Electromagnetic Wave PropagationLecture 2: Time harmonic dependence,
constitutive relations
Daniel Sjoberg
Department of Electrical and Information Technology
September 5, 2013
Outline
1 Harmonic time dependence
2 Constitutive relations, time domain
3 Constitutive relations, frequency domain
4 Examples of material models
5 Bounds on metamaterials
6 Conclusions
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Outline
1 Harmonic time dependence
2 Constitutive relations, time domain
3 Constitutive relations, frequency domain
4 Examples of material models
5 Bounds on metamaterials
6 Conclusions
3 / 53
Scope
I The theory given in this lecture (and the entire course) isapplicable to the whole electromagnetic spectrum.
I However, different processes are dominant in different bands,making the material models different.
I Today, you learn what restrictions are imposed by therequirements
1. Linearity2. Causality3. Time translational invariance4. Passivity
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Electromagnetic spectrum, c0 = fλ ≈ 3 · 108m/s
Band Frequency WavelengthELF Extremely Low Frequency 30–300Hz 1–10MmVF Voice Frequency 300–3000Hz 100–1000 kmVLF Very Low Frequency 3–30 kHz 10-100 kmLF Low Frequency 30–300 kHz 1–10 kmMF Medium Frequency 300–3000 kHz 100–1000mHF High Frequency 3–30MHz 10–100mVHF Very High Frequency 30–300MHz 1–10mUHF Ultra High Frequency 300–3000MHz 10–100 cmSHF Super High Frequency 3–30GHz 1–10 cmEHF Extremely High Frequency 30–300GHz 1–10mm
Submillimeter 300–3000GHz 100–1000µmInfrared 3–300THz 1–100µmVisible 385–789THz 380–780 nmUltraviolet 750THz–30PHz 10–400 nmX-ray 30PHz–3EHz 10nm–100 pmγ-ray >3EHz <100 pm
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Three ways of introducing time harmonic fields
I Fourier transform (finite energy fields, ω = 2πf)
E(r, ω) =
∫ ∞−∞
E(r, t)e−jωt dt
E(r, t) =1
2π
∫ ∞−∞
E(r, ω)ejωt dω
I Laplace transform (causal fields, zero for t < 0, s = α+ jω)
E(r, s) =
∫ ∞0E(r, t)e−st dt
E(r, t) =1
2πj
∫ α+j∞
α−j∞E(r, s)est ds
I Real-value convention (purely harmonic cosωt, preservesunits)
E(r, t) = Re{E(r, ω)ejωt}
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Some examples
Unit step function: u(t) =
{0 t < 0
1 t > 0
E(r, t) Fourier Laplace Real-value
e−αt2 √
παe−ω
2
4α — —
cos(ω0t) π(δ(ω + ω0) + δ(ω − ω0)) — 1
sin(ω0t) jπ(δ(ω + ω0)− δ(ω − ω0)) — −j
e−atu(t) 1jω+a
1s+a —
e−at cos(ω0t)u(t)jω+a
(jω+a)2+ω20
s+a(s+a)2+ω2
0—
e−at sin(ω0t)u(t)ω0
(jω+a)2+ω20
ω0
(s+a)2+ω20
—
δ(t) 1 1 —
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Different time conventions
Different traditions:
Engineering: Time dependence ejωt, plane wave factor ej(ωt−k·r).
Physics: Time dependence e−iωt, plane wave factor ei(k·r−ωt).
If you use j and i consistently, all results can be translated betweenconventions using the simple rule
j = −iIn this course we follow Orfanidis’ choice ejωt.
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Outline
1 Harmonic time dependence
2 Constitutive relations, time domain
3 Constitutive relations, frequency domain
4 Examples of material models
5 Bounds on metamaterials
6 Conclusions
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The need for material models
Maxwell’s equations are
∇×E(r, t) = −∂B(r, t)
∂t
∇×H(r, t) = J(r, t) +∂D(r, t)
∂t
This is 2× 3 = 6 equations for at least 4× 3 = 12 unknowns.Something is needed! We choose E and H as our fundamentalfields (partly due to conformity with boundary conditions), andsearch for constitutive relations on the form{
DB
}= F
({EH
})This would provide the missing 6 equations.
