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Recent Developments at the Brookhaven Source Development Laboratory Brian Sheehy National Synchrotron Light Source Brookhaven National Laboratory Beam Physics Seminar Jefferson Laboratory October 15, 2004
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Recent Developments at the Brookhaven Source Development Laboratory

Brian SheehyNational Synchrotron Light SourceBrookhaven National Laboratory

Beam Physics SeminarJefferson Laboratory

October 15, 2004

The SDL TeamG. L. Carr, E. D. Johnson, S. Krinsky, H. Loos , J. B. Murphy, J. Rose, T. Shaftan, B.

Sheehy, Y. Shen, X.-J. Wang, Z. Wu, L. H. YuNational Synchrotron Light Source; Brookhaven National Laboratory

• Facility Overview

•Diagnostics/Control

• High Gain Harmonic Generation (HGHG)• Cascading• Tunability

•Optical Compression and and Shaping coherent FEL output• SPIDER and CPA

•Other Sources• MV/cm peak field THz source

Facility Overview

AdjustableChicane

177MeV

RF zeroPhasingPhotoinjectorCTR Monitor

Normal incidence

77 MeV

FEL seedat 800 nm

Modulator Undulator

NISUS pop-inmonitors

FEL MeasurementEnergy, Spectrum, Synchronizationand Pulse Length Measurementsat 266 nm

s

Ion Pair ImagingExperimentat 88 nm

Nisus Wiggler

30 mJ Ti:SapphireAmplifier

DispersionMagnet Trim Chicane

• BNL Gun IV photoinjector, S-band, 4.5 MeV• 4 stage Linac up to 200 MeV

• upgrade to 250-300 MeV near completion• Magnetic Chicane Compressor R56 = 5 cm• Seed at λs= 800 nm in 1 m undulator K=1.67 , followed by dispersive section• NISUS undulator, 10 m, 256 period, K = 1.1

• fundamental at λs /3 = 266 nm, output 100 µJ• 1 µJ at third harmonic λs /9 = 89 nm

Diagnostics/Control

UnmatchedUnmatched

0

200

400

RM

S si

ze (u

m)

εn 4.78 ± 0.42 µmβ 3.73 ± 0.38 mα -0.95 ± 0.09

horizontal

0 2 4 6 8 100

200εn 4.12 ± 0.10 µmβ 4.03 ± 0.15 mα 0.51 ± 0.04

vertical

0

100

200

300

εn 4.00 ± 0.19 µmβ 3.26 ± 0.20 mα 0.09 ± 0.07

0 2 4 6 8 100

100

200εn 4.23 ± 0.15 µmβ 3.16 ± 0.16 mα 0.28 ± 0.05

Transverse beam parametersTransverse beam parameters

400400

Distance (m) MatchedMatched

Automated beam matching in NISUS

• over 30 Ce:YAG pop-in beam position monitors (BPM), including 17 in the radiator

•Automated beam matching and emittance measurements

• Optical

•longitudinal electron beam tomography

• CSR instability question

• temporal beam shaping

•electro-optic electron beam measurements

Diagnostics/Control

-10 -8 -6 -4 -2 0 2

-40-30

-20-10

010

2030

4000.51

1.52

Time (ps)

Phase matching

angle (mrad)

Sign

al

100 fs IR

5 ps UV

BBO crystal

250 fs blue

Power meter

BBO Crystal

Detector

ReferenceDetector

Micrometer delay stage

Wedged beam splitter

266 nm HGHGlight

Layout of the two-photon absorptionpump-probe autocorrelator

Photocathode Drive Laser: 250 fsec resolution cross – correlation with oscillator

• shaping: emittance, THz

• two photon absorption autocorrelator for 266 nm output

• picosecond resolution synchroscanstreak camera

• visible & XUV monochromators

• SPIDER: complete field measurement of FEL output

RF Zero PhaseRF Zero Phase

100 150 200 250 300

406080

100120140

100 150 200 250 300 350

406080

100120140160180

50 100 150 200 250 300 350 400

20406080

100120140160180200

Uncompressed beam on pop14

Mild compression

Strong compression.

