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Spin Liquid Phases?

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    Spin Liquid Phases ?

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    Valence Bond Crystals Valence Bond Crystals

    A si

    mple way to overcome frustration

    Crystal of singlets

    Fully optimized bonds and absence of m.-f. interactions

    How to overcome effect of frustration ?

    4-spin S=0 state

    J.B.Fouet et al. 2002, W. Brenig 2002

    P. Sindzingre 2003, E. Berg et al 2003

    LRO in singlet-singlet correl. fonct.

    (crystal)

    Modes of gapped excitations:

    integer(S=1, 0 excitations

    A product of singlet wave functions

    is a good app. of the N. body g.-s.

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    Quantum Spin Liquids

    No spin-spin long range order

    Singlet-singlet long range order

    Gapful spin integer excitations

    No LRO in spins

    No LRO in dimers

    and in any local correlation fctn

    Specificity of the g.-s. w.-f.

    Fractionalized spin excitations

    may be gapful or gapless

    Valence Bond Crystals

    e T(

    wG

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    Quantum Spin LiquidsResonating Valence Bond Liquids

    +

    EN )21( E+ terms

    P.W. Anderson, L. Balents,

    V. Elser, M.P.A. Fisher,

    E. Fradkin, S. Kivelson,

    C.L., G. Misguich,

    R. Moessner, S. L. Sondhi

    V. Pasquier, N. Read,D. Rokhsar, D. Sutherland, S.

    Sachdev, S. Senthil,

    D. Serban, P. Sindzingre

    .

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    Quantum Spin LiquidsResonating Valence Bond Liquids

    +

    EN )21( E+ terms

    No LRO in any local correlation

    fonctions (liquid) , spin gap

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    Quantum Spin LiquidsResonating Valence Bond Liquids

    +

    EN )21( E+ terms

    No LRO in any local correlation

    fonctions (liquid), spin gap

    Continuum of gapped unconfined

    spin excitations (spinons)

    By alphabetic order:

    P.W. Anderson,

    L. Balents,

    M.P.A. Fisher,

    E. Fradkin,

    S. Kivelson,N. Read,

    S. Sachdev,

    S. Senthil..

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    confined spinons in the

    V-B crystal

    unconfined spinons in

    the R.V.B. Spin Liquids

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    Quantum Spin LiquidsResonating Valence Bond Liquids

    +

    EN )21( E+ terms

    No LRO in any local correlation

    fonctions (liquid) , spin gap

    Continuum of gapped unconfined

    spin excitations (spinons)

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    Quantum Spin LiquidsResonating Valence Bond Liquids

    +

    EN )21( E+ terms

    No LRO in any local correlation

    fonctions (liquid) , spin gap

    Continuum of gapped unconfined

    spin excitations (spinons)

    Subtle phase coherence properties

    (Quantum liquid)

    and S=0 visons excitations

    An exactly solvable

    dimer liquid model

    Ising gauge theory

    G. Misguich et al. 02

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    Misguich et aldimer model (02)

    only kinetic energy: sum from 3 to six dimer moves around eachhexagon of the kagome lattice

    3

    6

    4

    H = 7 dimer moves from black to red config. + h.c.

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    Misguich et aldimer model (02)

    only kinetic energy: sum from 3 to six dimer moves around eachhexagon of the kagome lattice

    3

    6

    4

    H = 7 dimer moves from black to red config. + h.c.

    3

    6

    4

    H

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    Coherence Effects and S=0 Visons excitationsG. Misguich V. Pasquier & D. Serban P.R.L.02

    The Resonating Valence Bond ground-state:

    + .++

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    Coherence Effects and S=0 Visons excitationsG. Misguich V. Pasquier & D. Serban P.R.L.02

    The Resonating Valence Bond ground-state:

    b

    a

    An S=0 gapped excitation: the two-visons wave-function

    .+-

    + .++

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    Quantum Spin LiquidsResonating Valence Bond Liquids

    +

    EN )21( E+ terms

    No LRO in any local correlation

    fonctions (liquid)

    Continuum of gapped unconfined

    spin excitations (spinons)

    Subtle phase coherence properties

    (Quantum liquid)

    and S=0 gapped visons excitations

    Topological degeneracy

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    MSE Spin Liquid Spin gap & Topological degeneracy

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    MSE Spin Liquid Spin gap & Topological degeneracy

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    MSE Spin Liquid Spin gap & Topological degeneracy

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    MSE Spin Liquid Spin gap & Topological degeneracy

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    Topological degeneracy in SRRVB Spin

    Liquids

    a generic g.-s. configuration

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    Topological degeneracy in SRRVB Spin

    Liquids

    a generic g.-s. configuration

    draw an arbitrary cut

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    Topological degeneracy in SRRVB Spin

    Liquids

    ;x= 3

    a generic g.-s. configuration

    draw an arbitrary cut

    count the number of dimers

    across the cut

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    Topological degeneracy in SRRVB Spin

    Liquids

    ;x= 3 ;

    x=1

    Pijkl

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    Topological degeneracy in SRRVB Spin

    Liquids

    ;x= 3 ;

    x=1

    Parities of winding numbers (;x,;y) are good quantum numbers:

    4 unconnected topological subspaces on a 2-torus

    degenerate in the thermodynamic limit

    Pijkl

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    Topological degeneracy in SRRVB Spin

    Liquids

    ;x= 3 ;

    x=1

    Parities of winding numbers (;x,;y) are good quantum numbers:

    4 unconnected topological subspaces on a 2-torus

    degenerate in the thermodynamic limit

    4-fold degeneracy of low lying singlets

    Pijkl

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    Topological degeneracy in SRRVB Spin

    Liquids

    ;x= 3 ;

    x=1

    Parities of winding numbers (;x,;y) are good quantum numbers:

    4 unconnected topological subspaces on a 2-torus

    degenerate in the thermodynamic limit

    4-fold degeneracy of low lying singlets

    A topological quantum bit (Kitaev quant-phys/9707021) ?

