomerantz, P . , Rothberg.S. J. Research Nat. Bur . Stds. 47, 449-55, Doc. 1951.

STUDIES ON ISOTOPES. III. THE PERFORMANCE OF STAINLESS STEEL GAUZE RING PACKING IN THE . ISOTOPIC FRACTIONATION OF WATER. Mackenzie II. A. E. Malherbe P . N. J , S . African Chem, Inst. 4 ,69-78 ,1951 .

LOW TEMPERATURE HEAVY WATER PLANT. (Hydrocarbon Research Inc. USA), NYO-889. Mar . 15, 1951. .

OPTIMAL FLOW IN FRACTIONATING COLUMNS FOR ISOTOPE SEPARATION.'DostrovskyI. ' ,Gill is J . , Vromen B .H. Bull. Research Council I s rae l 2, 68-9,1952.

214

HYDROGEN - LIQUIFYING PLANT FOR SCIENTIFIC RESEARCH INSTITUTES. Malkov M. P . , Fradkov A . B . Zhur. Tekh. F iz . 22, 6, 1952. (In Russian)

ANALYTICAL METHODS FOR THE CALCULATION OF CASCADE SYSTEM OF RECTIFICATION COLUMNS. Zliavoronkov N. M., Zelvenskii Ya. D. Sbornik Protsess . i i Appara t i Khimicheskoi-' Tcklmologn. Goskhimizdat, Moscow 1953. (In Russian)

THE STEAM VENTS OF TUSCANY AND THE LARDERELLO PLANTS. Mazzoni A. 2nd. Ed. Calderini , .Bologna, 1954.(In Italian)

DW PLANT OPERATING CHARACTERISTICS. Blair J . A. (Du Pont do Nemours E . I . & Co.Savannah River Lab.-, Augusta Ga. USA) .TID-5337.June l8 , 1954. Deci . Mar . G, 1957.

TILE KUHN PRECISION RECTIFYING COLUMN. Sulsser Tech . . Rev. (Switz. )No. 2, 36-47, 1955.

A PRELIMINARY STUDY OF SOME ASPECTS OF A HEAVY WATER PLANT. Tech. Memo. No. 30. Vander Arend P . C. (NBS-AEC Eng. Lab . , Boulder, Colo. USA). NBS-3519. Feb . 11, 1955.

THE DESIGN OF ISOTOPE SEPARATION PLANTS. SOME DESIGN EQUATIONS FOR THE DISTILLATION PROCESS. Dostrovsky I. Presented at Symposium on Heavy Water . Rome, Italy, Mar. 31-Apr. 2, 1955. (CNRN Rome 1956)

THE DESIGN OF ISOTOPE SEPARATION PLANTS:SOME BASIC. DESIGN EQUATIONS FOR THE DISTILLATION PROCESS. Dosirovsky I . , Lehre r Y. 8,.P/774 (ISRAEL). 1st Geneva Conf. 1955

215

28. WATER DISTILLATION PROCESS FOR THE ISOLATION OF HEAVY WATER AS EMPLOYED BY E. I. DU PONT DE NEMOURS & CO. Inc. AT MORGANTOWN. Maloney-J. O.\ Quinn G. F . , Ray II. S. NNES-III-4 F, '55-83,1955.

29. SPRAY-PACK: A NEW INDUSTRIAL DISTILLATION AND AB-SORBPTION TOWER PACKING. McWilliams J. A. , Prat t U.R. G., Dell F . R . T r a n s . I n s t . Chem.Engrs . (London) 34, No. 1, 18-43,3 956.

30. THE CASCADING PROBLEM IN A WATER DISTILLATION PLANT FOR HEAVY WATER PRODUCTION. Cer ra i E . , Silves t r i M. , Villani S. Z . Naturforsch. I l a , G94-7Ü1, 1956.

31. PRELIMINARY PROJECT REPORT FOR THE NANGAL FERTI LIZER HEAVY WATER PROJECT. Saint Gobain, P a r i s , France . Apr. 195G.

32. PRELIMINARY PROJECT REPORT FOR THE NANGAL FERTILIZER HEAVY-WATER PLANT. Par t II. VLtro Engineering Div. New York. Aug. 195G.

33. FURTHER DEVELOPMENTS OF SPRAY-PACK : DISTILLATION COLUMN PACKINGS. McWilliams J . A. , Pra t t II. R. G. AERE. CE/R 1941. Nov. 15, 1956.

34. A DYNAMIC PROGRAMMING SOLUTION TO A PROBLEM IN HEAVY WATER PRODUCTION. Bellman R. (RAND Corp. , Santa 'Monica, Calif. USA). Nuclear Sci. and Eng, 2, 523-5, July 1957.

35. DESIGN ASPECTS OF PLANT FOR PRODUCTION OF HEAVY WATER BY DISTILLATION OF HYDROGEN. (Arthur D. Litt le Inc . , Cambridge, M a s s . USA).NYO-2134.Dec. 11, 1957.

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30. DESIGN CRITERION FOR WATER DISTILLATION PLANT FOR HEAVY WATER PRODUCTION. Canini R. P r o c . Int. Syinp, on Isotopes Separat ion 1957, North Holland Pubi, Co. Amste rdam 1958. (p. 360-82)

37, THE PILOT PLANT AT BOULDER. T immerhaus K. D . , Wcitzel D. II. , Flynn rr. M. Cliem, Eng. P rogr . 54, No, G, 36-4G, June 1958.

38. INDUSTRIAL SCALE HYDROGEN-DEUTERIUM DISTILLATION SEPARATION IN FRANCE. Chem. Engineering P r o g r . 54, No. 11, 12G, 128, 1958.

39. ON DISTILLATION COLUMNS FOR ISOTOPE SEPARATION, I-Iavlicek F. I. (J, Stephan Inst. Ljubljana, YUGOSLAVIA). Ene rg . Nucl. (Milan) 5, No. 8, 527-30, Aug. 1958.

40. A LABORATORY APPARATUS FOR DEUTERIUM ENRICHMENT BY THE RECTIFICATION OF LIQUID HYDROGEN, Weisser R. H. Sulzer Tcch.il. Rev. (Switzerland) 40, No. 3, 71-4 ,1958 .

4 1 . DESIGN OF THE FINAL STAGES OF. DEUTERIUM PRODUCING FLANTS. Lehrer Y . , Woissnian Y. ( Is rael Atomic Energy Comm i s s i o n ) ^ , P / l u l l . (ISRAEL). 2nd UN Geneva Conf. 1958.

PRODUCTION OF HEAVY HYDROGEN IN A LARGE-SCALE RECTIFICATION PLANT. Lehmer W. , Sel lmaier A . , Baldus W. Linde Ber . Tech. u. Wiss . 5, 3-14, 1959. (In German) (NP-tr -417)

HOW LINDE MAKES HEAVY WATER FROM HYDROGEN. Chem. Eng. GG, No. 4, 68, 70, 72, Feb . 23, 1959.

http://Tcch.il

217

THE PILOT PLANT FOR LIQUID HYDROGEN DISTILLATION AT TOULOUSE;StoulsE.Bul i r inf ;Sci . et Tech. (Paris) No. 40, 4-10, May 1960. (In French) • '"'

WATER DISTILLATION. THE PILOT PLANT OF SOULOM. Lazard B. Bull. Inf. Sei. et .Tech. (Par is ) No. 40, 11-13, May 1960. (In French)

PILOT PLANT DATA FOR HYDROGEN ISOTOPE DISTILLATION. Flynn T. M. (NBS, Boulder .Colo. USA). Chem. Eng. Progr . 56, No. 3, 37-42, Mar. I960.- •

. THE McCABE-THIELE DIAGRAM FOR ISOTOPE SEPARATION AND A GENERAL FORMULA FOR CALCULATING THE NUM-: ; BER OF THEORETICAL PLATES IN A MASS EXCHANGE COLUMN. Dietze M. , Pilz S. Chem. Techn.' 12, No. 2, 81-7, 1960. (In German)

McCABE-THIELE DIAGRAM .FOR THE IDEAL CASCADE. , Slirowiec A. J.. Ind. Eng. Chem.' 52, 789, 1960.

INDUSTRIAL INSTALLATION FOR PRODUCTION OF HEAVY-WATER AT LOW TEMPERATURES. Hanny J. Schweiz. A r c h . , Angew.Wiss .u .Tech . 26', 115-28, 1960. (CEA-tr-A-943)

A LOW-TEMPERATURE PLANT FOR THE PRODUCTION OF HEAVY WATER. Hanny/J. Sulzer ,Tech. Rev. (Switz; ) 42, No. 2 , . 9-24, 1960.

INDUSTRIAL INSTALLATION/FOR THE SEPARATION OF DEÙr.' TERIUM FROM LIQUID HYDROGEN BY RECTIFICATION. : Haenny J . P rob lems of Low Tempera tu re Physics and Thermo>v

dynamics.New York, McMillan Co.'Vol. 2.1960. (p. 29-45) '.

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218

52. ISOTOPIC DESIGN OF A PLANT FOR PRE-CONCENTRATION, OF HEAVY WATER BY DISTILLATION OF WATER, STARTING WITH NATURAL WATER. Ceri-ai E . , Si lvestr i M. , Villani S. j (CISE, Milan, ITALY). CISE-81. Sept. 1960. (In Italian) j

53. RECENT ADVANCES OF DISTILLATION TECHNICS. Brigoli j B . , Energia Nucleare;(Milan): Par t I, 7, No. 9, 590-G, Sept. 1960; ] Pa r t II. 7, No. 11, 7G1-8, Nov. 1960. j

* 54. CALCULATION METHODS FOR FRACTIONATING COLUMNS.

Brigoli B. Energia Nucleare (Milan) 7, No. 12, 845-8, Dec. I96 0.

55# ' HEAVY WATER PLANT MELDS NEW FEATURES. Chopey N. P . Chem. Eng. G8, No. 4, 118-21, Feb . 20,1961.

5 6 A DISTILLATION PLANT FOR H2OI8 ENRICHMENT. Adorni N . , Angelino G. , Brigoli B . C h e m . Age; of India 12, No. 4, 333-7, July -Aug.19G1.

57. PREDICTING TRAY EFFICIENCY IN DISTILLATION COLUMNS. Coates J . , P r e s s u n g B. S.Chcm. Engr. 68, 8 ,187-90 ,1961.

58. OPTIMUM REFLUX CONDITIONS FOR COLUMNS OF ISOTOPE SEPARATION. Olariu A. Stud. Cerce t . F iz . (Bucharest) 13, No. 6, 939-45,19G2.

59. KOCH-SULZER RECTIFICATION COLUMNS. Koch Engineering Co. New York, (USA). Bulletin KS-1.

§p•.•;• 60. HIGH PRECISION DISTILLATION COLUMNS. Kuhn W. Bull. Mp, ; Assoc . F r a n c . Techniciens Pe t ro l e 154, 559-91,1962. . t]

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219

CI. ON THE INDUSTRIAL ADAPTABILITY OF THE PACKINGS .OF THE HEAVY WATER DISTILLATION TOWER. Masami S. (Showa Dcnko K. K,, JAPAN), Shimizu M., Matsumoto S. Nippon Genshiryoku Gakkaishi 4(2), 85-94, Feb. 1962. (In Japanese)

G2. SOME ANALYSES ON • THE OPERATION OF WATER RECTIFICATION TOWER. Masami S. , Shinichi H. (Keio Univ., Tokyo, JAPAN). Nippon Genshiryoku Gakkaishi 4, 313-21, May 1962. (In Japanese)

G3. FINAL-AND RECONCENTRATION OF HEAVY WATER BY MEANS OF KUHN-SULZER COLUMNS. ThUrkauf M. (JEN, Madricl;EAES, Paris) . ColloquLum on Heavy Water, Madrid. Dec. 13-14, 1962. NP-1376G (p. 77-83)

G4. PERFORMANCE OF A COCURRENT DISTILLATION CONTACTING DEVICE. Angelino G., Brigoli B. »Silvestri M. Energia Nucleare (Milan) 10,85,1963.

65. SULZER RECTIFICATION PLANTS FOR SEPARATING D20 FROM H2O. Huber M., Sperandio A. Sulzer Tech. Rev. (Switz. ) 46,177-88,1964.

66. ANALYSIS OF OPERATING EXPERIENCE OF A HYDROGEN DISTILLATION PLANT; Gami D. C . , Rapial A. S. 12, P/754. (INDIA). 3rd UN Geneva Conf. 1964.

67. CHARACTERISTICS AND DESIGN OF A CO-CURRENT DISTILLATION COLUMN. Angelino G. , Brigoli B . , Silvestri M. Energia Nucleare (Milan) 12, 353, 1965. ..

68. INSTALLATION FOR HEAVY WATER PRODUCTION BY DISTILLATION IN THE CONCENTRATION RANGE OF 5-ütf, 8% DEUTERIUM. IFA (Bucharest). Rep. 1667/1967. (Unpublished)

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220

69. STAINLESS WELDING MEETS STRINGENT TEST ON HEAVY WATER PLANT. Can. Mach. Mctalwòrk. 79, 6G-7, May 1968.

70, RECTIFICATION OF HEAVY WATER IN COLUMNS IN PARALLEL. , Gisper t M. , Rojas J . L. (JEN Madrid, SPAIN).An.'Quim. 64, 7G5-74, Ju ly- Aug. 1968.

71 . HEAVY WATER RECOVERY PLANT. P rospec t .L inde A. G. 5 6 7 / 2 E . 1 9 6 8 /

72. NATURAL WATER DISTILLATION PLANT. Selecki A. (Warsaw Technical Univ . , P O L A N D ) . N u c l e a r - E n g . . . Int. 15, No. 172, 717-9, Sept. 1970.(CNEN Symp. Tur in , I ta l i . Sept. 30-Oct . 1, 1970)

7 3 EFFICIENCY OF AN EXCHANGE P L A T E IN CONCURRENT. Brigoli B. (CISE, Milan, ITALY) CNEN Symp. on Technical ed. Economic Aspec t s of Heavy Water Product ion . Tur in , Italy Sept. 3 0 - O c t . l , 1970.

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6 - P l a n t s based on Electrolysis df Water

1. APPARATUS FOR THE SEPARATION OF ISOHYDROGEN (DEUTERIUM) OXIDE BY ELECTROLYSIS. Harkins W. D . , Doede C. J . Am. Chem. Soc. 55,4330-1, 1933.

CONTINUOUS-FLOW METHODS OF CONCENTRATING DE.U-TERIUM. Anderson L. C . , Halford J . O. , Bates J. R. J. Chem. Phys .2 , 342-4, 1934.

3. PRODUCTION OF LARGE QUANTITIES OF HEAVY WATER. Tronstadt L. Nature 1.33, 872, 1934.

4. A LABORATORY SET-UP FOR THE ELECTROLYTIC FRACTIONATION OF HYDROGEN ISOTOPES. Erlenmayer H. , Gartner H'. II. Helv. Chim. Acta 17, 1226-31,1934. III. Helv. Chim. Acta '1TB, 419-20, 1935.

5. LABORATORY APPARATUS FOR THE ELECTROLYTIC CONCENTRATION OF THE ISOTOPE 2 OF HYDROGEN. Champetier G. Bull. Soc. Chim. France (5) 2; 162-7, 1935.

PLANT. O FOR THE PRODUCTION OF HEAVY WATER. Brown ; Wj. G. , Daggett A. F . J . Chem. Phys.,3, 216-8, 1935.

Sì AIP LE EQUIPMENT FOR ELECTROLYSING HEAVY WATER., Slack C. M. , Ehrke L. F . Rev. Sci. Insti-, 8, 39, 1937.

PRODUCTION OF HEAVY WATER. Alcksandrovich V. A. Novosti Teknniki No. 26-7, 5 0 - 1 , 1939.

INEXPENSIVE EQUIPMENT FOR THE PREPARATION AND CONCENTRATION OF PURE D2O DEUTERIUM RICH WATER. DESCRIPTION OF CONSTRUCTION AND OPERATION OF THE FORMER OHIO STATE UNIV. HEAVY-WATER PLANT. Johnston II. L . , Hall W.H.Ohio J . Sci . 41 , 357-65, 1941.

OPERATING MANUAL OF THE ELECTROLYTIC PLANT AT MORGANTOWN. Monier J . A. 1941

SECONDARY PLANT EVAPORATION. C a v e r s S .D. CMS Rep . 3, Sect . 953, May 18, 1944.

(On Deuter ium and Heavy Wa te r Analys i s ) . Wright M. M. T r a i l Rep. 63, Aug. 2Q, 1944.

ELECTROLYTIC P - 9 PRODUCTION OPERATING MANUAL. I la r ty W.'M.'(Du Pont de N e m o u r s E . I . & Co. Morgantown Ordnance Works , Morgantown, W..Va. USA) M-3132.Sept . 1, 1945. Dec i . Jan . 12, 1956.

PRE CON CENTRATION OF HEAVY WATER IN ELECTROLYSIS PLANT. Orsoni B . P r o c . X I Ins t . Congr . P u r e and Applied Chem. (London) 5, 1057-63, 1947. (Chim. e Indus t r . 30, 232-4,1948)

184 " CYCLOTRON DEUTERIUM ELECTROLYZER TESTS. Repor t No. l l . S t e p h a n W. 'J . (Univ. 'Berkeley, Cal i fornia ,Radiat ion Lab. U S A ) . M - 3 7 l 2 . M a r . 2 0 , 1947 .Dec i .Nov. 29, 1955.

223

IG. AUTOMATIC EQUIPMENT FOR ÉLECTROLYZING HEAVY WATER. Wanick R . W . Rev. 'Sci . I n s t r . 21 , 2G2, 1950.

17. ELECTROLYTIC CONCENTRATION OF HEAVY WATER.II CONTINUOUS OPERATION PLANTS. Or soni L.", S i lves t r i M." CISE-17.1050. '(In Italian)

18. AN AUTOMATIC HEAVY WATER'ELECTROLYSIS APPARATUS, Rabinovich E . S . , D o u g l a s J . 'E . Rev. S c i . I n s t r . 22 Z 9.Nov. 1951.

19. THE CONTINUOUS ISOTOPIC ENRICHMENT BY CASCADES. Walen R . R e c . Tx-av. Ins t . 'Rech. S t ruc tu re Mat ié re (Belgrade) 1,35-G7,1952.

20. A DEUTERIUM ELECTROLYSIS PLANT Lloyd J . T . J . Sci . I n s t r . 2 9 , N o . 5 , 1G4-5, 1952.

21 . OUTLINES OF SMALL-SIZED ELECTROLYTIC PLANT FOR D 2 0 AT HYGII DEGREE OF CONCENTRATION. C e r r a i E „ Orsoni L . , S i lves t r i M.CISE-32 , 1952. (In Italian)

22. I I 2 0 - D 2 0 SOLUTIONS NEUTRALIZATION AND DISTILLATION PLANT. C e r r a i E . , S i l ve s t r i M, CISE-33.1952. (In Italian)

23. ELECTROLYTIC SYSTEMS WITH COLUMNS FOR THE RECOVERY OF DEUTERIUM BY THE EXCHANGE REACTION. C e r r a i E . / M a r c h e t t i C . , S i lves t r i M . , Villani S. P a r t i ;CISE R e P ; 6 1 ( A E R E - T r a n s - 8 3 4 ) . P a r t i i ; CISE-62. :July 30, 1954. ( A E R E - T r a n s - 835) P a r t IIlJ STUDY OF FOUR-STAGE SYSTEMS WITH COLUMNS CONSISTING OF CONDENSATION PLATES, WITH PARTICULAR REFERENCE TO THE YIELD AND OTHER CHARACTERISTIC PARAMETERS.'ECONOMIC CONSIDERATION CONCERNING THE RECOVERY OF DEUTERIUM; CISÉ-63. July 1954. (AERE-Trans -836)

224

A METHOD FOR THE GRAPHICAL CALCULATION OF THE NUMBER O F THEORETICAL P L A T E S IN AN E L E C T R O L Y T I C PLANT WITH EXCHANGE TOWERS FOR THE PRODUCTION Oli' HEAVY WATERpinc l l i D. E n e r g i a N u c l e a r e (Milan) 2 , 4 2 6 - 3 3 , Aug. 15, 1055.(1» I tal ian) (AERE-Lib/Trans-GOfi)

CALCULATION METHODS FOR TRANSFER COLUMNS. Vil lani S. E n e r g . Nuc l . (Milan) 2, 5.04-18, 1955.

A MERCURY SAFETY VALVE FOR ELECTROLYSIS OF HEAVY WATER. Chauclliri II,' M. '{Government C o l l . , L a h o r e , PAKISTAN) P r o e . P h y s . S o c . (London) B-G'8, 1157-8 , D e c . 1, 1955.

R E P O R T ON RECENT ITALIAN E X P E R I E N C E S IN THE P R O D UCTION ON HEAVY WATER USING PROCESS ELECTROLYSIS AND P L A T E TOWERS. F inz i S . , Ronzoni R . , S i lves t r i M. P r o c e edings of the Scientif ic C o n g r e s s , N u c l e a r Sess ion , Ju ly 2 -6 , 1956, 3rd E l e c t r o n i c - N u c l e a r In te rna t iona l Rev iew. (Roma, Nat ional Commi t t ee for Nuc lea r R e s e a r c h ) . 1956.

DESIGN OF AN ELECTROLYTIC P L A N T FOR THE CONCEN- ' TRATION OF HEAVY WATER. Deshp ancle P . O . , Gami D.C." 4, P /1G69. (INDIA). 2nd UN Geneva Conf. 1958.

THE E L E C T R O L Y T I C C E L L FOR HEAVY WATER PRODUCTION. K a w a s h i m a N. Kogyo Kogaku Z a s s h i 62, 487-98 , 1959.

DESIGN OF A PLANT FOR FINAL ENRICHMENT OF AQUEOUS SOLUTIONS OF D 2 0 U P TO CONCENTRATIONS OF 99, 8%; F i n z i S . , M a r c h e t t i C. , Ronaoni R . , S i l v e s t r i M'. P a r t I . 'CHEMICAL DESIGN-PHYSICS OF THE P L A N T . CISE-76. ' Juno 1960. P a r t I I -A. DESIGN AND CONSTRUCTION OF THE T Y P E E L E MENTS. OPERATING E X P E R I M E N T S . CISE-77 ; June I 9 6 0 . P a r t I I - B . CONSTRUCTION DESIGN OF T Y P E ELEMENTS.! C I S E - 7 8 . J u n e I 9 6 0 . " P a r t . III . TECHNICAL DESIGN, CISE-79 . July 19G0.'

225

31. PRODUCTION OF '.HEAVY WATER BY THE ELECTROLYTIC METHOD. Tai Y. K . , Hsu Y.' C. (Taiwan Univ.' CHINA) Ho Tsu K'o I-Isueh 2, 10-8, 1960.

32. PRODUCTION OF LOW-TRITIUM DEUTERIUM. Drury J . ' S . , Guymon R. H . , Joseph E." F j (ORNL, Tenn. USA). Chem.' & P r o ces s Eng. '42, 220-4, May 1961.

33. ON THE OPTIMUM CASCADE OP MANUFACTURING OP HEAVY WATER AS A BY-PRODUCT IN THE WATER-ELECTROLYSIS PLANT.ELECTROLYSIS-EXCHANGE REACTION+WATER RECTIFICATION+RECOVERY ELECTROLYSIS. Shimizu Ml (3rd T e c h . Div . , Showa Denkó K j K , , JAPAN), Kawashima K' Nito S . , Matsumoto 'S . J . A t . E n e r g y Soc. Japan 3, 770-8, Oct,! 1961. (In Japanese)

34. THE INDUSTRIALIZATION'OF THE ELECTROLYTIC CONCENTRATION METHOD OF HIGHLY' ENRICHED HEAVY WATER. Shimizii M.', Nito S.', Harada A. (In Japanese) P a r t I . ELECTROLYTIC CONCENTRATION CASCADE AND C E L L . Nippon Genshiryoku Gakkaishi 4, No. 3, 180-7, 19G2. P a r t II . RECOMBINATION AND REMOVAL OF ALKALI. Nippon Gerehirypku Gakkaishi 4, No.' 4, 211-7, Apr . 1962.