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Examples of models
I Linear, isotropic materials (“standard media”):
D = εE, B = µH
I Linear, anisotropic materials (different in different directions):
D = (εxxx+ εyyy + εzzz) ·E ⇔
Dx
Dy
Dz
=
εx 0 00 εy 00 0 εz
ExEyEz
I Linear, dispersive materials (depend on the history):
Debye material Gyrotropic material
D = ε0E + P B = µ0(H +M)
∂P
∂t= ε0αE − P /τ
∂M
∂t= ωS z × (βM −H)
The models correspond to the physical processes in the material.11 / 53
Basic assumptions
To simplify, we formulate our assumptions for a non-magneticmaterial where D = F (E) and B = µ0H. We require themapping F to satisfy four basic physical principles:
Linearity: For each α, β, E1, and E2 we have
F (αE1 + βE2) = αF (E1) + βF (E2)
Causality: For all fields E such that E(t) = 0 when t < τ , wehave
F (E)(t) = 0 for t < τ
Time translational invariance: If D1 = F (E1), D2 = F (E2), andE2(t) = E1(t− τ), we have
D2(t) =D1(t− τ)
Passivity: The material is not a source of electromagneticenergy, that is, ∇ · 〈P〉 ≤ 0.
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The general linear model
The result of the assumptions is that all such materials can bemodeled as
D(t) = ε0
[E(t) +
∫ t
−∞χe(t− t′) ·E(t′) dt′
]+
∫ t
−∞ξ(t− t′) ·H(t′) dt′
B(t) =
∫ t
−∞ζ(t− t′) ·E(t′) dt′
+ µ0
[H(t) +
∫ t
−∞χm(t− t′) ·H(t′) dt′
]The dyadic convolution kernels χe(t), ξ(t), ζ(t), and χm(t) modelthe induced polarization and magnetization.
Linearity, causality, time translational invariance byconstruction. Passivity will be seen in frequency domain.
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Instantaneous response
Some physical processes in the material may be considerably fasterthan the others
This means the susceptibility function can be split in two parts
χ(t) = χ1(t) + χ2(t)
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Instantaneous response, continued
Assume that E(t) does not vary considerably on the time scale ofχ1(t). We then have
D(t)/ε0 = E(t) +
∫ t
−∞[χ1(t− t′) + χ2(t− t′)]E(t′) dt′
= E(t) +
[∫ t
−∞χ1(t− t′) dt′
]E(t) +
∫ t
−∞χ2(t− t′)E(t′) dt′
= E(t) +
[∫ ∞0
χ1(t′) dt′
]E(t)︸ ︷︷ ︸
=ε∞E(t)
+
∫ t
−∞χ2(t− t′)E(t′) dt′
The quantity ε∞ = 1 +∫∞0 χ1(t
′) dt′ is called the instantaneousresponse (or momentaneous response, or optical response).Thus, there is some freedom of choice how to model thematerial, depending on the time scale!
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Instantaneous response, example
0 5 10 15 20 25 30t
0.5
0.0
0.5
1.0
1.5
2.0P(t)/ε0
E(t)
χ(t)
D(t)/ε0
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Outline
1 Harmonic time dependence
2 Constitutive relations, time domain
3 Constitutive relations, frequency domain
4 Examples of material models
5 Bounds on metamaterials
6 Conclusions
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Constitutive relations in the frequency domain
Applying a Fourier transform to the convolutions implies
D(ω) = ε0 [ε∞ ·E(ω) + χe(ω) ·E(ω)] + ξ(ω) ·H(ω)
B(ω) = ζ(ω) ·E(ω) + µ0 [µ∞ ·H(ω) + χm(ω) · η0H(ω)]
or (D(ω)
B(ω)
)=
(ε(ω) ξ(ω)ζ(ω) µ(ω)
)·(E(ω)
H(ω)
)where we introduced the permittivity and permeability dyadics
ε(ω) = ε0 [ε∞ + χe(ω)] µ(ω) = µ0 [µ∞ + χm(ω)]
This is a fully bianisotropic material model.
