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Characterization of the loss of plasmonic modes in planar metalinsulatormetal waveguides by a coupling-simulation approach Chien-I Lin and Thomas K. Gaylord* School of Electrical and Computer Engineering, Georgia Institute of Technology, Atlanta, Georgia 30332-0250, USA *Corresponding author: [email protected] Received 13 October 2009; accepted 12 January 2010; posted 20 January 2010 (Doc. ID 118398); published 10 February 2010 Metalinsulatormetal (MIM) structures have been the subject of great interest as nanoscale plasmonic waveguides. The modeling and measurement of the loss in these waveguides is one of the critical issues in realizing the plasmon-based nanocircuitry. Due to the subwavelength size of the structure, the light injection and the measurement of the loss in MIM structures typically require tapered fibers or wave- guides, as well as multiple waveguide structures with various length scales [8,9] or scanning near-field optical microscopy. The transverse transmission/reflection (TTR) method is presented for determining the loss of plasmonic modes in MIM waveguides. The approach is based on determining the width of the reflection angular spectrum in the attenuated total reflection configuration. Owing to its transverse character, the TTR method potentially provides a more straightforward and simpler way to determine the loss of plasmonic modes in MIM structures. © 2010 Optical Society of America OCIS codes: 230.7370, 240.6680. 1. Introduction During the past few years, surface plasmon (SP)- based waveguides have been the subject of intensive research [16]. Due to the nanometer-scale confine- ment and the slow-wavenature of SP [37], SP- based waveguides have been considered as promising candidates in realizing optical nanocircuitry. How- ever, the loss in plasmonic waveguides is substantial owing to the intrinsic loss of the metal and is further magnified with enhanced transverse modal confine- ment [36], which is essential in integration of SP-based nanocircuitry. Therefore, the design, simu- lation, and measurement of the loss in plasmonic waveguides are critically important in the develop- ment of plasmonic waveguides. The MIM structure is one of the most intensively investigated of plasmonic waveguides. Despite its larger loss compared with its complementary struc- ture, the insulatormetalinsulator (IMI) plasmonic waveguide, the transverse modal size is significantly smaller in the former because of the relatively shal- low field penetration to the skin depth of the metal cladding. Such small penetration also makes the MIM structures less sensitive to interface/surface de- fects, index mismatch of cladding layers, and cross- talk. However, the modal profile of a typical MIM structure is usually below the diffraction limit [35]. Therefore, the excitation and the loss measurement of an MIM plasmonic mode typically requires end- firing of tapered fibers or waveguides, as well as mul- tiple waveguides structures with various length scales [8] or scanning near-field optical microscopy (SNOM) [1012]. The transverse transmission/reflection (TTR) method [13] presented here may significantly simpli- fy the loss measurement of the MIM plasmonic modes. Instead of conceptually injecting light from the end of the waveguides, e.g., finite-difference time-domain (FDTD) simulation [5,14,15], the TTR method excites a plasmonic mode in the transverse 0003-6935/10/060936-09$15.00/0 © 2010 Optical Society of America 936 APPLIED OPTICS / Vol. 49, No. 6 / 20 February 2010
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Page 1: Characterization of the loss of plasmonic modes in planar metal-insulator-metal waveguides by a coupling-simulation approach

Characterization of the loss of plasmonic modesin planar metal–insulator–metal waveguides

by a coupling-simulation approach

Chien-I Lin and Thomas K. Gaylord*School of Electrical and Computer Engineering, Georgia Institute of Technology,

Atlanta, Georgia 30332-0250, USA

*Corresponding author: [email protected]

Received 13 October 2009; accepted 12 January 2010;posted 20 January 2010 (Doc. ID 118398); published 10 February 2010

Metal–insulator–metal (MIM) structures have been the subject of great interest as nanoscale plasmonicwaveguides. Themodeling andmeasurement of the loss in these waveguides is one of the critical issues inrealizing the plasmon-based nanocircuitry. Due to the subwavelength size of the structure, the lightinjection and the measurement of the loss in MIM structures typically require tapered fibers or wave-guides, as well as multiple waveguide structures with various length scales [8,9] or scanning near-fieldoptical microscopy. The transverse transmission/reflection (TTR) method is presented for determiningthe loss of plasmonic modes in MIM waveguides. The approach is based on determining the width ofthe reflection angular spectrum in the attenuated total reflection configuration. Owing to its transversecharacter, the TTR method potentially provides a more straightforward and simpler way to determinethe loss of plasmonic modes in MIM structures. © 2010 Optical Society of America

OCIS codes: 230.7370, 240.6680.

