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Nonlocal resistance in graphene Origins of Nonlocal Resistance in Multiterminal Graphene: Spin Hall and Valley Hall vs. Other Competing Mechanisms Branislav K. Nikolić Department of Physics & Astronomy, University of Delaware, Newark, DE 19716, U.S.A. 1638–1655 RPGR 2017, Singapore https://wiki.physics.udel.edu/qttg
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  • Nonlocal resistance in graphene

    Origins of Nonlocal Resistance in Multiterminal Graphene: Spin Hall and Valley

    Hall vs. Other Competing Mechanisms

    Branislav K. NikolićDepartment of Physics & Astronomy, University of Delaware, Newark, DE 19716, U.S.A.

    1638–1655

    RPGR 2017, Singapore

    https://wiki.physics.udel.edu/qttg

  • Nonlocal resistance in grapheneRPGR 2017, Singapore

    Collaborators

    Dr. Jose H. García

    Juan M. Marmolejo-Tejada Dr. Chien-Liang Chen

    Dr. Alessandro Cresti Prof. Stephan Roche Prof. Ching-Ray Chang

    Dr. Po-Hao Chang Dr. Xian-Lei Sheng

    Dr. Xavier Waintal

  • Nonlocal resistance in grapheneRPGR 2017, Singapore

    “Ancient” History: Nonlocal Resistance in Quantum Hall Systems

    Landauer-Büttiker formula for quantum transport gains traction

  • Nonlocal resistance in grapheneRPGR 2017, Singapore

    Nonlocal Resistance in Graphene with Adatoms due to Direct and Inverse Spin Hall Effect (SHE)Nature Phys. 9, 284 (2013) and Nat. Commun. 5, 4748 (2015)

    Nature 511, 449 (2014)

    PRB 79, 035304 (2009)

    CONTROVERSYPRB 91, 165412 (2015)PRB 92, 161411 (2015)

    LB quantum transport theory

    removed in favor of semiclassical theory

    connecting RNL to bulk conductivities based on PRB 79, 035304 (2009)

  • Nonlocal resistance in grapheneRPGR 2017, Singapore

    Nonlocal Resistance in Graphene due to (?) Direct and Inverse Valley Hall Effect

    Science 346, 448 (2014)

    CONTROVERSYNat. Commun. 8, 14552 (2017)

    PRL 114, 256601 (2015)

    arXiv:1706.09361

  • Nonlocal resistance in graphene

    Physical Mechanisms of SHE: Extrinsic vs. Intrinsic

    RPGR 2017, Singapore

    strong SOC with the nuclei of the

    periodically arranged atoms is hidden behind the vacuum-like form

    skew-scattering (SS)

    side-jump (SJ)

    SOC in band structure

    PRB 72, 075335 (2005)

  • Nonlocal resistance in graphene

    Landauer-Büttiker (LB) Quantum Transport Theory for Charge and Spin Currents in Mulititerminal Circuits

    RPGR 2017, Singapore

    PRL 117, 176602 (2016)

    PRL 57, 1761 (1986)

    PRB 82, 081414(R) (2010)

    LB theory puts limits on the usage of Boltzmann equation for graphene

    PRB 72, 075361 (2005); PRB 89, 195418 (2014)

    https://kwant-project.org

  • Nonlocal resistance in graphene

    Kubo vs. LB Computed SH Angle of Graphene with SOC due to Adatoms

    RPGR 2017, Singapore

    Real-space Kubo formula via

    kernel polynomial method makes possible

    numerically exact calculations on

    ~500 nm x 500 nm square containing ≤ 10 million atoms

    PRL 117, 176602 (2016) Paper-pencil calculations: Which diagrams to consider?

    EPL 111, 37004 (2015)

    PRB 94, 201402(R) (2016)

    SS

    SJ

    Q

  • Nonlocal resistance in graphene

    LB Theory of Nonlocal Resistance in Multiterminal Graphene with Adatoms

    PRL 117, 176602 (2016)

    RPGR 2017, Singapore

  • Nonlocal resistance in graphene

    How to Get Nonlocal Resistance Due to Purely Direct and Inverse SHE in Graphene with Adatoms

    RPGR 2017, Singapore

    PRL 117, 176602 (2016)

  • Nonlocal resistance in grapheneRPGR 2017, Singapore

    First-Principles Bandstructure and Quantum Transport in Zigzag Nanowires of G/hBN vs. G

    arXiv:1706.09361

  • Nonlocal resistance in grapheneRPGR 2017, Singapore

    Ab Initio Tight-Binding Hamiltonian for Graphene-on-hBN Nanowires with Zigzag Edges

    Edge

    cur

    rets

    for

    TBH

    arXiv:1706.09361

  • Nonlocal resistance in grapheneRPGR 2017, Singapore

    Landauer-Büttiker Theory of Nonlocal Resistance and ρxx in Multiterminal Graphene/hBN

    arXiv:1706.09361

    RNL peak is seen in aligned G/hBNzigzag wires, never in nonaligned ones despite edge states being present

    ρxx peak value is metallic-like ρxx peak is wider than RNL peak RNL peak centroid is slightly shifted to

    the left of the DP

    COMPARE TO EXPERIMENT

  • Nonlocal resistance in grapheneRPGR 2017, Singapore

    Kubo Theory of Valley Hall Conductivity in Graphene/hBN

    nonlocal resistance obtained indirectly from σvxy +

    semiclassical diffusion

    arXiv:1706.09361real-space numerically exact Kubo formula

    Science 346, 448 (2014); PNAS 122, 10879 (2015)

    PRB

    94, 1

    2140

    8(R)

    (201

    6)

    PRL 99, 236809 (2007)

    JPSJ

    84,

    114

    705

    (201

    5)PRL 114, 256601 (2015)

  • Nonlocal resistance in graphene

    Conclusions in Pictures

    RPGR 2017, Singapore

    SHE

    VHE(?)

    Origins of Nonlocal Resistance in Multiterminal Graphene: Spin Hall and Valley Hall vs. Other Competing MechanismsCollaborators “Ancient” History: Nonlocal Resistance �in Quantum Hall SystemsNonlocal Resistance in Graphene with Adatoms due to Direct and Inverse Spin Hall Effect (SHE)Nonlocal Resistance in Graphene due to (?) �Direct and Inverse Valley Hall Effect Physical Mechanisms of SHE: �Extrinsic vs. IntrinsicLandauer-Büttiker (LB) Quantum Transport Theory for Charge and Spin Currents in Mulititerminal Circuits Kubo vs. LB Computed SH Angle of �Graphene with SOC due to Adatoms��LB Theory of Nonlocal Resistance in �Multiterminal Graphene with Adatoms��How to Get Nonlocal Resistance Due to Purely Direct and Inverse SHE in Graphene with Adatoms ��First-Principles Bandstructure and Quantum Transport in Zigzag Nanowires of G/hBN vs. G Ab Initio Tight-Binding Hamiltonian for Graphene-on-hBN Nanowires with Zigzag EdgesLandauer-Büttiker Theory of Nonlocal Resistance and ρxx in Multiterminal Graphene/hBNKubo Theory of �Valley Hall Conductivity in Graphene/hBNConclusions in Pictures ��


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