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Classification of materials
Type ε, µ ξ, ζ
Isotropic Both ∼ I Both 0An-isotropic Some not ∼ I Both 0Bi-isotropic Both ∼ I Both ∼ IBi-an-isotropic All other cases
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Modeling arbitriness
Assume the models
J(ω) = σ(ω)E(ω), D(ω) = ε(ω)E(ω)
The total current in Maxwell’s equations can then be written
J(ω) + jωD(ω) = [σ(ω) + jωε(ω)]︸ ︷︷ ︸=σ′(ω)
E(ω) = J ′(ω)
= jω
[σ(ω)
jω+ ε(ω)
]︸ ︷︷ ︸
=ε′(ω)
E(ω) = jωD′(ω)
where σ′(ω) and ε′(ω) are equivalent models for the material.Thus, there is an arbitrariness in how to model dispersivematerials, either by a conductivity model (σ′(ω)) or by apermittivity model (ε′(ω)), or any combination.
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When to use what?
Consider the total current as a sum of a conduction current Jc
and a displacement current Jd:
J tot(ω) = σc(ω)E︸ ︷︷ ︸Jc(ω)
+ jωεd(ω)E︸ ︷︷ ︸Jd(ω)
The ratio can take many different values (using f = 1GHz)
|Jc(ω)||Jd(ω)|
=|σc(ω)||ωεd(ω)|
=
109 copper (σ = 5.8 · 107 S/m and ε = ε0)
1 seawater (σ = 4S/m and ε = 72ε0)
10−9 glass (σ = 10−10 S/m and ε = 2ε0)
18 orders of magnitude in difference! Conductivity model goodwhen |Jc| � |Jd|, permittivity model good when |Jd| � |Jc|.
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Poynting’s theorem in the frequency domain
In the time domain we had
∇· (E(t)×H(t))+H(t) · ∂B(t)
∂t+E(t) · ∂D(t)
∂t+E(t) ·J(t) = 0
For time harmonic fields, we consider the time average over oneperiod (where 〈f(t)〉 = 1
T
∫ t+Tt f(t′) dt′):
∇·〈E(t)×H(t)〉+⟨H(t) · ∂B(t)
∂t
⟩+
⟨E(t) · ∂D(t)
∂t
⟩+〈E(t) · J(t)〉 = 0
The time average of a product of two time harmonic signals is〈f(t)g(t)〉 = 1
2 Re{f(ω)g(ω)∗}.
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Poynting’s theorem, continued
The different terms are
〈E(t)×H(t)〉 = 1
2Re{E(ω)×H(ω)∗} = 〈P〉⟨
H(t) · ∂B(t)
∂t
⟩=
1
2Re {−jωH(ω) ·B(ω)∗}⟨
E(t) · ∂D(t)
∂t
⟩=
1
2Re {−jωE(ω) ·D(ω)∗}
〈E(t) · J(t)〉 = 1
2Re {E(ω) · J(ω)∗}
For a purely dielectric material, we have D(ω) = ε(ω) ·E(ω) and
2Re {−jωE(ω) ·D(ω)∗}= −jωE(ω) · [ε(ω) ·E(ω)]∗ + jωE(ω)∗ · ε(ω) ·E(ω)
= jωE(ω)∗ · [ε(ω)− ε(ω)†] ·E(ω)
where ε(ω)† denotes the hermitian transpose of ε(ω).
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Poynting’s theorem, final version
Using a permittivity model (J = 0), we have
∇ · 〈P〉 = − jω
4
(E(ω)
H(ω)
)†
·(ε(ω)− ε(ω)† ξ(ω)− ζ(ω)†ζ(ω)− ξ(ω)† µ(ω)− µ(ω)†
)·(E(ω)
H(ω)
)Passive material: ∇ · 〈P〉 ≤ 0
Active material: ∇ · 〈P〉 > 0 ⇐= Definitions!
Lossless material: ∇ · 〈P〉 = 0
This boils down to conditions on the material matrix
jω
(ε(ω)− ε(ω)† ξ(ω)− ζ(ω)†ζ(ω)− ξ(ω)† µ(ω)− µ(ω)†
)= 2Re
{jω
(ε(ω) ξ(ω)ζ(ω) µ(ω)
)}= −2ω Im
{(ε(ω) ξ(ω)ζ(ω) µ(ω)
)}If it is positive we have a lossy material, if it is zero we have alossless material.