1. Introduction

During the past few years, surface plasmon (SP)-based waveguides have been the subject of intensiveresearch [1–6]. Due to the nanometer-scale confine-ment and the “slow-wave” nature of SP [3–7], SP-basedwaveguides have been considered as promisingcandidates in realizing optical nanocircuitry. How-ever, the loss in plasmonic waveguides is substantialowing to the intrinsic loss of the metal and is furthermagnified with enhanced transverse modal confine-ment [3–6], which is essential in integration ofSP-based nanocircuitry. Therefore, the design, simu-lation, and measurement of the loss in plasmonicwaveguides are critically important in the develop-ment of plasmonic waveguides.The MIM structure is one of the most intensively

investigated of plasmonic waveguides. Despite itslarger loss compared with its complementary struc-

ture, the insulator–metal–insulator (IMI) plasmonicwaveguide, the transverse modal size is significantlysmaller in the former because of the relatively shal-low field penetration to the skin depth of the metalcladding. Such small penetration also makes theMIM structures less sensitive to interface/surface de-fects, index mismatch of cladding layers, and cross-talk. However, the modal profile of a typical MIMstructure is usually below the diffraction limit [3–5].Therefore, the excitation and the loss measurementof an MIM plasmonic mode typically requires end-firing of tapered fibers or waveguides, as well as mul-tiple waveguides structures with various lengthscales [8] or scanning near-field optical microscopy(SNOM) [10–12].

The transverse transmission/reflection (TTR)method [13] presented here may significantly simpli-fy the loss measurement of the MIM plasmonicmodes. Instead of conceptually injecting light fromthe end of the waveguides, e.g., finite-differencetime-domain (FDTD) simulation [5,14,15], the TTRmethod excites a plasmonic mode in the transverse

0003-6935/10/060936-09$15.00/0© 2010 Optical Society of America

936 APPLIED OPTICS / Vol. 49, No. 6 / 20 February 2010

Page 2: Characterization of the loss of plasmonic modes in planar metal-insulator-metal waveguides by a coupling-simulation approach

direction. This can be realized by making one of themetal cladding sufficiently thin (e.g., three to fourskin depths) for light coupling. A high-index layer(e.g., prism) is then added adjacent to the thin metallayer to enable coupling. By plotting the fraction ofpower transmitted/reflected as a function of the nor-malized wave vector component of the incident wave,the Lorentzian maxima/minima are located at thereal parts of the propagation constants, and the half-widths at half-maxima/minima (HWHM) of theseresonances are equal to the imaginary parts of thepropagation constants of the allowed plasmonicmodes. Concisely stated, the TTR method providesa straightforward and simple approach for determin-ing the complex propagation constants by simulatinga coupled-waveguide structure. As a result, the TTRmethod has a similar configuration to the prism cou-pler introduced by Ulrich and Tien [16,17] and to theattenuated total reflection (ATR) configuration[18–20]. However, to the best of the authors’ knowl-edge, this is the first time such configuration has beenapplied to the plasmonic modes in a MIM structure.

2. Formulation

A. TTR Method Formulation

The transfer matrix provides the basis for a systema-tic approach for analyzing multilayer structures,such as that shown in Fig. 1. For a transverse mag-netic (TM) wave traveling in the þz direction inthe ith layer (xi−1 ≤ x ≤ xi), the magnetic field is

~Hi ¼ yHyiðxÞ exp½jðωt − γzÞ�, where y is the unit vectorin the þy direction and γ ¼ β − jα is the complex pro-pagation constant with β and α being the phase andattenuation propagation constants, respectively. Theeffective index Neff is defined as Neff ≡ β=k0, wherek0 ¼ 2π=λ0 and λ0 is the free space wavelength.The total magnetic field in the ith layer is the sum-mation ofþx and −x propagating waves, which can beexpressed as

HyiðxÞ ¼ Ai exp½−κx;iðx − xi−1Þ�þ Bi exp½þκx;iðx − xi−1Þ�; ð1Þ

where Ai and Bi are the complex field amplitudes cor-responding to the þx and −x propagating waves inthe ith layer, respectively, κx;i ¼ ðγ2 − k20εiÞ1=2 is thecomplex transverse wave vector in the ith layer,and xi defines the boundary between the ith and(iþ 1)th layers (Fig. 1). By matching the tangential

components of the electric and magnetic fields atevery interface, the field coefficient at the coverand the substrate can be related via the matrixequation

