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Radially symmetric nonlinear photonic crystals Noa Voloch,* Tal Ellenbogen, and Ady Arie School of Electrical Engineering, Department of Physical Electronics, Fleishman Faculty of Engineering, Tel Aviv University, Tel Aviv 69978, Israel * Corresponding author: [email protected] Received July 23, 2008; accepted September 23, 2008; posted October 16, 2008 (Doc. ID 99186); published December 15, 2008 Different types of quadratic, radially symmetric, nonlinear photonic crystals are presented. The modulation of the nonlinear coefficient may be a periodic or an aperiodic function of the radial coordinate, whereas the azi- muthal symmetry of the crystal may be either continuous or discrete. Nonlinear interactions within these structures are studied in two orientations, transverse and longitudinal, for which the interacting beams propa- gate either perpendicularly or in the plane of modulation. We show that radially symmetric structures can phase match multiple arbitrary processes in any direction. We study multiple wavelength three-wave mixing interactions and multiple direction interactions and analyze spatially dependent polarization states of the gen- erated harmonics. © 2008 Optical Society of America OCIS codes: 190.4360, 190.2620, 190.4160. 1. INTRODUCTION Frequency conversion processes resulting from second- order nonlinearity are usually inefficient due to disper- sion. The interacting light beams travel with different phase velocities, so intensity fails to build through their propagation path. Efficient construction of output beams can be achieved by a birefringence technique when the wave vector differences between three mixed waves— input pump beam, signal, and idler output beams—is k = k s + k i - k p =0. However, it also can be obtained by a quasi-phase- matching (QPM) [1] technique for which the sign of the nonlinear coefficient is modulated periodically or aperi- odically along the propagation path of the optical beams. This is realized by one-dimensional (1D) [2] or two- dimensional (2D) [3] domain poling of ferroelectrics. The obtained structures are quadratic nonlinear photonic crystals. The nonlinear interaction between waves in these structures can be regarded as a scattering [4] pro- cess for which the efficient scattering of the signal wave is formulated as a momentum conservation law; it can be satisfied up to a reciprocal lattice vector (RLV) G of the photonic structure [5], so G = k s + k i - k p . Different diffrac- tion conditions (or QPM orders) are obtained by different RLV vectors. The first modulation scheme to be studied was a 1D pe- riodic QPM [1]. This simple modulation is limited for the efficient phase matching of a single nonlinear process. Therefore, numerous schemes of periodic and aperiodic photonic structures [613] were suggested for the compli- cated task of phase matching multiple nonlinear pro- cesses simultaneously. By these schemes, nonlinear cas- cading [14,15] can be realized, i.e., the output of one nonlinear process can be used as the input of a second nonlinear process. Cascading nonlinear processes en- hance the possible applications that can be obtained by photonic structures, such as third-harmonic generation or polarization rotation. The annular, periodically poled, nonlinear photonic structure [16,17] shown in Fig. 1(a) has received consid- erable attention lately. It is characterized by a continuous radial symmetry, but it possesses no translation symme- try. The function that represents the binary modulation of the nonlinear coefficient is gr = signcos2r / . Its spa- tial spectrum contains rings located at discrete radii of q n =2 · n / . If the Ewald sphere [5] intersects with one of these rings the interaction is phase-matched. A very effi- cient collinear phase matching occurs if the phase mis- match k equals to 2 / , i.e., a first-order QPM. This process will be continuously phase-matched (because of radial symmetry) for each pump input angle. It was shown that by transverse phase matching (TRPM) [19,20], the annular periodic structure supports the generation of second-harmonic (SH) conical waves or Bessel beams, which propagate within the nonlinear crys- tal and eventually evolve into rings at the far field. It was also shown that spatiotemporal toroidal waves can be generated in the annular periodic structure using coun- terpropagating ultrashort pump pulses. Here we show that radial structures can be designed to support multiple processes for the purpose of cascading, nonlinear beam shaping, and nonlinear polarization switching. The periodic annular photonic structure that was recently investigated is only one specific example of a diverse family of radial photonic structures displayed in Fig. 1. The modulation of the nonlinear coefficient of these structures can be represented by gr, = mn signcosq n · r · signcosm · , 1 where q n is a set of spatial frequencies and m represents integers. Continuous radial symmetry structures shown in Fig. 1(a) and 1(b) generally may be represented by 42 J. Opt. Soc. Am. B/Vol. 26, No. 1/January 2009 Voloch et al. 0740-3224/09/010042-8/$15.00 © 2009 Optical Society of America
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42 J. Opt. Soc. Am. B/Vol. 26, No. 1 /January 2009 Voloch et al.

