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Spin Liquid Phases ?
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Valence Bond Crystals Valence Bond Crystals
A si
mple way to overcome frustration
Crystal of singlets
Fully optimized bonds and absence of m.-f. interactions
How to overcome effect of frustration ?
4-spin S=0 state
J.B.Fouet et al. 2002, W. Brenig 2002
P. Sindzingre 2003, E. Berg et al 2003
LRO in singlet-singlet correl. fonct.
(crystal)
Modes of gapped excitations:
integer(S=1, 0 excitations
A product of singlet wave functions
is a good app. of the N. body g.-s.
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Quantum Spin Liquids
No spin-spin long range order
Singlet-singlet long range order
Gapful spin integer excitations
No LRO in spins
No LRO in dimers
and in any local correlation fctn
Specificity of the g.-s. w.-f.
Fractionalized spin excitations
may be gapful or gapless
Valence Bond Crystals
e T(
wG
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Quantum Spin LiquidsResonating Valence Bond Liquids
+
EN )21( E+ terms
P.W. Anderson, L. Balents,
V. Elser, M.P.A. Fisher,
E. Fradkin, S. Kivelson,
C.L., G. Misguich,
R. Moessner, S. L. Sondhi
V. Pasquier, N. Read,D. Rokhsar, D. Sutherland, S.
Sachdev, S. Senthil,
D. Serban, P. Sindzingre
.
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Quantum Spin LiquidsResonating Valence Bond Liquids
+
EN )21( E+ terms
No LRO in any local correlation
fonctions (liquid) , spin gap
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Quantum Spin LiquidsResonating Valence Bond Liquids
+
EN )21( E+ terms
No LRO in any local correlation
fonctions (liquid), spin gap
Continuum of gapped unconfined
spin excitations (spinons)
By alphabetic order:
P.W. Anderson,
L. Balents,
M.P.A. Fisher,
E. Fradkin,
S. Kivelson,N. Read,
S. Sachdev,
S. Senthil..
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confined spinons in the
V-B crystal
unconfined spinons in
the R.V.B. Spin Liquids
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Quantum Spin LiquidsResonating Valence Bond Liquids
+
EN )21( E+ terms
No LRO in any local correlation
fonctions (liquid) , spin gap
Continuum of gapped unconfined
spin excitations (spinons)
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Quantum Spin LiquidsResonating Valence Bond Liquids
+
EN )21( E+ terms
No LRO in any local correlation
fonctions (liquid) , spin gap
Continuum of gapped unconfined
spin excitations (spinons)
Subtle phase coherence properties
(Quantum liquid)
and S=0 visons excitations
An exactly solvable
dimer liquid model
Ising gauge theory
G. Misguich et al. 02
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Misguich et aldimer model (02)
only kinetic energy: sum from 3 to six dimer moves around eachhexagon of the kagome lattice
3
6
4
H = 7 dimer moves from black to red config. + h.c.
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Misguich et aldimer model (02)
only kinetic energy: sum from 3 to six dimer moves around eachhexagon of the kagome lattice
3
6
4
H = 7 dimer moves from black to red config. + h.c.
3
6
4
H
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Coherence Effects and S=0 Visons excitationsG. Misguich V. Pasquier & D. Serban P.R.L.02
The Resonating Valence Bond ground-state:
+ .++
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Coherence Effects and S=0 Visons excitationsG. Misguich V. Pasquier & D. Serban P.R.L.02
The Resonating Valence Bond ground-state:
b
a
An S=0 gapped excitation: the two-visons wave-function
.+-
+ .++
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Quantum Spin LiquidsResonating Valence Bond Liquids
+
EN )21( E+ terms
No LRO in any local correlation
fonctions (liquid)
Continuum of gapped unconfined
spin excitations (spinons)
Subtle phase coherence properties
(Quantum liquid)
and S=0 gapped visons excitations
Topological degeneracy
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MSE Spin Liquid Spin gap & Topological degeneracy
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MSE Spin Liquid Spin gap & Topological degeneracy
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MSE Spin Liquid Spin gap & Topological degeneracy
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MSE Spin Liquid Spin gap & Topological degeneracy
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Topological degeneracy in SRRVB Spin
Liquids
a generic g.-s. configuration
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Topological degeneracy in SRRVB Spin
Liquids
a generic g.-s. configuration
draw an arbitrary cut
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Topological degeneracy in SRRVB Spin
Liquids
;x= 3
a generic g.-s. configuration
draw an arbitrary cut
count the number of dimers
across the cut
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Topological degeneracy in SRRVB Spin
Liquids
;x= 3 ;
x=1
Pijkl
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Topological degeneracy in SRRVB Spin
Liquids
;x= 3 ;
x=1
Parities of winding numbers (;x,;y) are good quantum numbers:
4 unconnected topological subspaces on a 2-torus
degenerate in the thermodynamic limit
Pijkl
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Topological degeneracy in SRRVB Spin
Liquids
;x= 3 ;
x=1
Parities of winding numbers (;x,;y) are good quantum numbers:
4 unconnected topological subspaces on a 2-torus
degenerate in the thermodynamic limit
4-fold degeneracy of low lying singlets
Pijkl
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Topological degeneracy in SRRVB Spin
Liquids
;x= 3 ;
x=1
Parities of winding numbers (;x,;y) are good quantum numbers:
4 unconnected topological subspaces on a 2-torus
degenerate in the thermodynamic limit
4-fold degeneracy of low lying singlets
A topological quantum bit (Kitaev quant-phys/9707021) ?