�As

Bs

�¼ Mj−1Mj−2 � � �M1M0

�Ac

Bc

¼�m11 m12

m21 m22

��Ac

Bc

�; ð2Þ

where the transfer matrix for the ith layer, Mi, isrepresented by

Mi ¼12

0BBB@

�1þ f i

κx;iκx;iþ1

�expð−κx;idiÞ

�1 − f i

κx;iκx;iþ1

�expðκx;idiÞ�

1 − f iκx;iκx;iþ1

�expð−κx;idiÞ

�1þ f i

κx;iκx;iþ1

�expðκx;idiÞ

1CCCA for i ¼ 0; � � � ; j − 1; ð3Þ

where for TE waves f i ¼ 1, while for TM wavesf i ¼ εiþ1=εi, and di is the thickness of the ith layer.By Eq. (2), the complex amplitude transmissionand reflection coefficients are represented as

cover incidence ðBs ¼ 0Þ:�ts0

¼�m11 m12

m21 m22

��1rc

�; ð4Þ

substrate incidence ðAc ¼ 0Þ:�rs1

¼�m11 m12

m21 m22

��0tc

�: ð5Þ

By algebraic manipulation,

Fig. 1. Geometry of a multilayer structure.

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Page 3: Characterization of the loss of plasmonic modes in planar metal-insulator-metal waveguides by a coupling-simulation approach

rc ¼ −m21

m22; rs ¼

m12

m22; tc ¼

1m22

;

ts ¼m11m22 −m12m21

m22:

ð6Þ

The fraction of the power reflected is

Rc ¼ jrcj2; Rs ¼ jrsj2: ð7Þ

The fraction of the power transmitted is

Tc ¼ Ts ¼ jtcj2κcκsεsεc

¼ jtsj2κsκcεcεs: ð8Þ

By Eqs. (6) and (8) we can also obtain

m11m22 −m12m21 ¼ κcκsεsεc: ð9Þ

The γ that makes the transmission and reflectioncoefficient infinite corresponds to the propagationconstant of a guided or leaky mode of the waveguidestructure [21].The essence of the TTR method is based on expres-

sing the fraction of the power transmitted approxi-mately as a rational function of the poles of thecomplex propagation constants γl for leaky modesand lossy modes [13,22]. That is,

T ¼���� 1m22

����2κcκsεsεc

≃UðβÞ���� 1QMp

l¼1ðβ − γlÞ

����2; ð10Þ

whereUðβÞ is a slowly varying function of β andMp isthe number of poles. The γl values that make thetransmission coefficients infinite correspond to thepropagation constant of a guided or leaky mode ofthe waveguide structure. This is consistent withguided modes and leaky modes being solutions ofm22 ¼ 0. Given that UðβÞ varies sufficiently slowlywith β, the TðβÞ has Lorentzian-type peaks locatedat β ¼ ReðγlÞ and has HWHM values equal toα ¼ ImðγlÞ. In the case that all the layers have zeroor negligible loss, i.e., jImðεÞj ≪ jReðεÞj, the fractionof power reflected can be approximated as R ¼ 1 − T[13]. Therefore the RðβÞ have Lorentzian-type mini-ma at β ¼ ReðγlÞ and have HWHM ¼ α ¼ ImðγlÞ.B. SP at a Single Metal/Dielectric Interface

Consider the structure shown in Fig. 2(a), which is atypical Otto configuration [23]. The SP is excited atthe metal/dielectric interface by frustrated total in-ternal reflection of the light incident upon the prism.The dispersion relation of the SP at a single metal/dielectric is given by

βSP ¼ k0

� εmεdεm þ εd

�1=2

; ð11Þ

which also implies that βSP > ε1=2d k0 and that such SPmode exists only when jεmj > −εd, ignoring the typi-cally small imaginary parts that lead to loss.

However, in the Otto configuration, the thicknessof the dielectric is not infinite, so part of the energy inthe SP mode at the metal/dielectric interface can becoupled back into the prism. Therefore, the SP modesupported by the Otto configuration is perturbed bythis leakage loss, which grows with decreasing gapdielectric thickness dg. The propagation constantγSP of the perturbed SP mode can be obtained bysolving the transfer matrix. The transfer matrix ofthis structure [Fig. 2(a)] is defined as

MSP ¼�m0

11 m012

m021 m0

22

�SP; ð12Þ

and the reflection coefficient is

rc;SP ¼ −m0

21

m022: ð13Þ

The propagation constant γSP is the solution ofm0

22 ¼ 0. As dg decreases, the loss of the SP modeincreases and the width of the fraction of power re-flected Rc;SP ¼ jrc;SPj2 increases, and the center of theRc;SP resonance moves from βSP to higher β. Examplecases are illustrated in Section 3.