Radially symmetric nonlinear photonic crystals

Noa Voloch,* Tal Ellenbogen, and Ady Arie

School of Electrical Engineering, Department of Physical Electronics, Fleishman Faculty of Engineering,Tel Aviv University, Tel Aviv 69978, Israel

*Corresponding author: [email protected]

Received July 23, 2008; accepted September 23, 2008;posted October 16, 2008 (Doc. ID 99186); published December 15, 2008

Different types of quadratic, radially symmetric, nonlinear photonic crystals are presented. The modulation ofthe nonlinear coefficient may be a periodic or an aperiodic function of the radial coordinate, whereas the azi-muthal symmetry of the crystal may be either continuous or discrete. Nonlinear interactions within thesestructures are studied in two orientations, transverse and longitudinal, for which the interacting beams propa-gate either perpendicularly or in the plane of modulation. We show that radially symmetric structures canphase match multiple arbitrary processes in any direction. We study multiple wavelength three-wave mixinginteractions and multiple direction interactions and analyze spatially dependent polarization states of the gen-erated harmonics. © 2008 Optical Society of America

OCIS codes: 190.4360, 190.2620, 190.4160.

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. INTRODUCTIONrequency conversion processes resulting from second-rder nonlinearity are usually inefficient due to disper-ion. The interacting light beams travel with differenthase velocities, so intensity fails to build through theirropagation path. Efficient construction of output beamsan be achieved by a birefringence technique when theave vector differences between three mixed waves—

nput pump beam, signal, and idler output beams—isk=ks+ki−kp=0.However, it also can be obtained by a quasi-phase-atching (QPM) [1] technique for which the sign of theonlinear coefficient is modulated periodically or aperi-dically along the propagation path of the optical beams.his is realized by one-dimensional (1D) [2] or two-imensional (2D) [3] domain poling of ferroelectrics. Thebtained structures are quadratic nonlinear photonicrystals. The nonlinear interaction between waves inhese structures can be regarded as a scattering [4] pro-ess for which the efficient scattering of the signal wave isormulated as a momentum conservation law; it can beatisfied up to a reciprocal lattice vector (RLV) G of thehotonic structure [5], so G=ks+ki−kp. Different diffrac-ion conditions (or QPM orders) are obtained by differentLV vectors.The first modulation scheme to be studied was a 1D pe-

iodic QPM [1]. This simple modulation is limited for thefficient phase matching of a single nonlinear process.herefore, numerous schemes of periodic and aperiodichotonic structures [6–13] were suggested for the compli-ated task of phase matching multiple nonlinear pro-esses simultaneously. By these schemes, nonlinear cas-ading [14,15] can be realized, i.e., the output of oneonlinear process can be used as the input of a secondonlinear process. Cascading nonlinear processes en-ance the possible applications that can be obtained by

0740-3224/09/010042-8/$15.00 © 2

hotonic structures, such as third-harmonic generation orolarization rotation.The annular, periodically poled, nonlinear photonic

tructure [16,17] shown in Fig. 1(a) has received consid-rable attention lately. It is characterized by a continuousadial symmetry, but it possesses no translation symme-ry. The function that represents the binary modulation ofhe nonlinear coefficient is g�r�=sign�cos�2�r /���. Its spa-ial spectrum contains rings located at discrete radii ofn=2� ·n /�. If the Ewald sphere [5] intersects with one ofhese rings the interaction is phase-matched. A very effi-ient collinear phase matching occurs if the phase mis-atch �k equals to 2� /�, i.e., a first-order QPM. This

rocess will be continuously phase-matched (because ofadial symmetry) for each pump input angle.

It was shown that by transverse phase matchingTRPM) [19,20], the annular periodic structure supportshe generation of second-harmonic (SH) conical waves oressel beams, which propagate within the nonlinear crys-

al and eventually evolve into rings at the far field. It waslso shown that spatiotemporal toroidal waves can beenerated in the annular periodic structure using coun-erpropagating ultrashort pump pulses.

