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Second-harmonic generation by off-axis propagation in an anisotropic optical waveguide

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Second-harmonic generation by off-axis propagation in an anisotropic optical waveguide D. V. Petrov Departamento de Fisica, Universidade Federal de Pernambuco, 50670-910, Recife, Brazil Received July 5, 1995; revised manuscript received June 20, 1996 Second-harmonic generation (SHG) by means of radiation modes (the C ˇ erenkov-type radiation scheme) in an anisotropic optical waveguide by off-axis propagation has been studied theoretically. If the second-harmonic wave is a leaky wave of the waveguide, the C ˇ erenkov-type SHG efficiency may be comparable with the effi- ciency of the guided-mode guided-mode SHG without critical control of the wave-vector-matching condition. The model presented predicts a strong modification of the radiation field by a change of the interaction length. A numerical simulation of the proposed type of SHG in a graded-index waveguide on the X-cut surface of LiNbO 3 is made. © 1997 Optical Society of America [S0740-3224(97)02001-8] 1. INTRODUCTION The use of integrated-optical structures to enhance non- linear effects, in particular, second-harmonic generation (SHG), is attractive because of the high optical power den- sities and long interaction lengths provided by guided- wave structures. 1 Moreover, they have another advan- tage in that all the components of the second-order nonlinear-optical coefficient tensor are, in principle, phase matchable by use of the modal dispersion in waveguiding structures. SHG in optical waveguides is classified into two types: One is conversion from a guided mode at the fundamental frequency into a second- harmonic (SH) guided mode (guidedguided type of SHG 25 ), and the other is conversion from a guided mode at the fundamental frequency into a SH radiation mode (so-called C ˇ erenkov-type SHG 611 ). The guided guided SHG has a large efficiency, but phase matching for a given wavelength requires critical control and uniformity of the waveguide dimensions. C ˇ erenkov-type SHG is free from the phase-matching constraint because this scheme uses radiation modes whose propagation constants can take arbitrary values. This type of SHG occurs when the phase velocity of the nonlinear SH polarization is larger than that of the free SH wave in the cladding material (substrate). The phase-matched SH wave is radiated into the substrate at an angle that satisfies the conservation of the wave-vector component parallel to the waveguide. The disadvantage of C ˇ erenkov-type SHG is a reduction in efficiency because of a small overlap of the modal fields of the fundamental wave and the SH wave. The C ˇ erenkov radiation scheme was demonstrated experimentally (see, for example, Refs. 6 9). Interest in C ˇ erenkov-type SHG has been generated by potential applications in short-wavelength light sources, generation of ultrashort SH pulses, 12 and all-optical switching by a x (2) :x (2) cascading process. 13 A leaky wave can propagate off axis in an anisotropic waveguide. 14,15 The phenomenon of leaky-wave propaga- tion in optical waveguides has been studied exten- sively. 1622 For waveguides on the X - and Y -cut surfaces of negative crystals a leaky wave is the wave of hybrid po- larization with an effective refractive index that is less than the substrate’s ordinary refractive index. The field of a leaky wave consists of two contributions with or- thogonal polarization. The contribution of the extraordi- nary polarization concentrates its power in the wave- guide. The contribution of the ordinary polarization has a radiative part, which is responsible for a leakage of the mode’s power into the substrate. Here we show how the C ˇ erenkov-type SHG process is modified if a leaky wave of an anisotropic waveguide is in- volved in the interaction. Assuming an anisotropic waveguide with an arbitrary graded-index distribution inside the waveguide layer, I present numerical results on an overlap integral that is responsible for the SHG ef- ficiency and the spatial distribution of the radiation field. 2. MODEL We consider a planar graded-index waveguide on the X -cut surface of a negative crystal [Fig. 1(a)] and a geom- etry in which the crystal optical axis Z is placed in the waveguide plane, forming an angle u with propagation di- rection z of the guided mode at the fundamental fre- quency v. We assume that an anisotropy ( n o 2 n e ) is large compared with typical graded-index refractive- index (RI) changes. (Here n o and n e are the substrate’s or- dinary and extraordinary RI’s, respectively.) In this case the hybrid waveguide modes are still mostly ordinary and extraordinary. The hybrid quasi-ordinary (quasi-TM) modes propagate as guided modes at any direction of the waveguide, whereas the hybrid quasi-extraordinary (quasi-TE) modes become leaky waves if their propaga- tion angles u are greater than the critical angles u c and their effective RI’s N TE ( u ) , n o . The critical angle is de- fined by the condition that N TE ( u c ) 5 n o . D. V. Petrov Vol. 14, No. 2 / February 1997 / J. Opt. Soc. Am. B 331 0740-3224/97/020331-08$10.00 © 1997 Optical Society of America
Transcript