HeadTail

HeadTail

HeadTail

Positive RF slope

Accelerate bunch at RF zero-crossing

Image at screen depends on energy spread

Bending magnet generates dispersion

Zero RF slope

Negative RF slope

Yikes!CSR Instability?

Use linac phase to ‘streak’ the bunch on screen

But!This is really an energy measurement,

not a current measurement

Longitudinal phase space tomography (H. Loos)

-400 0 400

-400 0 400

-400 0 400

-400 0 400

-400 0 400

-400 0 400

-400 0 400

-400 0 400

-400 0 400

-400 0 400

-400 0 400

-400 0 400

-400 0 400

-400 0 400

-400 0 400

-400 0 400

Spread (keV)

-4 -2 0 2 4

-20

-10

0

10

20

Time (ps)

Ener

gy (

keV

)

-6 -4 -2 0 2 4 6-10

0

10

∆E

(ke

V)

-6 -4 -2 0 2 4 60

25

50

Cur

rent

(A

)

-6 -4 -2 0 2 4 60

0.1

0.2

0.3

Time (ps)

Inte

nsity

t

EDrive laser

current

E-t corrEach value of the chirp manifests a different projection of the phase space.

The energy projection can be very deceptive

Huang & Shaftan NIMA 528, 345 (2004)Current and energy profiles of a chirped beam (a) without energy modulation, (b) with energy modulation.

• Degree of modulation observed inconsistent with CSR models• S. Heifets, G. Stupakov and S. Krinsky PRST-AB 5, 064401 (2002)• Z. Huang & H.-J.Kim PRST-AB 5, 074401 (2002)• Z. Huang T. Shaftan SLAC-PUB-9788, 329.

• Longitudinal Space Charge model: • small modulation in photocathode drive laser • small current modulations due to drive laser modulations at photocathode• longitudinal space charge forces result in enhanced energy modulations in the bunch• these dominate the horizontal distribution in zero-phase measurements• experimental confirmation

• lack of coherent enhancement of the IR in coherent transition radiation• modulation behavior with chicane strength, trans beam size, energy, etc• phase space tomography

potential threat for short pulse short wavelength FEL’s• can convert to current modulation; larger energy spresd • goes away for perfectly uniform laser temporal profile

Theory: Huang & Shaftan NIM A 528, 345 (2004)Experiment: Shaftan et al NIM A 528, 397 (2004)

Ti:Sapph Oscillator

Dazzler

Stretcher

Amplifier

Compressor

ω−tripler

800 nm9 nJ100 fsec

5 nJ200-400 psec

25 mJ170-350 psec

15 mJ0.1 - 30 psec

266 nm1.8 mJ

Time (psec)

Inte

nsity

(arb

uni

ts)

Temporal Shaping (in progress)At SDL in collaboration with SPARC

and SLAC

Amplified and compressed IR pulse

Millennia Laser

Tsunami Laser

Spec

trum

Ana

lyze

r

Aut

o-co

rrel

ator

OpticalIsolator

StretcherCompressor 1

Regenerative Amplifier

2-pass Amplifier

2-pass Amplifier

VariablePowerDivider

Phot

ocat

hode

GC

R-1

70 Y

AG

Las

er

GC

R-1

50 Y

AG

Las

er

Photodiode

Pow

erA

tten

ω+

ω

= 2ω

ω+

= 3ω

Autocor-rellator

SpotImaging

Power Mon

Optical Relay, 14 meters

Monument

PowerAtten

SpatialFilter

Compressor 2

Optical Relay, ~35 metersSeedingAnd Diagnostics

Daz

zler

ZnTeAccelerator

TrimModulator

Dipole

Monitor

Polarizer

Analyzer

λ/4 Plate

toNISUS

Spectro-meterFiber

Trim

Seed LaserDelay

ElectronsLaser

(800 nm)

Electro-Optic e-beam meaurements

( ) λε

πϕ+

=∆1

2 vac4130 lErn

Retardation induced by e-bunch field Evac

RTRT

+−

=∆ )sin( ϕ

Asymmetry in transmitted/reflected gives ∆ϕ

Chirp seed and spectrally resolve the asymmetry –single shot measurement (800 fsec resolution).