Here we show that radial structures can be designed toupport multiple processes for the purpose of cascading,onlinear beam shaping, and nonlinear polarizationwitching. The periodic annular photonic structure thatas recently investigated is only one specific example of aiverse family of radial photonic structures displayed inig. 1. The modulation of the nonlinear coefficient of thesetructures can be represented by

g�r,�� = �mn�sign�cos�qn · r�� · sign�cos�m · ����, �1�

here qn is a set of spatial frequencies and m representsntegers. Continuous radial symmetry structures shownn Fig. 1(a) and 1(b) generally may be represented by

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�r ,�� where m=0. Their spectra contain several ringspaced periodically or aperiodically. Up until now, onlyhe periodic annular structure with continuous radialymmetry shown in Fig. 1(a) [16] has been discussed. Dis-rete radial structures shown in Fig. 1(c) and 1(d) can beepresented by g�r ,��. A special case is the “fan” structurehown in Fig. 1(c) where qn=0. The spectra of the discretetructures contain azimuthally shaped intensity rings.he structure of Fig. 1(d) is a 2D, periodic, nonlinear pho-onic crystal in cylindrical coordinates, analogous to theD periodic structure in Cartesian coordinates [3,5,21]. Its worth noting that nonlinear devices possessing radialymmetry can also be realized using random, rather thanrdered, structures. One recent realization was done [18]y randomly rotating a unit lattice of a 2D nonlinear pho-onic crystal.

We start our discussion in Section 2 by giving an ex-mple of cascading two nonlinear processes in radialtructures. We analyze the generation of a radial third-armonic wave in two different configurations—ransverse and longitudinal QPM. In Section 3 we discussotential applications of radial structures by longitudinalPM. Generally they can be used for multidirectional

hird-harmonic generation or density shaping of noncol-inear processes. We present a novel structure: a quasi-eriodic radial structure. This structure possesses an im-ortant feature—it can be designed to support arbitraryonlinear processes in any direction. In Section 4 we dis-uss applications of these structures in transverse QPMonfigurations such as multicolored rings, azimuthal oradial polarization shaping, etc. In Section 5 we analyzepecial polarization states of output waves in radial struc-ures. We show that polarization effects must be takennto account when light waves interact in radially sym-

etric, nonlinear photonic crystals.

ig. 1. Family of radial photonic structures. The black andhite areas denote negative and positive signs of nonlinear coef-cients, respectively. (a) Periodic annular photonic structureharacterized by period �. (b) Aperiodic continuous radial photo-ic crystal characterized by several periods �n. (c) Discrete peri-dic radial photonic crystal characterized by azimuthal angle �.d) Discrete periodic radial photonic crystal characterized by azi-uthal angle � and radial period �.

. MULTIPLE PROCESSES WITH RADIALYMMETRYhere are numerous applications for phase matchingultiple processes simultaneously that can be done longi-

udinally or transversely. We introduce the concept ofhase matching multiple processes in radially symmetrictructures by a common example of third-harmonic gen-ration (THG).

Third-harmonic waves can be generated by cascading14] two nonlinear processes. The first process is second-armonic generation (SHG), where two pump photonsith frequency � are converted into one second-harmonichoton of frequency 2�. The following process is when onehoton of frequency � and another photon of frequency 2�onvert by sum frequency generation (SFG) into one pho-on of frequency 3�. For both of these processes we need

photonic structure that contains two RLVs—G1k2�−2k� and G2=k3�−k2�−k�.We suggest two experimental ways to achieve radial

HG. The first way is by longitudinal collinear QPM,hen the pump beam propagates in the modulation planes depicted in Fig. 2(a). For THG by longitudinal collinear

ig. 2. (Color online) THG with continuous radial symmetry. (a)ongitudinal QPM; the pump beam propagates in the modula-ion plane. (b) Wave vector diagram for THG. (c) TransversePM; the pump beam is orthogonal to the modulation plane. (d)ave vector diagram for simultaneous conical SHG and THG.

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44 J. Opt. Soc. Am. B/Vol. 26, No. 1 /January 2009 Voloch et al.