D. V. Petrov Vol. 14, No. 2 /February 1997 /J. Opt. Soc. Am. B 331

Second-harmonic generation by off-axispropagation in an

anisotropic optical waveguide

D. V. Petrov

Departamento de Fisica, Universidade Federal de Pernambuco, 50670-910, Recife, Brazil

Received July 5, 1995; revised manuscript received June 20, 1996

Second-harmonic generation (SHG) by means of radiation modes (the Cerenkov-type radiation scheme) in ananisotropic optical waveguide by off-axis propagation has been studied theoretically. If the second-harmonicwave is a leaky wave of the waveguide, the Cerenkov-type SHG efficiency may be comparable with the effi-ciency of the guided-mode–guided-mode SHG without critical control of the wave-vector-matching condition.The model presented predicts a strong modification of the radiation field by a change of the interaction length.A numerical simulation of the proposed type of SHG in a graded-index waveguide on the X-cut surface ofLiNbO3 is made. © 1997 Optical Society of America [S0740-3224(97)02001-8]

1. INTRODUCTIONThe use of integrated-optical structures to enhance non-linear effects, in particular, second-harmonic generation(SHG), is attractive because of the high optical power den-sities and long interaction lengths provided by guided-wave structures.1 Moreover, they have another advan-tage in that all the components of the second-ordernonlinear-optical coefficient tensor are, in principle,phase matchable by use of the modal dispersion inwaveguiding structures. SHG in optical waveguides isclassified into two types: One is conversion from aguided mode at the fundamental frequency into a second-harmonic (SH) guided mode (guided–guided type ofSHG2–5), and the other is conversion from a guided modeat the fundamental frequency into a SH radiation mode(so-called Cerenkov-type SHG6–11). The guided–guidedSHG has a large efficiency, but phase matching for agiven wavelength requires critical control and uniformityof the waveguide dimensions.Cerenkov-type SHG is free from the phase-matching

constraint because this scheme uses radiation modeswhose propagation constants can take arbitrary values.This type of SHG occurs when the phase velocity of thenonlinear SH polarization is larger than that of the freeSH wave in the cladding material (substrate). Thephase-matched SH wave is radiated into the substrate atan angle that satisfies the conservation of the wave-vectorcomponent parallel to the waveguide. The disadvantageof Cerenkov-type SHG is a reduction in efficiency becauseof a small overlap of the modal fields of the fundamentalwave and the SH wave. The Cerenkov radiation schemewas demonstrated experimentally (see, for example, Refs.6–9).Interest in Cerenkov-type SHG has been generated by

potential applications in short-wavelength light sources,generation of ultrashort SH pulses,12 and all-opticalswitching by a x(2):x(2) cascading process.13

A leaky wave can propagate off axis in an anisotropic

0740-3224/97/020331-08$10.00 ©

waveguide.14,15 The phenomenon of leaky-wave propaga-tion in optical waveguides has been studied exten-sively.16–22 For waveguides on the X- and Y-cut surfacesof negative crystals a leaky wave is the wave of hybrid po-larization with an effective refractive index that is lessthan the substrate’s ordinary refractive index. The fieldof a leaky wave consists of two contributions with or-thogonal polarization. The contribution of the extraordi-nary polarization concentrates its power in the wave-guide. The contribution of the ordinary polarization hasa radiative part, which is responsible for a leakage of themode’s power into the substrate.Here we show how the Cerenkov-type SHG process is

modified if a leaky wave of an anisotropic waveguide is in-volved in the interaction. Assuming an anisotropicwaveguide with an arbitrary graded-index distributioninside the waveguide layer, I present numerical resultson an overlap integral that is responsible for the SHG ef-ficiency and the spatial distribution of the radiation field.