C. SP in MIM Structures

Figure 2(b) shows a symmetric MIM structure. Thereare two possible plasmonic modes in such a struc-ture, one symmetric and one antisymmetric. The dis-persion relations of the two modes are given by

symmetric: tanh�κidi

2

�¼ −

κmκi

εiεm

; ð14Þ

antisymmetric: tanh�κidi

2

�¼ −

κiκm

εmεi

; ð15Þ

Fig. 2. (a) Schematic diagram of a single metal/dielectric inter-face-SP structure (Otto configuration). (b) Schematic diagram ofa symmetric MIM structure. (c) Schematic diagram of a prism-loaded MIM structure.

938 APPLIED OPTICS / Vol. 49, No. 6 / 20 February 2010

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where di is the thickness of the insulator. The sym-metric mode has no cutoff frequency. There is a sym-metric mode for any frequency above zero frequency.The antisymmetric mode has a cutoff frequency atwhich the mode makes a transition between oscilla-tory (inside the metal) mode to a plasmonic mode[24,25]. It should be noted that βs of the symmetricmode (TM0) is always larger than βSP of the metal/insulator interface, while βa of the antisymmetricmode (TM1) is always smaller than βSP. In this study,only the TM0 mode is of interest.The propagation constants γMIM of the TM0 modes

can also be obtained by solving the transfer matrix.The transfer matrix of the MIM structure [Fig. 2(b)]is defined as

MMIM ¼�m11 m12

m21 m22

�MIM

; ð16Þ

and the reflection coefficient is

rc;MIM ¼ −m21

m22: ð17Þ

The propagation constants γMIM are the solutions ofm22 ¼ 0. It should be noted that the plasmonic modescannot be directly excited from the metal cladding.Therefore, rc;MIM does not have a physically achiev-able value (e.g., jrc;MIMj > 1) near the resonances cor-responding to the plasmonic modes. In this study, oneside of the metal is made to be sufficiently thin forlight coupling. A high-index layer, such as prism,is added adjacent to the thin metal layer to enablelight coupling with a higher longitudinal wave vector.Detailed analysis on the prism-loaded MIM struc-ture is provided in Subsection 2.D.

D. Prism-Loaded MIM Structure

Based on the transfer matrix formulation, the prism-loaded MIM structure in Fig. 2(c) can be analyzed.The transfer matrix for this structure can be repre-sented as

M ¼�m11 m12

m21 m22

�MIM

�expð−κmdmÞ 0

0 expðκmdmÞ��

m011 m0

12m0

21 m022

�SP

¼�m12m0

21 expðκmdmÞ þm11m011 expð−κmdmÞ m12m0

22 expðκmdmÞ þm11m012 expð−κmdmÞ

m22m021 expðκmdmÞ þm21m0

11 expð−κmdmÞ m22m022 expðκmdmÞ þm21m0

12 expð−κmdmÞ�: ð18Þ

Therefore, the reflection coefficient for the lightincident at the prism is

rc ¼ −Mð2; 1ÞMð2; 2Þ ¼ −

m021

m022

1þ m21m011

m22m021expð−2κmdmÞ

1þ m21m012

m22m022expð−2κmdmÞ

¼ −m0

21

m022

�1þ

m21m22

m011m

022−m

012m

021

m022m

021

expð−2κmdmÞ1þ m21m0

12m22m0

22expð−2κmdmÞ

�: ð19Þ

In the case that ðm21m012Þ=ðm22m0

22Þ expð−2κmdmÞ ≪1, and usingm22 ≃ C · ðβ − γMIMÞ from Eq. (10), whereC is a constant and γMIM ≡ βMIM − jαMIM is the com-plex propagation constant of the TM0 mode in theMIM structure, Eq. (19) can be approximated as

rc ≃ −m0

21

m022

�1þm21

m22

m011m

022 −m0

12m021

m022m

021

expð−2κmdmÞ�

¼ rc;SP

�1þ VðβÞ

β − γMIM

�; ð20Þ

where the quantity VðβÞ ¼ m21Cðκpεm=κmεpÞ=ðm0

21m022 expð−2κmdmÞÞ, using m0

11m022 −m0

12m021 ¼

κpεm=κmεp, is a slowly varying function of β. Basedon Eq. (20), the fraction of power reflected Rc ¼ jrcj2can be expressed as