Jitter 150 fsec rms over 20 seconds

or chirp

High Gain Harmonic Generation (HGHG)

e-

• Self amplified Spontaneous Emission (SASE)Spontaneous emission microbunching enhanced emission

• Noisy• Broad Bandwidth• Not longitudinally coherent

• HGHG Seed modulates e- energy

coherent microbunching emission•Short wavelength : tune radiator to harmonic of seed•Stable•Narrow bandwidth, higher brightness•Longitudinal coherence

Spectrum

0 1 2 30

1

2

3

p(E

) σ= 41%

E/<E>0 1 2 30

5

10

p(E

) σ = 7%

Energy Fluctuations

SASE

HGHG

Cascading HGHG to soft X-ray wavelengths (L.H Yu)

1-ST STAGE 2-ND STAGE 3-RD STAGE FINAL AMPLIFIER

AMPLIFIER λw = 6.5 cm

Length = 6 m Lg = 1.3 m

AMPLIFIER λw = 4.2 cm

Length = 8 m Lg = 1.4 m

AMPLIFIER λw = 2.8 cm

Length = 4 m Lg = 1.75 m

MODULATOR λw = 11 cm

Length = 2 m Lg = 1.6 m

MODULATOR λw = 6.5 cm

Length = 2 m Lg = 1.3 m

MODULATOR λw = 4.2 cm

Length = 2 m Lg = 1.4 m

DISPERSION

dψ/dγ = 1

DISPERSION

dψ/dγ = 1

DISPERSION

dψ/dγ = 0.5

DELAY DELAY DELAY“Spent” electrons “Fresh”

electrons“Spent”

electrons“FRESH BUNCH”

CONCEPT

“Fresh” electrons

e- e-

266 nm SEED LASER

53.2 nm2.128nm10.64 nm÷5 ÷5 ÷5

400 MW 800 MW 70 MW

1.7 GW

500 MW

e- e-

LASER PULSE

AMPLIFIER λw = 2.8 cm

Length = 12 m Lg = 1.75 m

e-beam 750Amp 1mm-mrad2.6GeV σγ /γ=2×10 – 4 total Lw =36m

A proposed 2 stage cascade for the SDL

e-beam600Amp250 MeV2.7 mm-mradσγ / γ = 1.×10 - 4

Pin=1.5 MW266nm 66.5 nm

Pout=140 MW56 MW133nm

2m VISA

6 m NISUS0.8m MINI

Pulse length ~ 0.5ps 70µJ

A Novel Tunability scheme for HGHG (T. Shaftan)

Radiator DS Modulator

1 0 1174.5

175

175.5.

1 0 1174.5

175

175.5.

1 0 1174.5

175

175.5.

.

Seed with fixed λ

before FELafter Modulatorafter DS

E [MeV] E [MeV] E [MeV]

t [ps]

• Dispersive Section (DS) converts energy modulation into bunching• DS also compresses the energy modulation wavelength• a small but measureable effect in our machine, but could be optimized to yield a tuning range of 20%

(Dispersive Section)

Optimal tunability configuration

Klystron

Radiator DS ModulatorXRF XRF1 0 11

0

1

.

1 0 11

0

1

.1 0 11

0

1

.1 0 11

0

1

.1 0 11

0

1

. time

HGHG Seed with fixed λ

ener

gy

Compression or stretching in the dispersive section can be used to modify the period of the microbunching. This is ordinarily a small effect, but it could be optimized to yield ~20% tunability.