2. MODELWe consider a planar graded-index waveguide on theX-cut surface of a negative crystal [Fig. 1(a)] and a geom-etry in which the crystal optical axis Z is placed in thewaveguide plane, forming an angle u with propagation di-rection z of the guided mode at the fundamental fre-quency v. We assume that an anisotropy (no 2 ne) islarge compared with typical graded-index refractive-index (RI) changes. (Here no and ne are the substrate’s or-dinary and extraordinary RI’s, respectively.) In this casethe hybrid waveguide modes are still mostly ordinary andextraordinary. The hybrid quasi-ordinary (quasi-TM)modes propagate as guided modes at any direction of thewaveguide, whereas the hybrid quasi-extraordinary(quasi-TE) modes become leaky waves if their propaga-tion angles u are greater than the critical angles uc andtheir effective RI’s NTE(u) , no . The critical angle is de-fined by the condition that NTE(uc) 5 no .

1997 Optical Society of America

332 J. Opt. Soc. Am. B/Vol. 14, No. 2 /February 1997 D. V. Petrov

The effective RI of a leaky wave is a complex number,and its imaginary part describes a loss of mode energy inthe waveguide as a result of its radiation in thesubstrate.15–17 The loss coefficient is maximum near uc ,and it decreases with u.Usually the ordinary and the extraordinary RI’s have

different dispersion. Let the ordinary RI at v nov be

larger than the extraordinary RI at the double frequencyn e2v [see Fig. 1(b)]. (For example, in LiNbO3 this condi-

tion is satisfied in the near-infrared region for wave-lengths more than 1.1 mm.23) Assume that the wave at vis a guided quasi-TM mode. As Fig. 1(b) shows, allmodes at 2v with propagation constants bR

2v , ko2vno

2v

belong to radiation modes with continuous spectra of bR2v.

The wave-vector matching of the guided mode at v to theSH radiation mode exists for any propagation angle (theCerenkov-type SHG process).The effective RI of the leaky wave at 2v, NTE

2v (u), has areal and an imaginary part, and its real part is smallerthan n o

2v (dashed curve in Fig. 2). An angle us is definedby the condition Re@NTE

2v(us)# 5 NTMv , where NTM

v is theeffective RI of the guided mode at v. When the propaga-tion angle of the wave at v approaches u 5 us the SHGefficiency should increase considerably because of concen-

Fig. 1. (a) Anisotropic waveguide structure. x is the normal tothe waveguide’s surface; z is the propagation direction. (b) RI inthe waveguide plane versus propagation direction. The solidcurves correspond to the substrate’s RI’s. The dashed and dot-ted curves correspond to leaky and guided modes, respectively.uc is the critical angle at which the transition between the guidedwave and the leaky wave occurs. us is the angle, at which thephase matching of the guided wave at v and the SH leaky waveoccurs. The SH radiation modes are in the hatched region.

tration of the leaky-wave field in the waveguide layer.On the other hand, the radiative part of the leaky-wavefield provides the leakage of the SH wave into the sub-strate.Unlike guided modes and radiation modes, a leaky

wave does not constitute an eigenmode of waveguides be-cause it cannot be normalized.24 By a theoretical de-scription we should represent a leaky wave of the aniso-tropic waveguide as a sum of eigenmodes with differentpropagation constants, i.e., as a bundle of radiation modeswith hybrid polarization.25 Through nonlinear conver-sion from the guided mode at v, a continuum of the radia-tion modes at 2v is generated. The total radiation fieldcan be obtained by integration over all contributions.Hence we should consider the SHG of a leaky wave asCerenkov-type SHG by the specific set of the radiationmodes.Consider first the well-known expression for the SHG

efficiency. Assuming that the depletion of the wave at vcan be neglected, the efficiency of the guided–guided SHGin the coupled-wave formalism is given by2,10

P2v

Pv 5 AGGPvL2uIGG~bG

v , bG2v!u2

sin2@~bG2v 2 2bG

v !L/2#

@~bG2v 2 2bG

v !L/2#2,

(1)

where L is the interaction length, bGv and bG

2v are thepropagation constants of the fundamental guided modeand the SH guided mode, respectively, AGG is a constant,Pv and P2v are the intensity of the fundamental wave andof its second harmonic, respectively, and IGG(b G

v , b G2v) is

the overlap integral between the polarization wave withfrequency 2v and the SH guided mode:

IGG~bGv , bG

2v!

5 E dijkEjv~x, bG

v !Ekv~x, bG

v !Ei2v~x, bG

2v!dx, (2)

where dijk is the quadratic susceptibility tensor.In the guided–guided SHG, for a given propagation di-

rection, the propagation constants bGv and bG

2v cannot bechanged, and thus the overlap integral IGG(b G

v , b G2v) is a

constant. The factor sin c2 [(bG2v22bG

v L/2] is responsiblefor reducing the SHG efficiency if the wave-vector-matching condition bG

2v 5 2bGv is not satisfied.