Rc ≃ Rc;SP

�1þ 2 · Re

�VðβÞ

β − γMIM

¼ Rc;SP

�1þ 2

·ðβ − βMIMÞ · Re½VðβÞ� þ αMIM · Im½VðβÞ�

ðβ − βMIMÞ2 þ α2MIM

: ð21Þ

Equation (21) shows that Rc is similar to Rc;SP, whichhas a resonance near the pole of m0

22, but Rc has oneor more extra resonances that correspond to the plas-monic modes of the MIM structure near the poles ofm22. Equation (21) also implies that if the numeratorof the second component is a negative constant [i.e.,VðβÞ ¼ V expð3π=2Þ, where V is a positive constant],Rc=Rc;SP has a Lorentzian-type resonance centered atNMIM ¼ βMIM=k0 and a HWHM ¼ αMIM=k0. However,because VðβÞ is not a constant and the phase of VðβÞis shifted due to the material loss in the metal, theHWHM of Rc=Rc;SP is not precisely equal to αMIM=k0. Moreover, the approximation ðm21m0

12Þ=ðm22m022Þ

expð−2κmdmÞ ¼ 0 made in Eq. (20) also causes errorssince the metal thickness dm is finite. The detailederror analysis of these errors is given in Appendix A,

20 February 2010 / Vol. 49, No. 6 / APPLIED OPTICS 939

Page 5: Characterization of the loss of plasmonic modes in planar metal-insulator-metal waveguides by a coupling-simulation approach

and a step-by-step procedure for correcting for theerrors is given in Appendix B.

3. Example Cases

In this section, the simulation performance and accu-racy of the TTR method applied to various MIMstructures is examined. The TTR simulation resultsare compared with rigorous results calculated by theargument principle method (APM) [26]. The first ex-ample chosen is a silver–air–silver structure with a200nm core at λ ¼ 0:6328 μm. The second example isa silver–oxide–silver structure with a 50nm core atλ ¼ 1:55 μm. This structure has a relatively smallercore size and a higher βMIM; therefore the gap be-tween the prism and the MIM structure should befilled with high-index material (e.g., fluid) to facili-tate the light coupling. More details are discussedin Subsection 3.B.

A. Silver–Air–Silver Structure

The first example is a symmetric MIM structure witha 200-nm void core and silver claddings. At theoperating frequency λ ¼ 0:6328 μm, the silver hascomplex dielectric constant ~εAg ¼ −15:9 − j1:07, orequivalently, refractive index ~nAg ¼ 0:135 − j3:99[27]. The normalized propagation constant γMIM=k0of the TM0 mode calculated by APM is1:13412 − j0:00505, which corresponds to a loss of0:44dB=μm or propagation length of 10 μm.In order to apply the TTR method to this MIM

structure, one of the silver claddings has to be suffi-ciently thin for light coupling and a high-index layer(e.g., prism) has to be placed adjacent to the thin sil-ver cladding, as shown in Fig. 3. In this case, the skindepth of silver δ∼ 25nm, so dm is chosen to be 75nmand 100nm to allow the appropriate couplingstrength. The prism index np has to be sufficientlylarger than NMIM and is chosen to be 1.5.The plane-wave reflection power spectra of the

structure in Fig. 3 with dm ¼ 100nm and dm ¼75nm is plotted as functions of the effective indexNeff in Figs. 4 and 5, respectively, and summarizedin Table 1. The effective indexN 0

MIM of the TM0 modeis located at the minimum of the Rc=Rc;SP resonance,and the normalized attenuation coefficient α0MIM=k0

is equal to the HWHM, where the prime denotes re-sults obtained by the TTR method, in contrast to therigorous results obtained by APM. Rc;SP can be ob-tained by qualitatively subtracting out the TM0 reso-nance from Rc for each da. It is shown in Table 1 thatthe results obtained by the TTR method are in goodagreement with the rigorous result, especially in thecase of dm ¼ 100nm. The error in α0MIM < 5% in thecase of dm ¼ 100nm and ≲10% in the case ofdm ¼ 75nm. Larger dm causes a smaller TM0 reso-nance intensity and smaller perturbation, in agree-ment with the analysis of Subsection 2.D.

As described in Appendix A, the error in α0MIM canbe estimated. In the case of dm ¼ 100nm, the errordue to the finite thickness of the metal layer dm isusually smaller than the half-resonance strengthofRc=Rc;SP as da → 0, that is,≲2%. Following the pro-cedure described in Appendix B, the phase shift isfitted as ΔϕV ∼ 15°, and the normalized attenuationcoefficient after correction is α00MIM=k0 ∼ 0:00515. Si-milarly, in the case of dm ¼ 75nm, the error due tofinite dm is ≲8%. The fitted ΔϕV ∼ 15° andα00MIM=k0 ∼ 0:0051. It is shown that in both cases,the α00MIM values have less than 2% of error. It shouldbe noted that no explicit information about da or dmis needed in the correction procedure.