Repor t of the Colloquium on Heavy Water. ' J.' E.'N.' Madrid Dec '1962 (JEN and EASES). NP-13766:

35. A THEORETICAL STUDY ON THE UTILIZATION OF GAS SCRUBBERS IN A CASCADE OF ELECTROLYSERS AND ISO-TOPIC EXCHANGE. O te ro de l a Gandara J.' L . , M a r i a Arcoclia A . M . NP-13.766'(p.' 37-52);

36. A STUDY OF THE OPTIMUM HANDLING PROCEDURES OF A CASCADE OF ELECTROLYSERS AND ISOTOPIC EXCHANGE REACTORS BY MEANS OF AN ELECTRONIC COMPUTER. Otero de l a 'Ganda ra J . ' L . , Mar ia Arcocha A. M.NP-13766 (p. '53-76);

226

37. HEAVY WATER PRODUCTION. IN SPAIN.' DESCRIPTION OF THE. JEN-EIA PLANT AT SABINANIGO.'Gispert Bennach M.'(JEN, MadridjEAES, Paris) .NP-l3766.(p. '27-36).

38. STUDY ON THE PRODUCTION OF HEAVY WATER.'I.DESCRIPTION OF THE JEN-EIA INSTALLATION AT SABINANIGO.' Otero de.la Gandara J.'L.', Gispert Bennach M.(JEN, Madrid, SPAIN). Energia Nu ci . (Madrid) 8, No. 32, 4-11, Oct , -Dec. 1964. (In Spanish)

39. STUDIES. ON THE PRODUCTION OF HEAVY WATER. II. PILOT PLANT FOR ELECTROLYSIS AND BURNERS.'Otero de la' Gandara J . L . , Gispert Bennach Mi',Rojas J. 'L. 'Energia Nucl. (Madrid) 9, 90-4, M a r . - A p r . 1965. (In Spanish)

40. LABORATORY ELECTROLYZER WITH HIGH CURRENT CHARGE. Palibroda E . , Fodor T.' Rev. Chim. (Bucharest) 16, 94, 1965.

227

E - TECHNICAL AND EC ONO MIC-AS PEC TS

1. DUAL-TEMPERATURE HEAVY WATER PROCESS EVALUATION OF PROPOSED TESTING AND PRODUCTION PROGRAM AT WABASH RIVER ORDINANCE WORKS. (Gird ler Corp. Gas P r o c e s s e s Div . , Lu i sv i l l e , , USA), NYO-G81. Apr. .21, 1950, Deci . Feb . 27, 1957.

2. EVALUATION OF HEAVY WATER PRODUCTION AT GASEOUS DIFFUSION PLANT SITES. Blumkin S. , Dehoney R. W. , Shacter J . (Carbide and Carbon Chemica l s Co. K-25 Plant , Oak Ridge, Tenn. USA). K-843. Nov. 26, 1951. Deci . 27, 1955.

3. REPORT ON THE FEASIBILITY OF HEAVY WATER PRODUCTION IN INDIA. Brun J . June 1954.

4. DENSITY AND COST RELATIONS FOR D 2 0 AND SOLUTIONS OF UO2SO4 IN D2O. TBR Memorandum No. 2, Gaines A. L. (ORNL, Tenn. USA). CF-54-10-86 . 'Oct . 14, 1954.

5. CHEAP HEAVY WATER. Rae II. K. Chemis t ry in Can. 7, No. 10, 27-32, 1955.

G. ECONOMIC PROBLEMS IN THE PRODUCTION OF HEAVY WATER ' BY DISTILLATION OF NATURAL WATER, USING THERMOELECTRIC CENTER. Cas in i R. E n e r g i a nucl . (Milan) 3, 188-203,195G.

7. CHEAPER WAYS TO MAKE,D20. Ha r t eck .P . Nucleonics 14, No. 9,. 97^9,1956. . '•--. . ' • ' • ' ' .

228

CUTTING THE COST OF HEAVY WATER. Atomic World 9, No. 11, 382-5 , Nov. 19.58. . . .

CALCULATION OF D 2 0 ' COST. Atòmwir t scha r t 3, 36, Jan . 1958.

LESS D9O. Atòmwir t schar t 4, No. 5, 224,' May 1959.

SAVANNAH D 2 0 PLANT COSTS. Atomwir t scha f t 4, No. 10, 455, Oct. 1959.

SECRETS OF LOW COST HEAVY WATER. Labine R. A. Chem. Eng . G6 ,No .21 , 170-3 , Oct . 19","i~959.

EUROPEAN ATOMICS. F U E L GROWTH:U CONCENTRATES AND ENRICHED FUELS PRODUCTION IN INCREASING;MODERATORS AND OTHER AUXILIARIES ALSO GET ATTENTION. C h e m . E n g n g . News 37, No. 30, 64;1959.

TECHNICAL-ECONOMICAL STUDIES O F A PRIMARY UNIT FOR HEAVY WATER SEPARATION BASED ON 1SOTOP1C EXCHANGE REACTION AT HIGH PRESSURE AND SUSPENDED CATALYST. I F A - R e p o r t ( B u c a r e s t ) , F 5 , 1959. (Unpublished)

STUDIES O F THE MARKET FOR NUCLEAR MATERIALS. II. MODERATORS. B,HEAVY WATER. P a r i s , OEEC, 1959.

CHEMICAL AND BIOLOGICAL STUDIES WITH DEUTERIUM. Katz J . J . Am. Sc ien t i s t 48 , 544-80, Dec . 1960.

229

17. MODIFICATION IN THE PROCESS FOR THE PRODUCTION OF HEAVY WATER BY ELECTROLYSIS AND THE EXCHANGE REACTION. DECREASE IN THE STEAM CONSUMPRION. Gispert M. , Otero J . L. (JEN, Madrid, SPAIN). An. Real. Soc. Espan. F ì s . y Quim. (Madrid) Ser. E56, 559-68, I960. (In Spanish) (CEA-tr-X-411)

18. HEAVY WATER STAKES LURE NEW ENTRY. Chem. Eng. G7, No. 19, 92-4, Sept. 19,1960.

19. THE FUTURE FOR CHEAP HEAVY WATER. B a r r F . T . , Drews W. P. (Esso Res . and Eng. C o . , Linden, N. J . USA). Chem. Eng. P rogr .5G,No. 3 ,49-56, Mar. 196 0.

20. PRODUCTION AND APPLICATION OF HEAVY WATER. Kllchler L. (Farbwerke Hoechst AG, Frankfurt am Main, W. GERMANY). Chem. Ingr. Tech. 32, 773-81, Dec. I960. (NP-tr-647)

21. NATURAL ISOTOPES. II. SEPARATION CASCADES SOME PROBLEMS OF ECONOMICS AND ENGINEERING. Sclecki A. P r z e m y s l . Chem. Polska 40, No. 11,626-31, 19Gl.(In Polish)

22. THE ECONOMICS OF HEAVY WATER PRODUCTION. Proctor J . F . , Thayer V. R. (E. I. du Pont de Nemours & Co. Savannah River Laboratory) TID-139G4. Dec. 6, 1961.

23. THE PRODUCTION OF HEAVY WATER. Ruzicka J . Technika Hlubokych Teplot. CSAV Pubi. House, Prague 1961. (p. 43-108)

24. CHEAPER HEAVY'WATER A BONUS FOR AECL. Can. Chem. P r o c e s s . 46, 76-8 ,June 1962.

25. ECONOMICS OF HEAVY WATER PRODUCTION. Proctor J. F'. Thayer V. R. Chem. Eng. P rogr . 58, No. 4, 53,-61, Apr. 1962. (TID-15733) >

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2G. PRESENT STATE OF THE PRODUCTION AND OF THE MARKET OF URANIUM-235 AND HEAVY WATER. Villani S. (CISE, Milan,' ITALY). Energia Nucleare' ( Milan) 9, 212-25, Apr. 19G2. (In Italian) (AEC-tr-5200)

27. HEAVY WATER COST AND AVAILABILITY OF HEAVY WATER IN THE UK. Johnson K. D . , Walker P . T. AERE-R-3905. 19G2.

28. NUCLEAR MATERLALSrWHAT'S OUR FUTURE?Can. Chem. P r o c e s s . 47, G3, 65-G,Apr. 19G3.

29. POSSIBILITIES OF THE PRODUCTION OF HEAVY WATER IN ARGENTINA. Silber man E , , Crotella R. F . Commiss ion National de Energia Atomica Rep. No. 90. 19G3. (NP-13340)

30. WHY THE GS PROCESS STILL TOPS COMPETITORS. Law C. A. Can. NucLTeclmol. 3, 36-40, 19G4.

31. TECHNICAL-ECONOMICAL STUDIES ON INDUSTRIAL PILOT PLANT CONSTRUCTION FOR HEAVY WATER PRODUCTION AT U. F . S. Savinesti (Romania). Grecu E . , Mercea V. , Moraru N . , Olariu A . , Pal ibroda N . , Peculoa M. IFA Report (Bucharest) 033/ 13G4. (Unpublished)

Proceedings of the Third International Conference on the Peaceful Uses of Atomic Energy. Geneva Aug. 31-Sept. 9, 19G4:

32. PRODUCTION OF HEAVY WATER IN THE USA. Bebbington W. P . , P roc tor J . F . , S c o t t e n W . C . , Thayer V. R. 12, P/290(USA);

2 3 JL

33. TECHNICAL AND ECONOMICAL CONSIDERATIONS FORPRODUr CING200 t / y e a r OF HEAVY WATER IN INDIA. Deshpande P . G.',. Gami D, C.', Nagaraya Rao S. 12, P/753(INDIA).

34. ECONOMIC OPTIMUM OF A SATURATOR-SEPARATING COLUMN CONDENSER ASSEMBLY IN.AN ISOTOPE SEPARATION PROCESS.

' Peculea M. Rev. Roum.Phys; 10, No.'4, 393-402,1965.

35. HEAVY WATER-OUR STAKES IN THE FUTURE. Can. Chem. P r o c e s s . 50, 60;76, 1966.

36. COST OF HEAVY WATER PRODUCTION BY USING BITTERNS WATER. Kumar R. , Datta R. L. (Indian Inst, of Science, Bangalore, INDIA). Indian Chem. Eng. 8/No. 1,2-5, 1966.

3.7. ECONOMIC ASPECTS OF INDUSTRIAL PRODUCTION OF HEAVY . WATER. Malasek E . , &och O. Jad Energ . 12, 166-71, 1966. (In Czech)

•3.8. STUDIES ON THE ENERGETICAL OPTIMUM OF A ISOTOPIC SEPARATION COLUMN. Peculea M. Kernenergie 9, 351-5, 1966.

3.9. PRODUCTION OF HEAVY WATER AT THE NATURAL GAS FERTILIZER FACTORY, FENCHUGANJ. Shamsul A. K. M. (At. Energy Centre Dacca, Chemis t ry Div. PAKISTAN) AECD/CH-8. Feb.1966.

40. HEAVY WATER PRODUCTION.Report of an American Industrial Forum (A. I..F. ) Ad Hoc Commit tee . Apr i l 1966.

232

4.1. EXPERIMENTAL STUDY 'OF THE'.THERMOENERGETIC BEHAVIOUR OF AN ISOTOPIC SEPARATION INSTALLATION. Peculea M.'vBoiari' M.',' Fatu C . :Rev .Chim. (Bucharest) .'19, 524-9,1967.

42. A PRECISE ESTIMATION OF . PLANT AND' PRODUCTION COSTS FOR A HEAVY WATER PLANT(36, 2 t / y r ) ADDED TO A 545 t /day (600 sh . t /day) AMMONIA PLANT. Linde Aktiengesellschaft Werksgruppe, Munich:19&7.

4 3 ; THE OPTIMIZATION OF A CHEMICAL PROCESS WITH GREAT. ENERGY CONSUMPTION BY ENERGETICAL METHODS. Peculea M. 5th Coni. Ind. Power Economy, Prague 1967. (II/1-22)

44. D2Ò FROM SYNTHESIS GAS LOOKS PROMISING. Can. Chem. P r o c e s s . 5 2 , 71-4; 1968.

,'45. NEW LOW ENERGY PROCESS MAKES IMPACT ON HEAVY WATER PRODUCTION. Ellwood P . Chem Eng. (N.Y. ) 75, 56, 1968.

46. FLOODING BEHAVIOUR, OPTIMUM WORKING POINT, AND E F FICIENCY OF SEPARATION OF PACKED COLUMNS. Lentz H. C h e m . - I n g . - T e c h . 4 1 , 855-61,1968

47'. NELSON REFINERY COST INDEX. Nelson W.-L. (comp. )'Eri'g. ' News-Record 180, No. 12, 93, Mar. 21 , 1968.

.48. AECL WANTS A 400 t / y e a r ADDITION TO D 2 0 CAPACITY IN CANADA. Nucleonics Week 9, No. 12, 7, Mar. 21,1968.

•49. WORLD'S HEAVY WATER PINCH CREATES POLITICAL PROBLEMS. FOR AEC. Nucleonics Week 9, No. 18, 1-4, May 2,1968. ''

50: ALUMINIUM DESALTER'CUTS COST IN HALF. Water Newsletter , Water Inf. Center, Inc. Por t .Washington New'York (USA). Apr.' 22, 1968. . .

233

51. THE CANADIAN APPROACH TO CHEAPER HEAVY WATER '(1967,). Bancroft A. R. AECL-3044. Feb. 1968.

52. THE ECONOMICS OF HYDROGEN AND OXIGEN PRODUCTION BY WATER ELECTROLYSIS AND COMPETITIVE PROCESSES. Mrochck J. E. Conf. Abound. Nucl. Energy, Gatlinburg, Tenn. USA. Aug. 1068.

53. HEAVY WATER PRODUCTION IN CANADA. Law C. A. Nucl. Eng. 13; 510-2, Juno .1968.

54. HEAVY WATER. (Australian Atomic Energy Commission, r e s e a r c h Establishment Lucas Heights) Jan. 1970.

55. TECHNICAL STATUS OF THE LOW-TEMPERATURE PROCESS FOR HEAVY-WATER RECOVERY. ON THE ECONOMY OF THE LOW-TEMPERATURE PROCESS FOR HEAVY-WATER RECOVERY. Gutowski H. Kerntechnik 12, No. 516, 233-41, 1970.

CNEN Symp.on Tech. and Economic Aspects of Heavy Water Production^ Turin, Italy 1970:

56. ECONOMICS- OF HEAVY MANAGEMENT. Rüssel S. H. (AECL, Canada);

57. OPERATIONAL AND ECONOMIC ASPECTS OF HEAVY WATER PRODUCTION AT NANGAL BASED ON LIQUID HYDROGEN DISTILLATION. Bimbhat K. S. (India).

58. STUDIES AND TECHNICAL RESEARCH CONNECTED WITH DEUTERIUM AND NITROGEN-15 SEPARATION. Peculea M. Bull. St. Techn. Inst. Politechnic Timisoara , Romania. (In Press )

59. OPTIMIZATION OF A HEAVY WATER ENRICHMENT PLANT WITH A HOT/COLD OPERATING H2/NH3-EXCHANGE SYSTEM. Lang G.:, Schindewolf U. (Kernforschungszentrum, Karlsruhe(West Germany). (KFK-1483; p . 804-9). July 1971. (In German)

234

F - POTENTIAL PRODUCTION PROCESSES

1 - Chemica l Exchange P r o c e s s e s •

1 - Chemical Exchange between Hydrogtn and Deuter ium

THE KINETICS OF THE a - P A R T I C L E INDUCED EXCHANGE REACTION BETWEEN HYDROGEN AND DEUTERIUM. Mund W. , van Meersche M. Bull, c l a s s e sc i . Acad. roy. belg. 36, 47-G2, 1950.

HYDROGEN-DEUTERIUM EXCHANGE ACTIVITY OF CATALYSTS. Holm V . C . F . ,B lue R.W. Ind. Eng. Chem. 44 ,107-13 , 1952.

THE E F F E C T OF INHIBITORS ON THE HYDROGEN-DEUTERIUM EXCHANGE REACTION. Stephan M. J . , Danby C . J . (Univ. of Oxford, UK). P r o c . Roy. Soc. (London) A232, 271-7, Oct. 25, 1955.

THE OXYGEN-INDUCED HYDROGEN-DEUTERIUM EXCHANGE. Klein R . , Scheer M.D.' , Schoen L. J . (Bureau of Mines, P i t t sburg , USA) J . A m . C h e m . S o c . 7 8 , 4 7 - 9 , Jan . 5, 195G.'

HOMOGENEOUS EXCHANGE REACTION BETWEEN HYDROGEN AND DEUTERIUM.'Boato G . , C a r e r i G.'(1st.'di F is ica , Univ. di . Roma), Cimino A . , Molinari E . , Volpi G.G. ( Is t .d i Chimica Genera le ed Inorganica, Univ.'di Roma, Centro pe r la Chimica del CNR Roma) J , ' .Chem.Phys. '24, 783-91, Apr.'1956.'

THE ROLE OF IONS IN THE RADIATION INDUCED EXCHANGE OF HYDROGEN AND DEUTERIUM.'Thompson S.O.', Schaeffer Ö..:

A.'(BNL, Upton, N. 'Y. 'USA)J. 'Am.'Chem.'Soc. '80, 553-8, F e b ; 5 , 1958*

235

7, . THE CATALYTIC ACTIVITY OF GERMANIUM IN RELATION TQ THE ISOTOPIC EXCHANGE INACTION BETWEEN HYDROGEN AND DEUTERIUM. Boreskov G.K. , Kuchaev V. L. (Karpov Physico-Chemical Research Inst. USSR).Doklady Akad. Nauk SSSR 119, 302-4, Mar. 11, 1958, (In Russian) :

8. HYDROGEN-DEUTERIUM EXCHANGE REACTIONS CATALYZED BY NITROGENASE. Kelly M. Biochem. J . 109, 322-4,19G8.

237


1.- Chemical Exchange P r o c e s s e s

2 - Chemical Exchange between Hydrocarbons and Water

1 - Aroma t i c s /Wa te r

1. THE DEUTERIUM EXCHANGE REACTION BETWEEN p-XYLENE AND DEUTERIUM OXIDE CATALYZED BY SULPHURIC ACID. Tomiko Ueda (Osaka Univ. , Tokyo, JA PAN). Shokubay l ,No . . l , 1-7, 1959.

2. AROMATIC TRITIUM EXCHANGE IN WATER AND DEUTERIUM OXIDE. Gold V. , Lamber t R. W., Satchell D. P. N. (King's Col l . , '• London, UK). Chem. & Ind. No. 42, 1312-3, Oct. 17, 1959.

3. THE CATALYTIC DEUTERIUM EXCHANGE REACTION OF BENZENE AND ITS DERIVATIVES WITH DEUTERIUM OXIDE BY-Ni POWDERS. Kozo Hirota, Tomiko Ueda, Kciji Kuwata, Motoyosi Hata da. (Osaka Univ. JAPAN). Shokubai 2, 181-8, 19G0,

4. THE CATALYTIC DEUTERIUM EXCHANGE REACTION OF p-XYLENE AND ANISOLE WITH DEUTERIUM OXIDE ON-METALLIC CATALYST. Tomiko Ueda, Kozo Hirota. (Osaka Univ. , JAPAN). Shokubai(Tokyo) 3, No.'2, 122-6, 1961.

5# DEUTERIUM EXCHANGE REACTIONS WITH SUBSTITUTED AROMATICS. III. HETEROCYCLICS AND POLYCYCLIC HYDROCARBONS. Garnet). J . J,. . Sollicli W. A. (Univ. of Now South Wales Sidney, AUSTRALIA). Austral ian .!. Chcin. IB, No. 1, 56-04, Feb . 1962.

238

6. LABELLING OF HYDROCARBONS BY EXCI-IANGE CONDITIONS FOR HIGH YIELD. Gordon B. 'E . , Madison J . J . (Shell Co. Emeryvi l le , Calif. USA) Symp. on Advances in T r a c e r Methodology, Los Angeles, Calif. USA). Mar. 1963. (CONF-398-1)

7, THE SELECTIVITY OF CATALYSTS IN THE HYDROGEN EXCHANGE REACTION OF p-KYLENE WITH DEUTERIUM OXIDE. Tomiko Ueda, Kozo Hirota. (Osaka Univ. JAPAN). Nippon Kagaku Zassh i 84 ,882-6 , Nov.1963. (In Japanese)

239


1 - Chemica l Exchange P r o c e s s e s

2 - Chemica l Exchange between Hydrocarbons and Water

2 - Unsa tu ra ted A l i p h a t i c s / W a t e r

EQUILIBRIUM STUDIES ON THE EXCHANGE REACTION BETWEEN ACETYLENE AND HEAVY WATER.' R e y e r s o n L. H.'', Gi l lespie B. J . A m . Chem. Soc. 57, 2250-1 ,1935 .

EXCHANGE OF METHYL ACETYLENE WITH WATER-CATALYSIS' OF THE EXCHANGE, BY BASE OR BY ION.EXCHANGE RESINS. Stacey I. '{Columbia Univ . , N. Y. USA). P h . D . T h e s i s . 1956.

CATALYTIC ISOTOPIC EXCHANGE REACTION BETWEEN P R O P E N E AND DEUTERIUM OXIDE ON NICKEL CATALYSTS. Hi ro ta K . , Hi ronaka Y. {Osaka Univ. JAPAN). Shokubai (Tokyo) 4 / No. 1,41-6, .1962. {In J apanese ) .

THE ISOTOPIC HYDROGEN EXCHANGE BETWEEN PROPENE AND DEUTERIUM OXIDE CATALYZED BY NICKEL POWDER. Hi ro ta K . , Hironaka Y. (Osaka Univ. JAPAN). Bull. Chem, Soc. Japan 37 ,535 -42 , A p r . 1 9 6 4 .

INVESTIGATION OF THE EXCHANGE BETWEEN METHYL ACETYLENE AND WATER FOR CONCENTRATION OF DEUTERIUM. Mahadevan E . G . , T a y l o r T . I. {Columbia Univ. USA). NYO-755-1 ,Sep t . 1964.

EQUILIBRIUM IN THE DEUTERIUM EXCHANGE OF ACETYLENE AND WATER. Pype r J . W . ..Long F . A. (Cornel l Univ . , I thaca, N. Y;j USA). J . Chem. P h y s . 41 , 1890-6, Oct. 1, 1964.

240

7. ON THE MECHANISM OF H-D EXCHANGE IN ACETYLENE AT INTERMEDIATE TEMPERATURE: A RESPONSE. Bauer S. IL', Jeffers P . „ Z e v o s N.' J . ' P h y s . C h e m . 71,4412-G, 19G7.

8. RESEARCH PROPOSAL:SEPARATION OP HEAVY WATER UTILIZING THE ISOTOPE EXCHANGE REACTION BETWEEN METHYL-ACETYLENE AND WATER. Goldfrank J . C. Separa tion of Isotopes . CU-755-4 , Pape r HI B. 1967.

241



2 - Chemica l Exchange between Hydrocarbons and Water

3 - Sa tura ted Aliphat ic s / W a t e r

EXCHANGE OF DEUTERIUM OXIDE WITH BROMODICHLORO-METHANE AND C H L O R O D I B R O M O M E T H A N E . S h e r m a n R . i l . , B e r n s t e i n R. B. J . Am. Chem. Soc. 73 ,1376-7 . M a r . 1951. '

SEPARATION FACTOR FOR THE H/D EXCHANGE REACTION BETWEEN WATER AND ETHANE-DITHIOL-1 , 2.'Haul R. A.'W.', B ienemann D. Z . Phys ik . Chem.' (Frankfur t ) 23, 300-2, I960.' (In German) (CEA- t r -A-1381)

HYDROCARBONS FROM THE LOW-TEMPERATURE HEATING OF KEROGEN. Hoering T . C . , Abelson. P . H. (Carnegie Ins t . , Washington, D. C. USA). Carnegie Inst . W a s h . , P a p . Geophys. Lab . No. 1440, 2 5 6 - 8 , D e c . 19G4.

http://CHLORODIBROMOMETHANE.ShermanR.il

242

F - P O T E N T I A L PRODUCTION PROCESSES

1 - C h e m i c a l Exchange P r o c e s s e s

2 - C h e m i c a l Exchange be tween H y d r o c a r b o n s and W a t e r

4 - H e t e r o c y c l i c H y d r o c a r b o n s / W a t e r

ISOTOPIC EXCHANGE OF ACTIVE M E T H Y L HYDROGENS. II . DEUTERATION OF D I P H E N Y L - M E T H Y L P Y R Y I . I U M AND METIIYLTROPYLIUM SALTS. C a r d E . , Bal ly I . , Vas i l e scu A. et a l . (Inst , of Atomic P h y s i c s , B u c h a r e s t , ROMANIA). J . L a b e l . Compounds 1, 1H2- 8, J u l y - S e p t . 19G5.