Fig. 2. Guided-mode field at v in waveguide 1 at u 5 16.5°.The solid curve corresponds to Im Ex(x). The dotted anddashed curves correspond to Re Ey and Re Ez , respectively.

D. V. Petrov Vol. 14, No. 2 /February 1997 /J. Opt. Soc. Am. B 333

In guided-radiation-mode SHG the amplitude of the ra-diation mode with propagation constant bR

2v (the spectralamplitude) is given by10

B~bGv , bR

2v , L !

5 AGRPvIGR~bG

v , bR2v!L

sin@~bR2v 2 2bG

v !L/2#

@~bR2v 2 2bG

v !L/2#,

IGR~bGv , bR

2v!

5 E dijkEjv~x, bG

v !Ekv~x, bG

v !Ei2v~x, bR

2v!dx,

(3)

where AGR is a constant and IGR(b Gv , b R

2v) is the overlapintegral. The efficiency of the SHG of this radiationmode (the spectral efficiency) becomes

uB~bGv , bR

2v , L !u2

5 AGR2 ~Pv!2L2uIGR~bG

v , bR2v!u2

sin2@~bR2v 2 2bG

v !L/2#

@~bR2v 2 2bG

v !L/2#2.

(4)

The total power of a SH wave is the integral ofuB(b G

v , b R2v , L)u2 over bR

2v:

P2v~W/m ! 5 E2`

`

uB~bGv , bR

2v , L !u2dbR2v . (5)

The spatial distribution of the radiation field is givenby

E2v~x, z, t, L ! 5 E B~bGv , bR

2v , L !E~x, bR2v!

3 exp@i~2vt 2 bR2vz !#dbR

2v , (6)

where E(x, b R2v) is the field distribution of the radiation

mode with propagation constant bR2v.

In the guided-radiation mode SHG the factorsin c@(bR

2v 2 2bGv)L/2# defines the range of the propagation

constants of the radiation modes involved in the SHG.Because bR

2v can take arbitrary values, the overlap inte-gral IGR(b G

v , b R2v) is a function of bR

2v.In waveguides, where leaky waves cannot exist, the

overlap integral IGR(b Gv , b R

2v) depends only slightly onbR2v.10,11 In this case the half-width of the spatial distri-

bution of the radiating SH beam is reduced by an increaseof L. The main lobe of the SH energy distribution is di-rected into the substrate under the Cerenkov angle urad5 arccos@2bG

v/(ko2vno

2v)#. Integrating Eq. (5) in this case,one obtains that the efficiency of the Cerenkov-type SHGP2v is proportional to the interaction length L, not L2, asfor the guided–guided SHG.As is shown below, the overlap integral IGR(b G

v , b R2v)

by a given bGv has a maximum at bR

2v 5 bLW2v

5 ko2v Re@NTE

2v(u)#. The value of the overlap integral de-creases considerably as bR

2v deviates from bLW2v . The

half-width of the overlap integral depends mainly on theloss coefficient of the leaky wave. The angular distribu-tion of the radiation field P2v(b R

2v)/Pv is determined bythe interaction length L and by the relative position of themaximum of IGR(b G

v , b R2v) and the maximum of the

phase-mismatch function sin c2@(bR2v 2 2bG

v)L/2#. The

width of the phase-mismatch function is equal tokv@NR(2v) 2 NG(v)# 5 p/L, and at the fundamentalwavelength of 1 mm and by the interaction length of L5 1 cm it corresponds to DN 5 @NR(2v) 2 NG(v)#5 5 3 1025. As we shall see below, the width of theoverlap integral as a function of the radiation mode’s ef-fective RI may be comparable with the width of the phase-mismatch function. However, this cannot be so either inthe guided–guided interaction (where the overlap func-tion is the d function) or in the SHG of conventional ra-diation modes (where the overlap integral is almost con-stant over the width of the phase-mismatch function).