Fig. 3. Schematic diagram of the prism-loaded MIM structurewith a 200nm void core. Themetal is silver with complex dielectricconstant ~εm ¼ −15:9 − j1:07, or equivalently refractive index ~nm ¼0:135 − j3:99 [27]. The operating wavelength is 0:6328 μm.

Fig. 4. Plane-wave reflection power spectrum of the structure inFig. 3 with dm ¼ 100nm. The x axis is the effective indexNeff ≡ β=k0 ¼ np sin θ, and the y axis is the fraction of power re-flected. The resonances corresponding to the air gap-metal plas-monic mode and the TM0 mode of the MIM structure are labeled.

Fig. 5. Plane-wave reflection power spectrum of the structure inFig. 3 with dm ¼ 75nm.

940 APPLIED OPTICS / Vol. 49, No. 6 / 20 February 2010

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B. Silver–Oxide–Silver Structure

The second example is a symmetric MIM structurewith a 50nm SiO2 core and silver claddings. Atthe operating frequency λ ¼ 1:55 μm, the silver hascomplex dielectric constant ~εAg ¼ −86:6 − j8:74, orequivalently, refractive index ~nAg ¼ 0:469 − j9:32[27]. The normalized propagation constant γMIM=k0 of the TM0 mode calculated by APM is2:11140 − j0:02967, which corresponds to a loss of1:04dB=μm or propagation length of 4:2 μm. Thehigher NMIM in this case is the result of the higherindex and smaller size of the core insulator.In order to apply the TTRmethod to this structure,

one of the silver claddings is made thinner and aprism is placed adjacent to the MIM structure. Inthis case, the skin depth of silver is δ∼ 26nm, sodm is chosen to be 80nm to allow the appropriatecoupling strength. The prism index np is chosen tobe 2.5.The plane-wave reflection power spectrum of the

structure in Fig. 6 is shown in Fig. 7 and summarizedin Table 2. The N 0

MIM and α0MIM are obtained in thesame manner as in the previous example. It is shownin Table 2 that the results of the TTR method are ingood agreement with the rigorous result. The error inα0MIM < 5% for df ¼ 100 and 200nm and <10% fordf ¼ 0 and 50nm.Following Appendix A, the error of the HWHM can

be estimated. The error due to finite dm in this case is≲6%. The fitted phase shift ΔϕV ∼ 20°, and the

normalized attenuation coefficient after correctionis α00MIM=k0 ∼ 0:0297. The detailed fitting procedurefor this case is given in Appendix B.

4. Summary and Discussion

In this paper, a coupling simulation method, thetransverse transmission/reflection (TTR) method,is presented for the characterization of the plasmonicmodes in MIM structures. The TTR method is note-worthy for its simplicity and capability of character-izing plasmonic modes with a linkage to the physicalattenuated total reflection (ATR) configuration. Bysimulating such a structure, both the real part andthe imaginary part of the propagation constant ofa plasmonic mode can be characterized by the angleand width of the Lorentzian-type reflection reso-nance. It is shown in the example cases that appro-priate coupling strength can be obtained when thethickness of the metal is about three to four skindepths. The resulting errors in the attenuation coef-ficient are typically smaller than 10% and can beminimized using the analysis based on multiplereflection power spectra at various gap dielectricthickness.

To summarize, the TTRmethod presented here is apotentially powerful approach for characterizingplasmonic modes. Due to its transverse nature, a lossmeasurement based on the TTR method may obviatethe need of tapered end-couplers and the need ofmultiple waveguide samples or scanning near-fieldoptical microscopy (SNOM). A paper describing cor-responding experimental results by the authors hasrecently been submitted for publication.

Table 1. Normalized Complex Propagation Constantγ0MIM=k 0 Calculated by the TTR Method, for the MIM

Structure Shown in Fig. 3a

da dm TTR Method

0 100nm 1:1348 − j0:00530:25λ ” 1:1350 − j0:00530:50λ ” 1:1348 − j0:00510 75nm 1:1348 − j0:00550:25λ ” 1:1354 − j0:00570:50λ ” 1:1354 − j0:0053

aThe rigorous complex propagation constant for the TM0 modeof the MIM structure without the prism loaded (dm ¼ ∞)is γMIM=k0 ¼ 1:13412 − j0:00505.