DEUTERIUM EXCHANGE OF 4-PYRIMIDONES AND 4 - P Y R I -MIDTHIONES. 1. Wright G. E . , Baue r L . , Bel l C. h. (Univ. of I l l inois , Cli icago, USA). J . H c l e r o c y c l . Cheni . 3, 4 4 0 - 3 , D e c . 19GG.

ISOTOPI 0 EXCHANGE OF ACTIVE M E T H Y L HYDROGENS. V. REACTIVITY OF Ot-AND y - M E T H Y L GROUPS AND ß- . HYDROGENS IN PYRYLIUM SALTS. Ga rd E . , V a s i l e s c u A. ; Ma teescu G. D . , Balaban A. T . (Inst , of A tomic P h y s i c s , B u c h a r e s t , ROMANIA). J . L a b e l . Compounds 3, 19G-2Ü5, J u l y - S e p t . 19G7.

STUDIES ON HYDROGEN EXCHANGE. VIII. T H E BASE-CATALYSED HYDROGEN EXCHANGE OF M E T H Y L HYDROGENS OF METIIYLPYRIDAZINES AND THEIR N-OXIDES. Kawazoe Yutaka, Yoshioka Yuko, Y amada M u t s u m i , lge ta H i r o s h i . Chem. P h a r m . Bul l . (Tokyo), IH, 2000-2 , Doc. 19G7.

243


1 - Chemical Exchange P r o c e s s e s

2 - Chemical Exchange between Hydrocarbons and Water

5 - Alicyclic Hydrocarbons /Water

1# HYDROGEN-DEUTERIUM EXCHANGE IN SOME POLYAZAINDENES. Paudler W. W.', Helmick L. S. (Ohio Univ., Athens, USA). Chem. Commuti. No. 8, 377-8, 1967.

244


1 - Chemical Exchange Processes

3 - Chemical Exchange between Hydrocarbons and Hydrogen

1 - Aromatics/liyclrogcn

CATALYTIC DEUTERIUM EXCHANGE REACTIONS WITH ORGA-N1CS.X1V. DISTINCTION BETWEEN ASSOCIATIVE AND DISSOCIATIVE fT-COMPLEX SUBSTITUTION MECHANISMS. Garnelt J. L. , W. A. Sollich-Bauingarlncr (Univ. o! NSW, Sydney, AUSTRALIA). J. PJiys. Chcin. 0(3, 3.1.77-83, Nov. 19G4.

CATALYTIC DEUTERIUM-EXCHANGE REACTIONS WITH ORGANICS. XIX. Pi-COMPLEX ADSORPTION IN THE EXCHANGE OP THE ALKYLBENZENES.Garnctt J. L . , Sollich-Baumgartner W. A. (Univ. of NSW, Kensington, AUSTRALIA). J.Pliys.Chein.G'9, 1950-8, June .1 9G5.

NICKEL-CATALYSED HYDROGEN EXCHANGE OF ALKYLA-ROMATIC HYDROCARBONS AND TOLUIC ACID DERIVATIVES WITH DEUTERIUM OXIDE. MacDonalcl C. G. , Shannon J. S. (Commonwealth Scicnt. and Indus.Res. Organ. , Chatswood, NSW, AUSTRALIA). Australian J . Chem.18, 1009-21, July 19G5.

RADIATION-INDUCED ISOTOPE EXCHANGE IN SOME CG-HYDROCARBONS. Kroh J . , Ilankiewicz E. (Technical Univ., Lodz, POLAND). Bull. Acad. Pol. Sci. Ser. Sci. Chirn. 14, 243-4, 19G6.

2-1 ft

CATALYTIC DEUTERIUM EXCHANGE REACTIONS WITH ORGANICS. XXVII. THE ALKYLBENZENES ON SELF-ACTIVATED GROUP VIII TRANSITION METALS.F i she r B . D . , G a r n e t t J . L. (Univ. of NSW, Kensington, AUSTRALIA ). Au&lral. J . Chem. 19,2293-2310.000.196(5.

CATALYSIS OF HYDROGEN EXCHANGE IN in-DINITROBEN-ZENE. Bunccl E . , Zabel A. W. (Queen's Univ., Kingston, Ont, , CANADA). J . A m e r . Chem. Soc. 09, 3082-4, June 7, 1967.

KINETICS OF HYDROGEN ISOTOPE EXCHANGE IN BENZENE USING A HOMOGENEOUS PLATINUM CATALYST. Hodges R. J . , Gamct t J . L . (Univ. of NSW, Kensington, AUSTRALIA). J . Phys . Chum. 72, 1073-82, May 1068.

246




2 - Unsaturated Aliphatics/Hydrogen

THE EXCHANGE MECHANISM OF HYDROCARBON RADICALS WITH MOLECULAR DEUTERIUM. Voevodskii V. V . , Lavrovskaya G. K. , Mardaleishvili P. E . Doklady Akad. Nauk SSSR 81, 1951. (In Russian) (AEC-tr-1538;Tcch. Trans TT-358)

HYDROGEN EXCHANGE AND ISOMERIZATION OF SATURED HYDROCARBONS WITH SULPHURIC ACID. Stevenson D. P.', . Wagner C. D. , Bccck O., Otwos J . W. J. Am. Chem.'Soc.'74, 32G9-B2, July 5, 1952.

ISOTOPE EXCHANGE OF HYDROGEN IN FREE ALKYL RADICALS. Lavrovskaya G. L . , Mardaleishvili R. E . , Voevodskü V .V .ydsp rosy Khim. Kinetiki, Kataliza i Reaktsiónnoi Sposobnosti-Akad-. Nauk. SSSR, Otdel. Khim. Nauk 40-53, 1955. (TT-701) (In Russian)' "'

ISOTOPIC EXCHANGE BETWEEN DEUTERIUM AND HYDROCARBONS ON NICKEL-SILICA CATALYSTS.Burwell H.'.L.\ Tuxworth R.H. (Northwestern Univ.'Evanston.'Ill.USA) J. Phys. :

Chem. 60,1043-9, Aug.'1956. . ' ,

ON TWO MECHANISMS OF IIYDROGENATION AND EXCHANGE BETWEEN ETHYLENE AND DEUTERIUM ON PALLADIUM. Kazanskii V. B . , Voevodskii V. V. (Lomonosov Moscow State . Univ. USSR). Doklady Akad. Nauk SSSR 111, 125-8,;Nov. 1, 1956. . (In Russian)

247

ON THE ISOTOPIC EXCHANGE BETWEEN GASEOUS HYDROGEN AND SOLID POLYMERS UNDER THE ACTION OF NUCLEAR RADIATION.' Vnrs l invsku Ya. M. , Vasiliev G.' Ya, ' , Karpov V. L , , Lnmrkin Yu.'S.', Poti-ov J.' Ya. Doklucly Akad, Nauk SSSR 11 ti, 315-5, Jan.' 11, 1058. (Tn Russian)

REACTION BETWEEN DEUTERIUM AND METHYL RADICALS OBTAINED ACCORDING TO POLONYI METHOD.'Ivanov O.A.', Fok N.V"., Vocvodskii V.'V.'(Lomonosov State Univ.'Moscov, USSR) Doklady Akad. Nauk SSSR 11 8, 1142-5, Feb. 21, 1 958. (In Russian)

248




3 - Saturated Aliphatics/l-Iydrogen

1. HEAVY WATER PRODUCTION - DESCRIPTION OF PROCESS FOR THE PRODUCTION OF HYDROGEN AND WATER ENRICHED IN HEAVY WATER. Chrones J . (Nat. Res. Council of Canada. Atomic Energy Project , Chalk River, Ont. CANADA). XM-65. May 29,1951.

2. ON THE CHEMICAL, EXCHANGE BETWEEN HYDROGEN AND SATURATED HYDROCARBONS. Varshavskii Ya. M., Vaisberg-S .E . , Lozhkina M, G. Zhur. Fiz . Khim. 29, No. 4, 750-1, Apr. 1955.

KINETICS OF METHANE-DEUTERIUM EXCHANGE OVER NOBLE METAL, ALLOYS. McKee D. W., Trans . Faraday Soc. 61,2273-83,1965.

249



4 - Chemical Exchange between Amides, Aminoacids and Water

1 - Amines /Water

THE ISOTOPIC EXCHANGES EFFECTED, FROM A MIXTURE IN THE LIQUID OR VAPOR PHASE OF ALIPHATIC AMINES Ol OF DIMETHYLIIYDRAZTNE WITH HEAVY WATER. Pannetier G., Gucncbaut H . , Marsigny L . , Deschamps P.- J. Chim. Phys. 58, 790-G, Sept. 1961. (In French)

A THERMODYNAMIC STUDY OF THE TERNARY SYSTEM, TRIETHYLAMINE, WATER AND.HEAVY WATER, WITH SPECIAL REFERENCE TO ISOTOPE SEPARATION PROBLEMS. L inders t roem-Lang C. U. (Danish Atomic Energy Commission, Riso, DENMARK). Acta Chem. Scand. , 16,1730-50, 1962.

ISOTOPIC EXCHANGE OF DJ.FLUORAMINE WITH DEUTERIUM OXIDE AND TRIFLUOROACETIC ACID. Becker W. E . , Impastato F . J . (Ethyl Corp . , Baton Rouge, La. USA). Jan. 4, 19G5. (CONF-650401)

250

- POTENTIAL PRODUCTION PROCESSES


4 - Chemical Exchange between Amines, Aminoacids and Water

2 - Aniinoacicls/Water

EXCHANGE OF DEUTERIUM AND l 8 0 BETWEEN WATER AND OTHER SUBSTANCES. 2. ALTERNATIVE METHODS. Krause I. M. , Lindcrs t r j im-Lang K.' 3. DEUTERIUM EXCHANGE OF SHORT PEPTIDES, SANGER'S A-CHAIN AND INSULIN.' Ilvidt A . , L inders t r^m-Lang .Compt . rend. t r a v . lab. Ca r l sbe rg Ser. 'Chim. '29 JNo. '22-23, 367-402, 1955.

DEUTERATION OF PROTEINS AND POLYAMIDES IN DEUTERIUM OXIDE VAPOR. Jeffr ies R. {ShirleyInst. '; Manchester , Eng. UK). J . Po lymer . Sci. P t . A2, 5161-70, Dec. 1964..

DEUTERIUM-HYDROGEN EXCHANGE BETWEEN WATER AND SILK FIBROIN. Morr i son J . L. (Ontario R e s . Foundation, Toronto, CANADA). Can. J . Chem. 42, 1009-15, May 1964.

COMPARISON OF WATER SORPTION AND DEUTERIUM-HYDROGEN EXCHANGE SITE IN POLY- L- VA LINE. Brandt W. , Budrys R . S . (Univ. of Chicago, USA). J. Phys. Chcm.69, 1432-4, • Apr. 1965.

DEUTERIUM-HYDROGEN EXCHANGE IN AMIDE N-H GROUPS. Klotz I. M. , F rank B. II. (Northwestern Univ. , Evanston, 111. USA). J . A m . C h e m . S o c . 87, 2721-8, June 20, 1965.

HYDROGEN-DEUTERIUM EXCHANGE OF POLYPEPTIDES. (Thesis) . Leichtling B. II. (Northwestern Univ. , Evanstonj 111. LISA). 1966.

251

- P O T E N T I A L PRODUCTION PROCESSES


5 - Chemical Exchange between Amines, Amides and Hydrog

1 - Amines/Hydrogen

THE ISOTOPIC EXCHANGE OF GASEOUS HYDROGEN WITH LIQUID AMINES. Bar -E l i K . , Klein F . S. J. Chem. Sóc. London 3083-88, 19G2;

CATALYTIC HYDROGEN EXCHANGE- OF ANILINE ON SUPPORTED METAL CATALYSTS. Hagiwara Hiroshi, Echigoya Etsuro (Tokyo Inst, or Tech. JAPAN). Bull. Chem. Soc. Jap. 39, 1G83-9, Aug. 1966.

HEAVY WATER PRODUCTION BY A MINE-HYDROGEN EXCHANGE.'Bancroft A . R . , Rae H. K. (AECL, CANADA) CNEN Symposium on Technical and Economic Aspects of Heavy Water Production. Turin, Italy, Sept. 30 - Oct. 1, 1970.'

AECL'RESEARCH IN ENGINEERING.'(Atomic Energy of Canada Ltd . ,Cha lk River, Ontario). 1971. (AECL-3787)

HEAVY WATER PRODUCTION USING AMINE-HYDROGEN ISOTOPIC EXCHANGE. Holtslander W . J . AECL Research in Engineering 5-7, Sept. 1971. (AECL-3990)

CHEMICAL ENGINEERING RESEARCH AND DEVELOPMENT FOR FUEL REPROCESSING AND HEAVY WATER PRODUCTION. Rae H. K. (Atomic Energy of Canada Ltd. , Chalk River, Ontario. ' Chalk River Nuclear Labs . ) . Nov. 1971. (AECL-3911)

lù&lil. iAl.r.îiU.'Aì;;*

252


1 - Chemical Exchange P r o c e s s e s -

5 - Chemical Exchange between Aminos, Arn ims and Hydrogen

2 - Amides/Hydrogen

1.. THE HYDROGEN EXCHANGE OF ALKALI AMIDES AND HYDROXIDE WITH DEUTERIUM GAS. Claeys Y. M . , Dayton J. C. , Wilmarth W.K. J . C h e m . P h y s . 18, 759, 1950.

253

F. - POTENTIAL PRODUCTION PROCESSES


6 - Chemical Exchange between Organic Aci'cls and Water' or Hydrogen

1 - Organic Acids/Water

1. ; DEUTERIOXIDE-CATALYZED EXCHANGE REACTIONS.OF iviETHYLENECYCLOPROPANECARBOXYLIC ACIDS WITH DEUTERIUM OXIDE. Bottini A. T . , Davidson A. J, (Univ.-of Calif.,

• Davis, USA). J . Org. Chem. 30, 3302-8, Oct. 1965. •

BASE-CATALYZED HYDROGEN-DEUTERIUM EXCHANGE IN BIVALENT METAL-EDTA CHELATES. Terr i l l J,_B. , R'eilley' C.N.'(Univ. of North Carolina, Chapel Hill USA). Ana l ' chem. 38, 187G-81, Dec-, 19G6. • ' ' ' .

V • \ :

'• • 254


1 - Chemical Exchange Processes * •.

6 - Chemical Exchange between Organic Acids and Water or Hydrogen

2 - Organic Acids/Hydrogen

1. THE EFFECTS OF CERTAIN NITRO AND RELATED COMPOUNDS UPON THE RATE OF EXCHANGE OF DEUTERIUM GAS WITH ACETIC ACID OVER ADAMS PLATINUM CATALYST. Smith N. A. McDaniel E. L. (Univ. of Tenn; Knoxville, USA) J. Am. Chem. Soc. 77, 533-5;Feb. 5,1955.

.255

F - P O T E N T I A L PRODUCTION PROCESSES

1 - C h e m i c a l Exchange P r o c e s s e s

7 - C h e m i c a l E x c h a n g e between Hydr ides , Hydra t e s and • W a t e r

1 - Hydr ides , H y d r a t e s / W a t e r

PROPOSAL OF A NEW METHOD FOR THE SEPARATION OF HYDROGEN AND DEUTERIUM BY CHEMICAL EXCHANGE B E T W E E N SIMPLE HYDROGEN COMPOUNDS AND PALLADIUM HYDRIDE AND PALLADIUM DEUTERIDE. Salmon O.N. (KAPL,. Schenectady, N. Y. USA). KAPL-M-ONS-2(Del . . ) . F e b . 9, 1953. Dec i . de l . F e b . 25, 1957.

EXCHANGE BETWEEN HEAVY WATER AND CLAY MINERALS F a u c h e r - J . A . , T h o m a s H.'C. '(Yale Univ. ' ,New Haven, Conn. USA)r

J . P h y s . C h e m . 59, 189-91, F e b . 1955.

HYDROGEN AND. OXYGEN ISOTOPES A P P L I E D TO THE STUD"fr OF W A T E R - M E T A L REACTIONS.EXCHANGE O F D 2 0 1 8 WITH ALPHA ALUMINA MONOHYDRATE. B e r n s t e i n R. B."(Àrgonrie Nat . L a b . , Lemont , I l l inois , U S A h A N L - ^ S g . Aug. 1958.

ISOTOPIC EXCHANGE OF A HYDRIDOPLATINUM (II) COMPLEX WITH DEUTERIUM OXIDE. F a l k C. 'D. , Halpern J . (Univ. of.Chicago, USAK J . A m . C h e m . S o c . 8 7 , 3523-4, Aug. 5, 1965.

http://Chem.Soc.87

256


1 - Chemica l 'Exchange P r o c e s s e s

7 - Chemica l Exchange between Hydr ides , Hydra tes and Wate r

2 -r Phosph ine /Wate r

EQUILIBRIUM IN THE EXCHANGE OF HYDROGEN BETWEEN PHOSPHENE AND WATER. Weston R . E . , B ige le i sen J . J . Chem. Phys . 20, No. 9, 1.400, 1.052.

AN EVALUATION OF THE FEASIBILITY OF UTILIZING THE EXCHANGE OF HYDROGEN BETWEEN PI [OSPITINE AND WATER FOR-THE PRODUCTION .OF DgO. Bige le i sen J . , Weston R . E . J r . (Brookhavcn Nat. L a b . , Upton, N. Y. USA). BNL- 156. Feb . 1952. Dec i . Dec. 2, .1.955.

KINETICS OF THE EXCHANGE OF HYDROGEN BETWEEN PHOSPHINE AND WATER: A KINETIC ESTIMATE OF THE

.ACID AND BASE STRENGHTS OF PHOSPUINE. Weston R . E . J r . , Bigcic iscn ,1. (BroukhavcMi Nat . L a b . , Upton, N. Y. USA). BNL-1655 . 1953.

KINETICS OF THE EXCHANGE OF HYDROGEN,BETWEEN PHOSPHINE AND WATER : A KINETIC ESTIMATE OF THE ACID AND BASE STRENGHTS OF PIIOSPHINF^ Weston R . E . , Bigele isen J . J . Am. Chem. Soc. 7C, 3074-8, 1954.

JSOTOPIC EXCHANGE REACTIONS OF TRANS-HYDRID O-Gl 1LOROBIS (TI'METU YLPIIOS PHI.NE) PLATIN UM (II) . Falk C D . , IUilpern J . (Univ. of Chicago, USA). IAEA Symposium on Exchange K<!iu:l.i<MiK, llpLoii, N. Y. U.SA.SM-CÌ4/2H. | 965. (CON !•'-(;505-1 9- I 5)

257

DEUTERIUM EXCHANGE BETWEEN PHENYLPHOSPHONOUS ; ACID AND WATER. Reuben J . , Samuel D^Sllver B. L. (Weizmanri Inst.of Science, Rehovoth; ISRAEL). J .Äm. Chem.Soc. 85, . 3093-6, Oct. 20, 196a

258


1 " Chemical Exchange Processes

7 - Chemical Exchange between Hydrides, Hydrates and Water

3 - Arsine/Water

] , EQUILIBRIUM IN THE EXCHANGE OF HYDROGEN BETWEEN AUSINE AND WATER. Zcltman A. H., Gerhold G. (Los Alamos Sci, Lai)., N, Mexico, USA), J. Chcm, Phys. 31, 889-91, Oct, 1959.

259



•8 - Chemica l Exchange between Ilydi-ogen UnlirJes and Difrorcnt .Substanccs

1 - Hydrogen Ual idos /Water

A METHOD FOR INVESTIGATING THE ISOTOPIC EXCHANGE REACTION INA LIQUID DEUTERIUM FLUORIDE MEDIUM. Varshavski i Ya. M. , Lozhkina M. G. (Karpov Moscow. Pnysico-Chemical Insl. USSR). Zhur . F i / . Khiin. 31," Oil -4 , Apr. 1957. (hi Russ ian) .

TIIPM3XC11ANGE OF DEUTERIUM BETWEEN HYDROGEN CULO RIDE AND WATER. Pugh O. , Labaton V. Y. (Gt. Br i t . Capenhurst Works, Capcnliursl , Chcs . , Eng. UK). IGR-TN/CA-G52. Aug. 1957.

TWO-TEMPERATURE EXCHANGE OF DEUTERIUM IN THE SYSTEM WATER-HYDROGEN CHLORIDE. Vaishcrg S. E . , VarshavKkii Ya. M. Zhur . F i z . Kirim. 37, 307-9, 19G3.


1 - Chemical Exchange Processus

8 - Chemical Exchange between Hydrogen Halides ar:d Different Substances

2 - Hydrogen Halidos/llydrogen

1. . METHODS AND TECHNIQUES OF PHYSICOCHEMICAL INVESTIGATIONS. A METHOD OF STUDYING THE REACTION OF ISOTOPIC EXCHANGE OF HYDROGEN IN LIQUID DEU'I'ERIUM BROMIDE, Kaliuachenko V, R. , Varshavskiy Ya. M. , Shatenstein A.'I. Zhur.'Flz.'Khim,'30, 1140-3,195G. (In Russian) (AEC-tr-2976)

261



8 - Chomical Exchange between Hydrogen Halides and Different Substances

3 - Hydrogen I la l ides /Hydrocarbons

1. HYDROGEN ISOTOPE EXCHANGE IN HYDROCARBONS IN LIQUID DEUTERIUM FLUORIDE. Varshavski i 'Ya . M. , Shatenstein A. I. Doklady Akacl. Nauk SSSR 95, 297-9, 1954. (In Russian)

2. DETERMINATION OF THE COEFFICIENT FOR THE DISTRIBUÌ TION OF DEUTERIUM IN THE ISOTOPIC EXCHANGE OF HYDROGEN BETWEEN NAPHTALENE AND DEUTERIUM BROMIDE. Varshavskii. Ya. M. , Kalinaclienko V*. R. , Vaisberg S. E . , Shatenstein A . I . Zhur . F iz . Khim. 30, 1647-51, 1956.

3. HYDROGEN EXCHANGE BETWEEN AROMATIC HYDRO ~-CARBONS AND LIQUID DEUTERIUM BROMIDE. Shatenstein A. I . , Kalinachenko V. R. , Varshavski i Ya. M. (Karpov Moscow, Inst, of Phys .Chem. USSR). Zhur . F iz . Khim..30, 2093-7, Sept.

'1956.

4. HYDROGEN EXCHANGE BETWEEN BENZENE AND NAPHTALENE DERIVATES AND LIQUID DEUTERIUM BROMIDE. Shatenstein A. I., Kalinachcnko V. R. , Varshavski i Ya. M. (Karpov Moscow Inst, of Physical Chemis t ry , USSR). Zhur. E.iz! Khim. 30, 2098-2105, Sept. 1&5C.

262



8 - Chemical Exchange between Hydrogen Ilalicles and Different Substances

4 - Hydrogen Ilalicles/Organic Acids

HYDROGEN-DEUTERIUM EXCHANGE IN AQUEOUS SOLUTIONS OF GLYCOLIC:. ACID AND OF SODIUM FORMATE. Bok L . D . C . , PeUcrs L. B. J .Chem.Soc . 1524-5, Apr. 1952.

263



9 - Chemical Exchange between Ion Exchange Resins and Water

PURIFICATION OF HOMOGENEUS CHAIN REACTING SOLUTIONS PROTIUM-DEUTERIUM EXCHANGE .WITH AMBER U T E IR-L Adamson A. W. , Boyd G. E'. (Clinton Labs. , Oak Ridge, Tenn. USA). MonC-77.Apr. '2, 194G. Deci. Jan. 11/195C.

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ON THE REACTION OF DEUTERIUM OXIDES WITH CATION RESINS. Meleshko V. P . , Myagkoi O. N . , Bogatyrev K. S. (Voronezh State Univ. , USSR). Zliur, Neorg. Khim. 6, 9-14, Jan. 19G1. (In Russian) .

