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Laser spectroscopy of short -lived exotic nuclei at FAIR...Laser-desorption resonance ionization...

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Dubna NUSTAR meeting, Dubna, 5-10 October 2009 Iain Moore (for the LASPEC collaboration) University of Jyväskylä, Finland Laser spectroscopy of short-lived exotic nuclei at FAIR
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  • Dubna NUSTAR meeting, Dubna, 5-10 October 2009

    Iain Moore (for the LASPEC collaboration) University of Jyväskylä, Finland

    Laser spectroscopy of short-lived

    exotic nuclei at FAIR

  • Dubna NUSTAR meeting, Dubna, 5-10 October 2009

    The LASPEC collaboration

    In total: 8 countries; 13 institutes; 34 members

    Spokesperson: Wilfried Nörtershäuser (GSI) Deputy spokesperson: Iain Moore (JYFL) Technical Director: Christopher Geppert (GSI)

  • Dubna NUSTAR meeting, Dubna, 5-10 October 2009

    Hyperfine structure Isotope shift Isomer shift

    Investigation of Nuclear Ground State properties

    high-sensitivity & high selectivity… Why OPTICAL??

    providing model-independent nuclear data…

    Laser spectroscopy at NUSTAR

    Motivation:

    All proposed techniques are fully developed by the collaboration and have been adapted for on-line work

  • Dubna NUSTAR meeting, Dubna, 5-10 October 2009

    Isotope Shift (IS) Hyperfine Structure (HFS)

    AAr

    ′2δ

    Nuclear Spin I

    Magnetic Dipole Moment µI

    Electric Quadrupole Moment Qs

    Hyperfine Anomaly

    Mean Square Charge Radii

    However, sample preparation is crucial…..

    Nuclear ground state properties

    Deformation β Triaxiality

  • Dubna NUSTAR meeting, Dubna, 5-10 October 2009

    Good conditions for spectroscopy: highly successful and productive

    Target

    p+ or

    Light Ions

    Ion source

    Electromagnetic Separation

    100 keV

    T1/2 ~ 10 ms no reactive elements no refractory elements

    T1/2 ~ 1 ms reactive elements refractory elements very modest yields

    Ion guide Good conditions

    for spectroscopy only if the beam

    is cooled

    ISOL

    IGISOL

    Laser spectroscopy – “historically”

  • Dubna NUSTAR meeting, Dubna, 5-10 October 2009

    All elements produced chemically non-selective: T1/2 ~ 1 µs

    Thin Target

    1 GeV/u

    Heavy Ions Electromagnetic

    Separation Fragment Separator

    Low Quality High-Energy Ion Beam

    1 GeV/u

    In-flight fragmentation – towards LASPEC

    Laser spectroscopy at ISOL facilities is highly developed and has provided nuclear state properties for two decades. LASPEC offers the possibility to make these studies at the limits of stability and lifetime.

  • Dubna NUSTAR meeting, Dubna, 5-10 October 2009

    S-FRS

    LEB

    7

    FAIR – the facility layout

    SIS100/300

    SIS18 UNILAC

    HESR

    PANDA

    RESR/ CR

    NESR

    CBM

    FLAIR

  • Dubna NUSTAR meeting, Dubna, 5-10 October 2009

    energy buncher

    HISPEC

    DESPEC ‹―› Gas catcher

    MATS + LaSpec

    Layout at the Low Energy Branch

    AGATA

  • Dubna NUSTAR meeting, Dubna, 5-10 October 2009

    The device transforms high-energy ions from the Super-FRS into a high-quality low-energy ion beam.

    Design parameters

    Technical challenges

    Operation at high density: up to 0.20 mg/cm3, ~1 bar at room

    temperature for a cell of length 1 m. Inner diameter 0.25 m. Cryogenic (~60 K), high purity helium gas as stopping medium. At this temperature most of the impurities are frozen out, leading to a maximum extraction efficiency. Efficient transport of ions by DC and RF fields.

    High RF amplitude: few hundred Vpp

    Small RF electrode spacing: ≤0.25 mm High DC field: >100 V/cm

    outer chamber (room

    temperature)

    inner chamber (down to 60 K)

    DC ring electrodes

    exit-hole

    extraction RFQ

    insulation vacuum

    RF carpet DC grid electrode

    System design

    RF carpet

    500 rings

    4 electrodes/mm

    Exit hole : 0.6 mm

    Front

    Back

    The cryogenic ion catcher for high energy ions

  • Dubna NUSTAR meeting, Dubna, 5-10 October 2009

    Laspec atom beamline

    Laspec ion beamline β-NMR

    Laspec switchyard

    Gas catcher

    RFQ cooler & buncher section

    Common switchyard Multi-reflection TOF mass spectrometer

    Layout of MATS and LaSpec experiments (TDR)

    Top view

    Overview

    EBIT

    Spectroscopy station Penning traps

    - see talk of D. Rodriguez

  • Dubna NUSTAR meeting, Dubna, 5-10 October 2009

    http://www.gsi.de/forschung/ap/projects/laser/survey.html

    Clusters and Halos

    Refractory Elements around Shell Closures

    Further away from Stability

    Towards Superheavy Elements

    Present status and LASPEC regions of interest

    H.-J. Kluge & W. Nörtershäuser, Spectrochimica Acta B 58 (2003) 1031. J. Billowes & P. Campbell, J. Phys. G 21 (1995) 707.

    http://www.gsi.de/forschung/ap/projects/laser/survey.html

  • Dubna NUSTAR meeting, Dubna, 5-10 October 2009

    0 10 20 30 40 50 60 70 80 90 100 110 120 130 140

    10

    20

    30

    40

    50

    60

    70

    80

    90

    N

    Z01,0002,0003,0004,0005,0006,0007,0008,0009,00010,0011,0012,00Laser Spectroscopy

    Log Production Yield

    A variety of techniques to reach the limits

    Bunched beam spectroscopy

    ß-NMR

    Coincidence and decay tagged atom/ion spec.