Table 2. Normalized Complex Propagation Constantγ0MIM=k 0 Calculated by the TTR Method, for the MIM

Structure Shown in Fig. 6a

df dm TTR Method

0 80nm 2:1179 − j0:032650nm ” 2:1191 − j0:0329100nm ” 2:1178 − j0:0305200nm ” 2:1167 − j0:0296

aThe rigorous complex propagation constant for the TM0 modeof the MIM structure without the prism loaded (dm ¼ ∞)is γMIM=k0 ¼ 2:11140−j0:02967.

Fig. 7. Plane-wave reflection power spectrum of the structure inFig. 6 with dm ¼ 80nm.

Fig. 6. Schematic diagram of the prism-loaded MIM structurewith a 50nm SiO2 core. The metal is silver with complex dielectricconstant ~εm ¼ −86:6 − j8:74, or equivalently, refractive index ~nm ¼0:469 − j9:32 [27]. The operating wavelength is 1:55 μm.

20 February 2010 / Vol. 49, No. 6 / APPLIED OPTICS 941

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Appendix A: Detailed Error Analysis

The attenuation coefficient α0MIM obtained from theTTR method is specified by the HWHM of Rc=Rc;SP,which equals α0MIM=k0. Following Subsection 2.D, thequantity α0MIM differs from the rigorously calculatedattenuation coefficient αMIM. The error in α0MIM hasthree sources: (1) the finite metal thickness dm,(2) the phase shift of VðβÞ due to loss in the metal,and (3) the background variation in VðβÞ. A step-by-step procedure for obtaining the value of the at-tenuation coefficient α00MIM corrected for these errorsis given in Appendix B.The first error is caused by the approximation A≡

ðm21m012Þ=ðm22m0

22Þ expð−2κmdmÞ ¼ 0 in Eq. (20). Be-cause of the m22 in the denominator, jAj has a peaknear where m22 has a pole, which is also near whereRc=Rc;SP has a minimum. In the worst case, the reso-nance strength of Rc=Rc;SP is decreased by100jAjmax%, and its HWHM is broadened by similarpercentage. jAjmax can be estimated by comparingwith the value of ðm21=m22Þ½ðm0

11m022 −m0

12m021Þ=ðm0

22m021Þ� expð−2κmdmÞ ¼ VðβÞ=ðβ − γMIMÞ, which is

the resonance strength of Rc=Rc;SP. The transfer ma-trix MSP when the gap dielectric thickness dg → 0may be expressed as

MSPðdg → 0Þ ¼ 12

�1þm0

SP 1 −m0SP

1 −m0SP 1þm0

SP

�; ðA1Þ

wherem0SP ¼ ðn2

mκpÞ=ðn2pκmÞ, which is imaginary for a

lossless metal. For a low-loss metal, jðm011m

022 −

m012m

021Þ=ðm0

22m021Þj ¼ j4m0

SP=ð1 −m02SPÞj has values

between 1 and 2 for Neff ¼ 0 to ½n2mn2

pðn2m þ n2

pÞ=ðn4

m þ n4pÞ�1=2∼ np. Therefore, based on Eq. (21),

the value of jðm21=m22Þ expð−2κmdmÞj is between1=4 and 1=2 times the resonance strength ofRc=Rc;SP when dg → 0. Since the value of jm0

12=m022j

is between 1 and 2 for any dg, jAjmax at any dg ≲

1=2 times the resonance strength of Rc=Rc;SP whendg → 0. It should be noted that α0MIM obtained with-out the approximation A ¼ 0 [Eq. (19)] is alwayslarger than that with the approximation [Eq. (20)].The second source of error is caused by the mate-

rial loss in the metal. In the case of a lossless metal,ϕV ¼ 3π=2. However, ϕV is shifted when the metal islossy. Based on Eq. (21) and assuming VðβÞ ¼V exp½ð3π=2Þ þΔϕV �, where V is a positive constant,βmin at the minimum of the phase-shifted LorentzianRc=Rc;SP can be represented as

βmin ¼ βMIM þ αMIMcosðΔϕVÞ − 1sinðΔϕVÞ

; ðA2Þ

and βhm values at the half-minimum points are

βhm ¼ βMIM þ αMIM−2 sinðΔϕVÞ � f2½1þ cosðΔϕVÞ� þ sin2ðΔϕVÞg1=2

1þ cosðΔϕVÞ; ðA3Þ

where the positive and negative signs correspond tothe right and left half-minimum points, respectively.Figures 8(a) shows the variation of βmin and βhmvalues, and Fig. 8(b) shows the broadening effectof α0MIM as a function of ΔϕV.

