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#PRD2020 #CleanHydrogen - Europa

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#PRD2020 #CleanHydrogen
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Page 1: #PRD2020 #CleanHydrogen - Europa

#PRD2020#CleanHydrogen

Page 2: #PRD2020 #CleanHydrogen - Europa

#CleanHydrogen#EUHydrogenForum

#PRD2020#CleanHydrogen

LOWCOST-IC

General info

● H2020, FCH2

● Start: 1st of January 2019

● End: 30th of June 2022 (assuming extension)

● Budget: 2.34 mil. €

● Number of partners: 10 (7 companies, 3 research institutions)

Low Cost Interconnects with highly improved Contact Strength for SOC Applications

Page 3: #PRD2020 #CleanHydrogen - Europa

#CleanHydrogen#EUHydrogenForum

#PRD2020#CleanHydrogen

Objectives

● Decreasing cost of steel interconnects for SOFC and SOEC:

o New cheaper steels > 80 % cost reduction, same performance

• Development of coatings

o Test mass manufacturing processes

• Join roll-to-roll processes

● Increase lifetime by:

o Increasing strength of cell and interconnect interface by >200 %

• Development of contact layer

o Minimize stresses in interface between cell and interconnect

• Optimize flow distribution

Page 4: #PRD2020 #CleanHydrogen - Europa

#CleanHydrogen#EUHydrogenForum

#PRD2020#CleanHydrogen

The consortium

Page 5: #PRD2020 #CleanHydrogen - Europa

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#PRD2020#CleanHydrogen

Highlight 1:Roll-to-roll process test

Hydroforming of precoated IC

Coating is broken

Self-healing within ~50 hours

30 µm

25µm

Cross section

Page 6: #PRD2020 #CleanHydrogen - Europa

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#PRD2020#CleanHydrogen

Highlight 2:Performance of low cost coated steel

0

0.25

0.5

0.75

1

1.25

1.5

1.75

2

0 500 1000 1500 2000 2500 3000

Net

Mas

s ga

in (m

g/cm

2)

Time (h)

850 oC

441 850 Crofer 22 APU 850 44M 850

Corrosion mass gain similar in lab But degradation faster in stack test

Page 7: #PRD2020 #CleanHydrogen - Europa

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#PRD2020#CleanHydrogen

Highlight 3:High adhesion contact layers

Metal particles + binder

Oxidation and reaction

Homogenization

9·Mn (s) + 6·Cu (s) + 10·O2 (g) 5·Mn1.8Cu1.2O4 (s)

Mn (s) + 2·Co (s) + 2·O2 (g) MnCo2O4 (s)

Mn

Cu

0

5

10

15

20

Fra

ctu

re t

ou

gh

ne

ss (J/m

2)

Mn-Cu Mn-Co Ref.

Target

Reactive bonding principle

Conductive spinel

Cell

Interconnect

Page 8: #PRD2020 #CleanHydrogen - Europa

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#PRD2020#CleanHydrogen

Highlight 4:Fast multiphysics multiscale model

Fuel pressure variation Hydrogen molar fraction Temperature distribution

Mechanical stresses

oC• Build in Comsol

Multiphysics

• Using homogenization

• Runs in ~30 min

• 100 cell stack

• >100 times faster than SoA

• All physics included

• mass, heat, current, flows, etc.

• also solid mechanics, turbulent flow in manif.

ഥ𝛔

ഥ𝛔

Submodel for mechanical stresses

Page 9: #PRD2020 #CleanHydrogen - Europa

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Conclusions

● Feasibility of roll-to-roll process demonstrated feasible (coating, shaping)

o Due to self healing of coating

● Low cost steels showed to perform similar as high cost steels (in lab)

o Further research needed for the stack

● High robustness contact layers obtained

o Using reactive bonding

● Fast multiscale multiphysics modelled developed

o Will be used for flow geometry optimization

Page 10: #PRD2020 #CleanHydrogen - Europa

#CleanHydrogen#EUHydrogenForum

#PRD2020#CleanHydrogen

Acknowledgements

This project has received funding from the Fuel Cells and Hydrogen 2 Joint Undertaking (JU) under grant agreement No 826323. The JU receives support from the European Union’s Horizon 2020 research and innovation programmeand Denmark, France, Austria, Belgium, Sweden, Germany, Italy”

Thank you for the attention


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