    LD-RIS

  • Dubna NUSTAR meeting, Dubna, 5-10 October 2009

    LASPEC sub-projects

    Collinear laser spectroscopy of ions (P. Campbell, Manchester)

    Optical pumping and collinear laser spectroscopy on atoms (W. Nörtershäuser, Mainz)

    ß-nuclear magnetic resonance (G. Neyens, Leuven)

    Laser-desorption resonance ionization spectroscopy (M. Seliverstov, Mainz)

  • Dubna NUSTAR meeting, Dubna, 5-10 October 2009

    Collinear Spectroscopy Resonance Ionization (Mass) Spectrometry

    Fluorescence detection 104 ions/s β-NMR detection 103 ions/s Collisional ionization 102 ions/s

    Pulsed laser desorption 105 ions/s Nuclear radiation detection 1 ion/s Laser ion source 1 ion/s

    General applicability ISOL-type beams

    Very general applicability Daughter isotopes available

    CW lasers utilized High resolution

    Pulsed or cw laser applied Medium or high resolution

    Background – scattered light Isobaric contamination

    Background - non-resonant ions Very low (or zero) contamination

    The two workhorses of LaSpec

    See my talk tomorrow for details of these two methods !

  • Dubna NUSTAR meeting, Dubna, 5-10 October 2009 15 15

    Mainz TRIGA Reactor

    (University Mainz)

    Collinear Laser Spectroscopy and Mass Spectrometry

    of Long-Lived Trans-Uranium

    Elements up to Californium (SHE) +

    Short-Lived Fission Products of 235U and 249Cf

    (LASPEC & MATS)

    T R A P

    SOURCE Ketelaer, Krämer et al., Nucl. Instr. Meth. A 594, 162 (2008)

    K. Blaum

    Prototyping for FAIR: Mainz TRIGA reactor

    W. Nörtershäuser

  • Dubna NUSTAR meeting, Dubna, 5-10 October 2009

    quadrupole doublet & steerer plates

    retardation & charge exchange cell

    10° deflector chamber

    Status of the atomic beamline prototype

  • Dubna NUSTAR meeting, Dubna, 5-10 October 2009

    The IGISOL facility, JYFL

    50 – 5000 ions per sec

    On-going developments, new techniques (JYFL)

    P. Campbell, Hyp. Int. 171 (2007) 143

    Optical manipulation in an ion beam cooler-buncher (more tomorrow!)

  • Dubna NUSTAR meeting, Dubna, 5-10 October 2009

    Influencing F state population Survival of metastable in rfq

    Towards polarization

    Mn+ (Z=25)

    0 cm-1

    43378.510 cm-1

    9472.970 cm-1

    230.

    5714

    nm

    293.3913 nm

    J=3

    J=3

    J=2

    d5 p

    d5 s

    N=28

    3/2-5/2 5/2-7/2 7/2-9/2 9/2-11/2230.5705

    230.5710

    230.5715

    230.5720

    230.5725

    230.5730

    Pum

    ping

    wav

    elen

    gth

    (nm

    )

    Collinear laser hyperfine component

    Laser spectroscopy around the N=28 shell (2009)

  • Dubna NUSTAR meeting, Dubna, 5-10 October 2009

    Preparing for the new facility at JYFL (2010-2011)

    K = 130 MeV

    K = 30 MeV

    IGISOL

  • Dubna NUSTAR meeting, Dubna, 5-10 October 2009

    1980

    Looking back in time…collinear laser spectroscopy

    1976 1978

  • Dubna NUSTAR meeting, Dubna, 5-10 October 2009

    by 1990…

  • Dubna NUSTAR meeting, Dubna, 5-10 October 2009

    in 2000…

  • Dubna NUSTAR meeting, Dubna, 5-10 October 2009

    today !

  • Dubna NUSTAR meeting, Dubna, 5-10 October 2009

    at LaSpec in 201X, more elements, even further from stability

  • Dubna NUSTAR meeting, Dubna, 5-10 October 2009

    Operating facilities Facilities under

    construction or test Planned facilities

    TRIUMF

    MSU

    CARIBU

    IGISOL

    COLLAPS CRIS

    TRIGA-LASER

    LASPEC

    SLOWRI

    Collinear laser spectroscopy facilities worldwide

  • Dubna NUSTAR meeting, Dubna, 5-10 October 2009

    Thanks to Wilfried, Paul and Peter Dendooven for slides,

    and to you for your attention!

    Slide Number 1Slide Number 2Slide Number 3Slide Number 4Slide Number 5Slide Number 6Slide Number 7Slide Number 8Slide Number 9Slide Number 10Slide Number 11Slide Number 12Slide Number 13Slide Number 14Slide Number 15Slide Number 16Slide Number 17Slide Number 18Slide Number 19Slide Number 20Slide Number 21Slide Number 22Slide Number 23Slide Number 24Slide Number 25Slide Number 26


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