PM, the RLVs are �GL1�= �k2��−2�k�� and �GL2�= �k3���k2��− �k��. If the spectrum of the radial photonic struc-

ure contains rings with radii �GL1� and �GL2�, THG can bebtained for each incidence angle of the pump beam ashown in Fig. 2(b).

TRPM is when the pump beam propagates orthogo-ally to the modulation plane as shown in Fig. 2(c). ForHG by TRPM the spectrum of the structure should con-ain two RLVs:

�GT1� = ��k2��2 − �2k��2,

�GT2� = ��k3��2 − �3k��2 − �GT1�. �2�

he output beams that result from these transverse pro-esses are the SH cone wave and the TH cone wave ashown in Fig. 2(d). The transverse THG process is noncol-inear and resembles by its geometry the 1D scheme ofoncollinear THG [22], except that it is spanned radially.he spectrum of the radial structure should be designedo contain circles with the mentioned radii, which areenerally incommensurate. This can be achieved by de-igning radial photonic structures (periodic or aperiodic)hat are characterized by several radii as shown inig. 1(b).

. LONGITUDINAL QUASI-PHASEATCHING IN RADIAL STRUCTURES

. Radial Phase-Reversed Structuresenerally each radial structure can be characterized byeriods �n and azimuthal angles �m. With these charac-eristics, the Fourier space of these structures can be en-ineered so that it contains rings with several arbitraryesired radii. In addition, the intensity of these rings cane azimuthally modulated.We found that known 1D QPM modulation techniques

an be applied to construct radial nonlinear photonic crys-als that support multiple nonlinear processes simulta-eously. Here we demonstrate this by a phase-reversedPM technique [12]. However, it should be stressed that

ther modulation techniques, e.g., quasi-periodic [6,8]odulation, may be used as well.A periodic 1D binary modulation function of the nonlin-

ar coefficient g�z�=sign�cos�2�z /�QPM�� can be repre-ented by its Fourier series, g�z�=�m=−�

� Cmexp�iGm ·z�,here Cm=sinc�m� /2� and Gm=2� /�QPM. In phase-

eversed QPM a 1D QPM structure with period �QPM isultiplied with another 1D QPM structure with

eriod �phase. Thus the phase-reversed structure cane represented by a multiplication of two series:�z�=�m,n=−�

� Cmnexp�iGmn ·z�, where Cmn=sinc�m� /2�sinc�n� /2� and Gmn=2�m /�QPM+2�n /�phase .

A radial phase-reversed structure can be constructed inhe same way. The binary function of the radial phase-eversed structure can be represented by g�r�sign�cos�2�r /�QPM�� ·sign�cos�2�r /�phase��, where thehase-reversed radial structure can be represented byourier series [23]

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Cmn exp�iGmn · r�,

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here r=��x2+y2�, jinc�x�=J1�x� /x, and J1 is a Besselunction of the first kind. We conclude that the spatialpectrum of the phase-reversed structure contains circlesith different incommensurate radii Gmn. Thus, whenk=��kx

2+ky2�=Gmn, several different interactions can be

hase matched radially.We further conclude that if one wants to phase matchultiple processes with radial symmetry, all that needs to

e done is to construct a 1D structure with peaks at theesired phase mismatch values and to span it radially.We examined noncollinear phase-matching possibilities

ithin Fourier spectra by Ewald constructed of severalhase-reversed radial structures as presented in Fig. 3.ote that the studied cases are of longitudinal QPM SHG.hen the Ewald sphere (phase mismatch circle) inter-

ects with a circle on the Fourier space, the interaction ishase-matched. The walk-off angle mn between theump and SH beam can be obtained by the law of cosines:

cos�mn� =�2k��2 + �k2��2 − Gmn

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4k�k2�. �4�

e conclude that radial structures can be engineered sohat they support multiple processes in various discreteoncollinear configurations as shown in Fig. 3. Whereas

n the periodic annular structure, the different phase-atching orders (phase matched by different rings in the

eciprocal lattice) are typically separated by large walk-ff angles, in the phase-reversed radial structure theeparation between the walk-off angle can be made verymall (as shown in Fig. 3(c), where �QPM��phase). As anxample for doubling �=1.55 �m, we can build a “dense”adial structure with periods: �QPM=20.8 �m and �phase16.6 �m. The minimal domain resolution in such struc-

ure is 4 �m. This feature is convenient for diagnosticroperties of the crystal and the light beam, since all ofhese phase-matching orders are obtained simultaneously16].