The third source of error is caused by backgroundvariation of VðβÞ, and the effect is dependent onΔϕV .Assuming the phase-shifted Lorentzian is multipliedby a linearly varying function VðβÞ, Fig. 9 showsthe variation of α0MIM as a function of the percen-tage background variation, jVðβMIM þ αMIMÞ=VðβMIM − αMIMÞj − 1, at various ΔϕV values.

Appendix B: Method of Determining α00MIM

Based on the discussion in Appendix A, the correctedα00MIM can be obtained by using multiple Rc values atvarious dg values, utilizing the fact that the variationof α0MIM is proportional to the percentage backgroundvariation and that the slopes depend on the phaseshift ΔϕV (Fig. 9). From the α0MIM values obtainedfrom the VðβÞ variations, the quantity ΔϕV andthe corrected α00MIM can be estimated by the slope ofthe α0MIM versus the percentage background varia-tion. By definition, the variation of jVðβÞj is deter-mined by the variation of jðm0

11m022 −m0

12m021Þ=ðm0

22m021Þj and jðm21=m22Þ expð−2κmdmÞj; the former

is related to the prism–dielectric–metal structure,and the latter is related to the MIM structure. There-fore, the variation of jVðβÞj can be controlled by vary-ing the gap dielectric thickness dg, while thevariation of jðm21=m22Þ expð−2κmdmÞj stays constantand does not affect the slope of Fig. 9. The variationof jðm0

11m022 −m0

12m021Þ=ðm0

22m021Þj can be obtained by

using

Fig. 8. (a) Variation of βmin and βhm values as a function of thephase shift ΔϕV caused by the material loss of the metal. Theupper βhm corresponds to the right half-minimum point, and thelower one to the left half-minimum point. (b) Broadening ofα0MIM as a function of ΔϕV .

942 APPLIED OPTICS / Vol. 49, No. 6 / 20 February 2010

Page 8: Characterization of the loss of plasmonic modes in planar metal-insulator-metal waveguides by a coupling-simulation approach

����m011m

022 −m0

12m021

m022m

021

����¼����ts;SPtc;SPrc;SP

����≃Tc;SP ∝ 1 − Rc;SP;

ðB1Þ

where Rc;SP can be obtained by qualitatively sub-tracting out the TM0 resonance. It should be notedthat no explicit information about df or dm is needed,which means the correction procedure can be imple-mented by simply using multiple Rc values at var-ious dg values.The correction procedure of α0MIM is given by the

following steps. For illustration purpose, the proce-dure is applied to the example case in Subsection 3.B.

1. Calculate/plot Rc versus Neff at various df .2. Produce Rc;SP versus Neff by qualitatively sub-

tracting out TM0 resonance from Rc for each df .3. From Rc=Rc;SP versus Neff , estimate the error

due to the finite dm, which is the half-resonancestrength as df → 0. The error is ∼6% in this case.4. From Rc=Rc;SP versusNeff , calculate β0MIM from

the location of the minimum and α0MIM from theHWHM for each df . The quantity α0MIM should be sub-tracted by the broadening error due to the finite dmobtained in step 3.5. From Rc;SP versus Neff in step 2, calculate the

background variation, ½1 − Rc;SPðβ0MIM þ α0MIMÞ�=½1−

Rc;SPðβ0MIM − α0MIMÞ� − 1, for each df . The backgroundvariation is proportional to jVðβ0MIM þ α0MIMÞ=Vðβ0MIM − α0MIMÞj − 1 according to Eq. (B1). In thiscase, the background variation is ∼4%, −3%, −27%,and −30% for df ¼ 0, 50nm, 100nm, and 200nm,respectively.

6. From the plot of α0MIM versus the backgroundvariation (Fig. 10), estimate ΔϕV by comparing withFig. 9. In this case, ΔϕV ∼ 20°.

7. Calculate the corrected attenuation α00MIM from

α00MIM ¼ α0MIMðFig: 10Þðα0MIM=αMIMÞðFig: 9Þ

: ðB2Þ

In this case, α00MIM=k0 ∼ 0:0297.

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Fig. 9. Variation of α0MIM as a function of the linear backgroundvariation at various phase shift ΔϕV .

20 February 2010 / Vol. 49, No. 6 / APPLIED OPTICS 943

Page 9: Characterization of the loss of plasmonic modes in planar metal-insulator-metal waveguides by a coupling-simulation approach

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