SDL Experiment

• Chirp is provided by shifting beam off-crest in tank 4 (Emax = 58 MeV)

• Tank 4 phase shift: from +25° to -45°• DS is set to maximum current (200 A)• Nothing else was changed !• Spectrum of HGHG is measured

for different amounts of chirp

Gun 4.5 MeV

Tank 1Tank 2Tank 3Tank 435 MeV72 MeV130 MeV190 MeV

ModDSNISUS266 nm 0.8 um

.Tank 4 phase

Tank 4energygain

seed

HGHG output spectra for various tank 4 phases:

-45° -30°-10°

0°+10°

+25°

Wavelength, nm

HG

HG

inte

nsity

, a.u

.

Fit, based on R56(DS)=0.34 mm

0.8 0.6 0.4 0.2 0 0.2 0.4 0.6

263

264

265

266

Wavelength versus chirp

sin(phi4)

Wav

elen

gth

[nm

]

263.28

265.92

0.3 0.2 0.1 0 0.1 0.2 0.3

263

264

265

266

Wavelength versus energy

Energy detuning, %W

avel

engt

h [n

m]

∆λ/λ≈1 %FEL ρ

Fit including R56of DS and radiator

Additional compressionin the radiator

Spectral Phase Measurements; chirping and shaping FEL output

• Optical Compression and and Shaping coherent FEL output

• Measuring Spectral Phase• SPIDER technique• Application at 266nm for picosecond laser pulses

• Measurements HGHG• Unchirped, narrow bandwidth

•Near transform limit• Chirping and Compressing

High Gain Harmonic Generation (HGHG)and Chirped Pulse Amplification (CPA)

time

freq

uenc

y

time

e-en

ergy time

freq

uenc

y

ω

e- e-

Opticalcompressor

time

freq

uenc

y

Tb

T<<Tb

• Match optical seed chirp to electron energy chirp•Resonant frequency in modulator matches seed at each moment in the bunch

• Output pulse is also chirped• Longitudinal coherence permits optical compression to transform limit

• femtosecond pulses • Sensitive to spectral phase distortion• Li Hua Yu et al Phys Rev E 49, 4480 (1994)

Shaping HGHG

• Coherent control at short wavelengths• For both chirping and shaping, the question is:How will phase modulation in the seed transfer to HGHG?

•Can distortions be used as a probe of e- beam and radiator dynamics

Potential Problems / Interesting Questions• synchronization jitter • stability• noise & harmonics• optical field is bipolar, electron density is not.

(Walmsley group, Oxford)

266 nm

400 nm800 nm

Measuring the spectral phase: SPIDER(Spectral Interferometry for Direct Electric-Field Reconstruction)

ωc

D(ω

c) 2π/τ

C. Iaconis and I. A.Walmsley, Opt. Lett. 23, 792–794 (1998).

DOWNCONVERSION SPIDER LAYOUT

Spectrometer

800 nm(seed)

+266 nm

(HGHG)

Michelsoninterferometer

BBO

.

266

nm

800 nm

Filter

Compressor used as stretcher

DelayLine

400 nm

• Separate seed pulse (800 nm) and HGHG• stretch seed to 60 psec• make 2 HGHG pulse replicas in interferometer and separate by τ=3.5 psec• Downconvert to 400 nm in BBO• frequency shift is Ω=0.2 THz

• set spectrometer to λc=800 nm• measure 400 nm SPIDER trace in 2nd order• block seed, remove filter and measure 266 nm calibration trace in 3rd order

ang

Spidering a laboratory 266 nm source

-0.05 0 0.05-10

0

10

20

30

ω - ω0 (PHz)

radi

ans

amplitudephasefit chirpphase-chirp

-0.05 0 0.050

0.2

0.4

0.6

0.8

1

ω - ω0 (PHz)

inte

nsity

(arb

uni

ts)