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Example: “Standard media”
With the material model D = εE, J = σE, B = µH we have(ε(ω) ξ(ω)ζ(ω) µ(ω)
)=
((ε+ σ
jω
)I 0
0 µI
)
and
−ω Im
{(ε(ω) ξ(ω)ζ(ω) µ(ω)
)}=
(σI 00 0
)This model is lossy with electric fields present, but not with puremagnetic fields. In wave propagation, we always have both E andH fields.
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Lossless media
The condition on lossless media,(ε(ω)− ε(ω)† ξ(ω)− ζ(ω)†ζ(ω)− ξ(ω)† µ(ω)− µ(ω)†
)= 0
can also be written(ε(ω) ξ(ω)ζ(ω) µ(ω)
)=
(ε(ω) ξ(ω)ζ(ω) µ(ω)
)†That is, the matrix should be hermitian symmetric.
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Isotropic materials
A bi-isotropic material is described by(ε(ω) ξ(ω)ζ(ω) µ(ω)
)=
(ε(ω)I ξ(ω)Iζ(ω)I µ(ω)I
)The passivity requirement implies that all eigenvalues of the matrix
jω
(ε(ω)− ε(ω)∗ ξ(ω)− ζ(ω)∗ζ(ω)− ξ(ω)∗ µ(ω)− µ(ω)∗
)are positive. If ξ = ζ = 0 it is seen that this requires (using thatε(ω)− ε(ω)∗ = 2j Im ε(ω))
−ω Im ε(ω) > 0, −ω Imµ(ω) > 0
and if ξ and ζ are nonzero we also require (after more algebra)
|ξ(ω)− ζ(ω)∗|2 < 4 Im ε(ω) Imµ(ω)
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Kramers-Kronig dispersion relations
The causality requirement implies the Kramers-Kronig dispersionrelations (writing χ(ω) = χr(ω)− jχi(ω) for the real and imaginarypart)
χr(ω) =1
πp.v.
∫ ∞−∞
χi(ω′)
ω′ − ωdω′
χi(ω) = −1
πp.v.
∫ ∞−∞
χr(ω′)
ω′ − ωdω′
where the principal value of a singular integral is
p.v.
∫ ∞−∞
χi(ω′)
ω′ − ωdω′ = lim
δ→0
[∫ ω−δ
−∞
χi(ω′)
ω′ − ωdω′ +
∫ ∞ω+δ
χi(ω′)
ω′ − ωdω′]
The Kramers-Kronig relations prohibit the existence of a losslessfrequency dependent material.
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Some notes
I The Kramers-Kronig relations restrict the possible frequencybehavior of any causal material.
I It requires a model χ(ω) for all frequencies.
I Usually, our models are derived or measured only in a finitefrequency interval, ω1 < ω < ω2.
I We need to extrapolate the models to zero and infinitefrequencies, ω → 0 and ω →∞. Not a trivial task!
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Outline
1 Harmonic time dependence
2 Constitutive relations, time domain
3 Constitutive relations, frequency domain
4 Examples of material models
5 Bounds on metamaterials
6 Conclusions
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Randomly oriented dipoles
Consider a medium consisting of randomly oriented electric dipoles,for instance water. The polarization is
P = lim∆V→0
∑i pi
∆V
A typical situation is depicted below.
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Physical processes
We now consider two processes:
1. The molecules strive to align with an imposed electric field, atthe rate ε0αE.
2. Thermal motion tries to disorient the polarization. With τbeing the relaxation time for this process, the rate of changesin P are proportional to −P /τ .
This results in the following differential equation:
∂P (t)
∂t= ε0αE(t)− P (t)
τ
This is an ordinary differential equation with the solution(assuming P = 0 at t = −∞)
P (t) = ε0
∫ t
−∞αe−(t−t
′)/τE(t′) dt′
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Physical processes
We now consider two processes:
1. The molecules strive to align with an imposed electric field, atthe rate ε0αE.
2. Thermal motion tries to disorient the polarization. With τbeing the relaxation time for this process, the rate of changesin P are proportional to −P /τ .