    Pijkl

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    Quantum Spin LiquidsResonating Valence Bond Liquids

    +

    EN )21( E+ terms

    No LRO in any local correlation

    fonctions (liquid)

    Continuum of gapped unconfined

    spin excitations (spinons)

    Subtle phase coherence properties

    (Quantum liquid)

    and S=0 gapped visons excitations

    Topological degeneracy

    A topological quantum-bitA. Y. Kitaev 97, 03

    L. Ioffe and coll. 02

    G. Misguich et al 04

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    Quantum Spin LiquidsResonating Valence Bond Liquids

    +

    EN )21( E+ terms

    No LRO in any local correlation

    fonctions (liquid)

    Continuum of gapped unconfined

    spin excitations (spinons)

    Subtle phase coherence properties

    (Quantum liquid)

    and S=0 gapped visons excitations

    Topological degeneracy

    A topological quantum-bit

    What seems the most favorable

    conditions to observe

    Quantum Spin Liquids?

    triangular geometry

    importance of effective kinetic

    terms acting coherently on

    more than two spins

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    H = t ++ + ...+ ... + V

    on the triangular lattice 00

    MoessnerSondhi hard core quantum dimer model

    V / t0 1

    12 x 12 SRRVBVBC VBC

    On the square lattice the original model due to Rokhsar & Kivelson

    has no real spin liquid phase only a Q.C. point

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    Kagom-like ?

    SR-RVB

    Gapless LR-RVB ?

    H = 2 J2 7< i,j> Si . Sj+ J4 7 (Pijkl+ P-1

    ijkl )

    on the triangular lattice

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    Quantum behavior of models with

    infinite local degeneracy in the

    classical limitHeisenberg model on the kagom

    checkerboard and pyrochlore lattices

    Half integer odd spins versus integer ones

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    Classical Heisenberg Hamiltonian on

    the kagom lattice

    An infinite number of soft modes, an infinite T=0 degeneracy

    Same property on the checkerboard lattice, or the pyrochlore lattice

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    Quantum ground-state and first excitations

    of the Heisenberg model on the kagom lattice

    have a total spin S=0

    A gap < 10 -3 in the singlet

    sector(if any)!

    Very large extensive entropy

    from singlets at ultra-low T

    A small spin gap (~1/20)

    At low temperature Cv is insensitive to large magnetic fields

    ( Sindzingre et al.. PRL 00 , Ramirez et al.. PRL 00)

    pTCv!butT(w )exp(G

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    Spin-3/2 kagom Antiferromagnet

    No theoretical results

    Experiments: the spin liquid picture is plausible.

    Some features are very much alike the spin-1/2 system

    Dynamics of spins (Uemura et al 1994)

    Low lying local singlet excitations (Ramirez et al. 2000)

    A very tiny spin gap if any (Ramirez et al, Bono, Mendels et al.)

    Quasi-critical behavior of the spin susceptibility atintermediate temperatures (C. Mondelli, H. Mutka and coll.

    2002, A. Georges and coll. 2001)

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    Conclusion

    SU(2) magnets in 2d

    Semi-classical Nel phases

    Quantum phases: Valence Bond Crystals and Spin

    Liquids

    Quantum Spin Liquids

    A Realistic Spin Liquid : MSE on triangular latt.

    Open question: spin-1/2-Heisenberg model on the

    kagom lattice. A true new phase or a system near aQ.C. point?

    Half-odd integer spins versus integer ones

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    A toy model for a topological quantum-bitG. Misguich, V. Pasquier, F. Mila, C.L. cond-mat/0410693

    Z2 spin liquid on a cylinder: 2-fold degenerate g.s.

    a topological q-bit

    protected from any local perturbations

    How write and read it?

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    A toy model for a topological quantum-bitG. Misguich, V. Pasquier, F. Mila, C.L. cond-mat/0410693

    Z2 spin liquid on a cylinder: 2-fold degenerate g.s.

    a topological q-bit

    protected from any local perturbations

    How write and read it?

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    A toy model for a topological quantum-bitG. Misguich, V. Pasquier, F. Mila, C.L. cond-mat/0410693

    Z2 spin liquid on a cylinder: 2-fold degenerate g.s.

    a topological q-bit

    protected from any local perturbations

    How write and read it?

    Introduce a local perturbation

    which change the geometry

    from a cylinder to a plane

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    A toy model for a topological quantum-bitG. Misguich, V. Pasquier, F. Mila, C.L. cond-mat/0410693

    Z2 spin liquid on a cylinder: 2-fold degenerate g.s.

    a topological q-bit

    protected from any local perturbations

    How write and read it?

    gap

    perturbationVc

    exp(-L)

    1/L


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