Typical Spider Trace

Reconstructed phase and amplitude Comparison with x-correlation

• stretch a 100 femtosecond 800 nm Ti:Sapph chirped-pulse-amplification system• Frequency-triple in BBO to 266 nm(spoil phase matching to create an asymmetry in the time profile)• Compare scanning multishot cross-correlation of the 266 nm and a short 800 nm pulse with the average reconstruction, convolved with 250 fsec resolution of the x-correlator

-1 -0.5 0 0.5 1 1.50

0.2

0.4

0.6

0.8

1

time (psec)

inte

nsity

(arb

uni

ts)

spidercross correlation

900 fsec FWHM

UNCHIRPED HGHG

time

freq

uenc

y

time

e-en

ergy time

freq

uenc

y

Tb

ω

e- e-

• Stretch seed to 6 psec• optimize compression / minimize e- energy chirp• minimize output bandwidth

Frequency vs time

UNCHIRPED HGHG

* 3

Spectral Phase

• flat phase across the pulse• residual seed chirp not visible• frequency vs time constant

Temporal Phase

50 shots

0 5 10 150

2

4

6

8

10

12

rms spectral width σ (THz)

num

ber o

f sho

ts

0 0.2 0.4 0.6 0.80

5

10

15

20

rms temporal width σ (psec)

num

ber o

f sho

ts

σω=5.5 0.7THz

στ=0.20 0.01psec

•Define transform limit as the pulse when spectral phases are set to zero.• pulses are 1.4 0.1 times transform limit

widthtran ltd width

• σωστ = 1.1, twice transform limit for a Gaussian pulse• FWHM = 440 80 fsec• pulses are not Gaussian

207 fs rms

168 fs rmsUNCHIRPED HGHG

time

freq

uenc

y

time

e-en

ergy time

freq

uenc

y

Tb

ω

e- e-

CHIRPED HGHG

• Chirp e- bunch and optical seed together• optical seed: 3.8 THz/psec• e- bunch: 2.7 THz/psec (resonant frequency)• broader bandwidth already observed

Doyuran et al PRST AB 7, 050701 (2004)

CHIRPED HGHG

* 3

CHIRPED HGHG

* 3

CHIRPED HGHG

* 3

CHIRPED HGHG

* 3

Time (psec)

Freq

uenc

y (T

Hz)

Distribution of chirps fit over a 200 fs window around peak center

CHIRPED HGHG

seed chirp * 3

• Sources of instability• optical chirp / e- chirp mismatch• synchronization (150 fsec rms)• compression instability• rf curvature

•The seed chirp is clearly observed in the HGHG output over part of the pulse• distortion in the pulse wings deteriorates compressibility

Matching Electron and Optical Chirp

λ

t

γ

Optical BeamElectron Beam

•Electron beam has curvature due to sinusoidal acclerating field•If chirp is not matched, resonance occurs only over a short portion of the electron bunch – correlation between compressibility and uncompressed pulse length?•Mismatched is more sensitive to synchronization jitter.

Uncompressed rms pulse width (fsec)

Com

pres

sion

Fac

tor

correlation between compressibility and uncompressed pulse length

Compression factor

rms width‘compressed’ width

‘compressed width/transform limit

• most pulses compressible in principle to ~ twice transform limit•quadratic spectral phase (defines compressor) not determined only by chirp• a ‘reasonable’ fixed compressor compresses only 15% of pulses

Fit b for each shot and ‘compress’:

CPA Summary• Successfully demonstrated SPIDER at shortest wavelength and longest pulse lengths reported.