This results in the following differential equation:
∂P (t)
∂t= ε0αE(t)− P (t)
τ
This is an ordinary differential equation with the solution(assuming P = 0 at t = −∞)
P (t) = ε0
∫ t
−∞αe−(t−t
′)/τE(t′) dt′
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Dispersion or conductivity model
From the solution we identify the susceptibility function
χ(t) = u(t)αe−t/τ
This is monotonically decaying without oscillations.
Including allthe effects in the D-field results inD(t) = ε0
(E(t) +
∫ t
−∞αe−(t−t
′)/τE(t′) dt′)
J(t) = 0
and shifting it to J results inD(t) = ε0E(t)
J(t) = ε0αE(t)− ε0α
τ
∫ t
−∞e−(t−t
′)/τE(t′) dt′
Both versions have the same total current J(t) + ∂D(t)∂t .
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Dispersion or conductivity model
From the solution we identify the susceptibility function
χ(t) = u(t)αe−t/τ
This is monotonically decaying without oscillations. Including allthe effects in the D-field results inD(t) = ε0
(E(t) +
∫ t
−∞αe−(t−t
′)/τE(t′) dt′)
J(t) = 0
and shifting it to J results inD(t) = ε0E(t)
J(t) = ε0αE(t)− ε0α
τ
∫ t
−∞e−(t−t
′)/τE(t′) dt′
Both versions have the same total current J(t) + ∂D(t)∂t .
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Dispersion or conductivity model
From the solution we identify the susceptibility function
χ(t) = u(t)αe−t/τ
This is monotonically decaying without oscillations. Including allthe effects in the D-field results inD(t) = ε0
(E(t) +
∫ t
−∞αe−(t−t
′)/τE(t′) dt′)
J(t) = 0
and shifting it to J results inD(t) = ε0E(t)
J(t) = ε0αE(t)− ε0α
τ
∫ t
−∞e−(t−t
′)/τE(t′) dt′
Both versions have the same total current J(t) + ∂D(t)∂t .
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Response to different excitations
Consider two different excitation functions:
I One square pulse E(t) = 1 for 0 < t < t0, and zero elsewhere.
I A damped sine function, E(t) = e−t/t0 sin(ωat)u(t).
The response P (t) can be calculated by numerically performingthe convolution integral
P (t) = ε0
∫ t
−∞χ(t− t′)E(t′) dt′
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Debye model, square pulse excitation
0 5 10 15 20 25 30t
0.0
0.5
1.0
1.5
2.0
2.5
3.0
3.5P(t)/ε0
E(t)
χ(t)
D(t)/ε0
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Debye model, sine excitation
0 5 10 15 20 25 30t
1.0
0.5
0.0
0.5
1.0
1.5P(t)/ε0
E(t)
χ(t)
D(t)/ε0
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Debye material in frequency domain
The susceptibility kernel is χ(t) = αe−t/τu(t), with the Fouriertransform
χ(ω) =
∫ ∞0
αe−t/τe−jωt dt =α
jω + 1/τ=
ατ
1 + jωτ
The real and negative imaginary parts have typical behavior asbelow:
0.0 0.5 1.0 1.5 2.0 2.5 3.00.0
0.5
1.0
1.5
2.0
2.5real/neg imag
χ(ω)
and the relative permittivity is εr(ω) = 1 + χ(ω) = ε′ − jε′′.
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Harmonic oscillator
The archetypical material behavior is derived from an electronorbiting a positively charged nucleus. The typical forces on theelectron are:
1. An electric force F 1 = qE from the applied electric field.
2. A restoring force proportional to the displacementF 2 = −mω2
0r, where ω0 is the harmonic frequency.
3. A frictional force proportional to the velocity,F 3 = −mν∂r/∂t.
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Harmonic oscillator, continued
Newton’s acceleration law now gives
m∂2r
∂t2= F 1 + F 2 + F 3 = qE −mω2
0r −mν∂r
∂t
Introducing the polarization as P = Nqr, where N is the numberof charges per unit volume, we have
∂2P (t)
∂t2+ ν
∂P (t)
∂t+ ω2
0P (t) =Nq2
mE(t)
This is an ordinary differential equation, with the solution(assuming P = 0 for t = −∞)
P (t) = ε0ω2p
ν0
∫ t
−∞e−(t−t
′)ν/2 sin(ν0(t− t′))E(t′) dt′
with ωp = Nq2/(mε0) and ν20 = ω20 − ν2/4.