. Phase Matching with Continuous Angular Symmetryadial photonic structures can be engineered to phaseatch multiple processes with various discrete noncol-

inear geometries. Noncollinear processes with continu-us angular symmetry, i.e., phase matching for all direc-ions, can be achieved by a different radial photonictructure. The structure is designed so its Fourier spec-rum will contain the exact Ewald sphere (phase mis-atch circle). This cannot be obtained with a simple ra-

ial structure, because the center of an Ewald sphere ishifted from the center of the Fourier space by the k vec-ors of the input waves (2k� in case of SHG). However, wean shift the circle in the reciprocal lattice by multiplyinghe structure by an appropriate phase in the real space.e define: kshift=2k�, which represents the shift of the

ircle from the center of axis and kR=k2�, which repre-ents the radius of the desired circle. The binary modula-

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Voloch et al. Vol. 26, No. 1 /January 2009 /J. Opt. Soc. Am. B 45

ion that represents such a structure in real space (shownn Fig. 4(b) is

d�x,y� = sign�cos�x · kshift�� · sign�cos�r · kR��. �5�

The Fourier transform of this structure is shown in Fig.(a) is

D�k ,k � = ���k − k � + ��k + k �� � F�k �. �6�

ig. 3. (Color online) Density shaping of noncollinear processesy phase-reversed structures. Phase matching is obtained whenhe (black) circle (Ewald sphere) intersects with the (blue) circlesFourier spectrum circles). (a) Periodic annular structure. Theoncollinear processes are usually with large walk-off and theyre hard to detect experimentally. (b) Phase-reversed structurephase=3·�QPM. (c) Phase reversed structure �QPM��phase.

x y x shift x shift R

he Ewald construction coincides with a circle on theourier space; thus, the interaction is phase-matched forll propagation directions of the signal wave, with con-inuous angular symmetry. We simulated the aggregationf SH intensity along the propagation path of the beamsithin this photonic structure by a split-step Fourier nu-erical simulation in a stoichiometric lithium tantalate

SLT) [24]. The crystal’s length and temperature were L0.6 cm and T=100°C , respectively. We used a Gaussian

nput beam with wavelength and waist of �=3.496 �mnd �0=60 �m, respectively. The structure was designedy kR=7.5812·106 �1/m� and kshift=7.3763·106�1/m�.ig. 4(e) represents a scaled SH intensity accumulationlong the propagation path of the beam. Fig. 4(c) is the fareld of the output SH beam. The results were comparedith a propagating SH along a 1D (not annular) periodiconlinear photonic crystal. In this case, the simulationarameters were: L=0.6 cm, T=100°C, �=3.501 �m, and0=60 �m. The structure was designed by: kx2.0499·105 �1/m�. The propagating SH is displayed inig. 4(f). The conversion efficiency of this structure was.07·10−5 �1/W� and in the 1D periodic case was.45·10−4 �1/W�. It is clear that the action of phaseatching for all directions has widened the SH intensity

rofile. However, the conversion efficiency was reduced.he construction of energy was still highest at the beam’senter because of maximized interaction length. The two

ig. 4. (Color online) Phase matching with continuous angularymmetry. (a) Fourier spectrum of a photonic structure that sup-orts phase matching for all directions. The Ewald constructionred) circle coincides with a circle (blue) upon the Fourier space.b) Annular periodic photonic structure multiplied with 1D peri-dic structure. (c) Far-field simulation of SH beam at the crystalutput. (d) Far-field simulation of SH beam at the crystal outputn a 1D periodic structure. Note that the far-field image of theadial structure is wider than the far-field output of the 1D struc-ure. (e) Scaled intensity of SH accumulated along the propaga-ion path of the beams in z direction. (f) Scaled intensity of SHccumulated along the propagation path of the beams in z direc-ion in a 1D periodic structure.