3. NUMERICAL SIMULATIONWaveguides in anisotropic materials such LiNbO3 andKTiOPO4, produced by different diffusion processes, areused now in many applications, in particular for SHG inthe form of Cerenkov radiation and all-optical switchingusing cascading processes. Below we numerically simu-late the proposed type of SHG, assuming a graded-indexprofile distribution inside an anisotropic waveguide layer.Knowledge of the radiation mode field of such a wave-

guide is required. The set of radiation modes for a step-index slab waveguide is well known for both isotropic andanisotropic waveguides.24 Until now this set had beenused by a description of the SHG radiation processes ingraded-index waveguides.10,11 Here we apply a directnumerical procedure to evaluate the normalized radiationmode field of an anisotropic optical waveguide with arbi-trary ordinary and extraordinary index profiles.

A. Radiation Modes of an Anisotropic Graded-IndexWaveguideThe method employs an idea suggested in Ref. 18 bysearching for a leaky-mode field distribution for an aniso-tropic waveguide. Although in the proposed methodthere are no restrictions on the waveguide’s parametersand material symmetry, a waveguide on the X-cut surfaceof a negative birefringent crystal is considered [Fig. 1(a)].The crystal optic axis Z is placed in the waveguide plane,forming an angle u with a mode propagation direction z.The nonvanished components of the dielectric tensor aree11(x) 5 no

2(x), e22(x, u) 5 no2(x)cos2 u 1 ne

2(x)sin2 u, e333 (x, u) 5 ne

2(x)cos2 u 1 no2(x)sin2 u, and e23(x, u)

5 @ne2(x) 2 no

2(x)#cos u sin u, where no(x) 5 no 1 Dno3 (x) and ne(x) 5 ne 1 Dne(x) are the ordinary (o) andthe extraordinary (e) RI distributions in the waveguide,no,e are the o and e RI’s in the depth (i.e., at x ! 0), andDno,e(x) are the profile functions of o and e RI’s[Dno,e(x) 5 0 at x ! 0] [Fig. 1(b)].The longitudinal components of the fields Ez and Hz

can be represented as

H Ez~x, z, t !Hz~x, z, t !

J 5 H Ez~x !

Hz~x !J exp@i~vt 2 bRz !#, (7)

where N is the effective RI, bR 5 k0N is the propagationconstant, and k0 is the wave number in vacuum. Unlikein leaky waves, N for radiation modes is a real number.A radiation mode with ne(u) , N , no is the wave of hy-brid polarization. [Here ne

22(u) 5 no22 sin2 u 1 ne

22

3 cos2 u.] The field of extraordinary polarization oscil-

334 J. Opt. Soc. Am. B/Vol. 14, No. 2 /February 1997 D. V. Petrov

lates inside the waveguide layer and decreases exponen-tially in the substrate. The field of ordinary polarizationoscillates in both the waveguide layer and the substrate.We consider below only this type of radiation mode. Theair radiation modes with effective RI’s of less than unityhave no influence on the mode coupling considered here.We assume that the same argument applies to the sub-strate radiation modes with both ordinary and extraordi-nary fields oscillating in the substrate.At x ! 0 the longitudinal component of the field is

given by

Ez~x ! 5 ao2 exp~2igox ! 1 ao

1 exp~igox !

1 ae exp~gex !, (8)

where go 5 ko(no2 2 N2)1/2 and ge 5 ko(ne

2 cos2 u 1 no2

3 sin2 u)1/2no21@N2 2 ne

2(u)#1/2. ao2 , ao

1 , and ae are ar-bitrary constants. Other components of the electric andmagnetic fields are determined with the help of Maxwell’sequations. Unlike the field of the leaky wave in Ref. 18,field (8) includes the contribution ao

2 exp(2igox), whichdescribes a plane wave propagating from infinity to thewaveguide layer.The longitudinal components of the field inside the

waveguide layer are governed by four ordinary differen-tial equations, which follow from Maxwell’s equations:

]Ey~x !/]x 5 2ik0Hz~x !,

]Ez~x !/]x 5 ik0no22~x !@e11~x, u! 2 N2#Hy~x !,

]Hy~x !/]x 5 ik0e33~x, u!Ez~x ! 1 ik0e23~x, u!Ey~x !,

]Hz~x !/]x 5 2ik0@e22~x, u! 2 N2#Ey~x !