SEPARATION OF STAHLE ISOTOPES BY CHEMICAL AND ION EXCHANGE METHODS. Panchenkov G. M. J . Chem. Phys . 60, 107-13,1963.

264



10 - Chemical Exchange between Mercaptans and Water

EXCHANGE OF DEUTERIUM BETWEEN MERCAPTANS AND WATER. Hutchison C. , Gillies D. (Columbia Univ. , New York. Div. of War Research.-USA). A-754. July 9, 1943. Deci. Dec. 8, 1955.

SEPARATION FACTOR FOR THE Il /D EXCHANGE REACTION BETWEEN WATER AND ETHANE-DITHIOL-1, 2. Haul R. W.A. , Blcnneman D. Z. Physik. Chem. 23, 300-2, 1960. (CEA-tr-A-1381)

265

P - POTENTIAL PRODUCTION PROCESSES


11 - Chemical Exchange between Ketones and Water

ACID-AND BASE-CATALYZED HYDROGEN-DEUTERIUM EXCHANGE BETWEEN DEUTERIUM OXIDE AND SIMPLE KETONES. Bothner-By A . A . , Sun C. (Mellon Ins t . , Pit tsburgh, USA)..J. Org. Chcm.'32, 402-3, Feb. 1S61.

266

F - POTENTIAL PRODUCTION PRODUCTION

2 - Physical Separat ion P r o c e s s e s

1 - Absorptive Fract ionat ion •

1. PRELIMINARY STUDIES FOR THE SEPARATION OF HD FROM H2 BY RECTIFIED ABSORPTION. Hanson D.N. , I Iun t C .d 'A ; , Cook M . W . , Fiele J . L . (California. Univ., Berkeley. Radiation .,

. Lab. USA). UCRL-1723. Mar . 17,1952. Deci . Apr . 6, 1956.

THE SEPARATION OF HD AND H 2 BY ABSORTIVE FRACTIONATION. Augood D.R. T r a n s , Inst. Chem. Eng. 35,394-408, 1957.

267


2 - Physical Separation P r o c e s s e s

2 - Adsorption

THE SEPARATION OP HYDROGEN ISOTOPES BY FRACTIONAL DESORPTION. Taylor H.S. ,-Gould A . J . , Bleakney Wr. Phys.:Rev.,43, 496-7,1933.

QUANTITATIVE SEPARATION OF HYDROGEN ISOTOPES 3Y FRACTIONATED DESORPTION. P e t e r s K. , LohmarW. Z. physik. Chem.'(Leipzig) 180A, 51-7, 1937. (In German) ( CEA-tr-577)

THE ADSORPTION OF DEUTERIUM BY A PLATINUM CATALYST.'Bond G. C. (Princeton Univ. N. Y. USA). J . 'Phys. Chem.'60, 702-3, May 1956.

GAS CHROMATOGRAPHIC SEPARATION OF HYDROGEN ISOTOPES'. Glueckauf E . , Kitt G. P . Proc.pf • the.Intern. Symposium on Isotope' Separation. Amsterdam 1957. North Holland Pubi. Co. Amsterdam 1958. (p. 210-2G)

THE SEPARATION OF ISOTOPES AND'ORTHO-PARA HYDROGEN AND DEUTERIUM-BY PREFERENTIAL ADSORPTION AT LOW TEMPERATURE.THE THERMODYNAMIC PROPERTIES OF ORTHO-HYDROGEN AND PARA DE UTERIUM. White D.(Ohio State Univ. Research Foundation, Columbus, USA). TID-11621.' Dec.1960.

„jJJ^lIMI'Ù" ' , " r V' "". ' 'SI, - /-?".' ~.- »... . • -.1': . ! ->I«-Ì K- ji' '-iö ji t i f a s s i

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208

• ISOTOPE SEPARATION BY CHROMATOGRAPHIC METHODS. . Gliieckaiif" É. Separat ion of Isotopes. ' . .H.London ed, George Newness Ltd. London, 1^61.

ORTHO-PARA AND ISOTOPE SEPARATIONS BY PREFERENTIAL ADSORPTION AT LOW TEMPERATURES. White D . , Haubaeh W. J . , La s sc t t r e E . N. (Ohio State Univ. Columbus, USA). Pure and Appi. Chem. 2, Nos. 1-2, 323-4, 1961.

8. SEPARATION OF THE ISOTOPES HT AND ORTIIO-D2 BY ADSORPTION AT LOW TEMPERATURES. Kalorski A. , Ebcrhar t J . G. , White D. (Ohio State Univ. , Columbus, USA). J . Phys . Chem. 34,2189-90, June 1961.

9,i *:• THEORY OF ISOTOPE SEPARATION OF HOMO- AND HETERO r

NUCLEAR DIATOMIC MOLECULES BY ADSORPTION AT LOW TEMPERATURES. Katorsld A . , White D. J. Chem. Phys . CO,

"29-31, Jan. - F e b . 1903.

10. . SEPARATION OF ISOTOPES BY GAS AND ION EXCHANGE CHROMATOGRAPHY. Glucckauf E . J . Chem. Phys . CO, 73-80, J a n . - F e b . .I 9G3.

1 1 - ON THE HYDROGEN-DEUTERIUM EXCHANGE ACTIVITY OF SILICA G E L : ALUMINUM IMPURITY AND RADIATION E F F E C T . Kohh H.W. Catalysis 2, 208-10, June 1963.

12. THE CHROMATOGRAPHIC SEPARATION OF THE HYDROGEN ISOTOPES INCLUDING TRITIUM. King. J . J r . J . Phys . Chem. 67, 1337, June 1963.

13. THE SEPARATION OF H2 AND D 2 BY MOVING-BED ADSORP-. TION : CORROBORATION OF ADSORBER DESING EQUATIONS. Basmadjian D. (Univ. of Ottawa, CANADA). Can. J . Chem. Eng. 41;, 2G9-72, Dec. 1963.

269

14. PHYSICO-CHEMICAL SEPARATION OF ISOTOPES. Hotter F . , Mol inar i P . , Dir ian G. 12, P / 9 0 . (FRANCE) 3rd "UN Geneva Ccmf. 19G4.

15. THE LOW TEMPERATURE'CHROMATOGRAPHIC SEPARATION OF THE ISOTOP.IC HYDROGENS AT 25 AND 77°K. Haubach W. J . , Knobler C. M . , Ka to r sk i A . , While D. J . P h y s . Chem. 71, .1.393-402, 19(57.

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3 - Cent r i fugati on

1. B - A PROPOSES D2O FROM METHANE. Can. Chem. P rocess 49, No. 8,47-8. 56, Aùg,Ì965.

THE REACTION OF. METHANE AND DEUTERIUM ON EVAPORATED NICKEL CATALYSTS. Kemball C. Proc .Roy. Soc. (London) 207A,

'539-54/July 23, 1951.

EXPERIMENTS WITH A CENTRIFUGAL FORCE WITH SIMULTANEOUS PRODUCTION OF COLD AND HOT AIR. Ranque G.I . J . Phys. Radium 4, No. 7, 1125-55, July 1933.

THE EXPANSION OF GASES IN A CENTRIFUGAL FIELD. Ililsch R. Z. Naturforsch 1, 208-14, 1946. (In German)

271


2 - Phys ica l Separa t ion P r o c e s s e s

4 - Dist i l lat ion of Ammonia and Methane !

POSSIBLE DISTILLATION OR SIMILAR METHODS FOR THE RECOVERY OF D 2 O.Stedman D. C. (Na t .Res . Lab. CANADA). Repor t No. C50-49S, June 8/1949.

2. DISPROPORTIONATION IN DEUTERATED AMMONIA. Bigeleisen J . J . C h c m . P h y s . 2 0 , 1495-6,1952.

3^ DEUTERIUM SEPARATION STUDY.DISTILLATION OF AMMO-. NIA AND OF METHANE. P r o g r e s s Report No. 3 (on HEAVY WATER MANUFACTURE SURVEY). Drews W. P . (Esso R e s . and Engineer i r ig 'Có . |L inden , .N; . J .USA) .NYO-7522.0c t . 4, 1955.Decl . J an .12 ,195G. •

AMMONIA DISTILLATION FOR DEUTERIUM SEPARATION. P e t e r s e n G. T . , Benedic t 'M. (Mass . Inst.'of Tech. ^Cambridge, Mass . ;USA).NYO-2347.MaylG, I960.. ' •"'

5; DEUTERIUM ENRICHMENT IN THE DISTILLATION OF AMMONIA. P e t e r s e n G. T . , Benedict M. (MIT, Cambridge, M a s s . USA). N u c l . S c i . E n g . 15 ,90-7 , J a n . 1963. •

VAPOR.PRESSURE OF SATURATED LIQUID METHANE. Physica 32 ,1890-900,1964. . '

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272


2 - Physical Separation P rocesses

5 - Distillation of Other Compounds

FRACTIONATION OF THE HYDROGEN ISOTOPES IN THE DISTILLATION OF ETHYL ALCOHOL.'Widiger A.' H.', Brown W. G.' J.' Am.'Chem.'Soc.'ßl, 2453-4,1939.'

2. ' RECOVERY OF D 2 0 AND-U02F2 BY DISTILLATION.Fischer R. , Wattcnberg A. (Chicago Univ. Metallurgical Lab. USA). CC-3302. : Oct. 10, 1945. Deci. Dec. 22, 1955.

3 ; ENRICHMENT OF DEUTERIUM BY DISTILLATION OF DISSOCIARLE COMPOUNDS. Holimberg K. .R. (Atomenergy AB. , Stockholm).^" P/180. (SWEDEN)' 1st UN Geneve Coni'. 1955.

THE SEPARATION OF HYDROGEN ISOTOPES BY DISTILLATION OF ÀZEOTROPIC ACID-WATER MIXTURES. We'txclK.., Schlitze H., Kretzschman G:', Mtihle K. (Inst, i'ilr Physikalische . Stofftrennung, Leipzig , GERMANY). Naturwissenschaften 47, 374, 1960. (In German) '. ;

273


2 - Physical Separation P roces se s

6 - Diffusion

SEPARATION OF HYDROGEN ISOTOPES BY DIFFUSION THROUGH PALLADIUM.'Harris L . , Jost W., P e a r s e R. W. B. P roc .Na t l . Acàd. Sci. U . S . 19, 991-4, 1933.

PURIFICATION OF THE HYDROGEN ISOTOPES BY DIFFUSION. Hertz G.L.Naturwissenschaf ten 21, 884- 5 , 1933. (In German)

A DIFFUSION METHOD OF SEPARATION OF ISOTOPES. Urey H.C. Phys .Rev .44 , 314,1933.

ADDITIONAL EXPERIMENTS FOR THE SEPARATION OF ISOTOPES.'PRODUCTION OF PURE HEAVY HYDROGEN BY DIFFUSION . ' i larmsen H.', Hertz G.'L.', Schlitze W.' Z.'Physik 90, 703-11, .1934. (In German) (AEC-tr-4395)

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2 - Phys ica l Separation P r o c e s s e s

7 - The rma l Diffusion

1. RESEARCH ON THERMppiFFUSION IN THE LIQUID PHASE; THERM OD IFFUSION IN HEAVY WATER. Prigogine I. ,De Brouckère L. , B u e s s R.Physica. .18, 015-20, Nov. 1952.

2. THE SEPARATION OF HYDROGEN AND TRITIUM BY THERMAL DIFFUSION. Boorman C . , K r o n b e r g e r H . (UKAEA Ind. Group. Risley UK) P r o c . I n t . Symp. on Isotope Separation. Ams te rdam 1957. North Holland Pubi. Co. A m s t e r d a m 1958. (p.471-7)

3. THERMAL DIFFUSION FACTOR FOR HYDROGEN AND WATER MIXTURES. Saxena S. C. (Atomic Energy Establ ish. ' , Trombay, INDIA). Indian J . Phys. 34, 449-55, Oct. I960;:' '

4 / THE THERMAL DIFFUSION COLUMN. Vasaru Gh. , MMer. G. , Reinhold G. , Fodor; T. VEB Deutscher . Verlag der Wissenschaften, Ber l in 1969.

275


2 - Physical Separation P roces se s

8 - Solvent Extract ion

FINAL REPORT ON LABORATORY SEMIWORKS TESTS OF TRIETHY-LAMINE IN SOLVENT EXTRACTION. Bebbington W. P . SAMReport A-1916.Sept. 1943. '

LIGHT WATER SEPARATION WITH TRIETHYLAMINE. Hahn H. T . ; Street E; B . (General Elec t r ic Co.Hanford Atomic Products Operation, Richland, Wash. USA). HW-48735. Feb . 22, 1957.

276


2 - P h y s i c a l Separat ion P r o c e s s e s I

9 - Others

SEPARATION OF ISOTOPE MIXTURE BY NOZZLE PROCESS. Mikami 11., Oyama Y. Bull . Tokyo Inst . Technol . Spec. 49, 167-80, 1962.

SEPARATION OF GASES AND ISOTOPES IN A WHIRLING TUBE. Bornlccsscl 1C, Pilot J . Z. Physik. Clicm. 221, 177-84, 19G2.

CHARACTERISTICS OF A VORTEX TUBE. SokoloyJE.Y. T h e r m a l Eng. 13, No. 7, 84-91, 1 966. * > » • ; " '

277


3 - Others

1. ENRICHMENT OF HEAVY WATER BY BIOLOGICAL METHOD. Webb J . (Coll.' of Technology, Belfast, UK). Nature 177, 988-9, May 26,1956.'

2. PHOTOCHEMICAL SEPARATION OF ISOTOPES.'Rozenberg J. Isotop.' Radiat.' Technol.' 3, 200-5, Spring 1966.

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B - HEAVY WATER REACTORS IN NUCLEAR POWER PROGRAMS

1. NORVEGIAN ATOMIC RESEARCH. Gliom, and Eng. News 2G, 3780,Dec. 20, 1948.

2. AUSTRALIAN A . E . C . RESEARCH PROGRAMME. Walson-Munro C. N. (Australian Al.omic Energy Commiss ion, AUSTRALIA). Nuclear Eng. 1, 183-5, Aug. 195G.

3, REPORT FROM SPAIN: SENSE OF URGENCY GRIPS MADRID ON NUCLEAR POWER; CONVENTIONAL SOURCES TO BE FULLY EXPLOITED IN 10 YEARS. Nucleonics 15, No. 7, 2G, July 1 957.

4. NATURAL OR ENRICH KD URANIUM FOR POWER REACTORS?. Lewis \V. B. (Chalk River , Out . , CANADA). Atomwir lschaR 2, No. 9, 285, Ì957. (In Cprman)

5. ANALYTICAL CONTROL OF HEAVY WATER IN REACTOR. MODERATOR SYSTEM. Zcmyan E. M. (Du Pont de Nemours E. I. & Co.. Savannah River L a b . , Augusta, Ga. USA). Analytical Chemis t ry in Nuclear Reactor Rechnology Nov. 1957. Gatlinburg Tonn. USA. TID-7555. (p. 175-83)

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P r o c e e d i n g s Di'Ilio Second United .Nations In te rna t iona l ConJ'oren-cc on tlio Poacci'uJ l;s"K o l 'A lomk: E n e r g y , Geneva IDS!!:

G. HEAVY WATER MODERATED AND COOLED POWER REACTORS.

Eabeovk I). !•'. », P/fill) (USA):

7. TI!!1: NUCLEAR ENERGY PROGRAM AND E L E C T R I C POWER PROBLEMS IN SPAIN. Oloro N a v a s c u e s .1. i\l. J, P/2U3G. (SPAIN)

8. NUCLEAR. POWER PLANTS. P e l r o v . P . A. Gosene rgo r / r l a t , Moscow 1953. (In Russ ian)

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10. ESTIMATES OE NUCLEAR* ENERGY PRODUCTION IN E U R O P E 1958- L'Jfif). NATIONAL PROGRAMMES. BASIS FOR CALCULATING C A P I T A L COSTS-COSTS FACTORS. OECE P a r i s , 1959.

USAEC Sympos ium on l>2(-)- m o d e r a t e d r e a c t o r s . G e r m a n t o w n , My. USA. Alar. 1.959. T t D - 7 5 7 5 :

1 1 . ACCOUNTING P A R T I C L E S FOR. D 2 0 IN POWER - REACTOR OPERATION. Shephe rd 1:3. Ü / S A E C ) T T J . D - 7 5 7 Ö p. 11-1.4;

1.2. FUTURE REQUIREMENTS POR. D. ,0 . Lane J . A. (ORNL, Temi . I/SA):T!I>-7!V75 p. 15 WW;

285

l rJ. CAPABILITY OF ARC T O SUPPLY D 2 0 FOR FUTURE NEEDS. lUiUcrv/orlh A.-V. (UÖARC, Wash. I). C. ).TI.D-7r>7r> p. 2 3 - 7 .

14. ADVANCED COURSE OW HEAT EXTRACTION FROM BOILING WATER POWEII REACTORS AND ASSOCIATED DYNAMIC PROBLEMS, (PL II). Ne thc r l an t l s ' -Norwoginn R e a c t o r School. KjclJcr , Norway. 'Aug. 195)9. (NP-928G) .

15. HEAVY WATER IN HEAVY-WATER BASED NUCLEAR POWER PROGRAMMES. Or t i z F o r n a g u c r n R. («TEN, Madr id , SPAIN). EAES E n l a r g e d Sympos ium on He te rogeneous Heavy W a t e r Power R e a c t o r s , Majorca , Spain, Oct . 19G0. (CONF-4 J 0-1)

16. A CANADIAN APPROACH T O NUCLEAR POWER. G r a y J . L . A E C L - l t 5 5 . D c c . 1 9 G 0 . '

17. AN I l 2 0 - D 2 0 MODERATED REACTOR. H e b b i n g l o n W . . P . (Du Pont dc N e m o u r s E , I. & C o . , Aiken, S . C . USA). N u c l e a r S c i . a n d Eng . 8, '720, 'Doc. 1960.

18. REACTOR HANDBOOK. .2nd Ed. Rev i sed and E n l a r g e d . Vol . I. M a t e r i a l s . Tip ton J r . C. R. N'3W York , I n t o r s c i c n c c P u b l i s h e r s

•I960.

19. ECONOMIC POTENTIAL FOR D 2 0 POWER REACTORS. Isakoff 1. (Du Pont Co. Aiken, S. C . USA) D P - 5 7 0 . F e b . 1 961.

20 . S P K C I A L P H Y S I C O CHEMICAL PROBLEMS RELATED TO THE USE OF HEAVY WATER IN REACTORS.Di r i an G. Bul l . Inform. Sci . T e c h . ( P a r i s ) No. 87, 55-G7, Oct. 19G4.(In F r e n c h )

http://AECL-lt55.Dcc.19G0.'

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2 1 . ANALYSTS O F HEAVY WATER IN VIEW O F ITS I 'REPARATION AND USF, IN NUCLEAR REACTORS. Rolli E . Co l loqu ium on Heavy W a t e r . Madr id , Doc . 1962. ( J E N Madr id and EAES P a r i s ) . NP-.1.37GG. p . 135-54. (In F r e n c h )

22. HEAVY WATHIR POWFR REACTOR PROGRAM MONTHLY PROGRESS R E P O R T , .IANI/ARY 1364. (Savannah R i v e r O p e r a t ions Office, IJSAEC). SRO- 98 . , Ian . 19G4.

2 3 j T H E CSVTS 3rd C O N F E R E N C E ON NUCLEAR E N E R G E T I C S . M a i a s e k E. P r a g u e . 19(54. (in Czech)

24. ACCOUNTING SYSTEMS FOR HEAVY WATER AND FISSIONABLE MATERIALS. F l e t c h e r G. W . , Reid II. R . , J e n k i n s o n W. G. (AECL,

• Chalk R i v e r , Out. CANADA). A E C L - 2 2 0 2 . IAEA S y m p o s i u m on N u c l e a r M a t e r i a l s M a n a g e m e n t , Vienna ,Aug. 30 -Sep l . 3,19G5. (CONF-6 50803)

25. THtRD R E P O R T ON THE C O M P E T I T I V I T Y O F NUCLEAR ENERGY. S e r i e Studi E c o n o m i c i . CNEN 1 965. (In I ta l ian)

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27.. A COMPARATIVE EVALUATION OF. ADVANCED CONVERTERS. R o s e n t h a l M. W. et a l . ORNL-308(5. J a n . 1 9(55. . ,

28. DEMANDS FOR NUCLEAR F U E L S AND .COSTS OF D I F F E R E N T ; r REACTOR T Y P E S IN GERMANY. G r ü m m 11.,.Gupta D . , HhTelp W. et a l . KFK-3G(>. Soni. 19(55. :,, . . ; • .:-.,.-:

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ANALYSIS OF THE STUDIES ON THE ECONOMY" OF U-Th CYCLE. Scui ' icim CI. D . , Lav reticle D . , LIUTKHU A. , VendLUi P . E U R 2537Ì, 19GG.(In UnlLan)

ACHIEVEMENTS AND PROSPECTS OF HEAVY WATER REACTORS. Lewis W. B. (AECL, CANADA) D L - 7 3 . 1966.

THE ROLE AND REQUIREMENTS OF HEAVY WATER IN CANADA AND THE WOULD. Cochrane Ò. R. (Canadian Nuclear Assoc ia t ion , Toron to , Onl. CANADA)6G-CNA P a p o r r 3 0 1 . Annual Conference on Organic and Heavy Water R e a c t o r s , Winnipeg, Canada June 1966. (CONF-GGOolG-lü)

UTILIZATION O F DISCHARGED URANIUM IN HEAVY WATER REACTOUS. Grl lmm [I. Nuldeonik I), No. 8, 1 f)GG. (In German)

THOniÜM'BREEDERS AND CONVERTERS THEIR INFLUENCE ON F U E L CYC LE'ECONOMICS AND FUEL UTILIZATION. Kasten P . R . AEC Symposium on T h o r i u m Cycle Gat l inburg, T e n n . , USA. F e b . 19GG.

S U P P L E M E N T TO KFK-3GG:DEMANDS FOR NUCLEAR FUELS AND COSTS OF DIFFERENT REACTOR TYPES IN GERMANY. Gr l lmm It . , .Gupta D . , IlHfelc W. et a l . KFK-466, Sept. 1966. (In German)

,CANDU REACTORS TO 1980 AND IN THE LONG TERM. Gray J . L . , Lewis W. B . , Haywood L. R. 15 th" Sect ional Meeting of the World Power Conf. T r a n s a c t i o n s . Tokyo Oct. 15-20, 1966. Vol . Ill p . 1487-97.

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37. 11 R A W WATER POWER REACTORS. Mil lar C. IT.. (AEC, Chalk River , Out. CANADA). AEOL-2Ü27. Nov, 19CÌCJ.

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.the Kufure of Advanced Conver ters Portugal . Apr. 1 9G7.

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5 3 . TI I IS K C O N O M 1 C P O T E N T I A L O K D I F F K R 1 0 N T A D V A N C E D

R K A C T O R C O Ì V C K P T S I N A F U T U R E POWIOH. G E N E R A T I N G

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.STATUS OF HEAVY WATER REACTORS IN Till*] WORLD. Paul ieka I. (Boluinico Atomic Power Station, Czech. ). (Jn Slovak) (CONF-7012J4 , Paper No. 13. 5th conference on nuc lear power; P ios tany , Czechos lovakia , Doe. I 970)

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292

70. CIRENE PROTOTYPE. B r o m a t o A. (CNEN, Milan), Casagrande I . , Podret l t A. Com.Naz . Gncrg.Nucl. Notiz. 19, No. 3 ,28-42. Mar. 1973. (In Italian)

71. CIRENE RESEARCH AND DEVELOPMENT PROGRAM. Mancini C. (CNEN, Milan), Villani S. Com. Naz. Eiiorg. Nucl. Noti. 19, No. 3, 43-82. Mar. 1973. (In Italian)

72. PROSPECTS OF UTILIZATION OF THE CIRENE REACTORS. Barabaselii S. (CNEN, Milan), Cawtollt G. , Si lvest r i M.Com.Naz . Enui-K. Nucl. Noti-/.. 19, No. 3, «3-90. Mar, 1973. (In Italian)

73. APPROXIMATE CALCULATION METHOD FOR DESIGNING THE CORE SUPPORT STRUCTURE OF A PRESSURE TUBE REACTOR. Cravarolo L. , Zeiger P. (CISE, Segrato, Italy). Energ . nucl. (Milan) 20, No. 5, 280-292. May 1973.