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46 J. Opt. Soc. Am. B/Vol. 26, No. 1 /January 2009 Voloch et al.

imulations were operated with slightly different wave-engths because the maximal efficiency point is slightlyifferently for each structure.

. Quasi-periodic Radial Photonic Structureuasi-periodic structures are ordered, nonperiodic struc-

ures whose reciprocal lattice contains at least two incom-ensurate frequencies. Quasi-periodic 1D modulation of

he nonlinear coefficient was previously used to simulta-eously phase match several arbitrary collinear nonlinearrocesses [6,8]. Later it was shown that efficient 2D non-inear photonic quasi-crystals can phase match arbitraryrocesses in chosen discrete directions by the dual gridethod (DGM) [25]. The degree of freedom in this case is

n the lateral movement for which the geometry that theump beam experiences is unchanged under lateralranslation. Since the interaction occurs with a beam ofnite width, this degree of freedom is not critical. We sug-ested a different way to phase match arbitrary nonlinearrocesses in any direction (which are not fixed) by radiallyymmetric, nonlinear photonic quasi-crystals. By thisonfiguration we gain an important feature: arbitraryrocesses can be phase-matched for all pump input angleswith radial symmetry). However, we lose the lateralranslation symmetry since the input beams must passhrough the center of the radial structure.

A quasi-periodic radial photonic structure is schemati-ally presented in Fig. 5(a). It contains concentric rings

ig. 5. (Color online) Phase matching arbitrary multiple pro-esses in any direction by radial nonlinear photonic quasi-rystal. (a) Quasi-periodic radial nonlinear photonic crystal (b)umerical simulation results of SH efficiency of radial photonic

tructure (shown in the inset) that supports three nonlinear pro-ess of 1.53, 1.55, and 1.57 �m simultaneously. This phaseatching applies for each input angle of pump beam, i.e., with

adial symmetry. (inset) The Fourier coefficients of the source 1Duasi-periodic structure. (c) Nonlinear radial quasi-periodictructure spanned from 1D quasi-periodic structure (d) that wasonstructed by DGM. (e) Scheme of phase matching arbitraryrocesses in any direction.

ith radii given by a quasi-periodic sequence. This quasi-eriodic radial photonic structure can support any set ofrbitrary nonlinear processes in a radial fashion (for allump input angles).To illustrate its features we constructed a radial quasi-

rystal that phase matches three arbitrary processes. Werst designed a 1D quasi-crystal in Fig. 5(d) by DGM,hich longitudinally phase matches three SHG processesf 1.53, 1.55, and 1.57 �m [26]. The phase mismatches ofHG in SLT are 3.0467, 2.9673, and 2.8927 �105/m�, re-pectively. The structure’s building blocks were 6.87, 7.23,nd 7.47 �m. The duty cycles were 0, 1, and 0, respec-ively. Fourier coefficients of the 1D structure are shownn the inset of Fig. 5(b) (x axis represents spatial frequen-ies in �105/m� and y axis represents the Fourier coeffi-ients.) Then it was spanned radially as shown inig. 5(c).We simulated the efficiency of SHG in the radial struc-

ure by using the Fourier split-step method. The simula-ion parameters were: L=0.5 cm, T=25°C, and �020 �m. The simulation results are presented in Fig.(b). The conversion efficiencies for the three processeshere 3.45·10−4, 3.4·10−4, and 6.5·10−4 �1/W�, respec-

ively. These efficiencies were very similar to the efficien-ies of a 1D quasi-periodic structure: 2.8·10−4, 3.8·10−4,nd 6.1·10−4 �1/W�, respectively. The similarity of the re-ults is because a narrow stripe of a radial structure re-embles a 1D structure. The quasi-periodic structure effi-iently supports all three processes. This result isignificant since phase matching of several arbitrary pro-esses can be obtained efficiently for any pump inputngles, as illustrated in Fig. 5(e). This structure may belaced inside a ring resonator. Its rich spectrum canhase match multiple different processes, and its radialymmetry can facilitate the planning of the resonator’seometrical configuration.

. TRANSVERSE QUASI PHASE MATCHINGN VARIOUS GEOMETRIESn this section we present several applications of radialtructures that can be realized by TRPM. The first appli-ation is the multicolored SH rings visualized in Fig. 6(a).his application can be realized by structures similar to

he one shown Fig. 1(b). Each SH ring results from a dif-erent diffraction condition and thus appears with a dif-erent radius.