2ik0e23~x, u!Ez~x !. (9)

Using Eq. (8) as an initial condition by some set of theamplitudes ao

2 , ao1 , and ae (for example, ao

2 5 ao1

5 ae 5 1), we solve this system of equations numeri-cally, and the field is determined at any point of the wave-guide, including at the interface waveguide–air. Invacuum (x . 0) the tangential components of the fieldhave analytical solutions Ey(x) 5 A exp(2k0sx), Hy(x)5 B exp(2k0sx), Ez(x) 5 isB exp(2k0sx), and Hz(x)5 isA exp(2k0sx). Here A and B are arbitrary con-stants and s 5 (N2 2 1)1/2.The boundary conditions at x 5 0 are reduced to the

system of algebraic equations

F E y1o~0 !

E z1o~0 !

H y1o~0 !

H z1o~0 !

E y2o~0 !

E z2o~0 !

H y2o~0 !

H z2o~0 !

E ye~0 !

E ze~0 !

H ye~0 !

H ze~0 !

2100isG 3 F a01ao2ae

AG

5 F 0is10G 3 B. (10)

Here, for example, E z2o(0) 3 ao

2 means the value of thez component of the electric field at the interfacewaveguide–vacuum that originates from the initial condi-tion Ez(x) 5 ao

2 exp(2igox) at x ! 0. Unlike for theleaky-wave solution,10 we have no dispersion relation

leading to the discrete (complex) values of N, and wechoose N as an independent continuous variable. Thesystem of Eqs. (10) allows one to find the relationshipsamong the amplitudes ao

2, ao1, and ae and hence the ra-

diation mode field in the waveguide apart from a constantthat depends on the power normalization. For the nor-malization of the radiation modes the d function should beused24:

E2`

`

@E t,N8* ,~x ! 3 Ht,N~x ! 1 E t,N~x ! 3 H t,N8

* ~x !#dx

5 Pd~N 2 N8!, (11)

where P is the power flow per unit length and t refers thetransverse (x- and y-) field components.This type of normalization was described before only

for step-index slab waveguides, for which the d functioncan be recognized in Eq. (11) after substitution of analyti-cal expressions of the mode’s field.24 In our case of a nu-merical solution we find the normalization coefficientfrom an asymptotic expression for the field at x ! 0, aswas proposed in quantum mechanics for the normaliza-tion of the wave functions of continuous spectra.26

We can replace the field in Eq. (11) by its asymptoticvalue [Eq. (8)] for large negative x, taking as a lower limitof integration any finite value of x (say, zero). Thisamounts to neglecting a finite quantity rather than an in-finite one. The asymptotic form of the z component isEz(x ! 0) 5 2uao

1ucos(go x 2 f), where f is the phase.The integration of Eq. (11) gives the relationship betweenP and uao

1u 5 uao2u:

P 5 2Nuao1u2@1 1 ~kno tan u/go!

2#/tan2 u. (12)

B. Overlap Integral IGR(b Gv , b R

2v)The overlap integral IGR(b G

v , b R2v) determines the main

characteristics of the SH radiation field: the SHG effi-ciency and the angular distribution of the SH wave. Icalculated this integral for two-waveguides with differentparameters. The fundamental wavelength of 1.3 mm wasused.Parameters of the waveguide 1 (see Table 1) were cho-

sen in such a way that us and uc would be almost thesame. In this case the wave-vector-matching condition2bG

v 5 ko2v Re@NTE

2v(u)# is satisfied for a leaky wave with alarge loss coefficient. us is equal to 16.5°. The effectiveRI of the guided quasi-TM mode at v (2.19145) was foundby the shooting method.27 The nonzero components ofthe electric field are shown in Fig. 2. The x componentcontributes mainly in the field, i.e., the wave at v has aquasi-TM polarization.The field distribution of the SH radiation mode propa-

gated along u 5 16.5° was calculated for different N5 bR

2v/ko2v (Fig. 3). The y component of the electric field

increases strongly near N 5 2.19154, which is equal tothe real part of the effective RI of the leaky wave. Theamplitudes of the x and the z components do not changeessentially in the range of N used by the calculations.Hence the quasi-TE contribution concentrates its energyinside the waveguide layer. For radiation modes with Ndifferent from 2.19154 the main contribution in the field