74. SOURCE MATERIALS FOR NUCLEAR ENERGY. 1972 Atomic Energy Programs:Opera t ing and Development Functions;. (TID-26277, pp. 29-44)

293

C - TREATMENT OF DEGRADED HEAVY WATER

PURIFICATION OF D2O MODERATOR BY ION EXCHANGE. Hcston W. M,, BanicK- C, . 1 , , Wilson T. II. (E. I. du Pont de Nemrjiirs & Co.Savannah Riven- Lal>. Aiken S. C. USA). DP-73 . .Tune 1954.

APPLICATION OF MIXED-BED ION-EYCHANGE TO WATER PURIFICATION IN NUCLEAR REACTORS. SLvotz N . , Scheibelhut C.IJ. In<.I.Eiitf.Chem.47,No. I), 1020, 1955. (Pa r t I);Ind. Eng. Chem. 47/No. 10, 2140, 1955. ( l ' a r t If.)

RE-USE OF COOLING WATER IN AN AEC INSTALLATION. . Rilmloau A. L. Ind. Eng. Cl icm.48, No. 12, 2159, 195G.

BEHAVIOUR OF HEAVY WATER IN PILES OF CEA, Chenouard J . , Dirian G., Roth E. 9 /P /348 (FRANCE) 1st Geneva Conf. 1955.

PURIFICATION OF'THE HEAVY WATER OF REACTORS E L I AND EL2 BY ION EXCHANGE RESINS. Clienouard J . , Roth E. CEA-G73A. Sect. IV-VIII, p. 10-22, 1957. (AEC-tr-4G32)

DISTILLATION OF LIGHT WATER FROM HEAVY WATER MODERA TOR.Ber t schc E. C. (Du Pont do Nemours E. I. &Co. Savannah River Lab. Augusta, Ga. USA). DP-325. Dec.1958.

294

i l . I

i'l

ì

7. (On Heavy Water Epural iou). Natcr K .A. J e n e r Pubi. No. 17, .1959.

<L (On Heavy Water Epuratioii). Martiuola E . T e d i . Miti. 11, 412-G, 1959.

9. RECOVERY OF DgO FROM D.ET.ONIZERS. Ber tschc E. C. (Du Pont de Nemours E. I. fcCo. Savannah River L a b . , Augusta, Ga. USA). D P - 3 8 1 . Apr. .1959.

1 0. WATER TREATMENT PRO.iBLEMS IN NUCLEAR POWER PLANTS. Ellki G. (Budapest .Technical Univ . , 1IUNGARIA). Energia és Atnmted i . 13, 220-32, Apr, - May 19G0,(ln Hungarian)

3 1. THE USE OF HEAVY WATER IN NUCLEAR REACTORS. Chenouard J . Bull . Inforni. Sei. et T e d i . (Pa r i s ) No. 40, 3f>-47, May 19G 0. (In French)

12. RECOVERY OF DEGRADED HEAVY WATER AT THE SAVANNAH RIVER PLANT. Seotten W.C.(Du Pont t ic • Nemours E. I. &. Co. Savannah River L a b . , Aiken, S. C. USA USA). DP-470. July 19G0.

13. THE HEAVY WATER SYSTEM OF THE PROCESS DEVELOP MEN'I' PILE. Dunldoe A. E. (Du Poni eie Nemours 13.1. & Co.Savannah River Lab. , Aiken, S. C. USA). DP-5G7. June 1.961.

14. CHEMICAL AND RADIOCHEMICAL ANALYSIS AND PURIFICATION OF THE HEAVY WATER TAKEN FROM THE RA REACTOR. Maksimovie Z. P . , Ceranic T . , Marinkovic M. Bull. Inst. Nuel.Sei. "Tim-is Kidric:", Belgrade 13, J, 19G2.

295

MWtATU UE PURIFLCATI.ON l'UOGItl'ISS REPORT. I. DESCRIPTION OF EQUIPMENT, TESTS J.a, Hi, AND 1L. lir.nmuinnE. W. (I')u I'out di! Ni'inoiii'H K. I, to Co. Savuiiiinli Rivi-r Lnh, , Alki.-n; S.C. USA). DI'-fiYfl. Foli. JfUia.

TREATMENT ANT) ANALYSTS Ol-' 'ITIE WATER ANT) CAS IN •J l l l t -2 . (,1'apan At. KIHMVHUH, TUHL, Tokyo, ,TA PAN) J AERI-1024. Apr. 1 Wi'2. (In Jiipani'su)

SEPARATiVE WORK AS A PERFORMANCE CRITERION FOR A HEAVY WATER llECONCEN'rRATION UNIT, Scotton W. C. (Du PoiiL .du .No mourn. E . I . &Co, Savannah Hi vol Lab. /Aiken, S.C. USA). DÌ'-ti.Vi. May 19CÌ2.

CALCULATIONS FOR DISTILLATION OF DEGRADED HEAVY WATER..Svendsas P . (JEN, Madrid, SPATN;Europoan Atomic Energy Society, Par-is, FRANCE). NP-137GG (p. 85-93). Dec. 19G2.

PURIFICA'WON OF REACTOR. MODERATOR COOLANTS. P r o p o l i E .At . Energy Rcv . . l ,No . 1, 5-42, J 9G3. (In English)

TREATMENT OF WATER'.IN THE EXPERIMENTAL REACTORS OF T I IE C. E . A. Dolle L. ,Conan D. La Chimica del l 'Acqua noi Reattori Nuclear i , p.' 1 CI- 05. Symp. on Water Chemist ry in Reac to r s , Rome, CNJWN, J SCI«. (Ln French) (CONF-213)

HEAVY WATER CLEANUP BY ELECTROPHORESIS. Boyd.D. C. (Genoral E lec t r i c C o . , Jlanl'ord Atomic Products Operation, Richland, Wash: U S A ) ; H W - 7 7 Ö 5 0 . Aug. 1, 1 9G3.

••PitOB LE MS OF HEAVY WATER. PURI FTC ATJON BY ION EX-CIIANG'E METHOD. Tin Shw->uiitf, T'uny Ticn-c-lien, Ling- Fon-\i:\ni\ (Chincso Ai-adi-my '>r Srioiu-os, IVI.inj;. Iiisl. or Atomic Kniiff-y, c:111NA). NP-l(;(ii:t. I<HM.

296

23. HEAVY WATER HANDLING .EXPERIENCE IN THE SPERT II REACTOR F A C r U T Y , Montgomery C. Jl. (Phi l l ips Pe t ro l eum Co. Atomic Energy Div. , Idaho F a l l s , Idaho, USA). JDO-J «997. July 1 9fi4.

24. D 2 0 EXPERIENCE AT PU.C.F. Fishbaugor J. R. (General E l e c t r i c Co. Ilnnford Atomic Product« Operat ion, Richland, Wash. USA). HW-8M7:». J u l y 2 4 , 19(i4.

Proceeding« of Ilio Third Internat ional Conference on the P e a c e ful Usus of Atomic Energy, Geneva 1 9G4:

20. THE MANAGEMENT Ol-' HEAVY WATER .1<"OR RESEARCH AND POWER REACTORS. Mor r i son J . A. (Alomit: Energy of Canada Ltd. Chalk Rivor Nuclear Labs. , Chalk River , Out. ), Thomas M. I I . , Watson L. C . , Woodhoad L. W. 12. P / 2 9 (CANADA); (AECL-2029 . 1964)

2G. COMMERCIAL TECHNICAL METHODS FOR RECONCENTRA-TION AND PURIFICATION OF DEGRADED AND CONTAMCNED

. HEAVY WATER FOR NUCLEAR REACTORS.Sai to T . (Sliowa Denko K. K. , Tokyo), Sonoda S . , K u r iha r a Y., Takaniatsu T . , Morita T. 12, P / 4 3 3 . (JAPAN).

27. STUDIES ON TTIK RECONCENTRATJON OF DEGRADED HEAVY WATER. 11 a r ada A. , Kur lhara Y. (Showa Dunko C o . , L t d . , JAPAN) . Nippon Gcnshiryoku Gakkaishi (i, «28-32, Nov. 19G4. (In Japanese )

28.PURIFICATION OF HEAVY WATER BY ION EXCHANGE RESIN. Akishigc Harada , Yasuo Kur iha r a (Showa Denko C o . , L t d . , JAPAN) . Nippon Gcnshiryoku Gakkuishi G. G90-4, Dee . 19G4. (In Japanese )

2a.P(/R[FfCATION OF HEAVY WATER CONTAMINATED WITH : OIL. Paul S. D. , GaiH'san M. el a'l. (Alomic Kriorify Kstahl . , T r o m b a y , INDIA). Indian .1. 'IVHuiul. W, 2IÌ2-M, July 19(15.

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A HIGH SENSITIVITY HEAVY WATER LEAK D E T E C T O R . Bayly J . G. (AECL, Chalk R i v e r , Out. CANADA). A K C L - 2 2 0 1 . O c t . ] 0(55.

DECONTAMINATION OF TI 115 HEAVY WATER SYSTEM OF Till '; HA REACTOIl . MiiUaimovit' Z . H . , Nussonov P . M . , Nikolié li . M . , Miiviiìkuvii: JVI.J). /Elie L. IVI. Bull. B o r i s Kiclriu Ins t . Nuc.1. Sei . IG, 2 5 1 - 6 3 , Oct . 19G5. (In Russ i an )

PURIFICATION O F HEAVY WATER. 6th Ann . Rep . OECD, Halden R e a c t o r P ro j ec t 1 0 6 4 / 6 5 . .1065. (p. 151-7)

CHEMICAL ELIMINATION O F ALUMINA IN SUSPENSION IN HEAVY WATER O F NUCLEAR R E A C T O R S . Lecloux A. C E A - R - 2 9 9 0 . F e b . 1967.

CHEMICAL P R O B L E M S POSED BY THE OPERATION OF REACTORS. S y m p o s i u m on the C h e m i s t r y of R e a c t o r s , JÜLICH. Oct . 1966. V i l l a r d R. (CEA, P a r i s , F R A N C E ) . Rat l io-c h i m . Ac ta , C, 1-6, Sept. 19G7. (In F r e n c h )

PROCEDURES F O R HEAVY WATER RECONCENTRATION. Mi losev ic I t . , K o s a r i c .N. Nuld. E n c r g . 5, No. 3 -5 , 5 3 - 4 , 1000-69. (In S e r b o c r o a t i a n ) (CONF-G81079)

F U R T H E R D E V E L O P M E N T O F SULZER HEAVY WATER COLUMNS. WarlcriwciLl.Gr M. Sul'/.er T e c h . R e v . 53, 84-G, 1970

SULZER RECTIFYING P L A N T S FOR ENRICHING HEAVY WATER. Zmasek R. (Win t c r t hu r E n g i n e e r i n g W o r k s D i v . , S w i t z e r l a n d ) . S u l z e r T e c h . R e v . 54, No. 3 , 1 9 9 - 2 0 . 1 9 7 2 .

TRITIUM AND HYDROGEN EXTRACTION P L A N T S FOR ATOMIC POWER R E A C T O R S . D a m i a n i M. (Snlzer B r o t h e r s L td . / W i n t e r t h u r , S w i t z e r l a n d ) , Getra i td I I . , Sonn A . S u l z c r T e c h . Rev . 54, N o . 4 , 2 8 3 - 7 . 1972.

http://WarlcriwciLl.Gr

VI - LIST OF MAIN CONFERENCES ON HEAVY WATER

AND HEAVY WATER REACTORS

301

VI - LIST OF MAIN CONFERENCES ON HEAVY WATER AND IIBAVY .WATER UJSACTOHS

Simposium on Heavy Water Production oi-ganizcd by European Society of Atomic Energy. Rome Marcii 31-Apr i l 2, 1955.

Internat ional Conference on the Peaceful Uses of Atomic Energy (United Nations). Geneva, Aug. »-2 0, J 955. (1st Geneva Coni'. 1955). A/CONF 8 / l ' / 3 , 4 , 5,G,7, 34», 3 5 7 , 3 6 1 , 3 8 7 , 4 1 0 , 4 9 5 , 6 0 5 , 0 2 3 , 6 3 1 , 744, 790, 791, »19, H23,'839, Mil, 879, 8HG, 920, 923,927, 934, 958, 988, 1010, 1120.

T h i r d ElecLronic-Nucleal Internat ional Review. Scientific C o n g r e s s -Nuclear Sess ion: Colloquium on Heavy Water . Home, Italy, July 6,1956.

Internat ional Symposium on Isotope Separat ion. A m s t e r d a m , Netherlands. Apr . 23-27, 1957.

Second United Nations Internat ional Conference on the Peaceful Uses of Atomic Energy . Geneva, Sept. .1-13, 1958. (2nd Geneva Conf. 1958). A /CONF 15/P/135, .136, 151, 160, 180, 181, 188,208, 209, 210, 212, 231,24 5 ,246 ,255 ,259 ,334 , 335, 336, 340 ,423 ,424 ,491 ,559 ,572 ,575 , 500, UÓ0, 610, 723, 745, 703, 1000, 1063, 1065, .1150, 1154,'1.1 97, 1261, 1336, 1362, 1383, 1400, 1475,' 1476, 1524, l u l l , 1628, 1630, 1649, 1669, 1929, 1949, 2036, 2053,2094, 2105, 2250, 2323, 2336, 2424, 2471, 2495, 2538.

302

USAEC. Sympos ium on Heavy Wa te r Modera ted R e a c t o r s . G e r m a n -town, My. USA. March 3-4, 1959. (TID-7575)

A m e r i c a n Inst i tut ion of Chemica l E n g i n e e r s (A. I. Ch, E . ) Meeting. San Francisco, -Cal i f . USA. Dec . 1959

EAES En la rged Sympos ium on Heavy Wa te r P o w e r R e a c t o r s . Majorca, Spain. Oct. I960. (CONF-410)

[AEA Sympos ium on P r o g r a m m i n g and Uti l izat ion of R e s e a r c h Renclm-s. Vienna, Oct. 1G-21, 1961.

The Canadian Nuc lea r Assoc ia t ion Conference on Heavy Wa te r R e a c t o r s . Ottawa, Canada . May 1962.

Gth World P o w e r Conference . Melbourne , A u s t r a l i a . Oct. 20--'27, 1962.

Col loquium on Heavy Water , (Junta de E n e r g i a Nuc lea r Madrid and Eu ropean Atomic Energy Society, P a r i s ) Madrid , Spain. Dec. 13 -14 ,1962 .

IAEA Pane l on Heavy Wate r La t t i ce s .V ienna , F e b . 1963. (CONF-116)

The C'SVS Thi rd Conference on Nuc lea r E n e r g e t i c s . P r a g u e 1964.

Thi rd In te rna t iona l Conference 'on the Peacefu l Uses of Atomic E n e r g y . Geneva, Aug. 3.1-Sept. 9, 19G4. (3rd Geneva Conf. 1964) A / C O N F 2Ö/P/2, ' G, 7, 8, 9, 10, 11, 12, 29, 39, 40, 51 , 69, 70, 76, 78, 90, 91 , 116,129, 174, 17G, 209, 268,^290, 417, 433, 496, 522, 523, 525, 532, 557, 594, 595, 602, 603, G05, 608, 625, 630, 669, 673, 682, 683, 691 , 692, 697, 709, 711, 743, 744, 753, 754, 76-3, 777 ,778 , 779, 808, 809, 810, 833, 859,8G0,877.

303

Canadian Nuclear Association Annual Conference on Organic and Heavy Water Reactors . Winnipeg, Canada. May 30-Juno 1/196G. (CONF 6R051G-5)"

IAEA Symposium on Heavy Water Power Reactors . Vienna, Sept. 11-15, 106 7. (SM-99)

Brit ish Nuclear Society Conference on Steam Generating Heavy Water Reactors . London, UK. May 14-16, 1968.

IAEA Symposium on Economics of Nuclear Fuel . Gottwaldov, CSSR. May 27-31, 1968. (SM-Ì.05/8, 31, 32)

IAEA Panel on Utilization of Thorium in Power Reactors . Vienna, June 4-8, 19G8.

7th World Power Conference. Moscow, USSR. Aug. 20-25, 1968.

Reactor day 1969 of the German Atomforum. Frankfurt, F. R. G. Apr. 16.19G9:

Canadian Nuclear Association Annual Conference on the Status of Canadian Construction Pro jec t s . June 19G9.

Nuclex 69. International Nuclear Industries Fa i r and Technical Meetings. Basel, Switzerland. Oct. 6-11, 1969.

CNEN Symposium on the Technical and Economic Aspects of the Heavy Water Production. Turin, Italy. Sc-pt. 30-Oct, I, 1970.

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26. Fourt.li Intornntiotml Conference on the Peaceful Uses oj" AlomLc % Eucsvyy. (Teneva, Sept. (>-J(>, 1071. (4th Gonevu Coni'. 15)04) 8 A/CIONF. 4Ü/I ,/:I4G,0()7. , |

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307

Subject Index

I.. General

II. Bibliographies

III. Determination and Analyses of Deuterium and Heavy Water


A - Reviews of reparation processes B - Patent .Review - Patents selected from the files of

Brevatomc, P a r i s . - Addendum 1- Heavy Water Production by Chemical Exchange II2S-HDO 2- Heavy Water Production by Chemical Exchange NII3-IID 3- Heavy Water Production by Chemical.Exchange H2O-HD 4- Heavy Water Production by Chemical Exchange:

Equipment and Other Processes 5- Heavy Water Production by Hydrogen Distillation G- Heavy Water Production by Water Distillation 7- Heavy Water Production by Ammonia Distillation 8- Heavy Water Production by Methane Distillation 9- Heavy Water Production by Distillation of Other Compounds

10- Heavy Water Production by Electrolysis 11- Heavy Water Production by Other Processes

C - Actual Industrial Processes 1 - Chemical Exchange

1 - Bithcrmal Exchange between Hydrogen Sulphide and Water (HoS-IIDO)

2 - Chemical Exchange bci.wecn Ammonia and Hydrogen (NII3-HD)

3 - Hydrogen - Water Exchange (H20-HD) 2 - Distillation

1 - Distillation of Hydrogen 2 - Distillation of Water

3 - Electrolysis of Water D - Production Plants

1 - Table (Summary) 2 - Plants based on H2S-HDO Process 3 - Plants based on NII3-HD Process 4 - Plants based on II2O-HD 'Process 5 - Distillation Plants . G - Plants based on Electrolysis of Water

308

IC - Technical and economical a spec t s F - Potential Production P r o c e s s e s

1 - Chemical Exchange P r o c e s s e s 1 - Between Hydrogen and Deuter ium 2 - Between Hydrocarbons and Water

1 - Aromatic:« - II2O 2 - Unsafcurated Aliphatic» - 1I20 3 - .Saturatoci Aliplm.ti.es - II2O 4 - Heterocyclic: Hydrocarbons - H2O f) - Alicyclie Hydrocarbons - IT2O

3 - Between Hydrocarbons and Hydrogen 1 - Aroma t ics - Hydrogen 2 - Unsaturated AliphaU.cs - Hydrogen 3 - Saturated Alipliatj.es - Hydrogen

4 - Between Aminos , Aminoacids and Water 1 - Aminos - H2O 2 - Aminoaeicls - H20

!5 - Between Amines , A111i.noaci.ds and Hydrogen 1. - Amines - Hydrogen 2 - Amides - Hydrogen

6 - 'Between Organic Acids and Water or Hydrogen 1 - Organic Acids - H2O 2 - Organic Acids - Hydrogen ,

7 - 'Between Hydrides , Hydrates and Water .1. - Hydrides , Hydrates - HoO 2 - Phosphine - II2O 3 - Ars ine - II2O

ft - Between Hydrogen Halides and Different Substances 1 - Hydrogen Haliden - II2O 2 - Hydrogen Halides - Hydrogen 3 - Hydrogen Tlalidcs - Hydrocarbons 4 - Hydrogen HaJides - Organic Acids

0 - Between Jon Exchange Uesins and Water 10 - Between Mercaptans and Water ] I - Between Kolons and Water

2 - Physical Separation P roces se s 1 - Ahsorl ive 1'Vaclioiial.ion 2 - Adsorption 3 - Ceni ri fugai 4 - Inst i l la t ion of Ammonia and Methane 5 - Ins t i l la t ion of Other Compounds (i - Diffusion

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309

7 - Thermal Diffusion 3 - Solvent Extraction 0 - Others

3 - Other Polcntial Processes

Heavy Water Reactors

A - Table (Summary) B - Heavy Water Tfaactors in nuclear power programs C - Treatment of Degraded Heavy Water

Main Conferences on Heavy Water and Heavy Water Reactors

310

1 II III IV. A IV. 13 IV. B . IV. B.

IV. B. IV . 1.3. IV. B . IV. E . TV. B . IV. B . I.V. 13. IV. 13. IV. 13.

1 2 3 4 5 6 7 8 0

IC 1.1

Addend i IV. C . IV. C . IV. C. IV. C . IV. C . IV. C .

IV. D. IV. D. IV. 1").

iv. n. IV. "1"). IV. D. IV. D.

IV. E IV. F . IV. F . IV. F . IV. F . IV. F .

.1. 1. 1. 2_ 2,

3 1

1. 2

3 4 5 6

1. 1. 1. 1. 1.

)

m to 1?R 1 2

3 I 2

1

1 2..1 2 . 2 2 . 3 2 . 4

?, 33 43 75 97

sra 103 110 115 117 120 123 124 124 125 1.2 H

134 137 145 155 105 173 185 105-6 197-fì

ton 203 207 211 221 227 234 237 239

241 242

IV. F. IV. F. IV. F. IV. F. IV. F. IV. F. IV. F. IV. F. IV. F. IV. F. IV. F. IV. F. IV. F. IV. F. IV. F. IV. F. 1V.F. IV. F. IV. F. TV.F. IV. F. IV. F. I.V. F.

IV. F.

IV. F.

IV. F.

IV. IV.

IV. F,

IV. F,

V.A

V. 13 V.C VI

2. 3. 3. 3. 4. 4. 5. 5. 5. G. 7. 7. 7. 8. .1 8. 2

1.8. 3

1.8.4

1. 9

1. 10

1. 1 1

2. 1

2.2

2. 3

2.4

2.5

2.G

2.7

2.0

2. 9

3

243

244

246

248

249

250

251

252

253

254

255

256

258

259

20 0

261

262

26 3

264

205

266

267

270

271

272

273

274

275

276

277

281

283

293

301

Authors Index

311

A -

Abolson P. II.

Abernathoy lt. M.

Abraham B. M.

Aclamson A. W.

Addington N. G.

Adorni N.

Aerov M. E.

Agostini ,1. P .

Aharoni II.

Ahlbcrg «I.E.

Aie r e J .

Ailcin A . M .

Akar P .

Akhundov T . S .

Akishin P . A .

Aleksandrovich Y. A.

AlKii-Slatot' R. 13.

Alfreds on P . G.

Alkire G . J .

Allen R. E.

Alvrtroz-Oonaal.fi.s J . R.

A l y A. [. M.

Aiunnr id i II.

Ambrosi ni G .C .

Ainiek M.G.

IV (P. 1.2.3-3)

III (147)

IV (C. 2 .1 . -18 )

IV (P. 1.9-1)

IV (C. 2 .1 . -25 )

III (75, 80, 86, 88);IV (D. 5-56)

IV (C. 2 .1-37)

IV ( C I . 1.-54) .

IV (P.. 11-28)

IV (Ar23)

IV (C. 1.1-49)

V (B-43)

IV (A-125; C. 2. 1-33)

111(145,158)

I (146)

IV (C. 3 -12 ,40 ,53 ; D .6 -8 )

III (37)

IV (173)

ITI (49)

II (25)

IV (A-135; C I . 1-20; C . 2 . 2 . - 7 6 )

IV (C. 3-88,89)

IV ( C I . 1-19)

V (13-51)

IV (D.5-(!)

.11.