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Interpretation
The susceptibility function of the Lorentz model is
χ(t) = u(t)ω2p
ν0e−tν/2 sin(ν0t)
with typical behavior as below.
0 5 10 15 20 25 30t
0.8
0.6
0.4
0.2
0.0
0.2
0.4
0.6
0.8
1.0χ(t)
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Lorentz model, square pulse excitation
0 5 10 15 20 25 30t
1.0
0.5
0.0
0.5
1.0
1.5
2.0P(t)/ε0
E(t)
χ(t)
D(t)/ε0
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Lorentz model, sine excitation
0 5 10 15 20 25 30t
1.0
0.5
0.0
0.5
1.0
1.5P(t)/ε0
E(t)
χ(t)
D(t)/ε0
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Lorentz model, resonant excitation
0 5 10 15 20 25 30t
6
4
2
0
2
4
6P(t)/ε0
E(t)
χ(t)
D(t)/ε0
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Lorentz material in frequency domain
The susceptibility kernel is χ(t) =ω2p
ν0e−νt/2 sin(ν0t)u(t), with the
Fourier transform
χ(ω) =
∫ ∞0
ω2p
ν0e−νt/2 sin(ν0t)e
−jωt dt =ω2p
−ω2 + ω20 + jων
The real and negative imaginary parts have typical behavior asbelow:
0.0 0.5 1.0 1.5 2.0 2.5 3.03
2
1
0
1
2
3
4
5
6real/neg imag
χ(ω)
and the relative permittivity is εr(ω) = 1 + χ(ω) = ε′ − jε′′.44 / 53
Example: permittivity of water
Microwave properties (one Debye model):
Light properties (many Lorentz resonances):
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Handin 1
In the first handin, you will model and interpret the response of aferromagnetic material, when subjected to a magnetic field.
H
M
The magnetic moment of each atom precesses around the appliedmagnetic field, described by the Landau-Lifshitz-Gilbert equation
∂M
∂t= −γµ0M ×H + α
M
|M |× ∂M
∂t
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Outline
1 Harmonic time dependence
2 Constitutive relations, time domain
3 Constitutive relations, frequency domain
4 Examples of material models
5 Bounds on metamaterials
6 Conclusions
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What is a metamaterial?
I Engineered materials,designed to have unusualproperties
I Periodic structures
I Resonant inclusions
I Negative refractive index
I Negative or near zeropermittivity/permeability
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Some examples
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Typical frequency behavior of a dielectric
Frequency in Hz103 106 109 1012 1015
ε'
ε''
ε=ε'-jε''
atomic
dipolar
ionicelectronic
VIS UVinfraredmicrowave
ε(0)
ε(inf)
easy
hard
hard
Based on original Wikimedia image,courtesy of Prof. K. A. Mauritz.
Between the low- and high-frequency asymptotes (green region),there are no bandwidth limitations for metamaterial design.Outside the asymptotes (red regions), there are strong restrictionson bandwidth for metamaterials.
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Bounds on metamaterials
The requirements of linearity, causality, time translationalinvariance, and passivity, gives bounds on the relative bandwidth B(after some complex analysis involving Kramers-Kronig relations).
maxω∈B|ε(ω)− εm| ≥
B
1 +B/2(ε∞ − εm)
{1/2 lossy case
1 lossless case
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Outline
1 Harmonic time dependence
2 Constitutive relations, time domain
3 Constitutive relations, frequency domain
4 Examples of material models
5 Bounds on metamaterials
6 Conclusions
52 / 53
Conclusions
I Constitutive relations are necessary in order to fully solveMaxwell’s equations.
I Their form is restricted by physical principles such as linearity,causality, time translational invariance, and passivity.
I A Debye model is suitable for dipoles aligning with animposed field (relaxation model).
I A Lorentz model is suitable for bound charges (resonancemodel).
I There are restrictions on what kind of frequency behavior isphysically possible. If you want extreme behavior (outside low-and high-frequency asymptotes), you get small bandwidth.
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