D. V. Petrov Vol. 14, No. 2 /February 1997 /J. Opt. Soc. Am. B 335

Table 1. Waveguide’s Parameters Used in Calculations

Parameters Waveguide #1 Waveguide #2

lv 5 1.3 mm ne(x) 5 2.00 1 0.01 exp@2(x/2.6 mm)2# 2.1459 1 0.01 exp@2(x/2.6 mm)2#

no(x) 5 2.19 1 0.01 exp@2(x/2.6 mm)2# 2.2205 1 0.01 exp@2(x/2.6 mm)2#

l2v 5 0.65 mm ne(x) 5 2.05 1 0.01 exp@2(x/2.6 mm)2# 2.1989 1 0.01 exp@2(x/2.6 mm)2#

no(x) 5 2.20 1 0.01 exp@2(x/2.6 mm)2# 2.2819 1 0.01 exp@2(x/2.6 mm)2#

NTMv 2.19145 2.22211

us 16.5° 61.5°a(us) (cm21) 37 1.7Width of

IGR(b Gv , b R

2v)4.6 3 1024 4.0 3 1025

Maximum ofIGR(b G

v , b R2v)

0.78 7.9

has quasi-TM polarization. The fields of these modes os-cillate inside the waveguide layer.I evaluated the leaky-wave loss coefficient a

5 2ko2v Im@NTE

2v(u)# (Fig. 4), using the approximativeWKB expression from Refs. 16 and 17. For this wave-guide uc 5 9.8° and the loss coefficient is to 37 cm21 atu 5 16.5°.The dependence of IGR(b G

v , b R2v) on b R

2v/k o2v is shown

in Fig. 5. As expected, the integral has a maximum near2.19154, and the width of this curve, found by the Lorent-zian approximation, is to 4.6 3 1024.

Fig. 3. Distribution of the SH radiation mode field with differ-ent propagation constants (u 5 16.5°) (waveguide 1).

The parameters of waveguide 2 (see Table 1) were cho-sen as follows: The substrate’s RI’s are equal to the cor-responding values of LiNbO3.

24 A RI increase of 0.01and a diffusion depth of 2.6 mm were assumed by calcula-tions. These values are close to the experimental ones inLiNbO3 waveguides.The leaky-wave loss coefficient, the nonzero compo-

nents of the SH wave field, and the overlap integral areshown in Figs. 4, 6, and 5(b), respectively. The electricfield distribution of the wave at v is almost the same asfor waveguide 1. The SH radiation mode field changesconsiderably: the ratio of the quasi-TE component Ey(x)and the quasi-TM components [Ex(x) and Ez(x)] growsnear the maximum of Ey(x), which means that the radia-tion mode field with N 5 2.22211 is almost the same asfor any guided mode.

4. DISCUSSIONAs was predicted by the model proposed, the numericalsimulation shows a strong dependence of the overlap in-tegral on the propagation constant of the SH radiationmodes. This is an essential difference from the conven-tional Cerenkov-type SHG.10,11 For a given propagation

Fig. 4. Leaky-mode loss coefficient a versus propagation angle ufor 1, waveguide 1 and 2, waveguide 2. The points show the val-ues at the propagation angles for which the overlap integralswere calculated.

336 J. Opt. Soc. Am. B/Vol. 14, No. 2 /February 1997 D. V. Petrov

direction the range of bR2v where the overlap integral is

large depends on the leaky-wave loss coefficient. In fact,the difference in the widths of the curves in Figs. 5(a) and5(b) is ;1 order of magnitude. As shown in Fig. 4, a forwaveguide 1 (37 cm21) is ;20 times larger than for wave-guide 2 (1.7 cm21).The overlap integral in waveguide 2, where the leaky-

wave loss coefficient is small, depends strongly on thepropagation constant. Consequently we can consider themaximal value of this integral as the value of the overlapintegral in the guided–guided interaction. (In guided–guided SHG this dependence is described by the d func-tion.) The maximum value of the overlap integral is;1 order of magnitude less in waveguide 1 than in wave-guide 2. Nevertheless, it is much larger than the overlapintegral for radiation modes with propagation constantsother than that of the leaky wave. (For example, inwaveguide 1 the overlap integral is 0.09 for the radiationmode with N 5 2.1935, whereas the maximum value ofthe overlap integral is 0.78; i.e., the value of the overlapintegral decreases approximately eight times by detuningof ;DN 5 0.002. For the same detuning in waveguide 2the reduction is ;15 times.)Cerenkov-type SHG efficiency strongly depends on the

choice of optical parameters (diffusion depth and maxi-mum value of the refractive index in the waveguide; see,for example, Refs. 10 and 11). The proper choice of theseparameters can satisfy the wave-vector-matching condi-tion by u ' uc with a large value of the overlap integral.In this case the width of the overlap function should in-