We simulated transverse QPM on a phase-reversed ra-ial structure that was constructed to support two trans-erse radial SH processes of 1500 nm and 1600 nm. Theesults are presented in Fig. 6(b) and 6(c). We simulatedhe far-field output image of SH for each peak as shown inig. 6(d). We got different rings for each wavelength.here is also a possibility to plan a chirped radial struc-

ure that phase matches a range of processes and thusenerates adjustable and all optically controlled SH rings27].

By using structures similar to the one shown Fig. 1(d),e can shape azimuthally the intensity of the SH rings.he output rings will be similar to the one shown in Fig.(e). By inserting a light beam into a structure shown inig. 1(c) (the “fan” structure), we can design a multicol-red star beam.

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Voloch et al. Vol. 26, No. 1 /January 2009 /J. Opt. Soc. Am. B 47

. POLARIZATION STATES IN RADIALYMMETRY INTERACTIONS

n order to fully describe nonlinear interactions within ra-ially symmetric structures, we need to take into accounthe polarization states of the generated waves that essen-ially affect the efficiency of interactions and shape theenerated beams [20]. We will use this section to analyzehe polarization effects on single and cascaded three-waveixing processes with radial symmetry for longitudinal

nd transverse phase-matching configurations. We ana-yze in the following section the generated polarizationtates for crystals that belong to the 3 m symmetry pointroup, e.g., LiNbO3 and LiTaO3.

. Polarization States for Longitudinal Phase Matchingor longitudinal phase-matching configuration, as shownn Fig. 2(a), extraordinary waves polarized in the z direc-ion and ordinary waves polarized in the x–y plane can beenerated by [e-oo] or [e-ee] and [o-oo] or [o-eo] interac-ions, respectively. In this configuration, the polarizationf extraordinary waves generated by [e-oo] or [e-ee] inter-

ig. 6. (Color online) Applications of radial photonic crystals byransverse QPM. (a) Multicolored rings scheme. Each coloreding results from a different diffraction condition. (b) Simulationesults of the efficiency of phase-reversed structure that supportsransverse phase matching of 1500 nm and 1600 nm. (c) Simu-ated far-field output of each process–two SH rings of differentolors. (d) Discrete radial structure for azimuthal intensity shap-ng. (e) Azimuthal intensity shaping of SH rings.

ctions will always be perpendicular to the propagationirection of the waves; thus, the efficiency of generation issotropic.

However, for [o-eo] and [o-oo] the generated polariza-ion will be in the plane of propagation, and the efficiencyf interactions will have azimuthal dependence. This de-endence rises from the fact that the locally generated po-arization, i.e., the polarization of the SH wave is deter-

ined by the symmetry point group, while theolarization of the propagating SH field is determined byhe propagation direction, which is set by phase-matchingonditions. Only the projection of the locally generated po-arization on the plan normal to k2� will contribute to theotal generated efficiency [28]. Thus, when constructing atructure with continuous radial symmetry, which is sup-osed to collinearly phase match (one process or more) forll pump incidence angles as described above, we need toodify the analysis and to take into account that the ef-ciency of [o-eo] and [o-oo] interactions is azimuthally de-endent.For [o-eo] interactions the projection factor of the lo-

ally generated field on the propagating field can be cal-ulated to be cos��, where is the angle between theave vector of the ordinary pump wave k� and the waveector of the ordinary generated wave k2�, and it is deter-ined by the phase-matching conditions. Considering

his relationship, we can understand, for instance, that its not possible to use the [o-eo] interaction to generateaves that travel in perpendicular directions to the ordi-ary pump wave, even when using structures that sup-ort the phase mismatch in these directions, e.g., struc-ures shown on Fig. 3 and Fig. 4(b).

For the case of [o-oo] interactions, the local polarizationf the generated ordinary waves will have the form of

�local=sin�2 �x+cos�2 �y as shown on Fig. 7(a), and therojection factor will be sin �3 +�. This relation sets anzimuthal transparency window for the generated waves,hich has to be taken into account when considering lon-itudinal [o-oo] interactions. Fig. 7(b) shows the effect ofhe azimuthal transparency window in generating THGith continuous radial symmetry that is based on ordi-ary interactions. We can actually learn about the sym-etry group of an unknown crystal by poling it radially

nd measuring its azimuthal transparency window.