Amici S. 111(14 0)

Anderson C . E . 111(170)

Anderson L . C . IV (D. G-2)

Andreassen K. IV (C. 3-65)

Angelino G. C. IV (C. 2. 2-77; D. 5-5G, G4, G7)

Antipova N. P. Ili (94,97)

Antoncliik Yu . I . IH (114)

A r m s t r o n g F . S . II (40)

Arms t rong G. T. I (135); II (19)

Arnold H. Ti. IV (C. 1. 2 - 1 , 5, G; C. 1. 3-4)

Arn.stein TI. II. I (.11 fi)

Artaud J . 111(133)

Asada T. IV (C. 3-48)

Askins II. W. Ill (20G)

Aston F . W . I (49)

A u g o o d D . R . I (13G); IV (A-G2, 84; C . 2 . 1 - 2 2 ; F . 2 . 1 - 2 )

A y r o s J . A . I (234); IV (A-1G4)

•313

- B

Babcock D . F .

Babkov S. I,

Baortschi P.

Bailey B. M.

Hakin V. O.

Balaban A. T.

Balacoanu T.'C,

Baldctli S.

Bald us W.

Bully I.

Bamann E.

Bancroft A. R.

Banick C . J .

Banikiofco« G. C

Marabaschi. S.

HiU'aiiW.,1.

Barb D.

Barb ie r i W.

Bardwoll .1.

Ba r -E l i K.- : j

Barlow E . À.

ßarnocchi L.

Barr F . T.

Bar I hole my R.

Basmailjan 1).

Bales J. R.

Bate« R. G.

Bauche P .

IV (C. 1.1-9); V (B-G)

IV (C. 1.1-15)

I (223); III (112,201); IV (A-44; C. 2. 2-56, 63)

IV (C. 2 .1-29)

II (55)

IV ( F . 1 . 2 . 4 - 1 , 3 )

IV (C.1 .3 -15)

V (B-51)

IV (C.2.1-3G;D.5-42)

IV (F. 1.2.4-1)

I (36)

IV ( C . 2 . 2 - 5 5 ; E -51 ; F . 1.5. 1-3); V (B-41, 59)

V (C-.l)

IV (C.2 .1 -45)

V ( I1-72)

IV (C. 1.3-26)

IV (C. 1.2-59; C . 1 . 3 - 2 9 , 3 7 ; C.2.2-G7)

III (130,132)

IV (C.1 .3 -14)

n r ( B . 2-21); C. 1 .2-41; F . 1.5.1-1)

IV (D. 4-2)

IV (li. 11-3)

1 (114); IV (A-52; C. 1.2-29; E-19)

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Boorman C. IV (F. 2. 7-2)

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Bornlcessel K. IV (F. 2. 9-2)

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Botlmer-by A, A. IV (F. 1.11-1)

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Bottini A. T. IV ( F . l . 6 . 1 - 1 )

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Douglas J. E. IV (D. 6-18)

Doutsov P. Yu. Ill (93)

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Duncan J . F . I (225)

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Goldstein J . M. II (15, 16)

Goodal lC.A. •.,.,.. HI (49)

Goodman C. I (100) ' • ' • . .

Googin J! M. IV (C. 2. 2 -51 , 60)

Gordon B. E. IV (F . 1. 2. 1-6)

Gordon G. Ill (168)

Gossen W. Ill (51) ! ,

Goujon P. . I l l (141, 166)

Gould A. J . I (13); IV (F . 2. 2-1)

Grabowski E . J . IV (C. 1.1-3)

Graff J . I (93)

Gra f fo . ' IV (C. 2.1-17)

330

Grage rov I. P . I l l (79)

Grandcollot P . IV (C. 1. 2-44, 45)

Grane r J . IV (B. 6 -7 , 8, 16)

Gray J . L. V (B-13 ,36)

Graziarli G. V (B-45 ,55)

Grecu E. IV (A-99; 148,149; C . 1. 3-3G; E-31)

Green C . H . I (50)

Gregory II. S. IV (C. 3-42)

G r e i f f L . Y. 1(46)

G r e s k y A . T . I (233); IV (A-166)

Grooth S.R. de I (97)

G r o s s P . IV (C .3-35)

G r o s s e A. V. IV (C. 3-54) .

Groth W. I (120); IV (A-34,130)

Grove G. R. II (36)

Grauber G. H. 111(119)

G r u e m m H. V ( B - 2 8 , 3 3 , 35)

Grünspan S. I (193)

Gryson H. I (211)

Guenebaut H. IV (F . 1.4. 1-1)

Guenterschulzo A. IV (C. 3-29)

G u e r o n J . Il l (32, 41); IV (A-49)

Guggenlieim E. A. I (115) '

Guinot H. IV (C. 2. 2-16)

Guizoarn L. II (54) .

Gunderscn W. IV ( C . 3 - 6 8 , 6 9 , 7 2 )

Gupta D. IV ( C . 2 . 1 - 3 1 ) ; V (B-28, 35)

331

m

1 m M

Gutman J . R.

Gutovsky E. T. K.

Guymon R ,H .

Gverdisi tel i I. G.

IV (C. 1.2-28)

IV (C. 2.1-51)

IV.(D;6-32)

IV(A-145)

332

- II -

Haantjes J . I (27); IV (C.-2.1-3)

Habedank M. IV (C. 2 .2-69)

Haeffele W. V (B-28, 35)

H a e n n y J . IV (D. 5-49, 50, 51)

Hagiwara H. IV ( F . 1. 5 .1-2)

Hahn H.H. IV (B. 11-33)

H a h n H . T. IV ( F . 2 . 8-2)

Haiss insky M. 1(117)

H a l d e m a n R . G. 111(56)

H a l f o r d J . O . IV (D. 6-2)

Hall L. G. Ill (52); IV (C. 2 . 1-20)

H a l l N . F . IV (C. 2. 2-4)

H a l l W . H . I V ( D . 6 - 9 )

Hallaba E. IV (C. 3-88, 89)

Halle E . v a n IV (A-50)

Hal ler P . de IV (A-4 8)

Halpern J . IV (C. 1.3-52; F . 1 . 7 . 1 - 4 ; F . 1 .7. 2-5)

H a l p e r n O . IV (C.3-35)

Handley D. IV (D. 2-8)

Hankiewicz E . IV ( F . 1. 3 .1-4)

Hannerz K. IV (A-98; C. 1.3-11)

Hanson D. N. IV ( F . 2 .1-1)

Hansgirg F . IV (B . 3-1 ,2)

I-Iarada A. .,.' IV (C. 3-77, 78; D. 6-34); V (C.-27, 28)

Harada M. I l l (9); IV (C. 2. 2-7)

Harkins W. D. I (19); IV (D. 6-1)

333

Harmsen H. IV (P. 2. 6-4)

Harr is L. IV (P. 2.6-1)

Harrison J. M. IV (C. 2. 2-27, 30)

Hart R. G. 111(33)

Harteck P . Ill (19); IV (C.3-26; £-7)

Hartmann J. U. I (40)

Harty'H. V (B-46)

HartyW. M. IV (D. 6-13)

I-Iatada M. IV (P. 1. 2. 1-3)

Haubach W.J . IV (P. 2. 2-1, 15)

Haucke G. Ill (156)

HaulR.A.'W." IV (C. 1.1-16,27; C. 1. 2-36, 40, 42;

F . 1.2. 3-2; P . 1.1.0-2)

Havliqek F . IV (D. 5-39)

HaywarclW.H. Ill (123)

Haywood L. R. V(B-3G,43)

Hellmuth'D. IV (A-105)

He lmickL .S . IV (F. 1.2. 5-1)

Henslejv J . D . C . ' IV (D. 2-8)

Hering H. . 111(115)

Herr ick-C.B. IV (C. 1.1-2)

Hertz G.L . •;.'. • '• IV (F . 2. 6-2,4)

Hes tonW.M. V (C- l ) .

Heuberger M. t • II (40)

Heyningen W.E .von ' 111(20)

Heyrovsky J. IV (C.3-47)

Hi lbornH.S. ' "• IV,(D. 2-15, 16, 17, 19,20, 21)

334

Hllsch R. IV (P..2. 3-4).

Hippie J . A . J r . IV (C.3-34)

HironakaY. IV (P. 1. 2. 2 r 3 , 4)

Hlrota K. I (102); IV (F . 1. 2. 1-3, 4, 7; P . 1.2. 2-3,4)

His ano T. I (162)

Hiskcy C. F. I (89); IV (C. 1. 3-5; D. 2-1)

I-IoangT.F. 1(119)

Hodges R . J . IV (I 'M. 3. 1-7)

llodor I. IV (C. 1.3-54; D. 4-18)

Hoc ring T. C. IV (F. 1. 2 . 3 - 3)

Hojman .T.M. IV (0.3-02)

Itolcomb H..P. Ill (105)

H o l m V . C . F . IV (F. 1.1-2)

Ilolmbcrg K. E. I (214); IV (B. 9-1 2; P . 2. 5-3)

Holtslandur W.J . IV (F. ' l . 5. 1-6) ' -:/-n

Hondo E. TV (C. 3-4«) , y " .

Hori Y. IV (r:. 3-K!) ^

Horibe Y. Ill (125) 7 j "

Horiuti J . I (108,179); IV (C. 2 . 2 - 3 ; C. 3-45) .

Ilurnkc J . IV (C. 1;2-67; D.4-1G)

Howies on J . I (147)

Hsu H . P . III (92) "

Hsu Y. P . IV (D. 6-31)

Huber M. IV (D. 5-65)

Hucbener R. P . IV (C.1 .3 -17 ,20 , 31; D. 4-13)

Huebner H. . Ili'(188) •

Huffman J. R. IV (C. 2; 1-8, 9; C. 2. 2. -24; D. 5 -1 , 2, 3, 7, 8);

Hughes E . D . IV (C. 2 .2-6; D. 5-12,13)

Hughes H. E.

335

Hughes H. E.

Hull ILA.

Hunt C.d 'A.

limit II.

Hurst Jl.

Hutchinson C.

Hutchinson C A ,

Iluyskcns P .

Hvidt A.

IV (C. 2,1-25)

IV (D. 2-4)

IV (F. 2.1-1)

IV (C.3-15)

1(143); IV (A-G9)

IV (F . 1,1.0-1)

IV (C.2.2-2G)

IV (C.1.2-11)

IV (F. 1,4.2-1)

336

- I

Ica C. II. IV (A-130)

p o t a l i . IV (F . 1.2.4-4)

I h I e H « IV(C.1 .2 -3G)

Impastato F. J . IV (F . 1. 4 .1-3)

Indovina R, j (G4)

Ingoici C. K. HI (7);'lV (A-G); C. 2. 2-G)

Ingoici E. li m (Y)

I r s a A - P - IV ( C . l . 2-15, 16)

Isakofr t. v ( B - 1 9 )

' snida S. IV ( C I . 2-56)

I s h i d a T - IV ( C I . 3-44) Isberg P. I n ( 6 1 )

IvanovO.A. IV (F. 1. 3. 2-7)

Izrai levich E. A. \ (34g)

337

- J

Jackson D. P. IV (C.1.1-50)

Jacobs J. J. II (41) •

Jacobs J. AT. n (38,40)

Jacobson 0. HI(17)

Jacolin O. II (51)

Jaeger K. i n (175)

Jafrkc IT. IV (C. 2. 2-50)

James B .J . IV (C.1.3-52)

Jason A.C. 111(148)

Jaulmos P. IV (C. 2. 2-9)

Jerfcrs P. IV (P. 1.2. 3-7)

Jeffries R. IV (F. 1.4. 2-2)

-lenkinson W. G. V (B-24)

Jcnn J. T. IV (A-125)

Johanscn CI. Ill (17)

Johns T . F . IV (A-7G)

JohnsonB.S. IV (C. 2. 2-71)

JohnsonC.A. IV (C. 2. 2-34)

Johnson F. A. 1(174)

Johnson K. D, IV (22-27)

Johnson V. II.' II (30, 31, 34)

Johnston I-I.L. IV (C. 2.1-11, 12; D. 5-9; D.G-9)

Jones M. L. IV (C. 1. 3-50)

Jones T. O. IV (C.2.2-4)

Jones W. AT. HI (164)-'

Jo r i s G.G.

Joseph E. F .

Jos t W.

Julliot C.

Ju ra G.

IV (A-35; C. 1.3-5)

IV (D.G-32)

IV ( F . 2. 6-1)

II (110)

III (53)

>>*'.

339

1(178); IV (B. 10-3;

IV(A-77; F . 1.8.'2-

IV (C.1.2-51,55)

I (1); III (2)

IV (A-106)

IV (C.3-30)

IV (C. 2.1-30)

IV (B. 10-29)

111(106)

IV (C. 1.2-30)

IV (C. 1.2-15,16)

Kakihana II.

Kalinachenko V. R.

Kalinina S. E.

Kallmann H.

Kalyanasundaram C. V.

Kamienski B.

Kanda E.

Kandier L.

Kanekar C. R.

Kaneko J.

Kant A.

Kaplein A.

Kasten P. R.

Katclnikov S. G.

Katorski' A.

Kats M.ya.

K a t z J . J .

Kawashimn K.

Kawazoo Y.

Kazanskii V. B.

Ka'/avchinskii Yrx. 7,.

KecsomW.II.

Kokoh A.

K6)

V(B-34)

IV (C. 1.1-37)

IV (F. 2. 2-8, 9,15)

III (71,121)

IV (C. 1.1-21; E-lß)

IV (D. 6-20, 33)

IV (P. 1.2.4-4) : I V ( F . r . 3 . 2 - 5 )

1(188)

IV (C.2.1-3)

IV (A-158)

340

Keller F . IV (C.'3-20)

Keller W. 11. • IV (D.2-3); V (B-3?)

Kelly M. IV (F. 1.1-8)

Rombali C. IV (C.1.1-36; C.1.2-23,25; F . 2. 3-1)

Kcnyon A. R. IV (C. 1.2-50)

K c r w i n l . L. 111(103)

Kesselraum P . M. 1(188)

Kess le r R.W. IV (C. 1.3-17, 20, 31; D.4-13)

K e y c s D . B. IV (C. 2. 2 -21 , 39)

Kilcle G. I (74) '

Kimball A. H. II (5, 6)

Kimball G. E. IV (A-13,15)

Kimbrough D. J r . 111(206)

King. J . J r . IV (F. '2. 2-12)

K i r i l l i n V . A . I (188);'III (117)

Kirshenbaum I. I (93,125,127); II (6); IV (A-18J53;-,C'.l;l r10)

Kiss I. 1 (199) ' ' S ;

Kis temakcr J . 1(155)

Kitt G. P . IV (F . 2. 2-4)

Klein F . S. IV (B. 2-29; C. 1. 2-41; F . 1. 5.1-1)

Klein R. IV (F. 1.1-4)

Klomm A. I (01,151); IV (A-26; B . 10-5; C. 3-58)

Kliefoth W. I (141)

Klotz I .M. IV (F . 1.4.2-5)

Knaap II. F . P . I (205) ,

Knezevic Z .V. III (181)

K n o b l e r C . M . ., IV ( F . 2 . 2 - 1 5 )

Kno t tA ;R . 111(197)

341

K n o p L . . IV (C. 2 .2-58)

K n o w l e s A . E . IV (B.'10-4)

Kobayakawa M. 111(125) ,

Kocent A. HI (184)

Kodera T. l (159)

KohnH.W. IV (F . 2. 2-11)

Kol tsnyUZ. IV (D.2-28)

Kono M.' IV (A-94)

Kosar ic N. v (C-35)

Kot A.A. 1(195)

K r a m e r H. HI (207); V (B-53)

Krause I. M. IV (F . 1.4. 2-1)

K r e l l E . IV (A-147; C. 2.'1--41; C. 2. 2-68, 74)

K r e s g e A . J . IV (C. 1.3-19)

K r e t z c h m a n G . IV (A-111; c i 2. 2-66, 69; F . 2. 5-4)

Krogh A. m (13) ;

Kroh J. - , IV (F . 1 .3 .1-4)

Kronbergor II. IV (F . 2 .7-2)

Krumbicgel P . Ill (188)

Kruse E. * (145) •

Kubota M. , IV (C. 2 .1-30)

K u c h a e v V . L . IV (F . 1.1-7)

Kuechler L. !V (A-10Ó; C . 3 - 3 1 ; E-20)

K u e s s n c r A . ,'. '.IV (B. 10-25)

Kuhn W. IV (A-44; C. 2. 2-5G; D. 5-GO)

Kulicke P . IV (A-147)

Kumar R. Il l (113); IV (A-106; C. 3-84; E-36)

Kummer J . T. IV (C. 1.' 2-21)

342

K u m m e r e r K.

Kurchatov I. V.

Kurihara Y.

Kuwata K.

Kysela J .

III (14G)

1(157)

IV (A-12G, 127; C. ' l . '3-40); V (C-26, 27, 28)

IV (F . 1 -2.1-3)

III (211) "• •

• I

ni'«*!.',

343

L a b a t o n V . Y . IV (P."l." 8.1-2)

Labine R .A. IV (E-12)

Laidler K . J . I (84)

Lake G. R. IV (C. 2. 2-32)

Lamber t R. W. IV (F . 1.'2. 1-2)

Landsberg G. S. 1(3)

Lane J . A. V (B-12)

Lang G. IV (C. 1. 2-66; D. 3-11,16; E-59)

LangdonW.M. ;; IV (C. 2. 2-39)

Langer A. I (124)

Lantus E . H . - IV(A-174) .

Lapteva F . S. Ill (121) : ,

Large E . • ••'_•, IV (C. 2. 2-12)

Lasareff W. I (1); HI (2)/

L a s s e t t r e E . N. ; IV (F . 2 .2-7)

Las son A. T. IV (C. 3-72)

Lauder I. J . I (109) . ;

Lavrencic D. jV. IB-30,48)

Lavrovskaya G.K. ; •; III,(G2); IV ( F . 1. 3. 2 - 1 , 3)

L a w C . A . ; : IV (A-157; C. 1.1-39; E-30, 53)

Lawrence S. J . 11(11)

Lazard B. IV (A-86; C. 1.1-22; D. 5-45)

Lazurkin Yu .S . IV (F . 1 .3 .2-6)

Lazzar in i E . Ill (169)

Le Chate l ier J . IV (D. 3-5 , 7)

Leconte J . Ill (54)

344

Ledoux A.

Leo J . L.

Lees A.

Lefrancois B ,

L e h m c r W.

L e h r e r Y.

Leichtl ing B , H .

Lentz H.

Lepoutre G.

Le ra t J. M.

Lewins D. M.

Lewis D.

Lewis G. N.

Lewis G. P .

Lewis W. B.

Leyden D. E,

Libby W. F .

L ich tens te in R. M.

Liforov V. G.

Lifshi tz A.

L i n d e r s t r o e m - L a n g C . U .

L i n d e r s t r ö e m - L a n g K.

Lindner J .

Ling F . L.

• L i u . w T . C ,

Llewcll in .D. R.

V (C-33)

IV (C. 1.2-37)

111(148)

IV (A-134, 171; C. 1. 2 -33 , 34, 49, 60; D. 3-4, 7,14)

IV (C. 2. 1-36 ,48 ,49; D. 5-42)

IV (D. 5-27, 41)

IV ( F . 1.4. 2-6)

IV (C. 2. 2-83; E-46)

IV (C. 1.2-43)

I (193);.IV (A-134)

, IV(A-1G7, 173)

IV (C. 1.1-48)

I (7); I V ( C . 2 . 2 - 1 ; C . 3 - 2 , 6 )

IV (C. 3-80)

V ( B - 4 , 3 1 , 3 6 , 4 4 , 6 7 )

III (180)

IV (C. 2 .1-10)

I (102)"

111(151)

IV ( C . 1 . 1 - 4 8 )

IV (A-Ì18 ; F . 1 .4 .1 -2 ; F . 1.4. 2-1)

III (17)

1(21)

V (C-22) ••"•••• ^

HI (160," 161) / r'

IV (C.'2. "2-43, 47; D .5 -13)

/

345

Lloyd J. T. IV (D. 6-20)

L o C . F . ' III (161)

Lohmar W. IV (F . 2. 2-2)

London H. I (175)

Long F . A. IV ( F . 1.2. 2-6)

Lor ies R. IV (C .1 .2 -11)

Lousiart A. 111(110)

Loveridge B .A . 111(58)

Lozhkina M. G. IV (F . 1. 3. 3-2; F . 1. 8. 1-1)

Lumetti A. V (B-30)

Lundberg L. I l l (61)

Lundkvist B. . I (198)

Lunelund H. 1.(53)

Lyon A .M. IV (C. 2. 2-26)

L y o n C . J . IV (A-104; D. 2-8)

346

M -

Mac Donald A. I l l (81)

Mac Donald C. G. IV (F . 1. 3. 1-3)

Mackenzie H . A . E . IV (C. 2. 2-44, 45; D. 5-17)

Madison J . J . IV (F . 1. 2. 1-6)

Mahadevan E. G. I l l (113, 191); IV (C. 1. 3-39; F . 1. 2. 2-5)

Mjzovb M. Ill (186)

M a k i s h i m a S . IV (C. 1.3-21)

Maksimovic Z . B. V (C-14 , 31)

Malan-Nelson A. M. I (44)

Malasek E. IV (E-37); V (B-23)

Malherbe P . N . IV (C. 2. 2-45; D. 5-17)

M a l k o v M . P . IV (A-89; C. 2. 1-14, 32 ,40; D. 5-20)

Mal leroy A. IV (A-162)

M a l o n e y J . O . IV (C. 2. 1-19, 25; D. 4 - 3 , 4 ; D. 5-28)

M a l y u s o v V . A . IV (C. 2. 1-37) • ,.

Mancini C. V (B-71)

Manciulescu A. 'IV'(A-159)

Mandel H. V (B-58)

Manowitz B . 1(229)

M a r a z a n N . IV (C. 1.3-38)

M a r c h e t t i C . I (29); III (43, 47); IV (C. 1. 3-8; D. 6-23,30)

M a r c u s W . C . d e IV (A-50)

Marda le i shv i l i 11. E. IH (G2); IV (F . 1. 3. 2 - 1 , 3)

Margincanu P . IV (C. 1. 3-25, 30, 32, 37, 38, 47, 57, 59)

M a r i a - A r c o c h a A. M. IV (A-135; C. 1. 1-20; D. 6-35 , 36)

Marinkovic M. D. V (C-14, 31)

Mark II. 1 (41 ,52 )

347

Marsigny L. IV (F. 1. 4. 1-1) .

Martin TI. . I (113); IV (C. 3-60)

Martin IT. Z. IV C. 1. 2-29)

Martin W. IV (C. 2. 2-12)

Marcinola F . V (C-8)

Marx R. IV (C. 1.1-26)

Masami S. • IV (D. 5-61, 62)

Mateescu F . IV (F. 1.2. 4-3)

MathurS .C. HI (106)

Matsugashita T. IV (C. 2. 1-30)

Matsumoto S. IV (D. 5-61; D. 6-33)

Matsushima T. IV (C. 1.3-53)

Mat tauchJ . 1(29,54,81,86)

Mat te r 'G.L IV(C .2 .2 -22 )

MaughanG.L ' II (39)

Mayer I L L . I (87); IV (A-17, 24, 25; C. 1. 2-7, 8, 10)

Mayer M.'G. • IV (A-29)

Mazzoni A.' IV (D. 5-22)

M c C l u r e D . C . IV (C. 1.1-2)

Mc Daniel E . L . IV (F . 1. G. 2-1)

Mc Donald R. T. IV (C. 3-6)

Mc Donough R. Ill (59)

Me Fadden C. II (32)

M c K e e D . W . IV (F. 1. 3. 3-3)

Mc Lain S. I (143): IV (A-69)

Mc Manus C. J . IV (C.'2. i -13)

Mc Williams J . A. • IV (D. 5-29, 33)

Meersche M. van ' IV (F .1 .1 -1 )

348

IVIeleshko V. P . IV (F . 1. 9-2)

Mcnes F . I (193)

Mcrcca J . Ill (204); IV (C. 1. 3-32)

Mercca V. I (213); IV (A-99, 148, 149, 1G0; C. 1. 3-29,

32, 3G, 37, 47, GO; D . 4 - 1 5 , 17; E-31)

M e r i e l Y . IV (A-133)

Mer l iva t L. IV (C. 2. 2-72)

Meyer F . I (134)

Mikami II. IV ( F . 2. 9-1)

Miliaila A. II (59); IV (A-155)

Mikkelcit W. Ill (15G)

Mikolic S. S. I (5)

M i l l a r C . H . V (13-37)

Mi l le r A. I. I (215)

Mil ler R. W. IV (C. 2. 2-38)

. M i l l c r S . L. IV (C. 1.3-1.8)

Mil ls G. F . " II (10); IV (C .2 .2 -4G)

M i l h c r A . M. • IV (C. 2. 2-44)

Milosevic R. V (C-35)

Missbach D. IV (À-U.7) . •

Mi tchel l J . J r . IV(C:2.-2- .18) '.