Fig. 5. (a) Overlap integral versus propagation constant of theSH radiation mode. (b) Overlap integral for waveguide 2 shownon a different scale. Dotted curves represent the Lorentzian ap-proximation.

crease, but the SHG efficiency is still comparable with theguided–guided SHG efficiency. The wave-vector-matching condition will not be so strictly important formaintaining high efficiency because the width of the over-lap integral function is broad.Consider now the angular spectrum of the radiation

modes. Even without calculation of the final integral[Eq. (6)] one can see that the angular distribution of theradiation field E2v(x, z, t, L) is determined by L and bythe relative position of the maximum of IGR(b G

v , b R2v)

and the maximum of sin c2@(bR2v 2 2bG

v)L/2#. If the peaksof these two functions of bR

2v are not coincident (bR2v

5 2bGv Þ bLW

2v ), for small L the radiation modes with bR2v

in the vicinity of bLW2v provide the main contribution to the

total radiation field at 2v. The main lobe of the radiationfield is directed into the substrate under the angle u*5 arccos@bLW

2v /(ko2vno

2v)# (Fig. 7). However, as L in-creases, the half-width of the function sin c2@(bR

2v

2 2bGv)L/2# becomes narrow, and the radiation modes

with bR2v in the vicinity of the phase-matching point 2bG

v

provide the main contribution to the total radiation fieldat 2v. The SH wave radiates into the substrate mainlyunder the angle urad (see Fig. 7). Obviously this shiftdoes not occur when the peaks of the two above-

Fig. 6. Distribution of the SH radiation mode field with differ-ent propagation constants (u 5 61.5°) (waveguide 2).

D. V. Petrov Vol. 14, No. 2 /February 1997 /J. Opt. Soc. Am. B 337

Fig. 7. Radiation of the SH wave into the substrate for (a)DbL ! 1 and (b) DbL @ 1. Db 5 (bR

2v 2 2bGv ). The solid ar-

rows are the double wave vector at v; the dashed arrows are thewavevector of the SH wave.

Fig. 8. Product f(bR2v) 5 IGR(b G

v , b R2v) 3 sin c2@(bR

2v 2 2bGv)

3 L/2] as a function of bR2v for different interaction lengths

L: (a) 2bGv Þ bLW

2v , (b) 2bGv 5 bLW

2v .

mentioned functions are coincident. Hence the overlapintegral IGR(b G

v , b R2v) is responsible in our case for the

efficiency of the SHG as well as for the angular distribu-tion of the radiating SH field. In conventional Cerenkov-type SHG in the waveguide2,10 the main lobe of the radi-ating field distribution becomes narrow with increasinginteraction length, but it does not change its direction.The product sin c2@(bR

2v 2 2bGv)L/2#IGR(b G

v , bR2v) as a

function of the propagation constants of the SH radiationmode is shown in Fig. 8 for different interaction lengths.As this figure shows, if the wave-vector-matching condi-tion is not satisfied (2bG

v Þ bLW2v ) the radiation field with

propagation constant bLW2v radiates into the substrate for

small interaction lengths @(bR2v 2 2bG

v )L ! 1#. As (bR2v

2 2bGv )L @ 1, the SH radiation field has the propagation

constant 2bGv . In an intermediate range of the interac-

tion lengths the radiation field can form two or morebeams. If 2bG

v 5 bLW2v [Fig. 8(b)] the radiation field has

the propagation constant 2bGv for any interaction length.

5. CONCLUSIONSecond harmonic generation in an anisotropic opticalwaveguide has new features if leaky waves are involvedin the interaction. In particular, Cerenkov-type SHG ef-ficiency can be comparable with the SHG efficiency of twoguided modes, and it can be observed without critical con-trol of the phase-matching condition. The direction ofthe main lobe of the Cerenkov radiation field distributiondepends on the interaction length and the initial choice ofthe propagation direction. These results can be used inthe construction of short-wavelength light sources, gen-eration of ultrashort second-harmonic pulses, and studyof x(2):x(2) cascading process.

ACKNOWLEDGMENTThis research was supported by the Brazilian AgencyConselho Nacional de Desenvolvimento Cientıfıco e Tech-nologico.Permanent address, The Institute of Semiconductor

Physics, 630090, Novosibirsk, Russia; current address,Department of Signal Theory and Communications, Uni-versitat Politecnica de Catalunya, UPC-D3, 08034, Barce-lona, Spain.

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