. Polarization States of Transverse Phase Matchinge assume that, owing to the relatively small propaga-

ion angles, interactions involving d33 and d31 can be ne-lected [20]. However, polarization states of [o-oo] inter-ctions (using the d22 element of the ��2� tensor) atransverse phase-matching configurations show uniquend interesting properties. As in the case of longitudinalhase matching, the local generated polarization of theecond-harmonic wave will have the form of P� localsin�2 �x+cos�2 �y, which sets an angle of � /2−2 coun-

erclockwise to the x direction. If we now consider sumrequency generation of two pump beams with differentngles of polarizations 1 and 2, the local generated po-arization will have an angle of � /2− 1− 2. Using theseelations we can understand that a polarization rotationf the generated waves will occur for =m� /3 , and that

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48 J. Opt. Soc. Am. B/Vol. 26, No. 1 /January 2009 Voloch et al.

qually polarized generation will occur for =� /6+m� /3.cascaded interaction, e.g., SHG and THG, will result in

he following angels ��� of polarization states for the gen-rated beams:

�SH��pump = � = �/2 − 2 , �7�

�TH��pump = ,�SH = �/2 − 2 � = �/2 − − ��/2 − 2 � = .

�8�

It is also interesting to examine the states of polariza-ions generated by radially symmetric beams, e.g., radi-lly polarized beams [see Fig. 8(a)] or azimuthally polar-zed beams [Fig. 8(b)], when using radially symmetrictructures in transverse configurations. For small anglenteractions the SH waves in both cases will have theame azimuthal polarization dependence, � /2−2�, ashown in Fig. 8(c) where � is the azimuthal angle with re-pect to the x direction. However in a cascaded interactionhe TH wave will gain back the polarization state of theump wave, i.e., a radial pump will generate a radial THave, and an azimuthal pump will generate an azimuthalH wave.

. SUMMARY AND CONCLUSIONSe have presented a new family of nonlinear photonic

tructures having either continuous or discrete radialymmetry. Their symmetry is useful for phase matchingonlinear interactions in any direction. Moreover, aperi-dic radial modulations enable us to simultaneouslyhase match multiple wavelength interactions. It washown that the density of noncollinear processes can behaped by constructing a crystal with an appropriate Fou-ier spectrum.

We have discussed the possibility of continuous angularhase matching (for all directions) by designing a struc-ure spectrum that contains an exact Ewald sphere. Nu-erical simulation showed that even though the SH was

hase matched for all directions, it was built very effi-iently in the collinear direction due to longer, effective in-eraction length. We have proposed schemes for construct-ng multiwavelength converters, multicolored rings, andzimuthal beam shaping using phase-reversed or quasi-eriodic modulation in radial coordinates. These devicesan be used for generating multiple harmonics in arbi-rary directions.

Finally, we have shown that polarization effects muste taken into account (especially for [o-oo] interactions)nd that interactions in a continuous radial structure cane spatially dependent. We have discussed interesting po-arization states of beams generated in radial structuresnd have shown that polarization states can be shaped inadially symmetric structures.

This work was partially supported by the Israeli Sci-nce Foundation grant 960/05 and by the Ministry of Sci-nce, Culture, and Sports.

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ig. 7. (Color online) Azimuthal transparency window for [o-oo]nteractions. (a) Polarization and propagation directions of inter-cting waves in [o-oo] interactions. The polarization of SH gener-ted wave is P� local=sin�2 �x+cos�2 �y. The projection of the gen-rated polarization onto the direction of the propagating wave isin�3 +�. (b) Transparency window for longitudinal THG withontinuous radial symmetry using [o-oo] interactions for 3 mymmetry point group crystals.

ig. 8. (Color online) Special polarization states by transversePM in radial structures. (a) and (b) Radial and azimuthal po-

arization states of pump beams, respectively. (c) Generated/2−2� polarization state of the SH for both pump polarization

tates (radial or azimuthal) shown in (a) and (b). In case of THGhe TH wave will maintain the polarization state of the pump.

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