Miyahara K. IV (C. 1 . 2 - 3 1 , 4G)

Mizusliina T. - IV (A-94)

Moggi S. ' I (71)

Mol inar i Ph. I (193); IV (F . 2. 2-14)

Mongini L. 1 (139)

Monier .I .A. IV (D. 5-5; D .6 -10 )

Monna G. IV (C. 2. 1-30)

Montarna l R. IV (C. 1. 3-15)

349

Montgomery C R . V (C-23)

Montgomery G. W. IV ( C 2. 2-30)

Moraru N. IV (C. 1. 2-53; C. 1. 3-54; E-31)

Moravec J. Ili (211)

Morcau C. IV (C. 1.2-43)

Morgan T. D. Ili (147)

MorLta N. Ili (12): IV (C. 1.3-22)

Morlta T. V (C-26) \

Morowitz I-I. J. II (17) • . ' • • : • • •

MorozovN. M. IV (C. 1.3-33)

Morphcw A. T. II (9)

Morris J .W. IV (A-117; C. •]. 1-9, 34)

Morrison J. A. V (C-25) :

Morrison J. U IV (F. 1. 4. 2-3)

MrochekJ . È. IV (E-52)

Muhele K. IV (A-147; C. 2. 2-66, 69; F . 2. 5-4)

Mueller G. I (200); IV (F. 2. 7-4)

Mucllcnpfordt J . I (209)

Mund W. IV ( C I . 2-11; F . 1. 1-1)

Murphy C. M. I (2, 125, 127); III (3, 5); IV (A-53; C. 2. 2-2)

MiirronhoffA. P. T (1 90); TV (A-1 31, 132) *

Muyllo R. 1. ( I 08)

MyagkoiO.N. IV (F. 1. 9-2)

Myhrc K. IV (C. 3-713)

350

N -

Nacl imanovich M . L . IV (C. 1. 3-33)

N a g a r a j a - R a o S. IV (E-33)

Nagra thna R. A. II (Gl)

Naito Y. I l l (100)

Nakanishi A. IV (A-94)

Namba S. I l l (83)

N a s s o n o v P . M . V (C-31)

N a l c r K . A . V (C-7)

Na t ta G. IV (C. 2. 2-22)

N e d u m o v a E . S . TV (C. 1.3-46)

Nelson W. L . IV (E-47)

Nepi 0 . V (B-5.1)

Neumann K. . IV (C. 2. 2-13)

Neumann L. I (196)

Newel l J . L . I V ( C . 3 - 3 ) / ; :

Newell W . C . IV (C .3 -42 ) . - , ,

Newton C. L . IV (C. 2 , 1 - 5 0 )

Nicho las C M . .• ; 1 (173) ' : . / : • • • ;

N i e f G . ••• . : III (126,144); IV (A-86, 121; C. 2. 2-72)

N i c r A . O . C . I (155); III ' (21) '

Nikolaev M. N. 111(151)

M k o l a c v P. N. IV (A-59)

N i k o U c R . M . V (C-31)

Nito S. IV (C. 3-77 , 78; D. G-33, 34)

M t s c h k e E. IV (A-175; J J . 3 - 1 2 ; D . 4 - 1 3 )

Noguclii T. IV (C. 3-36 ,51)

Nordemann. D. Ill (110)

I ?

351

I Normand J . I11 <133)

I Norton E .R . IV (C.1 .1-46 , 47)

I Norton W . J . IV (C. 1.1-6)

I Novakovic M. IV (C. 2.2-57)

! Nowak E . S . 111(205)

352

O -

Obi nata I.

Oddio T. II.

Ugo K.

Okahc: T.

Okaj ima Y.

Okajnoto CI.

Olar iu A.

Oppenhe im I,

Orch in M.

Orlov V . V .

u r s o n i B.

Or son i L.

Or tego J . M.

O r t i z - F o r n a g u e r a R.

Ota Y.

Otero de la Gamlara J . L.

Ote ro N a v a s c u e s J . M.

O t h m c r D. F .

Otwos J . W .

Ou ei le t C.

Oulibin S. A.

Oyama Y.

I V ( B : 1 0 - 2 8 )

IV ( C . 3 - 3 8 )

VIB-GG)

HI (.1.39)

IV (C.3-GC)

IV ( C . 2 . 2 - 8 ; C . 3 - 4 5 )

IV (A-149, 1G9; C. 1. 3-32, 37, 38, 47 , 57, 59; C , 2 . 2-G7; D. 5-58; E-31)

il (34)

111(3 0)

III (151)

IV (D.G-14)

III (3G); IV (C. 3-59; D. 6 -17 , 21)

IV (C. 2. 2-79)

V (B-15)

IV (C. 3 - 2 1 , 37)

III (1.11, 142, 150, 171 ,177 , 192); IV (A-72 , 135; C. 1. 1-20; C . 2 . 2 - 7 6 ; C. 3-67, 73; D . 6 - 3 5 , 3 G , 3 8 , 3 9 ; E-17)

V (B-7)

IV ( C . 2 . 2 - 1 9 , 20, 23)

IV ( F . 1 .3 . 2-2)

1 (22)

111(117)

IV ( F . 2. 9-1)

353

- P -

Paabo M. 1(228); 111(202)

P a e m e l O. van I (99)

Paladi M. IV (C. 1. 3-55)

Pa l ibroda N. . IV (A-148; C. 1. 3-36, 42; D. 4 -15 ,17 ;

E-31)

Panchcnkov. G. M. I (14G); IV (F . 1. 9-3)

Panne t ie r G. IV (F . 1. 4 . 1 - 1 ) P a o l u z i G . I V ( F . 1 . 4 . 1 - D

P a r f e n o v V . A . 111(151)

P a r k J . L. II (16)

P a r k e r A. 111(136)

P a r r a v a n o G. I (101)

P a r r u c i n i M. Ill (59)

P a t t e r s o n W. A. 111(59)

P a u d l e r W . W . IV ( F . ' l . 2. 5-1)

Pau l S.D. V (C-29)

Paul icka I. V (B-6J)

Pau l sen F . R. IV (C. 1.2-35)

Pavlov K . F . IV (C. 1.2-14)

Pavlovic B. IV (C. 1.3-9)

P e a r s e R. W. B. IV (F. 2 .6-1)

Peculea M. I V ( A - 9 9 , 1 4 3 C. 1 .3-36, 54 D . 4 - 1 4 , 1 5 , 18 E - 3 1 , 3 4 , 3 8 , 4 1 , 4 3 , 5 0 )

P e d r e t t i A. V (B-70)

P e g r a m G. B. IV (D. 5 - 1 , 2)

P e i s a c h M. I (169) III (140)

P e p p e r D. IV (C. 1 .2-47,50) '

P e r i l l i M. L. V (B-54)

.354

Per lman M. L. Ill (48, 50); IV (C. 1. 2-15, 16, 18, 19, 27)

Pcrpero l H. IV (A-3 3)

P e r r y J . II. ' 1(85)

Pc r s son T. I (198)

Pe t e r s K. IV (F . 2. 2-2)

P o t l e r s e n G . T . IV (C. 2. 2-73; F . 2. 4-4 , 5)

Pctrov I .Ya. IV (F. 1. 3. 2-6)

Pctrov P .A . V (B-8)

P e t t e r s L . B. IV (F. 1. 8. 4-1)

Phill ips J . C. IV (C. 2. 2-29)

Pierot t i G . J . IV (C. 2. 2-38)

Pigford R. 1.(15 0)

Pilot J . IV (F. 2. 9-2)

Pilz S. IV(A-92; D. 5-47)

Pimentel G. C. 111(53)

P i r e t E . L . 1(158)

Pi r inger O. IV (C..1. 3-25, 55)

P l a s k u r a W . I (207)

Pohl I-I. A. I &72); IV (C. 1.1-28, 30, 31,32; D. 2-4)

Pohler G.M. IV (C. 2. 2-23)

Polanyi 'M. I (48); II (4); IV (C. 3-9)

Po las t r i F . IV (D. 3-15)

Pomerantz P . IV (C. 2. 2-42; D. 5-16)

Pot te r R. A. Ill (24, 27, 28, 29)

Powel l ' J . I (229)

Prasad N . B . IV (C.2 .1-31)

P ra t t H . R . C . I (170); IV. (A-67 f 141; C. 2. 2-54; D. 2-8;

D.5-29 ,33)

P r e s s u n g B. 3 IV (D. 5-57)

P re to r ius R. m (210)

P re to r ius V. IV (B. 11-33)

355

Prigogine I. IV (F . 2. 7-1)

P roc to r J. P . IV (D. 2-13; E-22 , 25, 32)

P roksch E . Ill (162); V (C-19)

P rosov i t s P . I (47)

P r o s s e r II. C. Ill (48, 50); IV (C. 1. 2-16)

P r o t t e r S . R . 111(195)

Puddington I . E . Ill (31)

Pugh 0 . IV (F . .1 .8 . 1-2)

Pu rca ru C.I . I (153)

Pu rce l l R.I-I. IV (C. 3-42)

Pyper .T .W. IV (F . 1. 2. 2-6)

35fi

Q

Qu inn F . G . I.V (C. 1. 2-2, 9; C. 2. 1-19; D. 4.-4; D. 5-28)

357

- R -

Rabinovich I. B. IV (A-59)

Rabinovitch B. S. IV (D. 6-18)

R a d u l e s c u C . 1(161)

Rae II. K. IV (A-138, 142,165; C. 1. 1-44: C. 2. 2-52,

53, 55; E - 5 ; F . 1. 5. 1-3,6); V (B-59)

Raman M.S. IV (C. 3-76, 84)

Rampey W. P . Ill (208)

Randall M. IV (C. 2. 2-17)

Rank D.H. IV (C. 3-7)

Ranque G.I . IV ( F . 2 . 3 - 3 )

RapLalA. S. IV (D. 5-66)

Rapoport L. L. IV (C. 1.2-51)

R a v o i r e J . IV (C. 1. 2-44, 45 , 54, 65)

R a y H . S . IV (D. 4-4 ; D. 5-28)

R e a s e r P . B. 111(108)

Rebora P . L. IV (C. 1. 2-38)

Reed R. I . 111(81)

R e g i m b a l J . J . Ill (123)

Reid A . F . IV (A-32)

ReidPI. B. V (B-24)

R e i l l e y C . N . Ill (180); IV (F . 1. 6. 1-2)

Reinhold G. .IV (F . 2. 7-4)

Reitz O. • .1.(55)

Renzon iR. IV (C. 1. 3-8, 12, 16, 20; D. 4 -8 , 9;D. 6-27, 30)

Reuben J. IV (F . 1. 7. 2-6)

Reyerson L. H. ' IV (F . 1. 2. 2-1)

358

Reynolds P . Il l (58,65)

Reynolds T. G. IV (C. 1. 2. -2)

Ribnikar S. IV (C. 1.3-9)

Rich E . H . IV (C. 2. 2-42)

Richter E. L. Ill (174)

Ridoal E. K. I (24)

Riedinger M. IV (C. 2. 2-78)

Riosenfeld E . H . I (G5)

Riualclini C. V (B-45 , 55)

Rishcr C. IV (C. 2 .1-13)

Rit tenbcrg D. IV (C. 1. 3-18)

Rivldn S. L. I (.1.88); III (145,158)

Rober ts E . R. TV (C .1 ;2 -14)

Robinson II. K: 111(196)

Robinson R . D . IV (D. 2-25)

Rock S. M. Ill (37)

R o d d e n C . J. I (192)

Rogiinski S.S. • I (182)

Rojas de Diego J . L. Ill (150 ,171,177, 182, 192); IV (A-135; C. 1. 1-20; C. 2. 2-79, 80, 81; D. 5-70; D.6-39)

Rolle W. Ill (188)

Romaniw M. IV (B. 6 - 1 , 2; B . 11-1)

Rosatzin II. I (223); III (201)

Rosebury F . 111(20)

Rosenthal M. W. V (B-27)

Roseo L ; iy--(C. l . 3-7,8)

Rosta P . Z . I (235)

Rostaing M. IV (A-136, 168;C. 1. 1-38;D. 3-6)w .;

Roth E. 1(142, 193;202);III (41,54, 153);IV(A-58, 68, 86, 101, 119, 134, 136, 166, 168, 171;C. 1.2-39, 62); V (B-21;C-4 , 5)

359

Rothberg S. . IV (D. 5-16)

Rowland P . R. 111(193,197)

Royen P . I (72)

Rozen A.'M. I (154); IV (A-57, 109; C. 2. 1.-21)

Rozenborg J . IV ( F . 3 - 2 )

Rozental K. I. IV (C. 3-5G, 57)

Rubin L. C. IV (C. 2. 2-33,34)

Rubissow G. A. IV (B. 11-27)

Ruderman I. W. I (152)

Ruhtz E. IV (C. 3-60)

Rusk inS . L. IV (B. 11-16)

Rüssel S. II. IV (E-55)

R u s t F . G . D . IV (C. 2. 2-71)

Rustad B. 1X1(21)

Rutherford E . 1(12,33)

Ruzicka J . IV (C. 2 .1 -35 ; E-23)

RyanR.-K.'"' IV (A-151)

Rypar V. I (196)

360

Saclhukhan H. K.

Sage B. II.

Saito E.

Sa ito II.

Saito T.

Sakharovski i Yu. A.

Sakodynskii K. I.

Salmon O. N.

Samoilov L. N.

Sampaleanu L.

Samuel F ;

Sandroni S.

Sands t rocm A. E .

Sansone M.

Santos-Macedo C. M.

Sap i r s tc in L. A.

Sara V.

Sataka O.

Satchel'l D. P . N.

Sato S.

Sato T.

Sat t le r H.

Savard J .

Savie P .

Sawayanagi S.

IV (D. 2-27)

IV ( C . l . 1 - 1 1 )

I (193)

IV ( C . l . 3-22)

V (C-26)

IV ( C I . 2-61)

I (187); IV (A-88, 95 ,103 , C 1. 1-15).

IV (F . 1 .7 .1-1)

I (189)

IV (A-143; C. 1.3-54)

IV ( F . 1 . 7 . 2 - 6 )

III (127, 132)

III (45)

V (B-54)

IV (A-93)

II (38)

III (211)

IV ( C I . 3-22)

IV (F. 1 .2 .1-2)

IV (C. 2 .1-30)

IV ( C 2. 1-30)

IV (C. 2. 2-12)

IV (C.3-55)

IV (C. 1.3-9; C 2. 2-57)

IV ( C I . 3-40)

361

SaxenaS ' .C. IV (F . 2. 7-3)

Sayama H. IV (A-94)

Scatchard G. IV (C. 2, 2-25)

Schacher l F . IV (A-4)

Schaeffer O. A. IV (F . 1.1-6)

Schaumburg K. 111(199)

Scheepors L. Ill (8); IV (C. 3-18)

Scheer M.D. IV (F . 1.1-4)

Scheibelhut C .H. V (C-2)

Schenkel G. • HI(129)

Schierholz H. IV (C. 1.2-36)

Schindcwolf U. IV (C. 1. 2-48, 53, 66, 67;C. 1. 3-34; D. 3-2, 11, 16 ; .D.4-13 , 16; E-59)

Sc la t t e re r R. IV (C. 2 .1-36)

Schmid L . C . V (B-50)

Schmidt W. A. 111(174)

Schmieschek U. IV (B. 11-22)

Schnette R. I (212)

S c h o e n L . J . IV (F . 1.1-4)

Schoenborn E. M. ... IV (C. 2. 2-35)

Schoenemann K. IV (B. 1-19, 20)

Scholz.W. IV (C. 2 .1-43)

Schuetze II. IV (A-147; C. 2. 2-66, 69; F . 2. 5-4)

Schuetze W. , IV (F . 2 .6-4)

Schumann K. D. ,-..IV (C.-3-74) ., ,

Schwartz K. ' = IV (C. 3-31)

Scoüeld R. . : ; . ; : , . ; • i y ( D . 5 - 1 4 )

S c o t t R . B . : ' 1(110); IV (C. 2.1-4) , .

362

Scottcn W . C . IV (A-117, 157; C. 1 .1-34, 42; E-32) ;

V ( C - 1 2 , 1 7 )

Scur ic in i G. B. V ( B - 3 0 , 4 8 )

Seat t les J . C. IV (B. 10-20, 22)

Sehgal I . J . S . IV (D. 2-27)

Seidel D. I (212)

Seito E. I (66)

Sekowski S. I (163)

S c l a k P . J . IV (A-43)

Selecki A. I (204); IV (A-156; C. 1. 3-23, 24; C. 3-79;

D . 5 - 7 2 ; E-21)

Selleck F . T. IV (C. 1. 1-11)

Se l l e r s E. S. IV (C. 2 .1-22)

Se l lma ic r A. IV (D. 5-42)

Selmi L. I l l (42,44)

S e l w o o d P . W . I (80); IV (C. 3-34)

S e m e n o v V . A . 111(151)

Semiokhin I .A. I (146) Senn A. V ( C - 3 8 )

Senvar C . E . I (203)

Shacter J . IV (A-79; E-2)

Shah P . G.S. II (52)

Shalnikov A. I. Il l (102)

Shamsul A. K. M. IV (E-39)

Shank R . C . Ill (137,167)

S h a n n o v J . S . IV ( F . 1 .3 . 1-3) '

S h a r m a K . C . IV ( C . 2 . 1-31)

Shatenstein A. I. I (148); III (84, 94, 96, 97, 98, 114); IV (A-77; F . l . 8 . 2 - 1 ; F . 1.8. 3 - 1 , 2, 3,4)

Shaw A . J . IV (A-9)

363

Shaw B . IV (C. 2. 2-26)

Sheffield E . L . IV (C. 2. 2-25)

Sheinl in A. E . : I (188)

She lud 'ko M. K. IV (C. 3 -12 , 40, 53)

Shephe rd E . V ( B - l l )

S h e r m a n A. I (8)

S h e r m a n lt . H. IV. ( F . 1. 2. 3-1)

Shimizu M. IV (C. 3 -77 , 78; D . 5 - 6 1 ; D. 6 - 3 3 , 34)

Shinichi H. IV (D. 5-62)

S h i r e s R . N . .. i y (C. 2 . 2 - 3 8 )

Shlypnilcov S. V. TV ( C . 1 . 1 - 3 7 )

Shp i l r a in E, E . 1 (188)

Sh tukkenberg Y u : M . . . 1 ( 2 2 4 ) ; :

S i l b e r m a n E . - I l l (72); IV (E-29)

S i lve r B . I-,. IV ( F . 1. 7. 2-6)

S i l v e r m a n L. I l l (51) ,

S i l v e s t r i M. I (129); III (36, 4 3 , 47, 75, 80, 85, 86, 88); : .';.•; . IV (A-27 , 66; C. 1. 3 - 8 , 1 2 , 16, 20; C .2 .2 -77 ;

C. 3-59; D. 4 - 7 , 8, 9; D. 5-30, 52, 64, 67; D . C - 1 7 i 2 1 , 2 2 , 2 3 , 2 7 , 30); V (B-71)-,. .•• .-.-....

S imone t G. IV (C. 2. 1 -33 ,44 , 46)

Sinev M . N . I (219)

Singleton J . H . I V ( C . 1 . 2 - 1 4 )

Sivetz N. • i •• . •'-•• V (C-2)

S k a r r e O . K . I (70)' ' :; , : > . : :

Skr inn ikova H. P . • : ; ::IV (C. 3-33)

S l a c k C . M . ;;:;. I V . ( C 3-49; . p . 6-7)

SUn'ko M. G.,. IV ( C . l . 3-46)

S lu t skaya N. M. I l l (10, 1 1 , 16); IV (C. 3 -12 , 40)

364

Small P .A . IV (C, 1.1-13)

Smirnov B. I . Ill (15.1)

Smith D.M. IV (C.'2.2-18)

Smith E .R. Ill (C); IV (C. 2. 2-2, 3; C. 3-5)

Smith F . A . IV (C.'3-20) .

Smith H.A. IV ( 0 . 2 . 2 - 5 1 , 6 0 , 65)

Smith N. A. IV (F.'1.'G.2-1)

Smith S.R. IV (D. 5-11)

Smythc II. D. I (112)

Snyder J . A. IV (C.1 .1-12)

SokolovE. Y. I V ( F . 2 . ö - 3 )

Solli R. IV (C. 3-68)

Soll ich-Baumgartner W. A. IV (F. 1. 2. 1-5; F. 1. 3, 1-1, 2)

Solomon E. IV (C. 2. 2-34)

Solomon J . 111(105)

Sonderhoff R. Ill (15)

Sonoda S. V (C-26)

Soudors J r . M. IV (C. 2. 2-38)

Souza-Reis F . de - 1(71)

S p a c i l l l . S . IV (C.3-85)

Spaepcn J . I l l (82).

SperandioA. IV (D. 5-65)

S p e v a c k J . S . IV (A-14,16; B. 1-4,18; C. 1 .1-1, 3,4, 5, 53)

Spraklcn S. B. Ill (63)

Spray P. H. G. IV (D. 2-26,28)

Stacey I. IV (F. 1. 2. 2-2)

Starke K. IV (C.2 .1-15)

365

Staschcwski D. 111(203)

StasovLch B. M. - 111(71)

S t o d m a n D . C . IV (F . 2. 4-1)

Stcdman D. F . IV (C. 1. 2-22; C. 2. 1-5)

Steinberg M. I (229)

Ste iner I-I. IV (C. 3-31)

SteLnert B. I (76)

Steinert C. V (B-42, 52)

Storming A. H. IV (C. 2. 2-53)

Stephan M. J . IV (F . 1.1-3)

Stephan W . J . IV (D. 6.-15)

Stephens W. E. 1(124)

Stern F . IV ( C . 2 . 2 - 5 8 )

Stevens C M . 111(21)

Stevens W.U. 111(60,104,118,138,149,163)

Stevenson D. P . IV ( F . 1 . 3 . 2 - 2 )

Steward D.W. I (98)

•Stiehl G. IV(A-147)

Stockmaycr W. II. IV (A-13,15)

Stoeckl K. I (59 )

Stoicovici L. IV (D. 4-17)

Stouls L. IV (A-83, 86; C. 2. 1-44,46; D. 5-44)

S t r a u l e a R . S . IV (D. 4-18)

S t ree t E. E. . IV (F . 2. 8-2)

Striganov A. It. ' , 111(93)

Strugaru D. IV ( C . 1 . 3-55)

Stumper R. IV (C. 2. 2-11)

Stutheit J . S . Ill (208) '

Stziganov A. R. 111(78)

366

Subranianian G.S. IV (C. 3-G4)

Suda N. V (B-GG)

Sucss II. I (G8, 107); IV (C. 1. 3-G)

Sulima L. V. IV (C. 1.2-12)

SunC . IV (F .1 .11-1)

Surowicc A . J . IV (D. 5-48)

Sus lovB.N. 1(156)

Suzdaltseva S. F . Ill (94, 97)

Svendsas P . V (C-18)

Svenke E. IV (A-150)

Swain C.G. IV (C. 1. 3-.19)

Swaroop J . IV (A-170)

Swiatowski W. IV (C. 2. 2-70)

Swislochi M. HI (37)

SychevV.V. 1(188)

Symons W.J . 111(196)

S z e M . C . IV (C. 2.1-45)

Szentgyorgyi P . 11 (59); IV (C. 1 .3-25 ,30 ,41 ,48 ,61)

367

- T -

Tai Y.K. IV (D.G-31)

Takamatsu T. IV (A-94); V (C-2G)

Tamaru K. IV (C. 1. 2-56)

Tanaka K. IV (C .1 .2 -56)

Tash i ro T. IV (C. 2. 1-30)

Taylor E . H . IV (A-35)

T a y l o r H . S . I (14, 94); IV (A-35; C.3-8, 34; F.2.2-1)

Taylor J . K . Ill (198)

Taylor T . I . I (201); IV (A-129; F . 1. 2. 2-5)

Tatevski i V. M. IV (C. 1. 1-8)

T e a l G . K . II (3)

Temkin M. I (38); IV (C. 1. 3-33)

T e r r i l l J . B . IV (F . 1. 6. 1-2)

T e r r y E . A. 111(136)

Thayer V .R . IV (A-41, 42, 90, 115; C. 1.1-.17, 35; C. 2. 2-62; D. 2 -11 , 12, 13; E-22, 25, 32)

T h i e l S - IV (A-147; C .2 . 2-74)

Thiele E . W . IV (C. 2. 1-6, 7)

T h o d e H . G . IV (D. 5-11)

Thomas B .W. Ijj (35)

Thomas C .O. IV (A-78; C. 2. 2-65)

Thomas H.. II (15)

Thomas H. C. IV (F . 1. 7 .1-2)

Thomas J . R. 11(39),

3C>8

Thomas M.H, V (C-25)

Thompson S. O. IV (P . 1.1-G)

Thompson T . J .