• Characterized spectral phase of High Gain Harmonic Generation

• near transform limited

• Chirped Pulse Amplification• Imparted positive chirp commensurate with seed chirp• poorly matched electron chirp• sensitivity to other factors still unclear

• shown the viability of CPA and potential for more complex pulse shaping

GaAs

Typical Laser-based THz Source

UF laserTHz

• Transient current is subpicosecond, Ea ~ 10 kV/cm• Relaxation is slow: half-cycle pulse• THz yields: 1 nJ (250 kHz) to 1 uJ (1 kHz), • size scaling limit 1 - 10 uJ• optical rectification yields are similar w/ higher freqs.

photocathodeelectron gun

dipole chicanecompressor~ 300 fs, 700pC electron bunches

(can be shorter w/ less charge)

Coherent THz transitionradiation

Note: <10 Hz rep. rateCoherent THz dipole radiation

SDL LINAC-based THz Source

• bunch length ~ λ, coherent enhancement• energy of 80 uJ measured in this setup ( E ~ 1 MV/cm)

• 2 orders of magnitude larger than other sources • Scales as Ne-

2

• spectral content to 2 THz• higher for shorter bunches

• This machine is not optimized for THz production 0 2

Inte

nsity

Frequency (THz)

Coherent Transition Radiation

Transition radiation occurs when an electron crosses the boundary between two different media. For a relativistic electron (β ≡ v/c ≅ 1) incident on a perfect conductor, the number of photons emitted per solid angle and wavelength range is:

( )θβθθβ

λπα

λ 22

222

2 cos1cossin

−=

ΩdddN

Intensity is 0 on axis, peaks at θ ~ 1/γ.Polarization is radial

Coherent radiation emission:

-50 -25 0 25 50

Inte

nsity

(rel

.)

Angle (mrad)

Far field distribution for γ = 200

dWN /dω = N2 dW1 /dω | f (ω)|2

( ) ( )2

/ˆ∫∞

∞−

⋅= drrSef crniωωwhere (Nodvick & Saxon)

Electro-Optic measurement of THz field

•Polarization of synchronized optical field is retarded by instantaneous THz field in the ZnTe crystal by Pockels effect• analyzer gives time resolved 2-dimensional distribution of electric field component

CCDZnTe AnalyzerPolarizer

Lens

Electron Beam

Vacuum Window

Paraboloid

Coupling Hole, 2 mmTi:Sa Laser

Delay

λ/4

EO Detection method:T.F. Heinz/Columbia & X.-C. Zhang/Rensselaer Accelerators:Yan, Van der Meer et al PRL 2000Wilke et al PRL 2002Loos et al PAC 2003Chirped sampling:Jiang and Zhang, APL (1998)

Pixels

Pix

els

100 200 300 400 500 600

100

200

300

400

Horizontal (mm)

Verti

cal

(mm

)

-2 -1 0 1 2

-2

-1

0

1

2

Image Processing for electric field recovery

Use compensator waveplate to detect sign of polarization change.Reference IR (left) and Signal IS (right) obtained simultaneously.Rescale and normalize both.Calculate asymmetry A of Signal.Subtract asymmetry pattern w/o THz.

A = 2IS/IR - 1

Coherent THz Transition Radiation Pulses from the SDL Linac

0.0 0.5 1.00

20

40

60

80

Pyr

oele

ctric

Det

ecto

r Res

pons

e [µ

J]

Time [ms]

Up to 80 µJ (!) per pulse -> consistent with calculation

0 20 40 600

2

4

6

8

10

Inte

nsity

[arb

.]

Frequency [cm-1]

0 1 2 Frequency [THz]

Intensity to 2 THz (higher with shorter bunches)

photocathodeelectron gun

dipole chicanecompressor~ 300 fs, 700pC electron bunches

(can be shorter w/ less charge)

Coherent THz transitionradiation

Note: <10 Hz rep. rateCoherent THz dipole radiation

THz beam path and analyzer

Beam Paths in Analyzer

OAPOAP ZnTeZnTe

BSBS

λ/4λ/4 Pol.Pol.RefRef

SignalSignal

CameraCamera

CTR simulation (H. Loos)

30 m

m

Decompose electron beam coulomb field in Gauss-Laguerre modes.

