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O AK R IDGE N ATIONAL L ABORATORY U.S. D EPARTMENT OF E NERGY Nanoscale Electronics /...

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OAK RIDGE NATIONAL LABORATORY U.S. DEPARTMENT OF ENERGY Nanoscale Electronics / Single-Electron Transport in Quantum Dot Arrays Dene Farrell SUNY Binghamton Research Alliance for Minorities www.csm.ornl. gov Oak Ridge National Laboratory Mentor: Jack Wells, Ph.D.
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OAK RIDGE NATIONAL LABORATORYU.S. DEPARTMENT OF ENERGY

Nanoscale Electronics / Single-Electron Transport in Quantum Dot Arrays

Dene Farrell

SUNY Binghamton

Research Alliance for Minorities

www.csm.ornl.gov

Oak Ridge National Laboratory

Mentor: Jack Wells, Ph.D.

OAK RIDGE NATIONAL LABORATORYU.S. DEPARTMENT OF ENERGY

Introduction

Nanotechnology – what is it? Science, technology and engineering dealing in

nanometer sized dimensions A nanometer is 1x10-9 meters

Nanoscale Electronics Devices of this type are different from their

macroscale counterparts Importance

Research is basic, not applied Scientists need nanoscale information processors

OAK RIDGE NATIONAL LABORATORYU.S. DEPARTMENT OF ENERGY

Project Overview

Goal Understanding how to observe Coulomb

blockade effect in a single-electron device Procedure

Working mainly on a computational level Defining transistor properties and

analyzing behavior Results

Greater understanding of Nanoelectronics

OAK RIDGE NATIONAL LABORATORYU.S. DEPARTMENT OF ENERGY

Island (3)

Source (1)

Drain (2)

C13 C32

R13 R32

Capacitance

Electrons Electrons

Conductance

Single-Electron Transistor

OAK RIDGE NATIONAL LABORATORYU.S. DEPARTMENT OF ENERGY

Monte-Carlo Single-Electronics Simulator (MOSES)

FORTRAN based simulator program Utilizing Monte-Carlo method to project

transistor performance Generating Current-Voltage characteristics

OAK RIDGE NATIONAL LABORATORYU.S. DEPARTMENT OF ENERGY

Background

Research of single electron transistors involved exposure to new concepts

Background research was major component of the internship

Key concepts:

Electron Tunneling Quantum Dots Coulomb Blockade Coulomb Staircase

OAK RIDGE NATIONAL LABORATORYU.S. DEPARTMENT OF ENERGY

Electron Tunneling In classical mechanics, if E < V (the maximum height of the

potential barrier), the particle remains in the well forever If E > V , the particle escapes

OAK RIDGE NATIONAL LABORATORYU.S. DEPARTMENT OF ENERGY

Electron Tunneling, Cont. In Quantum Mechanics, the electron can escape even if its energy

E is below the height of the barrier V Quantum tunneling has no counterpart in classical physics

OAK RIDGE NATIONAL LABORATORYU.S. DEPARTMENT OF ENERGY

Quantum Dots

“Artificial Atoms” Quantum Dots Are Clusters of Atoms Behave like single atom, concerning electron

tunneling Arrays

Single-electron devices often use more than one quantum dot in one, two-dimensional patterns

OAK RIDGE NATIONAL LABORATORYU.S. DEPARTMENT OF ENERGY

Requirements: Electron enters or departs island only via “quantum

tunneling”Well isolated conductor

High resistance tunnel junctions, (Rt >> Rk = h/e2)

Charging energy must exceed the energy of thermal fluctuations kbT

Ec e2/C >> kbT

Very small conductor as C (size)

The Coulomb Blockade and the Coulomb Staircase

OAK RIDGE NATIONAL LABORATORYU.S. DEPARTMENT OF ENERGY

Finding The Right Conditions

OAK RIDGE NATIONAL LABORATORYU.S. DEPARTMENT OF ENERGY

The Coulomb Ladder

OAK RIDGE NATIONAL LABORATORYU.S. DEPARTMENT OF ENERGY

Effects of Heat on a Nanoelectronic System

OAK RIDGE NATIONAL LABORATORYU.S. DEPARTMENT OF ENERGY

Directed Bioassembly of Nanoelectronic Arrays

Atomic force microscope image of gold nanoparticle attached to DNA

(a) DNA-nanoparticle assembly, Functionalized gold clusters attached to DNA chain via peptide bonds.

(b) Optimized structure of the Au38(SCH3)24 cluster, obtained by quantum molecular dynamics computed on IBM supercomputer at ORNL

OAK RIDGE NATIONAL LABORATORYU.S. DEPARTMENT OF ENERGY

Neuromorphic Signal Discrimination Two-dimensional quantum-dot array showing currents as input

channels Iin and output channels Iout

Processors for advanced sensors Requires special algorithms Success would result in the first-in-kind application

OAK RIDGE NATIONAL LABORATORYU.S. DEPARTMENT OF ENERGY

Acknowledgments

This research was performed under the Research Alliance for Minorities Program administered through the Computer Science and Mathematics Division, Oak Ridge National Laboratory. This Program is sponsored by the Mathematical, Information, and Computational Sciences Division; Office of Advanced Scientific Computing Research; U.S. Department of Energy. Oak Ridge National Laboratory is managed by UT-Battelle, LLC, for the U.S. Department of Energy under contract DE-AC05-00OR22725.

This work has been authored by a contractor of the U.S. Government under contract DE-AC05-00OR22725. Accordingly, the U.S. Government retains a nonexclusive, royalty-free license to publish or reproduce the published form of this contribution, or allow others to do so, for U.S. Government purposes.

OAK RIDGE NATIONAL LABORATORYU.S. DEPARTMENT OF ENERGY

Thank you

A special thanks to Debbie McCoy and Cheryl Hamby for being so caring and helpful and to my mentor, Jack Wells, Ph.D. you were great to work with.

OAK RIDGE NATIONAL LABORATORYU.S. DEPARTMENT OF ENERGY

Current Modulation via External AC Potential

Novel Computational ParadigmChallenge:1nm-size islands not accessible

individuallyCannot modulate current in analogy to

Field Effect Transistors (FETs)

Idea:Control transport with external AC

potentialAdapt tunneling rate by phase locking to a

variable AC potential

Supported by experimental evidence

Wybourne, et al., Jpn. J. Appl. Phys., (1997)

Clarke, et al., APL 71 (1997)

OAK RIDGE NATIONAL LABORATORYU.S. DEPARTMENT OF ENERGY

Simulation of PAT in QD Arrays Simulations of PAT in Single-Electron Transport

Modified MOSES to include PAT transition rates Effective modulation of current by external field

Qualitative agreement with experiments by Wybourne et al


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