Thompson \V.I . IV (C. 1.2-17)

Thornton V. HI (39)

Thucrkauf M. HI (112); IV (C. 2. 2-G3; D. 5-G3)

Thurs ton W. M. n i '(GO, 163)

T i a S . Y . V (C-22)

Tillol A. IV (C. 1.1.-22; D. 3-7)

T i m m e r h a u s K . D . IV (C.2.1-24,28; C.2.2-G1; D. 5-37)

T imro t D . L . i (188)

Tipton J r . C .R . I (1G5); V (B-18)

Ti tani T . I l l (12); IV (C. 2. 2-7)

Tohmfor G. IV (C. 2. 2-13) , v

Tomaskova L. Ill (200)

Tomkins F . S . I l l (25)

Topley B . IV ( C . 3 - 4 , 1 7 , 2 3 )

T r a u r o u d e r It. , IV (A-171)

T r e n n e r N . R . Ill (4G)

Tre tyakova N . N . IV (A-59)

Tri l l ing C .A . 1(234)

Trcwistand L. n i (18); IV (B. 10-0; C. 3-32; D. 6-3)

Trubi t syn B. A. IV (C. 1. 2-55)

Tuchòlski T. IV (C. 2. 2-5)

Tuck R. IV ( C . 2 . 1 - 1 3 )

Tung T. C. V (C-22)

•Turchia V . F . m (151)

Türkin V.K. . I (144)

Tuxworth R. H. IV (P . 1. 3. 2-4)

369

U -

Uclovichcnko P . M .

Ucda T.

Ugajin II.

Uhlmarm W.

Updike O. L. J r .

Urey' .H.C.

,.Ursu D.

Uruguchi Y.

Ussing II.

I (219)

IV (F . 1.2. 1 -1 ,3 ,4 ,7 )

IV (C. 1.3-28)

•IV (C. 3-24)

IV (C .2 .2 -39 )

I (2, 15, 16, 42, 46, 77, 78, 79, 95, 96, 125, 127); II (3, 6); III (3, 5); IV (A-10, 20, 53; C. 1.2-4, 5; C . l . 3 - 3 , 4 ; C .2 . 1-1,2; C. 2, 2-10; C . 3 - 1 , 10, 25, 54; D. 5 - 1 , 2, 3; F . 2 .6-3)

II (59)

IV (B.6-3)

III (13)

370

- V -

Vaccaro G. IV (D. 3-15)

Vagncr J . 111(211)

Vaisberg S. E. I (138)- IV (A-45, 9G, 128; C. 1. 3-13, 35;

F . 1. 3. 3-2; F . 1. 8. 1-3: F . 1. 8. 3-2)

Valant P . V (B-48)

Vancler-Aroncl P . C. IV (C. 2. 1-47; D. 5-25)

Vaniscotte C. IV (C. 1. 2-33, 34) Varbcrg T. IV (C. 3-G3,68,69)

Varshnvski i Ya. M. I (138,148); II (84, 96); IV (A-45, 96,128; C. 1. 3-13, 35; F . 1, 3. 2-6; F . 1. 3. 3-2; F . 1. 8. 1-1,3; F . 1 .8 .2 -3 ; F . 1. 8. 3 - 1 , 2 , 3,4)

Vasaru G. I (186,191, 227); II (56, 57, 59, 60); IV (A-140, 144, 155; C. 1. 2-68; C. 3-86; F . 2 . 7-4)

Vasatkova J . Il l (184)

Vasi lcscu A. IV (F. 1. 2 . 4 - 1 , 3 )

Vasil iev A. M. I (37)

Vasiliev G. Ya. IV (F . 1. 3. 2-6)

Vasilyev D. I . Il l (102)

Veil S. I (31)

Venditti P . V (B-30,49)

Vers ino B. I l l (131)

V e r t e r s s i a n K .A . IV (C. 2. 2-15)

Via l la id R. Ill (34,40)

Vic R. Jit (133)

Vielst ich W. IV (B. 10-19)

371

Villani S. I (176); IV (A-74; C. 1. 1-20;.C. 1.3-8, IG; D. 2-10; D. 4-G, 7; D. 5-30, 52; D. ß-23 , 25; E-2G); V (B-71)

Villard R. V (C-34)

Viratol le J . IV (A-171)

Vladimirski i K. V. 111(71)

Vlasov N. A. I (189)

Voevodski V. V. I l i (62); IV (F. 1. 3. 2 - 1 , 3, 5, 7)

Volpi G.G. IV (F . 1.1-5)

VoskuylR. J . 111(24,27,29)

Voyer R. D. I (215)

V r o m e n B . H. IV (C. 2. 2-47; D. 5-19)

372

W

Wagomann K,

Wagenc r K.

Wagner C D .

Wagner II. G.

Wahl M. II.

Waincrd i E . II.

Wa lchc r W.

Wald AI.

Waiden G.

Wald mann L .

Walen R.

W a l k e r P . T.

Wa lke r II . W.

Wa lke r W.

Wallung F . O.

W a l t e r A.

W a l t e r S.

Walton U . F .

Wanick R .W.

W a n s b r o u g h - J o n e s O. H.

Ward D . E .

.War ren J .

War t enwe i l e r M.

Washburn E . W .

Washburn [I .W.

Watson U . E . -ß''

V (B-53)

IV (C. 3-83)

IV (F . 1 .3 . 2-2)

IV (C. 2. 2-83)

IV (C. 2. 2-10; C. 3 -10 ,25)

III (210)

1 (75 ,105)

1(52)

IV ( C . 3 - 5 4 )

1(90)

I (130); IV (D.G-19)

IV (A-114; D . 2 - 8 ; E -27 ) .. ,-

III (4G)

IV (A-116)

IV (D. 5-11)

I (169)

IV (C. 1 .2 -48 , 53; D. 3 - 2 , 1 2 ; D .4 -13)

IV ( G . 3 - 4 1 , 4 3 , 4 6 , 52)

IV (D. 6-16)

1(17)

IV ( C . 2 . 1 - 2 6 )

IV (C. 1.1-12)

V (C-3G)

III (6); IV ( A - 1 ; C .2 .2 -2 , 3; C. 3-1, 5, 20)

III (52); IV (C. 2. 2-2,3)-

IV (C. 2. 2-49)

373

Watson L . C . V (C-25)

Watson-Munro C.N. V (B-2)

Wattenberg A. I (92); IV (F. 2. 5-2)

W e b b G . M . IV (A-19)

Webb J. IV (F .3-1)

W e b b R . J . 111(120)

Webb W. A. IV (A-2; B. 10-2; C.2.2-17; C.3-14)

Wei C.W. Ili (160)

Weight M.M. IV (D. 4-1)

Weinberg A.M. 1(221)

W e l n g a e r t n e r E . I (183); III (76, 113)

Weise G. IV (A-147)

Weiss G. IV (C. 1.1-14, 18)

Weisser R. IT. IV (D. 5-40)

Weissman Y. IV (D. 5-41)

Weitzel D.H." 111(69); IV(C.2.1r28; C.2.2-61; D. 5-37)

Welch L .M. IV (C. 2. 2-31)

Wender I. IH (30)

Wenwor thT .O . IV (C. 2. 2-19, 23)

Weston R. E. jr . . IV (F; 1; 7. 2 -1 , 2, 3, 4)

Wetzel K. I (210); IV ( A - l l l , 147; B. G-14; C. 2. 2-64,

G6,G9; C.3-74; F . 2.5-4)

Whateley T.'L. HI (189)

Wheat J.'A. . Ili (176)

Whcts.ol H .B . II (10)

Whitaker II, III (7)

White A ,S . IV (A-85)

White D. IV (F . 2. 2-5, 7, 8, 9, 15)

374

White D.W. IV (C. 3-85)

White L . E . 111(69)

White R. R. IV (C. .2 .2-37)

Whit tem R. N. III (189)

Whytlawgray R. III (7)

Wicke E. IV (B. 10-25)

W i d i g e r A . H. IV (F . 2. 5.-1)

Wi lmar th W. K. IV (C. 1. 2-26; F . 1. 5. 2-1)

Wilson C . L . IV (A-26; C . 2 . 2 - 6 )

Wilson R, L. IV (C. 1. 1-36)

Wilson T. IL V ( C - l ) ; ;

Winnaker K. 1(232)

WinsGl A. IV (C .3 -81 )

Winter E . R . S. IV (C. 1.2-14)

Wir t z K. 1(62); IV (C. 1.3-1)

W o h l K . IV (C. 2 .2 -41)

Wolczek O. IV (A-3 0)

Wolfenclen J . H. IV (C. 3-22 , 4 1 , 4 3 , 52)

Wood J . I. IV (A-163)

Woodhead L. W. : V (C-25)

Wooley H.W. '.-.'; I (110) ;

Wright C . R . 111(197)

Wright G. E. IV ( F . 1.2. 4-2)

Wright M. M. IV (D. 6-12)

Wroblenska M. III (143)

Wullum T. IV (A-1G3)

375

Yagi S.'

Yak: nonlco L. M.

Yakovleva E. A.

Yamada M."

Ya mat ora I-I.

Yoneda Y.

Yoshida A.

Yoshilcawa Y.

Yoshioka Y.

Young A. R.

Young J . R.

IV (B. G-3)

IV (A-7 7)

I (148); III (77, 97)

IV (F . 1.2.4-4)

III (168)

IV (C. 1.3-21)

IV (A-94)

IV (C.3-66)

IV (F . 1.2. 4-4)

11(2)

IV (C. 2 .2-82 ,84)

376

a

Zabcc A.W,

Zanantoiii C,

ZavattarclH .fl.

Zeldovirch A, G,

Zeiger P.

Zellmann E.

Zelvenskii Ya. D.

Zemyan E.M.

Zevos N.

Zhavoronkov N.M.

Zinn W. H.

Zinovyeva N. P .

Zlotowski ,T,

Zmasek R.

Znamirovsclii V.

Zoch O.

Zvyagintseva 13. N.

IV ( F . 1 . 3 , 1-6)

V (B-45, 55)

IV (D.4-9)

IV (C. 2,1-32, 40)

V (ß-73)

IV ( I M . 7, 3-1)

IV (A-137; C, 1, 2-61; D. 5-21)

V (B-5)

tV (F 1.2.2-7)

I (187); IV(A-05,103, 107,122; C. 1. 1-15; 17.5-21)

1(92,100)

III (C8)

III (143)

IV (D. 5-74); V (C-37)

IV (C. 3-07)

IV (A-173; ' 12-37)

1(148); III (08)

377

Societies Index

A. E . C . Ltd

Air Liquido

Air Products & Chemicals

Allmanna Svcnska Elokt r i ska A. B.

Amer ican Security & T r u s t Co.

A . M . F .

Asahi Kasci Kogyo K. K.

Atlantic Refining Co.

Atomic Fuel Corp .

Badisdio Anilin & Soda Fab r ik A.G.

Br i t i sh Amer i can Oil Cy Ltd

Canadian General E l ec t r i c Co.

Cas sella F a r b w e r k e

C . E . A .

IV (R.2-4G; B. 10-35)

IV (B. 1-10; B . 2-9, 2 7 , 3 1 , 3 2 , 4 0 , 4 1 , 42 ,45 ; B. 3-23; B.5-12)

IV (B. 5-21)

IV (B. 1-14, IG)

IV (B. 10-1)

IV (B.11-32)

IV (B. 10-33, 34)

IV (B. 11-25)

IV (B. 10-33)

IV (B. 2-23)

IV (B.8-1)

IV (B. 1-22, 31)

IV (B .11-9 ,13) '

IV (B. 1-7, 8, 9, 11 , 23,24;' B. 2-13 , IG, 17;18, 19, 20, 27, 31, 32, 34, 3 7 , 3 8 , 4 0 , 4 1 , 4 2 , 4 3 , 4 4 , 4 5 ; B. 5 -22 ,23 ; B .10-27 ; B. 11-5 , 30, 38) !

378

C . F . T .H.

Cie de Construction Mecanique

C . I . S . E .

Constructors John Brown Ltd & N.W. Roberts

Costain John Brown Ltd

Degussa

Dow Chemical Co.

Esso Research &. Eng. Co.

Fe r t i l i z e r s &. Chemicals Ltd

Fluor Corp.

F . Uhde GmbH

General E lec t r i c Co.

Gesellschaft für Kernforschung

Gesellschaft 'fUr Lindc's Eis machinen A. G.

Gulf General Atomic Inc.

Hoechst

Houdry P r o c e s s Corp .

Ilouilleros du Bass in du Nord et du Pas -dc-Ca la i s

IV (B. 10-30)

IV (B. 2-27, 31, 32,40,41, 42, 45)

IV (B. 3-11)

IV (B. 1-15; B.2-10; B. 7-3)

IV (B.2-4; B.7-1)

IV (B. 3-26, 30, 32; B. 5-17; B. 1.1-4,11)

IV (B.1-21)

IV ÜB.1-25)

IV (B. 11-28) ^'••P"

IV (B. 11-24)' '

IV (B. 2-5, 8, 12, 25, 26, 28, 30, 33, 35; B. 3-17, 27, 34, 35, 38; B.10-16)

IV (B. 11-31)

mbH IV (B.2-33; B.3-38; B. 11-29)

IV (B. 5-15,18,19,20)

'-._: IV (B.11-37) &:

IV (ß.'5-10)

IV (B. 3-15)

IV (B. 2-14,17, 18, 27, 31, 32, 40, 41, 42,45; B. 10-27)

379

I. G. -Farbonindustric A. G. IV (B. 10-3)

Johnson, Matthey & Cy Ltd IV (B. 10-32)

Junta de Energia Nuclear IV (B.10-15)

Lonza IV (B.5-8)

Lummus Co. IV (B.'1-26)

Metalgescllschaft A. G. IV(B. '3-31)

Norsk Hydro-Elekt r i sk Kvaelstofaktiesclskab IV ( B . l - 1 7 ; B. 2 -21 ; B .3 -14 ; .

B." 10-6, 17,23)

Oerlikon IV ( B . 5 - 4 , 5 , 6 ; B .10-11 ,12 ,13)

Office National Industr ie l del 'Azote IV (B.3-33)

Osterreichische-St ickstoffwerke A.G.IV (B.2-11)

Pact ide Corp. IV(B.C-18)

Pin tsch-Bamag A. G. . IV (B. 1-13)

Quartz &Silice i IV (B. 9-3)

Rensse laer Polytechnic Institute IV (B. 1-5, G)

I luhrchemie A. G. IV (B. 3-20, 29; B . 10-18, 24, 2C;

B . 11-15, 17)

S i e m c n s A . G . / . IV (B. '10-31; B. 11-7, 26)

S.N. P . A. • IV (B.' 11-30)

Société de Produi ts Azoté ' • IV (B. 7-2)

Société d'Etudes pour l 'Obtention du Deuter ium IV (B. 1-12)

380

Sociótó Industriel le & Commercia le de la Cie des Salines du Midi

Socony Mobil Oil

South American Coal Oil and Gas Corp. Ltd

S. R . T . I .

Stamicarbon N. V.

Stcinkolilun Elektr izi taet A . C .

Sulzer

U . K . A . E . A .

Union Carbide Corp.

Union Oil Co.

U.S . A . E . C .

Varta A. G.

Veb Vakutronik

Western Elec t r ic Co.

Zaidan Ilojin Iloguchi Kcnkyu Jo

IV (B .6 -9 ,15 ,17 ; B.11-18)

IV (B. 3^37)

IV (B.11-10)

IV (B. 11-34,35)

IV ( B . 5 - 1 , 2 , 3 , 7 , 1 1 )

IV (B. 3-20; B. G-20; B. 10-18, 2G)

IV (B. 2-15, 27, 31, 32, 40, 41 , 42, 45, 47; B . 4 - 3 , 4 , 5, 6 ,7 , 8, 9, 11, 1.2, B .5-16 ; B.G-10,11 ,12 ,13 ,19)

IV (B. 2-6, 7, 22) 24,-36, 39; B. 3-18, 19, 21, 24,25; B . 5 - 9 , 1 4 ; B .6 -6 ; B. 10-7,8; B. 11-6, 8)

IV (B.4-10)

IV (B.11-2)

IV (B. 1-1,2, 3,27, 28, 29,30; B. 2- l ,2 ; > 3; B. 3-3, 4, 5, G, 7, 8, 9, 10;"B. 4 -1 ,2 ; B. 5-13; B. 6-5; B. 10-10; B.11-12)

IV (B. .10-31)

•IV (B.3-36)

IV (B.11-19)

IV (B.10-21)

A N N E X

FLOW DIAGRAMS OF HEAVY WATER PRODUCTION PLANTS

F igu res in parenthes is show plant number in Table IV. D. 1;

FIRST STAGE

(3 IN PARALLELI

A, 8 & C

SECOND STAGE THIRD STAGE

HOT TOWER COLD TOWER

HYDROGEN SULPHIDE DEPLETED

IN DEUTERIUM

FEED WATER

COLD SECTION 90°F

DEUTERIUM ENRICHED

WATER ID20)

HYDROGEN SULPHIDE

ENRICHED IN DEUTERIUM

HOT SECTION 26J°F

DEPLETED WATER

HYDROGEN SULPHIDE

GAS FLOW

WATER FLOW

ENRICHED WATER

r T0

FINISHING SECTION

CANADA: Simplified process diagram (2,3)

*\trJ*Ó**ì-àì3~?Wve*iw»fi J^T*Hf?trtCt ,&a^ a*îgfa;g'-lfihc**—• W^r^^»*iS. i.'Vâi»'

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1

1 1

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Supplementary

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t

d pump Production tonk

F R A N C E : Block diagx-am of Lacq facili ty (4)

araaiafjfiaaag

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GERMANY'R. F . rF lowshce t of-German H2S - I-IDO pilot plant (6)

IV

Closed water cycle

Open water cycle

SWEDEN : Kvarntorp pilot plant. (13)

Wa, 4

M l - I

Feed

r*

CT-I

""I

.1/

r-i n V

n , :r t .

Product

Q j \ J

Flow diagram of a SRP GS Unit

I-egend

•Liquid - (Jail and Vnp<>r

Meat llecovcf.i

T m i c . l Uiv-r U j t i v 0 O'.V.

«feg V flslit

WJJ.II-T r A'.ilcr

V/////////'/////'/_\

Trjln A ^ ! i l Train H ^ — — L * - — T - l — J — ,

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h'astc 4. SI

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n: mv PLANT

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I F l'LANT (Electrolytic)

Currently Oneratine j j Dote Shut Pt.wn P % $ )

% Indicatali moie % U 0 0 "

History of Operation of SRP GS Plant

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SYNTHESIS GAS B 0 B B m / 1 ) „ .EFFLUENT - _ - | - | | - . | - ^ - - .

F IRST STAGE N H J - M J

EXCHANGE

2 1 4 4 7 Mj

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SECCNO STAGE FINAL STAGE D j O FORMATION N K J - H J EXCHANGE N H , O IST ILLATION NH , COMBUSTION

SOS N H , G.8 N H ,

I 1 ( 7 3 G 0 0 ) 1

O.907 0 , 0

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HEAVY WATER

{ 4 5 0 0 1 '

I spm) IN PARENTHESIS

t

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L L.

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7 0 TONS

SYNTHESIS

0 ? 0 /

GAS

vr FEED

CANADA : Chalk River planned pilot plant (20)

jj^^Sl^^^sm-s^^ms^^sss^s^^s

VII

Arrfvfl* d% g<ti hydfogin*»

Hxv>

• r-0 I Séparottur

V Capaci >•

-DXJ—,

Sépoiataur Boutfill«

DjpKUgwalawr colotìfug«

Bolliti l i« •chaft l i l lonH,

u CZÌ

Mil« a l'air

:FRANCE: Small pilot plant UCMa (21)

T JJÜ

To SfnlM*li

T( , ? , K . r , . „ , . , „ni M

. 1 , i t . . . . .

H

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c ' ^ ) —

plow diagram

Gos mixture (N2+3HZ) . far ommonia synthesis

Ammonio ••«»•/production

Final concentration: distinction ot

fijmmonia

v PURIFICATION

Cracking

ISOTOPE EXCHANGE

RECOVERY AND TREATMENT OF CATALYST

Heavy woter

FINAL ' PROCESS

Schematic arrangement

FRANCE: Mazingarbe heavy water plart ^

f f *

Syntticsegn -,

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: V»rrdl!>l>p|iji|ii>r für <|en'ini(|l'" Ammoniak und Amld-I.fiMini|Ph, / Aininniiiiik-Vpriliiitipfrr, "i IPPII» KH-loniicn&tü<fc, n HinktwiiririOiiilMniiMlirf, o Hi'klri-idipr Anf-hcizrr.

GERMANY R. F. .:' Flow diagram of semiindustrial plant for the system H2/li<luid NH3 exchange

X

AMMONIA

Sil r

Nl-Ig - HD exchange section

H

-&~

T J

} 33-

u-rj- -fr-1

a ~Q-

Nllg distillation section

U. K. : Construction John Brown Ltd. Project (29)

lo Chemical Plani /"rei/ Waler

Catalyst (ledi.

inox?/;?!1,

\ üi/ii/r Cap Plolos

jlj•_. I J.\.> GosSupcrheoler

I

Electrolytic Celti .. 0, \ - l

J-, .Humidifier i • — H //,

V-^;i (

lo Higher Stages

^Condenser

XI

Schematic d iagram of T r a i l exchange plant, based on the hydrogen/water system with gas-phase ca ta lys i s

Watir t l r luiRI ' i I 'rt iniry rianl n u n » - " " "1

-, 1 J*™, | »>cJ i l f t t r

f 'rt iniry 5*l»ni

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CANADA :; Diagram of the Secondary Plant at T r a i l for Concentrating D 2 0 by a Cascade of Elec t ro ly t ic Cel ls . Tra i l Plant

XII

Cold Columns Cooler

Hydrogen

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GERMANY It. F . : Diagram of pilot plant, lor the system hydrogen/aqueous, catalyst suspension, built by .;.' Fi-iccli-ich Uhclc G. m. b. II (34)

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FRANCE: 2, 5 t /y pilot plant Toulouse"- Semplified diagram (35)

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GERMANY 11. F . : Block diagram of the Farbwerke Hoechst 4 t /y heavy-water plant based on IT, distillation (38)

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INDIA :Combin.ition or walor e lectrolysis and low-tempera-ture II2 distillation in Nangal plant. (39)

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URSS : Side and Top Views of USSR Hydrogen Distillation Pilot Plant

A Low Tempera tu re Block, Including Distillation Column and Heat Exchangers opera ted at t empera tu re s below 80°K

13 Block- containing Heat Exchangers and F i l t e r s operated at t e m p e r a t u r e s above 80°K (43)

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USA ;l;'low Diagram of Water Dist i l lat ion Unit of tlie MOW P r i m a r y Plant (53)

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NORWAY : The Norsk Plant for Producing D2O by a Combination of E l e c t r o l y s i s of Water and U D - 1120 Catalytic Exchange

XX

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Product

SWITZERLAND':' Flow-sheet of hydrogen distillation plant built by the firm Gebrüder Sulzer (41)

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ITALY : Electrolyt ic .plant at Nera Montoro (Soc. Terni) Lay-out of the fourth stage of an isotopie exchange unit

(58)

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