Calculate complex transmission factors through experiment for THz spectral range.

Use bunch form factor to reconstruct time dependence.

20 ps

Cross section of E-field at focus as a function of time

E-field along horizontal plane

Note: opposite sides are asymmetric, as shown (radial polarization)

Measurement

Calculation (mm)

Temporal-spatial E-field profile of coherent transition radiation pulse at ~ f/1.5 focus

Opportunities in Magnetism for THz pulses(Epeak = 1 MV/cm → Bpeak = 3 kilogauss)

magneticviscosity

field(gauss)

Ultra-Short Pulses and/or High Fields -- D. Arena / NSLSCurrent state of the art for “ultra-fast” dynamics experiments:

10

-15

10

-12

10

-9

10

-6

Excitation / Interaction

exchange interaction

Stoner excitations

spin waves

(low q limit)

spin-lattice relaxation

in manganites

precessional rotation

and damping

spin coherence

and spin diffusion

Coercivity / Saturation

time(sec)

10

5

10

4

10

1

10

2

10

3

soft

manganites

permallo

y

transit

ion

metals & allo

ysa″

Fe 16N 2

dilute

magnetic se

micond.

rare-earth

magnets

Role forTHz!

Time: ~100 fs (lasers)~100 ps (synchrotron)

Field: ~10 – 100 gauss (stripline)

Soft Modes in Ferroelectrics & Perovskites (PbTiO3)G. L. Carr

Use half-cycle pulse to coherently drive atoms, probe motion as a function of time (needs diffraction probe).

THz

HCP

ETH

z HC

P

ETH

z HC

P

E

E(t)

Observe “shift” in diffraction spot(s)

DOE Workshop on Ultrafast X-rays

Why Make Terahertz Pulses ?

• Imaging/Remote Ranging– non-ionizing

– medical– safely use to monitor public or battlefield environments

– CHEMICALLY AND BIOLOGICALLY SENSITIVE– explosives, weapons detection– phonon modes in DNA (Woolard et al Phys Rev E 65, 051903)

– remote ranging with bacterial species identification – a lot of work remains in sources, detection, and characterization.

explosives

weaponsWoolard et al THz Differential Absorption Radarmodel (Bio early warning)

1 km

Some More Reasons•Ultra-fast dynamics (< 1 ps time scale)

– directly measure complex dielectric response of sample – strong coupling of optical/THz excitations in correlated e- systems (e.g. high-Tc superconductors)

•Low frequency, non-linear properties of materials– nanoparticles / quantum dot arrays in dielectrics

– Optronics: Ultrafast components in all-optical circuits– faster, EMP resistant

•Orienting Molecules– spectroscopy and chemistry from coherent rovibrational states– manipulate internal molecular fields / fundamental measurements & coherent control

•Structural transitions–Large E-field to coherently “shove” atoms

THz Summary

• The DUVFEL THz source pulse energy exceeds other sources by 2 orders of magnitude (DUVFEL 80 uJ, Laser sources 1 uJ, JLab ERL 0.5 uJ)

• fundamental dynamics ( magnetic systems, strongly correlated e- systems, nanoparticles…) • large area imaging• single shot detection• explore nonlinear effects• THz as pump in pump-probe experiments

•MV/cm E-fields and kilogauss B-fields •THz pulse shaping (through e-beam and optically)

• Accelerator sources have not been optimized for THz production

Global Summary

SDL continues to be an important test bed for FEL science and technology development, as well as a user facility

•answers to important questions of beam dynamics for next generation sources

HGHG is an extremely promising candidate for producing longitudinally coherent short wavelength ultrafast pulses

•tunability•chirped pulse amplification and Shaping•cascading is in the works

The THz production is a truly unique source capable of opening a new regime of dynamics to study


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