Pijkl
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Quantum Spin LiquidsResonating Valence Bond Liquids
+
EN )21( E+ terms
No LRO in any local correlation
fonctions (liquid)
Continuum of gapped unconfined
spin excitations (spinons)
Subtle phase coherence properties
(Quantum liquid)
and S=0 gapped visons excitations
Topological degeneracy
A topological quantum-bitA. Y. Kitaev 97, 03
L. Ioffe and coll. 02
G. Misguich et al 04
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Quantum Spin LiquidsResonating Valence Bond Liquids
+
EN )21( E+ terms
No LRO in any local correlation
fonctions (liquid)
Continuum of gapped unconfined
spin excitations (spinons)
Subtle phase coherence properties
(Quantum liquid)
and S=0 gapped visons excitations
Topological degeneracy
A topological quantum-bit
What seems the most favorable
conditions to observe
Quantum Spin Liquids?
triangular geometry
importance of effective kinetic
terms acting coherently on
more than two spins
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H = t ++ + ...+ ... + V
on the triangular lattice 00
MoessnerSondhi hard core quantum dimer model
V / t0 1
12 x 12 SRRVBVBC VBC
On the square lattice the original model due to Rokhsar & Kivelson
has no real spin liquid phase only a Q.C. point
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Kagom-like ?
SR-RVB
Gapless LR-RVB ?
H = 2 J2 7< i,j> Si . Sj+ J4 7 (Pijkl+ P-1
ijkl )
on the triangular lattice
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Quantum behavior of models with
infinite local degeneracy in the
classical limitHeisenberg model on the kagom
checkerboard and pyrochlore lattices
Half integer odd spins versus integer ones
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Classical Heisenberg Hamiltonian on
the kagom lattice
An infinite number of soft modes, an infinite T=0 degeneracy
Same property on the checkerboard lattice, or the pyrochlore lattice
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Quantum ground-state and first excitations
of the Heisenberg model on the kagom lattice
have a total spin S=0
A gap < 10 -3 in the singlet
sector(if any)!
Very large extensive entropy
from singlets at ultra-low T
A small spin gap (~1/20)
At low temperature Cv is insensitive to large magnetic fields
( Sindzingre et al.. PRL 00 , Ramirez et al.. PRL 00)
pTCv!butT(w )exp(G
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Spin-3/2 kagom Antiferromagnet
No theoretical results
Experiments: the spin liquid picture is plausible.
Some features are very much alike the spin-1/2 system
Dynamics of spins (Uemura et al 1994)
Low lying local singlet excitations (Ramirez et al. 2000)
A very tiny spin gap if any (Ramirez et al, Bono, Mendels et al.)
Quasi-critical behavior of the spin susceptibility atintermediate temperatures (C. Mondelli, H. Mutka and coll.
2002, A. Georges and coll. 2001)
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Conclusion
SU(2) magnets in 2d
Semi-classical Nel phases
Quantum phases: Valence Bond Crystals and Spin
Liquids
Quantum Spin Liquids
A Realistic Spin Liquid : MSE on triangular latt.
Open question: spin-1/2-Heisenberg model on the
kagom lattice. A true new phase or a system near aQ.C. point?
Half-odd integer spins versus integer ones
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A toy model for a topological quantum-bitG. Misguich, V. Pasquier, F. Mila, C.L. cond-mat/0410693
Z2 spin liquid on a cylinder: 2-fold degenerate g.s.
a topological q-bit
protected from any local perturbations
How write and read it?
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A toy model for a topological quantum-bitG. Misguich, V. Pasquier, F. Mila, C.L. cond-mat/0410693
Z2 spin liquid on a cylinder: 2-fold degenerate g.s.
a topological q-bit
protected from any local perturbations
How write and read it?
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A toy model for a topological quantum-bitG. Misguich, V. Pasquier, F. Mila, C.L. cond-mat/0410693
Z2 spin liquid on a cylinder: 2-fold degenerate g.s.
a topological q-bit
protected from any local perturbations
How write and read it?
Introduce a local perturbation
which change the geometry
from a cylinder to a plane
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A toy model for a topological quantum-bitG. Misguich, V. Pasquier, F. Mila, C.L. cond-mat/0410693
Z2 spin liquid on a cylinder: 2-fold degenerate g.s.
a topological q-bit
protected from any local perturbations
How write and read it?
gap
perturbationVc
exp(-L)
1/L